scholarly journals Estimation of the fossil fuel component in atmospheric CO<sub>2</sub> based on radiocarbon measurements at the Beromünster tall tower, Switzerland

2017 ◽  
Vol 17 (17) ◽  
pp. 10753-10766 ◽  
Author(s):  
Tesfaye A. Berhanu ◽  
Sönke Szidat ◽  
Dominik Brunner ◽  
Ece Satar ◽  
Rüdiger Schanda ◽  
...  
Keyword(s):  
Nuclear Power ◽  
Power Plants ◽  
Large Scale ◽  
Fossil Fuel ◽  
Transport Model ◽  
Vertical Mixing ◽  
Fuel Component ◽  
Mixing Ratios ◽  
Tall Tower

Abstract. Fossil fuel CO2 (CO2ff) is the major contributor of anthropogenic CO2 in the atmosphere, and accurate quantification is essential to better understand the carbon cycle. Since October 2012, we have been continuously measuring the mixing ratios of CO, CO2, CH4, and H2O at five different heights at the Beromünster tall tower, Switzerland. Air samples for radiocarbon (Δ14CO2) analysis have also been collected from the highest sampling inlet (212.5 m) of the tower on a biweekly basis. A correction was applied for 14CO2 emissions from nearby nuclear power plants (NPPs), which have been simulated with the Lagrangian transport model FLEXPART-COSMO. The 14CO2 emissions from NPPs offset the depletion in 14C by fossil fuel emissions, resulting in an underestimation of the fossil fuel component in atmospheric CO2 by about 16 %. An average observed ratio (RCO) of 13.4 ± 1.3 mmol mol−1 was calculated from the enhancements in CO mixing ratios relative to the clean-air reference site Jungfraujoch (ΔCO) and the radiocarbon-based fossil fuel CO2 mole fractions. The wintertime RCO estimate of 12.5 ± 3.3 is about 30 % higher than the wintertime ratio between in situ measured CO and CO2 enhancements at Beromünster over the Jungfraujoch background (8.7 mmol mol−1) corrected for non-fossil contributions due to strong biospheric contribution despite the strong correlation between ΔCO and ΔCO2 in winter. By combining the ratio derived using the radiocarbon measurements and the in situ measured CO mixing ratios, a high-resolution time series of CO2ff was calculated exhibiting a clear seasonality driven by seasonal variability in emissions and vertical mixing. By subtracting the fossil fuel component and the large-scale background, we have determined the regional biospheric CO2 component that is characterized by seasonal variations ranging between −15 and +30 ppm. A pronounced diurnal variation was observed during summer modulated by biospheric exchange and vertical mixing, while no consistent pattern was found during winter.

scholarly journals Estimation of the fossil-fuel component in atmospheric CO<sub>2</sub> based on radiocarbon measurements at the Beromünster tall tower, Switzerland

2017 ◽  
Author(s):  
Tesfaye A. Berhanu ◽  
Sonke Szidat ◽  
Dominik Brunner ◽  
Ece Satar ◽  
Rudiger Schanda ◽  
...  
Keyword(s):  
Power Plants ◽  
Large Scale ◽  
Fossil Fuel ◽  
Transport Model ◽  
Vertical Mixing ◽  
Fuel Component ◽  
Mixing Ratios ◽  
Tall Tower ◽  
Emission Ratios

