scholarly journals Combined effects of surface conditions, boundary layer dynamics and chemistry on diurnal SOA evolution

2012 ◽  
Vol 12 (15) ◽  
pp. 6827-6843 ◽  
Author(s):  
R. H. H. Janssen ◽  
J. Vilà-Guerau de Arellano ◽  
L. N. Ganzeveld ◽  
P. Kabat ◽  
J. L. Jimenez ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Atmospheric Boundary Layer ◽  
Land Surface ◽  
Large Scale ◽  
Organic Aerosol ◽  
Layer Growth ◽  
Combined Effects ◽  
Free Troposphere ◽  
Surface Conditions ◽  
Boundary Layer Dynamics

Abstract. We study the combined effects of land surface conditions, atmospheric boundary layer dynamics and chemistry on the diurnal evolution of biogenic secondary organic aerosol in the atmospheric boundary layer, using a model that contains the essentials of all these components. First, we evaluate the model for a case study in Hyytiälä, Finland, and find that it is able to satisfactorily reproduce the observed dynamics and gas-phase chemistry. We show that the exchange of organic aerosol between the free troposphere and the boundary layer (entrainment) must be taken into account in order to explain the observed diurnal cycle in organic aerosol (OA) concentration. An examination of the budgets of organic aerosol and terpene concentrations show that the former is dominated by entrainment, while the latter is mainly driven by emission and chemical transformation. We systematically investigate the role of the land surface, which governs both the surface energy balance partitioning and terpene emissions, and the large-scale atmospheric process of vertical subsidence. Entrainment is especially important for the dilution of organic aerosol concentrations under conditions of dry soils and low terpene emissions. Subsidence suppresses boundary layer growth while enhancing entrainment. Therefore, it influences the relationship between organic aerosol and terpene concentrations. Our findings indicate that the diurnal evolution of secondary organic aerosols (SOA) in the boundary layer is the result of coupled effects of the land surface, dynamics of the atmospheric boundary layer, chemistry, and free troposphere conditions. This has potentially some consequences for the design of both field campaigns and large-scale modeling studies.

scholarly journals Combined effects of surface conditions, boundary layer dynamics and chemistry on diurnal SOA-evolution

2012 ◽  
Vol 12 (4) ◽  
pp. 9331-9375 ◽  
Author(s):  
R. H. H. Janssen ◽  
J. Vilà-Guerau de Arellano ◽  
L. N. Ganzeveld ◽  
P. Kabat ◽  
J. L. Jimenez ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Atmospheric Boundary Layer ◽  
Land Surface ◽  
Large Scale ◽  
Organic Aerosol ◽  
Layer Growth ◽  
Combined Effects ◽  
Free Troposphere ◽  
Surface Conditions ◽  
Boundary Layer Dynamics

Abstract. We study the combined effects of land surface conditions, atmospheric boundary layer dynamics and chemistry on the diurnal evolution of biogenic secondary organic aerosol in the atmospheric boundary layer, using a model that contains the essentials of all these components. First, we evaluate the model for a case study in Hyytiälä, Finland, and find that it is able to well reproduce the observed dynamics and gas-phase chemistry. We show that the exchange of organic aerosol between the free troposphere and the boundary layer (entrainment) must be taken into account in order to explain the observed diurnal cycle in organic aerosol (OA) concentration. An examination of the budgets of organic aerosol and terpene concentration shows that the former is dominated by entrainment, while the latter is mainly driven by emission and chemical transformation. We systematically examine the role of the land surface, which governs both the surface energy balance partitioning and terpene-emissions, and the large-scale atmospheric process of vertical subsidence. Entrainment is especially important for the dilution of organic aerosol concentrations under conditions of dry soils and low terpene-emissions. Subsidence suppresses boundary layer growth while enhancing entrainment. Therefore it influences the relationship between organic aerosol and terpene-concentrations. Our findings indicate that the diurnal evolution of SOA in the boundary layer is the result of coupled effects of the land surface, dynamics of the atmospheric boundary layer, chemistry, and free troposphere conditions. This has potentially some consequences for the design of both field campaigns and large-scale modeling studies.

scholarly journals Surface heterogeneity impacts on boundary layer dynamics via energy balance partitioning

2010 ◽  
Vol 10 (7) ◽  
pp. 17815-17851 ◽  
Author(s):  
N. A. Brunsell ◽  
D. B. Mechem ◽  
M. C. Anderson
Keyword(s):  
Boundary Layer ◽  
Heat Flux ◽  
Latent Heat ◽  
Latent Heat Flux ◽  
Land Surface ◽  
Surface Heterogeneity ◽  
Length Scales ◽  
Surface Conditions ◽  
Boundary Layer Dynamics

