scholarly journals Aerosol nucleation and its role for clouds and Earth's radiative forcing in the aerosol-climate model ECHAM5-HAM

2010 ◽  
Vol 10 (22) ◽  
pp. 10733-10752 ◽  
Author(s):  
J. Kazil ◽  
P. Stier ◽  
K. Zhang ◽  
J. Quaas ◽  
S. Kinne ◽  
...  

Abstract. Nucleation from the gas phase is an important source of aerosol particles in the Earth's atmosphere, contributing to the number of cloud condensation nuclei, which form cloud droplets. We have implemented in the aerosol-climate model ECHAM5-HAM a new scheme for neutral and charged nucleation of sulfuric acid and water based on laboratory data, and nucleation of an organic compound and sulfuric acid using a parametrization of cluster activation based on field measurements. We give details of the implementation, compare results with observations, and investigate the role of the individual aerosol nucleation mechanisms for clouds and the Earth's radiative forcing. The results of our simulations are most consistent with observations when neutral and charged nucleation of sulfuric acid proceed throughout the troposphere and nucleation due to cluster activation is limited to the forested boundary layer. The globally averaged annual mean contributions of the individual nucleation processes to total absorbed solar short-wave radiation via the direct, semi-direct, indirect cloud-albedo and cloud-lifetime effects in our simulations are −1.15 W/m2 for charged H2SO4/H2O nucleation, −0.235 W/m2 for cluster activation, and −0.05 W/m2 for neutral H2SO4/H2O nucleation. The overall effect of nucleation is −2.55 W/m2, which exceeds the sum of the individual terms due to feedbacks and interactions in the model. Aerosol nucleation contributes over the oceans with −2.18 W/m2 to total absorbed solar short-wave radiation, compared to −0.37 W/m2 over land. We explain the higher effect of aerosol nucleation on Earth's radiative forcing over the oceans with the larger area covered by ocean clouds, due to the larger contrast in albedo between clouds and the ocean surface compared to continents, and the larger susceptibility of pristine clouds owing to the saturation of effects. The large effect of charged nucleation in our simulations is not in contradiction with small effects seen in local measurements: over southern Finland, where cluster activation proceeds efficiently, we find that charged nucleation of sulfuric acid and water contributes on average less than 10% to ultrafine aerosol concentrations, in good agreement with observations.

2010 ◽  
Vol 10 (5) ◽  
pp. 12261-12308 ◽  
Author(s):  
J. Kazil ◽  
P. Stier ◽  
K. Zhang ◽  
J. Quaas ◽  
S. Kinne ◽  
...  

Abstract. Nucleation from the gas phase is an important source of aerosol particles in the Earth's atmosphere, contributing to the number of cloud condensation nuclei, which form cloud droplets. We have implemented in the aerosol-climate model ECHAM5-HAM a new scheme for neutral and charged nucleation of sulfuric acid and water based on laboratory data, and nucleation of an organic compound and sulfuric acid using a parametrization of cluster activation based on field measurements. We give details of the implementation, compare results with observations, and investigate the role of the individual aerosol nucleation mechanisms for clouds and the Earth's radiative budget. The results of our simulations are most consistent with observations when neutral and charged nucleation of sulfuric acid proceed throughout the troposphere and nucleation due to cluster activation is limited to the forested boundary layer. The globally averaged annual mean contributions of the individual nucleation processes to total absorbed solar short-wave radiation via the direct, semi-direct, indirect cloud-albedo and cloud-lifetime effects in our simulations are −1.15 W/m2 for charged H2SO4/H2O nucleation, −0.235 W/m2 for cluster activation, and −0.05 W/m2 for neutral H2SO4/H2O nucleation. The overall effect of nucleation is −2.55 W/m2, which exceeds the sum of the individual terms due to feedbacks and interactions in the model. Aerosol nucleation contributes over the oceans with −2.18 W/m2 to total absorbed solar short-wave radiation, compared to −0.37 W/m2 over land. We explain the higher effect of aerosol nucleation on Earth's radiative budget over the oceans with the larger area covered by ocean clouds, due to the larger contrast in albedo between clouds and the ocean surface compared to continents, and the larger susceptibility of pristine clouds owing to the saturation of effects. The large effect of charged nucleation in our simulations is not in contradiction with small effects seen in local measurements: over southern Finland, where cluster activation proceeds efficiently, we find that charged nucleation of sulfuric acid and water contributes on average less than 10% to ultrafine aerosol concentrations, in good agreement with observations.


2015 ◽  
Vol 2015 ◽  
pp. 1-15 ◽  
Author(s):  
Britta Jänicke ◽  
Fred Meier ◽  
Marie-Therese Hoelscher ◽  
Dieter Scherer

The evaluation of the effectiveness of countermeasures for a reduction of urban heat stress, such as façade greening, is challenging due to lacking transferability of results from one location to another. Furthermore, complex variables such as the mean radiant temperature(Tmrt)are necessary to assess outdoor human bioclimate. We observedTmrtin front of a building façade in Berlin, Germany, which is half-greened while the other part is bare.Tmrtwas reduced (mean 2 K) in front of the greened compared to the bare façade. To overcome observational shortcomings, we applied the microscale models ENVI-met, RayMan, and SOLWEIG. We evaluated these models based on observations. Our results show thatTmrt(MD = −1.93 K) and downward short-wave radiation (MD = 14.39 W/m2) were sufficiently simulated in contrast to upward short-wave and long-wave radiation. Finally, we compare the simulated reduction ofTmrtwith the observed one in front of the façade greening, showing that the models were not able to simulate the effects of façade greening with the applied settings. Our results reveal that façade greening contributes only slightly to a reduction of heat stress in front of building façades.