Abstract. Fossil fuel CO2 (CO2ff) is the major contributor of anthropogenic CO2 in the atmosphere, and accurate quantification is essential to better understand the carbon cycle. Since October 2012, we have been continuously measuring the mixing ratios of CO, CO2, CH4 and H2O at five different heights at the Beromünster tall tower, Switzerland. Air samples for radiocarbon (Δ14CO2) analysis have also been collected from the 212.5 m sampling inlet of the tower on a bi-weekly basis. A correction was applied for 14CO2 emissions from nearby nuclear power plants (NPPs), which have been simulated with the Lagrangian transport model FLEXPART-COSMO. The 14CO2 emissions from NPPs offset the depletion in 14C by fossil-fuel emissions resulting in an underestimation of the fossil-fuel component in atmospheric CO2 by about 16 %. An average observed ratio (RCO) of 13.4 ± 1.3 mmol/mol was calculated from the enhancements in CO mixing ratios relative to the clean air reference site Jungfraujoch (ΔCO) and the radiocarbon-based fossil-fuel CO2 mole fractions. This ratio is significantly higher than both the mean anthropogenic CO/CO2 emission ratios estimated for Switzerland from the national inventory (7.8 mmol/mol for 2013), and the ratio between in-situ measured CO and CO2 enhancements at Beromünster over the Jungfraujoch background (8.3 mmol/mol). Differences could not yet be assigned to specific processes and shortcomings of these two methods but may originate from locally variable emission ratios as well as from non-fossil emissions and biospheric contributions. By combining the ratio derived using the radiocarbon measurements and the in-situ measured CO mixing ratios, a high-resolution time series of CO2ff was calculated exhibiting a clear seasonality driven by seasonal variability in emissions and vertical mixing. By subtracting the fossil-fuel component and the large-scale background, we have determined the regional biospheric CO2 component that is characterized by seasonal variations ranging between −15 to +30 ppm. A pronounced diurnal variation was observed during summer modulated by biospheric exchange and vertical mixing while no consistent pattern was found during winter.

Planning of Large-Scale In-Situ Gas Generation Experiment in Korean Radioactive Waste Repository

2010 ◽  
Author(s):  
Juyoul Kim ◽  
Sukhoon Kim ◽  
Jin Beak Park ◽  
Sunjoung Lee
Keyword(s):  
Radioactive Waste ◽  
Nuclear Power ◽  
Power Plants ◽  
Nuclear Power Plants ◽  
Large Scale ◽  
Radioactive Waste Disposal ◽  
Gas Generation ◽  
Radioactive Waste Repository ◽  
Waste Repository

In the Korean LILW (Low- and Intermediate-Level radioactive Waste) repository at Gyeongju city, the degradation of organic wastes and the corrosion of metallic wastes and steel containers would be important processes that affect repository geochemistry, speciation and transport of radionuclides during the lifetime of a radioactive waste disposal facility. Gas is generated in association with these processes and has the potential threat to pressurize the repository, which can promote the transport of groundwater and gas, and consequently radionuclide transport. Microbial activity plays an important role in organic degradation, corrosion and gas generation through the mediation of reduction-oxidation reactions. The Korean research project on gas generation is being performed by Korea Radioactive Waste Management Corporation (hereafter referred to as “KRMC”). A full-scale in-situ experiment will form a central part of the project, where gas generation in real radioactive low-level maintenance waste from nuclear power plants will be done as an in-depth study during ten years at least. In order to examine gas generation issues from an LILW repository which is being constructed and will be completed by the end of December, 2012, two large-scale facilities for the gas generation experiment will be established, each equipped with a concrete container carrying on 16 drums of 200 L and 9 drums of 320 L of LILW from Korean nuclear power plants. Each container will be enclosed within a gas-tight and acid-proof steel tank. The experiment facility will be fully filled with ground water that provides representative geochemical conditions and microbial inoculation in the near field of repository. In the experiment, the design includes long-term monitoring and analyses for the rate and composition of gas generated, and aqueous geochemistry and microbe populations present at various locations through on-line analyzers and manual periodical sampling. A main schedule for establishing the experiment facility is as follows: Completion of the detailed design until the second quarter of the year 2010; Completion of the manufacture and on-site installation until the second quarter of the year 2011; Start of the operation and monitoring from the third quarter of the year 2011.

scholarly journals On the Root Causes of the Fukushima Daiichi Disaster from the Perspective of High Complexity and Tight Coupling in Large-Scale Systems

Symmetry ◽  
2021 ◽  
Vol 13 (3) ◽  
pp. 414
Author(s):  
Atsuo Murata ◽  
Waldemar Karwowski
Keyword(s):  
Nuclear Power ◽  
Power Plants ◽  
Large Scale ◽  
High Complexity ◽  
Tight Coupling ◽  
Large Scale Systems ◽  
Safety Issues ◽  
Loss Of Coolant ◽  
Station Blackout ◽  
Fukushima Daiichi