Abstract. The role of land-atmosphere interactions under heterogeneous surface conditions is investigated in order to identify mechanisms responsible for altering surface heat and moisture fluxes. Twelve coupled land surface – large eddy simulation scenarios with four different length scales of surface variability under three different horizontal wind speeds are used in the analysis. The base case uses Landsat ETM imagery over the Cloud Land Surface Interaction Campaign (CLASIC) field site for 3 June 2007. Using wavelets, the surface fields are band-pass filtered in order to maintain the spatial mean and variances to length scales of 200 m, 1600 m, and 12.8 km as lower boundary conditions to the model. The simulations exhibit little variation in net radiation. Rather, a change in the partitioning of the surface energy between sensible and latent heat flux is responsible for differences in boundary layer dynamics. The sensible heat flux is dominant for intermediate surface length scales. For smaller and larger scales of surface heterogeneity, which can be viewed as being more homogeneous, the latent heat flux becomes increasingly important. The results reflect a general decrease of the Bowen ratio as the surface conditions transition from heterogeneous to homogeneous. Air temperature is less sensitive to surface heterogeneity than water vapor, which implies that the role of surface heterogeneity in modifying the local temperature gradients in order to maximize convective heat fluxes. More homogeneous surface conditions, on the other hand, tend to maximize latent heat flux. Scalar vertical profiles respond predictably to the partitioning of surface energy. Fourier spectra of the vertical wind speed, air temperature and specific humidity (w, T and q) and associated cospectra (w'T', w'q' and T'q'), however, are insensitive to the length scale of surface heterogeneity, but the near surface spectra are sensitive to the mean wind speed.

scholarly journals The anatomy of large-scale motion in atmospheric boundary layers

2018 ◽  
Vol 858 ◽  
pp. 1-4 ◽  
Author(s):  
G. G. Katul
Keyword(s):  
Boundary Layer ◽  
Atmospheric Boundary Layer ◽  
Turbulent Flows ◽  
Land Surface ◽  
Large Scale ◽  
Cloud Condensation Nuclei ◽  
Surface Heating ◽  
Flow State ◽  
Scale Motion ◽  
Large Eddies

The atmospheric boundary layer is the level of the atmosphere where all human activities occur. It is a layer characterized by its turbulent flow state, meaning that the velocity, temperature and scalar concentrations fluctuate over scales that range from less than a millimetre to several kilometres. It is those fluctuations that make dispersion of pollutants and transport of heat, momentum as well as scalars such as carbon dioxide or cloud-condensation nuclei efficient. It is also the layer where a ‘hand-shake’ occurs between activities on the land surface and the climate system, primarily due to the action of large energetic swirling motions or eddies. The atmospheric boundary layer experiences dramatic transitions depending on whether the underlying surface is being heated or cooled. The existing paradigm describing the size and energetics of large-scale and very large-scale eddies in turbulent flows has been shaped by decades of experiments and simulations on smooth pipes and channels with no surface heating or cooling. The emerging picture, initiated by A. A. Townsend in 1951, is that large- and very large-scale motions appear to be approximated by a collection of hairpin-shaped vortices whose population density scales inversely with distance from the boundary. How does surface heating, quintessential to the atmospheric boundary layer, alter this canonical picture? What are the implications of such a buoyancy force on the geometry and energy distribution across velocity components in those large eddies? How do these large eddies modulate small eddies near the ground? Answering these questions and tracking their consequences to existing theories used today to describe the flow statistics in the atmospheric boundary layer are addressed in the work of Salesky & Anderson (J. Fluid Mech., vol. 856, 2018, pp. 135–168). The findings are both provocative and surprisingly simple.

scholarly journals South East Pacific atmospheric composition and variability sampled along 20° S during VOCALS-REx

2011 ◽  
Vol 11 (11) ◽  
pp. 5237-5262 ◽  
Author(s):  
G. Allen ◽  
H. Coe ◽  
A. Clarke ◽  
C. Bretherton ◽  
R. Wood ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Land Surface ◽  
Large Scale ◽  
Trajectory Analysis ◽  
Model Simulation ◽  
Atmospheric Composition ◽  
Back Trajectory ◽  
Free Troposphere ◽  
Back Trajectory Analysis ◽  
East Pacific

