scholarly journals Advances in understanding mineral dust and boundary layer processes over the Sahara from Fennec aircraft observations

2015 ◽  
Vol 15 (14) ◽  
pp. 8479-8520 ◽  
Author(s):  
C. L. Ryder ◽  
J. B. McQuaid ◽  
C. Flamant ◽  
P. D. Rosenberg ◽  
R. Washington ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Mineral Dust ◽  
Cloud Condensation Nuclei ◽  
Deep Convection ◽  
Dust Particles ◽  
Cold Pool ◽  
Boundary Layer Processes ◽  
Aircraft Observations ◽  
Scientific Results ◽  
The Uk

Abstract. The Fennec climate programme aims to improve understanding of the Saharan climate system through a synergy of observations and modelling. We present a description of the Fennec airborne observations during 2011 and 2012 over the remote Sahara (Mauritania and Mali) and the advances in the understanding of mineral dust and boundary layer processes they have provided. Aircraft instrumentation aboard the UK FAAM BAe146 and French SAFIRE (Service des Avions Français Instrumentés pour la Recherche en Environnement) Falcon 20 is described, with specific focus on instrumentation specially developed for and relevant to Saharan meteorology and dust. Flight locations, aims and associated meteorology are described. Examples and applications of aircraft measurements from the Fennec flights are presented, highlighting new scientific results delivered using a synergy of different instruments and aircraft. These include (1) the first airborne measurement of dust particles sizes of up to 300 microns and associated dust fluxes in the Saharan atmospheric boundary layer (SABL), (2) dust uplift from the breakdown of the nocturnal low-level jet before becoming visible in SEVIRI (Spinning Enhanced Visible Infra-Red Imager) satellite imagery, (3) vertical profiles of the unique vertical structure of turbulent fluxes in the SABL, (4) in situ observations of processes in SABL clouds showing dust acting as cloud condensation nuclei (CCN) and ice nuclei (IN) at −15 °C, (5) dual-aircraft observations of the SABL dynamics, thermodynamics and composition in the Saharan heat low region (SHL), (6) airborne observations of a dust storm associated with a cold pool (haboob) issued from deep convection over the Atlas Mountains, (7) the first airborne chemical composition measurements of dust in the SHL region with differing composition, sources (determined using Lagrangian backward trajectory calculations) and absorption properties between 2011 and 2012, (8) coincident ozone and dust surface area measurements suggest coarser particles provide a route for ozone depletion, (9) discrepancies between airborne coarse-mode size distributions and AERONET (AERosol Robotic NETwork) sunphotometer retrievals under light dust loadings. These results provide insights into boundary layer and dust processes in the SHL region – a region of substantial global climatic importance.

scholarly journals Advances in understanding mineral dust and boundary layer processes over the Sahara from Fennec aircraft observations

2015 ◽  
Vol 15 (1) ◽  
pp. 199-290 ◽  
Author(s):  
C. L. Ryder ◽  
J. B. McQuaid ◽  
C. Flamant ◽  
R. Washington ◽  
H. E. Brindley ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Mineral Dust ◽  
Deep Convection ◽  
Dust Particles ◽  
Cold Pool ◽  
Boundary Layer Processes ◽  
Airborne Measurement ◽  
Aircraft Observations ◽  
Scientific Results ◽  
The Uk

