scholarly journals The Cluster Low-Streams Regression Method for Fast Computations of Top-of-the-Atmosphere Radiances in Absorption Bands

2020 ◽  
pp. short25-1-short25-9
Author(s):  
Ana del Aguila ◽  
Dmitry Efremenko

Atmospheric composition sensors provide a huge amount of data. A key component of trace gas retrieval algorithms are radiative transfer models (RTMs), which are used to simulate the spectral radiances in the absorption bands. Accurate RTMs based on line-by-line techniques are time-consuming. In this paper we analyze the efficiency of the cluster low-streams regression (CLSR) technique to accelerate computations in the absorption bands. The idea of the CLRS method is to use the fast two-stream RTM model in conjunction with the line-by-line model and then to refine the results by constructing the regression model between two- and multi-stream RTMs. The CLSR method is applied to the Hartley-Huggins, O2 A-, water vapour and CO2 bands for the clear sky and several aerosol types. The median error of the CLSR method is below 0.001 %, the interquartile range (IQR) is below 0.1 %, while the performance enhancement is two orders of magnitude.

2021 ◽  
Author(s):  
Steven Compernolle ◽  
Athina Argyrouli ◽  
Ronny Lutz ◽  
Maarten Sneep ◽  
Jean-Christopher Lambert ◽  
...  

<p>Space-born atmospheric composition measurements, like those from Sentinel-5p TROPOMI, are strongly affected by the presence of clouds. Dedicated cloud data products, typically retrieved with the same sensor, are therefore an important tool for the provider of atmospheric trace gas retrievals. Cloud products are used for filtering and modification of the modelled radiative transfer.</p><p>In this work, we assess the quality of the cloud data derived from Copernicus Sentinel-5 Precursor TROPOMI radiance measurements. Three cloud products are considered: (i) L2_CLOUD OCRA/ROCINN CAL (Optical Cloud Recognition Algorithm/Retrieval of Cloud Information using Neural Networks; Clouds-As-Layers), (ii) L2_CLOUD OCRA/ROCINN CRB (same; Clouds-as Reflecting Boundaries), and (iii) the S5p support product FRESCO-S (Fast Retrieval Scheme for Clouds from Oxygen absorption bands for Sentinel). These cloud products are used in the retrieval of several S5p trace gas products (e.g., ozone columns and profile, total and tropospheric nitrogen dioxide, sulfur dioxide, formaldehyde). The quality assessment of these cloud products is carried out within the framework of ESA’s Sentinel-5p Mission Performance Centre (MPC) with support from AO validation projects focusing on the respective atmospheric gases.</p><p>Cloud height data from the three S5p cloud products is compared to radar/lidar based cloud profile information from the ground-based networks CLOUDNET and ARM. The cloud height from S5p CLOUD CRB and S5p FRESCO are on average 0.6 km below the cloud mid-height of CLOUDNET measurements, and the cloud top height from S5p CLOUD CAL is on average 1 km below CLOUDNET’s cloud top height. However, the comparison is different for low and high clouds, with S5p CLOUD CAL cloud top height being only 0.3 km below CLOUDNET’s for low clouds.  The radiometric cloud fraction and cloud (top) height are compared to those of other satellite cloud products like Aura OMI O<sub>2</sub>-O<sub>2</sub>. While the latitudinal variation is often similar, offsets are encountered.</p><p>Recently, major S5p cloud product upgrades were released for S5p OCRA/ROCINN (July 2020) and for S5p FRESCO (December 2020), leading to a decrease of the ROCINN CRB cloud height and an increase of the FRESCO cloud height on average. Moreover, a major change in the ROCINN surface albedo treatment leads to a clear improvement of the comparison with CLOUDNET at the complicated sea/land/ice/snow site Ny-Alesund.</p><div></div>


2015 ◽  
Vol 15 (18) ◽  
pp. 10597-10618 ◽  
Author(s):  
M. J. M. Penning de Vries ◽  
S. Beirle ◽  
C. Hörmann ◽  
J. W. Kaiser ◽  
P. Stammes ◽  
...  