Abstract. The VAMOS Ocean-Cloud-Atmosphere-Land Regional Experiment (VOCALS-REx) was conducted from 15 October to 15 November 2008 in the South East Pacific (SEP) region to investigate interactions between land, sea and atmosphere in this unique tropical eastern ocean environment and to improve the skill of global and regional models in representing the region. This study synthesises selected aircraft, ship and surface site observations from VOCALS-REx to statistically summarise and characterise the atmospheric composition and variability of the Marine Boundary Layer (MBL) and Free Troposphere (FT) along the 20° S parallel between 70° W and 85° W. Significant zonal gradients in mean MBL sub-micron aerosol particle size and composition, carbon monoxide, sulphur dioxide and ozone were seen over the campaign, with a generally more variable and polluted coastal environment and a less variable, more pristine remote maritime regime. Gradients in aerosol and trace gas concentrations were observed to be associated with strong gradients in cloud droplet number. The FT was often more polluted in terms of trace gases than the MBL in the mean; however increased variability in the FT composition suggests an episodic nature to elevated concentrations. This is consistent with a complex vertical interleaving of airmasses with diverse sources and hence pollutant concentrations as seen by generalised back trajectory analysis, which suggests contributions from both local and long-range sources. Furthermore, back trajectory analysis demonstrates that the observed zonal gradients both in the boundary layer and the free troposphere are characteristic of marked changes in airmass history with distance offshore – coastal boundary layer airmasses having been in recent contact with the local land surface and remote maritime airmasses having resided over ocean for in excess of ten days. Boundary layer composition to the east of 75° W was observed to be dominated by coastal emissions from sources to the west of the Andes, with evidence for diurnal pumping of the Andean boundary layer above the height of the marine capping inversion. Analysis of intra-campaign variability in atmospheric composition was not found to be significantly correlated with observed low-frequency variability in the large scale flow pattern; campaign-average interquartile ranges of CO, SO2 and O3 concentrations at all longitudes were observed to dominate over much smaller differences in median concentrations calculated between periods of different flow regimes. The campaign climatology presented here aims to provide a valuable dataset to inform model simulation and future process studies, particularly in the context of aerosol-cloud interaction and further evaluation of dynamical processes in the SEP region for conditions analogous to those during VOCALS-REx. To this end, our results are discussed in terms of coastal, transitional and remote spatial regimes in the MBL and FT and a gridded dataset are provided as a resource.

scholarly journals The HD(CP)<sup>2</sup> Observational Prototype Experiment (HOPE) – an overview

2017 ◽  
Vol 17 (7) ◽  
pp. 4887-4914 ◽  
Author(s):  
Andreas Macke ◽  
Patric Seifert ◽  
Holger Baars ◽  
Christian Barthlott ◽  
Christoph Beekmans ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Atmospheric Boundary Layer ◽  
Water Vapour ◽  
Land Surface ◽  
Critical Evaluation ◽  
Boundary Layer Height ◽  
Microphysical Properties ◽  
Boundary Layer Dynamics ◽  
Macrophysical Properties ◽  
Microwave Radiometers

Abstract. The HD(CP)2 Observational Prototype Experiment (HOPE) was performed as a major 2-month field experiment in Jülich, Germany, in April and May 2013, followed by a smaller campaign in Melpitz, Germany, in September 2013. HOPE has been designed to provide an observational dataset for a critical evaluation of the new German community atmospheric icosahedral non-hydrostatic (ICON) model at the scale of the model simulations and further to provide information on land-surface–atmospheric boundary layer exchange, cloud and precipitation processes, as well as sub-grid variability and microphysical properties that are subject to parameterizations. HOPE focuses on the onset of clouds and precipitation in the convective atmospheric boundary layer. This paper summarizes the instrument set-ups, the intensive observation periods, and example results from both campaigns. HOPE-Jülich instrumentation included a radio sounding station, 4 Doppler lidars, 4 Raman lidars (3 of them provide temperature, 3 of them water vapour, and all of them particle backscatter data), 1 water vapour differential absorption lidar, 3 cloud radars, 5 microwave radiometers, 3 rain radars, 6 sky imagers, 99 pyranometers, and 5 sun photometers operated at different sites, some of them in synergy. The HOPE-Melpitz campaign combined ground-based remote sensing of aerosols and clouds with helicopter- and balloon-based in situ observations in the atmospheric column and at the surface. HOPE provided an unprecedented collection of atmospheric dynamical, thermodynamical, and micro- and macrophysical properties of aerosols, clouds, and precipitation with high spatial and temporal resolution within a cube of approximately 10  ×  10  ×  10 km3. HOPE data will significantly contribute to our understanding of boundary layer dynamics and the formation of clouds and precipitation. The datasets have been made available through a dedicated data portal. First applications of HOPE data for model evaluation have shown a general agreement between observed and modelled boundary layer height, turbulence characteristics, and cloud coverage, but they also point to significant differences that deserve further investigations from both the observational and the modelling perspective.

scholarly journals The HD(CP)2 Observational Prototype Experiment HOPE – An Overview