Abstract. The Fennec climate program aims to improve understanding of the Saharan climate system through a synergy of observations and modelling. We present a description of the Fennec airborne observations during 2011 and 2012 over the remote Sahara (Mauritania and Mali) and the advances in the understanding of mineral dust and boundary layer processes they have provided. Aircraft instrumentation aboard the UK FAAM BAe146 and French SAFIRE Falcon 20 is described, with specific focus on instrumentation specially developed and relevant to Saharan meteorology and dust. Flight locations, aims and associated meteorology are described. Examples and applications of aircraft measurements from the Fennec flights are presented, highlighting new scientific results delivered using a synergy of different instruments and aircraft. These include: (1) the first airborne measurement of dust particles sized up to 300 microns and associated dust fluxes in the Saharan atmospheric boundary layer (SABL), (2) dust uplift from the breakdown of the nocturnal low-level jet before becoming visible in SEVIRI satellite imagery, (3) vertical profiles of the unique vertical structure of turbulent fluxes in the SABL, (4) in-situ observations of processes in SABL clouds showing dust acting as CCN and IN at −15 °C, (5) dual-aircraft observations of the SABL dynamics, thermodynamics and composition in the Saharan heat low region (SHL), (6) airborne observations of a dust storm associated with a cold-pool (haboob) issued from deep convection over the Atlas, (7) the first airborne chemical composition measurements of dust in the SHL region with differing composition, sources (determined using Lagrangian backward trajectory calculations) and absorption properties between 2011 and 2012, (8) coincident ozone and dust surface area measurements suggest coarser particles provide a route for ozone depletion, (9) discrepancies between airborne coarse mode size distributions and AERONET sunphotometer retrievals under light dust loadings. These results provide insights into boundary layer and dust processes in the SHL region – a region of substantial global climatic importance.

scholarly journals Resolution Dependence of Initiation and Upscale Growth of Deep Convection in Convection-Allowing Forecasts of the 31 May–1 June 2013 Supercell and MCS

2015 ◽  
Vol 143 (11) ◽  
pp. 4331-4354 ◽  
Author(s):  
Russ S. Schumacher
Keyword(s):  
Boundary Layer ◽  
Numerical Models ◽  
Deep Convection ◽  
Squall Line ◽  
Cold Pool ◽  
Model Resolution ◽  
Grid Spacing ◽  
Boundary Layer Processes ◽  
High Impact Weather ◽  
Supercell Thunderstorm

Abstract On 31 May 2013, a supercell thunderstorm initiated in west-central Oklahoma and produced a deadly tornado. This convection then grew upscale, with a nearly stationary line developing early on 1 June that produced very heavy rainfall and caused deadly flash flooding in the Oklahoma City area. Real-time convection-allowing (Δx = 4 km) model forecasts used during the Mesoscale Predictability Experiment (MPEX) provided accurate guidance regarding the timing, location, and evolution of convection in this case. However, attempts to simulate this event at higher resolution degraded the forecast, with the primary supercell failing to initiate and the evolution of the overnight MCS not resembling the observed system. Experiments to test the dependence of forecasts of this event on model resolution show that with grid spacing smaller than 4 km, mixing along the dryline in northwest Texas was more vigorous, causing low-level dry air to move more quickly eastward into Oklahoma. This drying prevented the supercell from initiating near the triple point in the higher-resolution simulations. Then, the lack of supercellular convection and its associated cold pool altered the evolution of subsequent convection. Whereas in observations and the 4-km forecast, a nearly stationary MCS developed parallel to, but displaced from, the supercell’s cold pool, the higher-resolution simulations instead had a faster-moving squall line that produced less rainfall. Although the degradation of convective forecasts at higher resolution is probably unusual and appears sensitive to the choice of boundary layer parameterization, these findings demonstrate that how numerical models treat boundary layer processes at different grid spacings can, in some cases, have profound influences on predictions of high-impact weather.

scholarly journals Occurrence and growth of sub-50 nm aerosol particles in the Amazonian boundary layer

2021 ◽  
Author(s):  
Marco A. Franco ◽  
Florian Ditas ◽  
Leslie Ann Kremper ◽  
Luiz A. T. Machado ◽  
Meinrat O. Andreae ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Meteorological Data ◽  
Cloud Condensation Nuclei ◽  
Deep Convection ◽  
Potential Temperature ◽  
Meteorological Conditions ◽  
Subsequent Growth ◽  
Wet Season ◽  
Particle Injection ◽  
Continuous Growth