Abstract. Detecting the optical properties of aerosols using passive satellite-borne measurements alone is a difficult task due to the broadband effect of aerosols on the measured spectra and the influences of surface and cloud reflection. We present another approach to determine aerosol type, namely by studying the relationship of aerosol optical depth (AOD) with trace gas abundance, aerosol absorption, and mean aerosol size. Our new Global Aerosol Classification Algorithm, GACA, examines relationships between aerosol properties (AOD and extinction Ångström exponent from the Moderate Resolution Imaging Spectroradiometer (MODIS), UV Aerosol Index from the second Global Ozone Monitoring Experiment, GOME-2) and trace gas column densities (NO2, HCHO, SO2 from GOME-2, and CO from MOPITT, the Measurements of Pollution in the Troposphere instrument) on a monthly mean basis. First, aerosol types are separated based on size (Ångström exponent) and absorption (UV Aerosol Index), then the dominating sources are identified based on mean trace gas columns and their correlation with AOD. In this way, global maps of dominant aerosol type and main source type are constructed for each season and compared with maps of aerosol composition from the global MACC (Monitoring Atmospheric Composition and Climate) model. Although GACA cannot correctly characterize transported or mixed aerosols, GACA and MACC show good agreement regarding the global seasonal cycle, particularly for urban/industrial aerosols. The seasonal cycles of both aerosol type and source are also studied in more detail for selected 5° × 5° regions. Again, good agreement between GACA and MACC is found for all regions, but some systematic differences become apparent: the variability of aerosol composition (yearly and/or seasonal) is often not well captured by MACC, the amount of mineral dust outside of the dust belt appears to be overestimated, and the abundance of secondary organic aerosols is underestimated in comparison with GACA. Whereas the presented study is of exploratory nature, we show that the developed algorithm is well suited to evaluate climate and atmospheric composition models by including aerosol type and source obtained from measurements into the comparison, instead of focusing on a single parameter, e.g., AOD. The approach could be adapted to constrain the mix of aerosol types during the process of a combined data assimilation of aerosol and trace gas observations.


2020 ◽  
Vol 12 (8) ◽  
pp. 1250 ◽  
Author(s):  
Ana del Águila ◽  
Dmitry S. Efremenko ◽  
Víctor Molina García ◽  
Michael Yu. Kataev

Current atmospheric composition sensors provide a large amount of high spectral resolution data. The accurate processing of this data employs time-consuming line-by-line (LBL) radiative transfer models (RTMs). In this paper, we describe a method to accelerate hyperspectral radiative transfer models based on the clustering of the spectral radiances computed with a low-stream RTM and the regression analysis performed for the low-stream and multi-stream RTMs within each cluster. This approach, which we refer to as the Cluster Low-Streams Regression (CLSR) method, is applied for computing the radiance spectra in the O2 A-band at 760 nm and the CO2 band at 1610 nm for five atmospheric scenarios. The CLSR method is also compared with the principal component analysis (PCA)-based RTM, showing an improvement in terms of accuracy and computational performance over PCA-based RTMs. As low-stream models, the two-stream and the single-scattering RTMs are considered. We show that the error of this approach is modulated by the optical thickness of the atmosphere. Nevertheless, the CLSR method provides a performance enhancement of almost two orders of magnitude compared to the LBL model, while the error of the technique is below 0.1% for both bands.


2015 ◽  
Vol 15 (9) ◽  
pp. 13551-13605
Author(s):  
M. J. M. Penning de Vries ◽  
S. Beirle ◽  
C. Hörmann ◽  
J. W. Kaiser ◽  
P. Stammes ◽  
...  

Abstract. Detecting the optical properties of aerosols using passive satellite-borne measurements alone is a difficult task due to the broad-band effect of aerosols on the measured spectra and the influences of surface and cloud reflection. We present another approach to determine aerosol type, namely by studying the relationship of aerosol optical depth (AOD) with trace gas abundance, aerosol absorption, and mean aerosol size. Our new Global Aerosol Classification Algorithm, GACA, examines relationships between aerosol properties (AOD and extinction Ångström exponent from the Moderate Resolution Imaging Spectroradiometer (MODIS), UV Aerosol Index from the second Global Ozone Monitoring Experiment, GOME-2) and trace gas column densities (NO2, HCHO, SO2 from GOME-2, and CO from MOPITT, the Measurements of Pollution in the Troposphere instrument) on a monthly mean basis. First, aerosol types are separated based on size (Ångström exponent) and absorption (UV Aerosol Index), then the dominating sources are identified based on mean trace gas columns and their correlation with AOD. In this way, global maps of dominant aerosol type and main source type are constructed for each season and compared with maps of aerosol composition from the global MACC (Monitoring Atmospheric Composition and Climate) model. Although GACA cannot correctly characterize transported or mixed aerosols, GACA and MACC show good agreement regarding the global seasonal cycle, particularly for urban/industrial aerosols. The seasonal cycles of both aerosol type and source are also studied in more detail for selected 5° × 5° regions. Again, good agreement between GACA and MACC is found for all regions, but some systematic differences become apparent: the variability of aerosol composition (yearly and/or seasonal) is often not well captured by MACC, the amount of mineral dust outside of the dust belt appears to be overestimated, and the abundance of secondary organic aerosols is underestimated in comparison with GACA. Whereas the presented study is of exploratory nature, we show that the developed algorithm is well suited to evaluate climate and atmospheric composition models by including aerosol type and source obtained from measurements into the comparison, instead of focusing on a single parameter, e.g. AOD. The approach could be adapted to constrain the mix of aerosol types during the process of a combined data assimilation of aerosol and trace gas observations.