2016 ◽  
Author(s):  
Andreas Macke ◽  
Patric Seifert ◽  
Holger Baars ◽  
Christoph Beekmans ◽  
Andreas Behrendt ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Atmospheric Boundary Layer ◽  
Land Surface ◽  
Critical Evaluation ◽  
Microphysical Properties ◽  
Intensive Observation ◽  
Boundary Layer Dynamics ◽  
Macrophysical Properties ◽  
Microwave Radiometers

Abstract. The "HD(CP)2 Observational Prototype Experiment" (HOPE) was executed as a major 2-month field experiment in Jülich, Germany, performed in April and May 2013, followed by a smaller campaign in Melpitz, Germany in September 2013. HOPE has been designed to provide a critical evaluation of the new German community atmospheric Icosahedral non-hydrostatic (ICON) model at the scale of the model simulations and further to provide information on land-surface-atmospheric boundary layer exchange, cloud and precipitation processes as well as on sub-grid variability and microphysical properties that are subject to parameterizations. HOPE focuses on the onset of clouds and precipitation in the convective atmospheric boundary layer. The paper summarizes the instrument set-ups, the intensive observation periods as well as example results from both campaigns. HOPE-Jülich instrumentation included a radio sounding station, 4 Doppler lidars, 4 Raman lidars (3, 3, and 4 of these provide temperature, water vapor, and particle backscatter data, respectively), 1 water vapour differential absorption lidar, 3 cloud radars, 5 microwave radiometers, 3 rain radars, 6 sky imagers, 99 pyranometers, and 5 Sun photometers operated in synergy at different supersites. The HOPE-Melpitz campaign combined ground-based remote sensing of aerosols and clouds with helicopter- and balloon-based in-situ observations in the atmospheric column and at the surface. HOPE provided an unprecedented collection of atmospheric dynamical, thermodynamical, and micro- and macrophysical properties of aerosols, clouds and precipitation with high spatial and temporal resolution within a cube of approximately 10 × 10 × 10 km3. HOPE data will significantly contribute to our understanding of boundary layer dynamics and the formation of clouds and precipitation. The datasets are made available through a dedicated data portal.

scholarly journals Wind speed response of marine non-precipitating stratocumulus clouds over a diurnal cycle in cloud-system resolving simulations

2016 ◽  
Vol 16 (9) ◽  
pp. 5811-5839 ◽  
Author(s):  
Jan Kazil ◽  
Graham Feingold ◽  
Takanobu Yamaguchi
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Large Scale ◽  
Layer Growth ◽  
Radiative Properties ◽  
Cloud Base ◽  
Latent Heat Release ◽  
Marine Stratocumulus ◽  
Stratocumulus Clouds ◽  
Boundary Layer Growth

Abstract. Observed and projected trends in large-scale wind speed over the oceans prompt the question: how do marine stratocumulus clouds and their radiative properties respond to changes in large-scale wind speed? Wind speed drives the surface fluxes of sensible heat, moisture, and momentum and thereby acts on cloud liquid water path (LWP) and cloud radiative properties. We present an investigation of the dynamical response of non-precipitating, overcast marine stratocumulus clouds to different wind speeds over the course of a diurnal cycle, all else equal. In cloud-system resolving simulations, we find that higher wind speed leads to faster boundary layer growth and stronger entrainment. The dynamical driver is enhanced buoyant production of turbulence kinetic energy (TKE) from latent heat release in cloud updrafts. LWP is enhanced during the night and in the morning at higher wind speed, and more strongly suppressed later in the day. Wind speed hence accentuates the diurnal LWP cycle by expanding the morning–afternoon contrast. The higher LWP at higher wind speed does not, however, enhance cloud top cooling because in clouds with LWP ⪆ 50 g m−2, longwave emissions are insensitive to LWP. This leads to the general conclusion that in sufficiently thick stratocumulus clouds, additional boundary layer growth and entrainment due to a boundary layer moistening arises by stronger production of TKE from latent heat release in cloud updrafts, rather than from enhanced longwave cooling. We find that large-scale wind modulates boundary layer decoupling. At nighttime and at low wind speed during daytime, it enhances decoupling in part by faster boundary layer growth and stronger entrainment and in part because shear from large-scale wind in the sub-cloud layer hinders vertical moisture transport between the surface and cloud base. With increasing wind speed, however, in decoupled daytime conditions, shear-driven circulation due to large-scale wind takes over from buoyancy-driven circulation in transporting moisture from the surface to cloud base and thereby reduces decoupling and helps maintain LWP. The total (shortwave + longwave) cloud radiative effect (CRE) responds to changes in LWP and cloud fraction, and higher wind speed translates to a stronger diurnally averaged total CRE. However, the sensitivity of the diurnally averaged total CRE to wind speed decreases with increasing wind speed.

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