Abstract. New particle formation (NPF), referring to the nucleation of molecular clusters and their subsequent growth into the cloud condensation nuclei (CCN) size range, is a globally significant and climate-relevant source of atmospheric aerosols. Classical NPF exhibiting continuous growth from a few nanometers to the Aitken mode around 60–70 nm is widely observed in the planetary boundary layer (PBL) around the world, but not in central Amazonia. Here, classical NPF events are rarely observed in the PBL, but instead, NPF begins in the upper troposphere (UT), followed by downdraft injection of sub-50 nm (CN< 50) particles into the PBL and their subsequent growth. Central aspects of our understanding of these processes in the Amazon have remained enigmatic, however. Based on more than six years of aerosol and meteorological data from the Amazon Tall Tower Observatory (ATTO, Feb 2014 to Sep 2020), we analyzed the diurnal and seasonal patterns as well as meteorological conditions during 254 of such Amazonian growth events on 217 event days, which show a sudden occurrence of particles between 10 and 50 nm in the PBL, followed by their growth to CCN sizes. The occurrence of events was significantly higher during the wet season, with 88 % of all events from January to June, than during the dry season, with 12 % from July to December, probably due to differences in the condensation sink (CS), atmospheric aerosol load, and meteorological conditions. Across all events, a median growth rate (GR) of 5.2 nm h−1 and a median CS of 0.0011 s−1 were observed. The growth events were more frequent during the daytime (74 %) and showed higher GR (5.9 nm h−1) compared to nighttime events (4.0 nm h−1), emphasizing the role of photochemistry and PBL evolution in particle growth. About 70 % of the events showed a negative anomaly of the equivalent potential temperature (∆θ'e) – as a marker for downdrafts – and a low satellite brightness temperature (Tir) – as a marker for deep convective clouds – in good agreement with particle injection from the UT in the course of strong convective activity. About 30 % of the events, however, occurred in the absence of deep convection, partly under clear sky conditions, and with a positive ∆θ'e anomaly. Therefore, these events do not appear to be related to downdraft injection and suggest the existence of other currently unknown sources of the sub-50 nm particles.

Saharan Dust Records and Its Impact in the European Alps

2021 ◽  
Author(s):  
Marion Greilinger ◽  
Anne Kasper-Giebl
Keyword(s):  
Mineral Dust ◽  
Cloud Condensation Nuclei ◽  
Ice Cores ◽  
Atmospheric Particulate Matter ◽  
Saharan Dust ◽  
Cloud Formation ◽  
Dust Particles ◽  
European Alps ◽  
Airborne Dust ◽  
Dust Events

Mineral dust is one of the main natural sources of atmospheric particulate matter, with the Sahara being one of the most important source regions for the occurrence and deposition of mineral dust in Europe. The occurrence of dust events in the European Alps is documented via measurements of airborne dust and its deposits onto the glaciers. Dust events occur mainly in spring, summer, and early autumn. Dust layers are investigated in ice cores spanning the last millennium as well as in annual snow packs. They strongly affect the overall flux of dust-related compounds (e.g., calcium and magnesium), provide an alkaline input to wet deposition chemistry, and change the microbial abundance and diversity of the snow pack. Still airborne mineral dust particles can act as ice nuclei and cloud condensation nuclei, influencing the formation of cloud droplets and hence cloud formation and precipitation. Dust deposits on the snow lead to a darkening of the surface, referred to as “surface albedo reduction,” which influences the timing of the snowmelt and reduces the annual mass balance of glaciers, showing a direct link to glacier retreat as observed presently in a warming climate.

Regional modelling of aerosol interaction with deep convection and the effect on new particle formation over Amazonia

2020 ◽  
Author(s):  
Xuemei Wang ◽  
Daniel Grosvenor ◽  
Hamish Gordon ◽  
Meinrat O. Andreae ◽  
Ken Carslaw
Keyword(s):  
Boundary Layer ◽  
Cloud Condensation Nuclei ◽  
Deep Convection ◽  
Particle Formation ◽  
Nucleation Mechanism ◽  
Transport Processes ◽  
Radiative Properties ◽  
Free Troposphere ◽  
New Particle Formation ◽  
New Particles