Sensors ◽  
2021 ◽  
Vol 21 (2) ◽  
pp. 345
Author(s):  
Pyung Kim ◽  
Younho Lee ◽  
Youn-Sik Hong ◽  
Taekyoung Kwon

To meet password selection criteria of a server, a user occasionally needs to provide multiple choices of password candidates to an on-line password meter, but such user-chosen candidates tend to be derived from the user’s previous passwords—the meter may have a high chance to acquire information about a user’s passwords employed for various purposes. A third party password metering service may worsen this threat. In this paper, we first explore a new on-line password meter concept that does not necessitate the exposure of user’s passwords for evaluating user-chosen password candidates in the server side. Our basic idea is straightforward; to adapt fully homomorphic encryption (FHE) schemes to build such a system but its performance achievement is greatly challenging. Optimization techniques are necessary for performance achievement in practice. We employ various performance enhancement techniques and implement the NIST (National Institute of Standards and Technology) metering method as seminal work in this field. Our experiment results demonstrate that the running time of the proposed meter is around 60 s in a conventional desktop server, expecting better performance in high-end hardware, with an FHE scheme in HElib library where parameters support at least 80-bit security. We believe the proposed method can be further explored and used for a password metering in case that password secrecy is very important—the user’s password candidates should not be exposed to the meter and also an internal mechanism of password metering should not be disclosed to users and any other third parties.


2021 ◽  
Vol 13 (3) ◽  
pp. 434
Author(s):  
Ana del Águila ◽  
Dmitry S. Efremenko

Fast radiative transfer models (RTMs) are required to process a great amount of satellite-based atmospheric composition data. Specifically designed acceleration techniques can be incorporated in RTMs to simulate the reflected radiances with a fine spectral resolution, avoiding time-consuming computations on a fine resolution grid. In particular, in the cluster low-streams regression (CLSR) method, the computations on a fine resolution grid are performed by using the fast two-stream RTM, and then the spectra are corrected by using regression models between the two-stream and multi-stream RTMs. The performance enhancement due to such a scheme can be of about two orders of magnitude. In this paper, we consider a modification of the CLSR method (which is referred to as the double CLSR method), in which the single-scattering approximation is used for the computations on a fine resolution grid, while the two-stream spectra are computed by using the regression model between the two-stream RTM and the single-scattering approximation. Once the two-stream spectra are known, the CLSR method is applied the second time to restore the multi-stream spectra. Through a numerical analysis, it is shown that the double CLSR method yields an acceleration factor of about three orders of magnitude as compared to the reference multi-stream fine-resolution computations. The error of such an approach is below 0.05%. In addition, it is analysed how the CLSR method can be adopted for efficient computations for atmospheric scenarios containing aerosols. In particular, it is discussed how the precomputed data for clear sky conditions can be reused for computing the aerosol spectra in the framework of the CLSR method. The simulations are performed for the Hartley–Huggins, O2 A-, water vapour and CO2 weak absorption bands and five aerosol models from the optical properties of aerosols and clouds (OPAC) database.


2021 ◽  
Author(s):  
Miriam Latsch ◽  
Andreas Richter ◽  
John P. Burrows ◽  
Thomas Wagner ◽  
Holger Sihler ◽  
...  