1971 ◽  
Vol 10 (58) ◽  
pp. 101-104 ◽  
Author(s):  
M.P. Langleben

AbstractTwo Kipp hemispherical radiometers mounted back to back and suspended by an 18 m cable from a helicopter flying at an altitude of about 90 m were used to make measurements of incident and reflected short-wave radiation. The helicopter was brought to a hovering position at the instant of measurement to ensure that the radiometers were in the proper attitude and a photograph of the ice cover was taken at the same time. The observations were made in 1969 during 16 flights out of Tuktoyaktuk, Northwest Territories (lat. 69° 26’N., long. 133° 02’W.) over the fast ice extending 80 km north of Tuktoyaktuk. Values of albedo of the ice cover were found to decrease during the melting period according to the equation A = 0.59 —0.32P where P is the degree of puddling of the surface.


1974 ◽  
Vol 20 (4) ◽  
pp. 434-438
Author(s):  
E. M. Golubev ◽  
N. N. Ogurtsova ◽  
I. V. Podmoshenskii ◽  
P. N. Rogovtsev

2005 ◽  
Vol 36 (4-5) ◽  
pp. 381-396 ◽  
Author(s):  
A. Rutgersson ◽  
A. Omstedt ◽  
Y. Chen

In this paper, which reports on part of the BALTEX project, various components of the heat balance over the Baltic Sea are calculated using a number of gridded meteorological databases. It is the heat exchange between the Baltic Sea surface and the atmosphere that is of interest. The databases have different origins, comprising synoptic data, data re-analysed with a 3D assimilation system, an ocean model forced with gridded synoptic data, ship data and satellite data. We compared the databases and found that the greatest variation between them is in the long- and short-wave radiation values. However, considerable upward long-wave radiation is followed by considerable downward short-wave radiation, so the total radiation component is partly compensated for in the total budget. The variation in the total heat transport in the databases therefore appears smaller (1.5±3 W m−2) as the average and one standard deviation. The turbulent heat fluxes estimated from satellite data have very low values; this can largely be explained by the method of calculating air temperature, which also produces an unrealistic stratification over the Baltic Sea. The ERA40 data was compared with measured values: there, we found a certain land influence even in the centre of the Baltic proper. The indicated turbulent heat fluxes were too large, mainly in the fall and winter, and the sensible heat flux was too large in a downward direction in spring and summer.


2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Henrik Svensmark ◽  
Jacob Svensmark ◽  
Martin Bødker Enghoff ◽  
Nir J. Shaviv

AbstractAtmospheric ionization produced by cosmic rays has been suspected to influence aerosols and clouds, but its actual importance has been questioned. If changes in atmospheric ionization have a substantial impact on clouds, one would expect to observe significant responses in Earth’s energy budget. Here it is shown that the average of the five strongest week-long decreases in atmospheric ionization coincides with changes in the average net radiative balance of 1.7 W/m$$^2$$ 2 (median value: 1.2 W/m$$^2$$ 2 ) using CERES satellite observations. Simultaneous satellite observations of clouds show that these variations are mainly caused by changes in the short-wave radiation of low liquid clouds along with small changes in the long-wave radiation, and are almost exclusively located over the pristine areas of the oceans. These observed radiation and cloud changes are consistent with a link in which atmospheric ionization modulates aerosol's formation and growth, which survive to cloud condensation nuclei and ultimately affect cloud formation and thereby temporarily the radiative balance of Earth.


2021 ◽  
Author(s):  
Georges Djoumna ◽  
Sebastian H. Mernild ◽  
David Holland

<p>The surface radiation budget is an essential component of the total energy exchange between the atmosphere and the Earth’s surface. Measurements of radiative fluxes near/on ice surfaces are sparse in the polar regions, including on the Greenland Ice Sheet (GrIS), and the effects of cloud on radiative fluxes are still poorly studied. In this work, we assess the impacts of cloud on radiative fluxes using two metrics: the longwave-equivalent cloudiness, derived from long-wave radiation measurements, and the cloud transmittance factor, obtained from short-wave radiation. The metrics are applied to radiation data from two automatic weather stations located over the bare ground near the ice front of Helheim (HG) and Jakobshavn Isbræ (JI) on the GrIS. Comparisons of meteorological parameters, surface radiation fluxes, and cloud metrics show significant differences between the two sites. The cloud transmittance factor is higher at HG than at JI, and the incoming short-wave radiation in the summer at HG is 50.0 W m−2 larger than at JI. Cloud metrics derived at the two sites reveal   a high dependency on the wind direction. The total cloud radiative effect (CREnet) generally increases during melt season at the two stations due to long-wave CRE enhancement by cloud fraction.  CREnet decreases from May to June and increases afterward, due to the strengthened short-wave CRE. The annually averaged CREnet were 3.0 ± 7.4 W m-2 and 1.9 ± 15.1 W m−2 at JI and HG.  CREnet estimated from AWS indicates that clouds cool the JI and HG during melt season at different rates.</p>


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