&lt;p&gt;It has been estimated that over 50% of the present-day global low-level cloud condensation nuclei (CCN) are formed from new particle formation (NPF), and that this process has a substantial effect on the radiative properties of shallow clouds (Gordon et al. 2017). In contrast, we have a very limited understanding of how NPF affects deep convective clouds. Deep clouds could interact strongly with NPF because they extend into the high free troposphere where most new particles are formed, and they are responsible for most of the vertical transport of the nucleating vapours. Andreae et al. (2018) hypothesised from ACRIDICON-CHUVA campaign that organic gas molecules are transported by deep convection to the upper troposphere where they are oxidised and produce new particles, which are then be entrained into the boundary layer and grow to CCN-relevent sizes.&lt;/p&gt;&lt;p&gt;Here we study the interaction of deep convection and NPF using the United Kingdom Chemistry and Aerosols (UKCA) model coupled with the Cloud-AeroSol Interacting Microphyics (CASIM) embedded in the regional configuration of UK Met Office Hadley Centre Global Environment Model (HadGEM3). We simulate several days over a 1000 km region of the Amazon at 4 km resolution. We then compare the regional model, which resolves cloud up- and downdrafts, with the global model with parameterised convection and low resolution.&lt;/p&gt;&lt;p&gt;Our simulations highlight three findings. Firstly, solely using a binary H&lt;sub&gt;2&lt;/sub&gt;SO&lt;sub&gt;4&lt;/sub&gt;-H&lt;sub&gt;2&lt;/sub&gt;O nucleation mechanism strongly underestimates total aerosol concentrations compared to observations by a factor of 1.5-8 below 3 km over the Amazon. This points to the potential role of an additional nucleation mechanism, most likely involving biogenic compounds that occurs throughout more of the free troposphere. Secondly, deep convection transports insoluble gases such as DMS and monoterpenes vertically but not SO&lt;sub&gt;2&lt;/sub&gt;&amp;#160;or H&lt;sub&gt;2&lt;/sub&gt;SO&lt;sub&gt;4&lt;/sub&gt;. The time scale for DMS oxidation (~ 1 day) is much longer than for monoterpene (1-2 hours), which points to the importance of simulating biogenic nucleation over the Amazon in a cloud-resolving model, while lower-resolution global models may adequately capture DMS effects on H&lt;sub&gt;2&lt;/sub&gt;SO&lt;sub&gt;4&lt;/sub&gt; nucleation. Finally, we also examine the Andreae et al (2018) hypothesis of aerosol supply to the boundary layer by quantifying cloud-free and cloudy up- and downdraft transport. The transport of newly formed aerosols into the boundary layer is 8 times greater in cloud-free regions than in the clouds, but these transport processes are of similar magnitude for large aerosols.&lt;/p&gt;

scholarly journals Impact of mineral dust on cloud formation in a Saharan outflow region

2011 ◽  
Vol 11 (12) ◽  
pp. 32363-32390 ◽  
Author(s):  
L. Smoydzin ◽  
A. Teller ◽  
H. Tost ◽  
M. Fnais ◽  
J. Lelieveld
Keyword(s):  
Radiative Forcing ◽  
Mineral Dust ◽  
Eastern Mediterranean ◽  
Cloud Condensation Nuclei ◽  
Coupled Model ◽  
Cloud Formation ◽  
Dust Particles ◽  
Ice Nuclei ◽  
Outflow Region ◽  
The Impact

Abstract. We present a numerical modelling study investigating the impact of mineral dust on cloud formation over the Eastern Mediterranean for two case studies: (i) 25 September 2008 and (ii) 28/29 January 2003. On both days dust plumes crossed the Mediterranean and interacted with clouds forming along frontal systems. For our investigation we used the fully online coupled model WRF-chem. The results show that increased aerosol concentrations due to the presence of mineral dust can enhance the formation of ice crystals. This leads to slight shifts of the spatial and temporal precipitation patterns compared to scenarios where dust was not considered to act as ice nuclei. However, the total amount of precipitation did not change significantly. The only exception occurred when dust entered into an area of orographic ascent, causing glaciation of the clouds, leading to a local enhancement of rainfall. The impact of dust particles acting as giant cloud condensation nuclei on precipitation formation was found to be small. Based on our simulations the contribution of dust to the CCN population is potentially significant only for warm phase clouds. Nevertheless, the dust-induced differences in the microphysical structure of the clouds can contribute to a significant radiative forcing.