<p>The first European Sentinel satellite for monitoring the composition of the Earth’s atmosphere, the Sentinel 5 Precursor (S5p), carries the TROPOspheric Monitoring Instrument (TROPOMI) to map trace species of the global atmosphere at high spatial resolution. Retrievals of tropospheric trace gas columns from satellite measurements are strongly influenced by clouds. Thus, cloud retrieval algorithms were developed and implemented in the trace gas processing chain to consider this impact.</p><p>In this study, different cloud products available for NO<sub>2</sub> retrievals based on the TROPOMI level 1b data version 1 and an updated TROPOMI level 1b test data set of version 2 (Diagnostic Data Set 2B, DDS2B) are analyzed. The data sets include a) the TROPOMI level 2 OCRA/ROCINN (Optical Cloud Recognition Algorithm/Retrieval of Cloud Information using Neural Networks) cloud products CRB (cloud as reflecting boundaries) and CAL (clouds as layers), b) the FRESCO (Fast Retrieval Scheme for Clouds from Oxygen absorption bands) cloud product,  c) the cloud fraction from the NO<sub>2</sub> fitting window, d) the VIIRS (Visible Infrared Imaging Radiometer Suite) cloud product, and e) the MICRU (Mainz Iterative Cloud Retrieval Utilities) cloud fraction. The cloud products are compared with regard to cloud fraction, cloud height, cloud albedo/optical thickness, flagging and quality indicators in all 4 seasons. In particular, the differences of the cloud products under difficult situations such as snow or ice cover and sun glint are investigated.</p><p>We present results of a statistical analysis on a limited data set comparing cloud products from the current and the upcoming lv2 data versions and their approaches. The aim of this study is to better understand TROPOMI cloud products and their quantitative impacts on trace gas retrievals.</p>


2008 ◽  
Vol 1 (1) ◽  
pp. 103-125 ◽  
Author(s):  
T. von Clarmann ◽  
C. De Clercq ◽  
M. Ridolfi ◽  
M. Höpfner ◽  
J.-C. Lambert

Abstract. Limb remote sensing from space provides atmospheric composition measurements at high vertical resolution while the information is smeared in the horizontal domain. The horizontal components of two-dimensional (altitude and along-track coordinate) averaging kernels of a limb retrieval constrained to horizontal homogeneity can be used to estimate the horizontal resolution of limb retrievals. This is useful for comparisons of measured data with modeled data, to construct horizontal observation operators in data assimilation applications or when measurements of different horizontal resolution are intercompared. We present these averaging kernels for retrievals of temperature, H2O, O3, CH4, N2O, HNO3 and NO2 from MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) high-resolution limb emission spectra. The horizontal smearing of a MIPAS retrieval in terms of full width at half maximum of the rows of the horizontal averaging kernel matrix varies typically between about 200 and 350 km for most species, altitudes and atmospheric conditions. The range where 95% of the information originates from varies from about 260 to 440 km for these cases. This information spread is smaller than the MIPAS horizontal sampling, i.e. MIPAS data are horizontally undersampled, and the effective horizontal resolution is driven by the sampling rather than the smearing. The point where the majority of the information originates from is displaced from the tangent point towards the satellite by typically less than 10 km for trace gas profiles and about 50 to 100 km for temperature, with a few exceptions for uppermost altitudes. The geolocation of a MIPAS profile is defined as the tangent point of the middle line of sight in a MIPAS limb scan. The majority of the information displacement with respect to this nominal geolocation of the measurement is caused by the satellite movement and the geometrical displacement of the actual tangent point as a function of the elevation angle. In none of the cases investigated, propagation of the horizontal smoothing on the vertical profile shape has been observed.


2018 ◽  
Author(s):  
Jean-François Müller ◽  
Trissevgeni Stavrakou ◽  
Jozef Peeters

Abstract. A new chemical mechanism for the oxidation of biogenic volatile organic compounds (BVOCs) is presented and implemented in the Model of Atmospheric composition at Global and Regional scales using Inversion Techniques for Trace gas Emissions (MAGRITTE v1.0). With a total of 99 organic species and over 240 gas-phase reactions, 67 photodissociations and 7 heterogeneous reactions, the mechanism treats the chemical degradation of isoprene – its main focus – as well as acetaldehyde, acetone, methylbutenol and the family of monoterpenes. Regarding isoprene, the mechanism incorporates a state-of-the-art representation of its oxidation scheme accounting for all major advances put forward in recent theoretical and laboratory studies. The model and its chemical mechanism are evaluated against the suite of chemical measurements from the SEAC4RS (Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys) airborne campaign, demonstrating a good overall agreement for major isoprene oxidation products, although the aerosol hydrolysis of tertiary and non-tertiary nitrates remain poorly constrained. The comparisons for methylnitrate indicate a very low nitrate yield (


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