scholarly journals Surface modification of mineral dust particles by sulphuric acid processing: implications for CCN and IN abilities

2011 ◽  
Vol 11 (3) ◽  
pp. 7235-7289 ◽  
Author(s):  
P. Reitz ◽  
C. Spindler ◽  
T. F. Mentel ◽  
L. Poulain ◽  
H. Wex ◽  
...  
Keyword(s):  
Sulphuric Acid ◽  
Mineral Dust ◽  
Cloud Condensation Nuclei ◽  
Particle Surface ◽  
Surface Modifications ◽  
Dust Particles ◽  
Ammonia Vapour ◽  
Ice Nuclei ◽  
Aerosol Mass ◽  
Acid Processing

Abstract. The ability of coated mineral dust particles to act as cloud condensation nuclei (CCN) and ice nuclei (IN) was investigated at LACIS (Leipzig Aerosol Cloud Interaction Simulator) during the FROST1- and FROST2-campaigns (Freezing of dust). Sulphuric acid was condensed on the particles which afterwards were optionally humidified, treated with ammonia vapour and/or heat. By means of aerosol mass spectrometry we found evidence that processing of mineral dust particles with sulphuric acid leads to surface modifications of the particles. These surface modifications are responsible for the observed reduction of the IN activation of the particles. The observed particle mass spectra suggest that different treatments lead to different chemical reactions on the particle surface. Possible chemical reaction pathways and products are suggested and the implications on IN and CCN efficiency of the treated dust particles are discussed.

scholarly journals Assessing the mineral dust indirect effects and radiation impacts on a simulated idealized nocturnal squall line

2012 ◽  
Vol 12 (11) ◽  
pp. 29607-29655 ◽  
Author(s):  
R. B. Seigel ◽  
S. C. van den Heever ◽  
S. M. Saleeby
Keyword(s):  
Indirect Effects ◽  
Mineral Dust ◽  
Synergistic Effects ◽  
Atmospheric Modeling ◽  
Dust Particles ◽  
Squall Line ◽  
Cold Pool ◽  
Freezing Level ◽  
Warm Rain Process ◽  
The Individual

Abstract. Mineral dust is arguably the most abundant aerosol species in the world and it plays a large role in aerosol indirect effects (AIEs). This study assesses and isolates the individual responses in a squall line that arise (1) from radiation, (2) from dust altering the microphysics, as well as (3) from the synergistic effects between (1) and (2). To accomplish these tasks, we use the Regional Atmospheric Modeling System (RAMS) set up as a cloud-resolving model (CRM). The CRM contains aerosol and microphysical schemes that allow mineral dust particles to nucleate as cloud drops and ice crystals, replenish upon evaporation and sublimation, be tracked throughout hydrometeor transition, and scavenge by precipitation and dry sedimentation. Factor separation is used on four simulations of the squall line in order to isolate the individual roles of radiation (RADIATION), microphysically active dust (DUST MICRO), and the nonlinear interactions of those factors (SYNERGY). Results indicate that RADIATION acts to increase precipitation, intensify the cold pool, and enhance the mesoscale organization of the squall line due to changes in microphysics beginning from cloud top cooling. Conversely, DUST MICRO decreases precipitation, weakens the cold pool, and weakens the mesoscale organization of the squall line due to an enhancement of the warm rain process. SYNERGY shows little impact on the squall line, except near the freezing level, where an increase in mesoscale organization takes place. The combined effect of the mineral dust AIE due to both DUST MICRO and SYNERGY is to weaken the squall line.

Measurements of Saharan Dust in Convective Clouds over the Tropical Eastern Atlantic Ocean*

2015 ◽  
Vol 72 (1) ◽  
pp. 75-81 ◽  
Author(s):  
Cynthia H. Twohy
Keyword(s):  
Mineral Dust ◽  
Cloud Condensation Nuclei ◽  
Saharan Dust ◽  
Dust Particles ◽  
Tropical Storms ◽  
Liquid Droplets ◽  
Particle Type ◽  
Convective Clouds ◽  
Ice Nuclei ◽  
Eastern Atlantic Ocean

Abstract Mineral dust particles have been shown to act as cloud condensation nuclei, and they are known to interact with developing tropical storms over the Atlantic downwind of the Sahara. Once present within liquid droplets, they have the potential to act as freezing ice nuclei and further affect the microphysics, dynamics, and evolution of tropical storms. However, few measurements of mineral dust particles in tropical convective clouds exist. This study indicates that about one-third of droplets sampled in small convective clouds in the tropical eastern Atlantic contained dust particles, and dust was the dominant residual particle type sampled in ice crystals from anvil outflow. However, estimated number and mass concentrations of dust in anvil ice were small compared to the amount of dust available within the Saharan air layer itself.

scholarly journals Aircraft observations of aerosol, cloud, precipitation, and boundary layer properties in pockets of open cells over the southeast Pacific

2014 ◽  
Vol 14 (15) ◽  
pp. 8071-8088 ◽  
Author(s):  
C. R. Terai ◽  
C. S. Bretherton ◽  
R. Wood ◽  
G. Painter
Keyword(s):  
Boundary Layer ◽  
Cloud Condensation Nuclei ◽  
Surface Wind ◽  
Cloud Droplet ◽  
Cloud Base ◽  
Cold Pool ◽  
Accumulation Mode ◽  
Aerosol Cloud ◽  
Wide Range ◽  
Southeast Pacific

Abstract. Five pockets of open cells (POCs) are studied using aircraft flights from the VOCALS Regional Experiment (VOCALS-REx), conducted in October and November 2008 over the southeast Pacific Ocean. Satellite imagery from the geostationary satellite GOES-10 is used to distinguish POC areas, and measurements from the aircraft flights are used to compare aerosol, cloud, precipitation, and boundary layer conditions inside and outside of POCs. Conditions observed across individual POC cases are also compared. POCs are observed in boundary layers with a wide range of inversion heights (1250 to 1600 m) and surface wind speeds (5 to 11 m s−1) and show no remarkable difference from the observed surface and free-tropospheric conditions during the two months of the field campaign. In all cases, compared to the surrounding overcast region the POC boundary layer is more decoupled, supporting both thin stratiform and deeper cumulus clouds. Although cloud-base precipitation rates are higher in the POC than the overcast region in each case, a threshold precipitation rate that differentiates POC precipitation from overcast precipitation does not exist. Mean cloud-base precipitation rates in POCs can range from 1.7 to 5.8 mm d−1 across different POC cases. The occurrence of heavy drizzle (> 0 dBZ) lower in the boundary layer better differentiates POC precipitation from overcast precipitation, likely leading to the more active cold pool formation in POCs. Cloud droplet number concentration is at least a factor of 8 smaller in the POC clouds, and the ratio of drizzle water to cloud water in POC clouds is over an order of magnitude larger than that in overcast clouds, indicating an enhancement of collision–coalescence processes in POC clouds. Despite large variations in the accumulation-mode aerosol concentrations observed in the surrounding overcast region (65 to 324 cm−3), the accumulation-mode aerosol concentrations observed in the subcloud layer of all five POCs exhibit a much narrower range (24 to 40 cm−3), and cloud droplet concentrations within the cumulus updrafts originating in this layer reflect this limited variability. Above the POC subcloud layer exists an ultraclean layer with accumulation-mode aerosol concentrations < 5 cm−3, demonstrating that in-cloud collision–coalescence processes efficiently remove aerosols. The existence of the ultraclean layer also suggests that the major source of accumulation-mode aerosols, and hence of cloud condensation nuclei in POCs, is the ocean surface, while entrainment of free-tropospheric aerosols is weak. The measurements also suggest that at approximately 30 cm−3 a balance of surface source and coalescence scavenging sinks of accumulation-mode aerosols maintain the narrow range of observed subcloud aerosol concentrations.

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