This study explores the root causes of the Fukushima Daiichi disaster and discusses how the complexity and tight coupling in large-scale systems should be reduced under emergencies such as station blackout (SBO) to prevent future disasters. First, on the basis of a summary of the published literature on the Fukushima Daiichi disaster, we found that the direct causes (i.e., malfunctions and problems) included overlooking the loss of coolant and the nuclear reactor’s failure to cool down. Second, we verified that two characteristics proposed in “normal accident” theory—high complexity and tight coupling—underlay each of the direct causes. These two characteristics were found to have made emergency management more challenging. We discuss how such disasters in large-scale systems with high complexity and tight coupling could be prevented through an organizational and managerial approach that can remove asymmetry of authority and information and foster a climate of openly discussing critical safety issues in nuclear power plants.

Development of 1500-r/min 75-Inch Ultra-Long Last Stage Blades for Nuclear Steam Turbine

2017 ◽  
Author(s):  
Deqi Yu ◽  
Jiandao Yang ◽  
Wei Lu ◽  
Daiwei Zhou ◽  
Kai Cheng ◽  
...  
Keyword(s):  
Nuclear Power ◽  
Power Plants ◽  
Large Scale ◽  
Vibration Monitoring ◽  
Steam Turbines ◽  
Element Analysis ◽  
Rotating Blade ◽  
Lifetime Analysis ◽  
Computational Fluid Dynamics Cfd ◽  
Last Stage

The 1500-r/min 1905mm (75inch) ultra-long last three stage blades for half-speed large-scale nuclear steam turbines of 3rd generation nuclear power plants have been developed with the application of new design features and Computer-Aided-Engineering (CAE) technologies. The last stage rotating blade was designed with an integral shroud, snubber and fir-tree root. During operation, the adjacent blades are continuously coupled by the centrifugal force. It is designed that the adjacent shrouds and snubbers of each blade can provide additional structural damping to minimize the dynamic stress of the blade. In order to meet the blade development requirements, the quasi-3D aerodynamic method was used to obtain the preliminary flow path design for the last three stages in LP (Low-pressure) casing and the airfoil of last stage rotating blade was optimized as well to minimize its centrifugal stress. The latest CAE technologies and approaches of Computational Fluid Dynamics (CFD), Finite Element Analysis (FEA) and Fatigue Lifetime Analysis (FLA) were applied to analyze and optimize the aerodynamic performance and reliability behavior of the blade structure. The blade was well tuned to avoid any possible excitation and resonant vibration. The blades and test rotor have been manufactured and the rotating vibration test with the vibration monitoring had been carried out in the verification tests.

In situ gamma spectrometry using portable HPGe detector. Radiological characterization and environmental surveillance around an operating nuclear power plant. Possibilities and limits

2021 ◽  
Author(s):  
Jose Angel Corbacho ◽  
A Baeza
Keyword(s):  
Power Plant ◽  
Nuclear Power Plant ◽  
Gamma Spectrometry ◽  
Nuclear Power ◽  
Power Plants ◽  
Activity Concentration ◽  
Versatile Tool ◽  
Ge Detector ◽  
Radiological Characterization

Abstract In situ technique for measuring radionuclides in the soil using a portable Ge detector is a highly versatile tool for both the radiological characterization and for the monitoring of operating nuclear power plants. The main disadvantage of this technique is related to the lack of knowledge of the geometry of the source whose activity concentration is to be determined. However, its greatest advantage is the high spatial representability of the samples and the lower time and resource consumption than gamma spectrometry lab measurements. In this study, the possibilities and limits offered by in situ gamma spectrometry with a high resolution gamma portable detector in two common uses are shown: First, the radiological background characterization and its relationship with the geology of an area of 2700 km2 are assessed; Secondly, its potential for monitoring man-made activity concentration in soils located around an operating nuclear power plant in Spain for surveillance purposes is evaluated. Finally, high accuracy radiation maps have been prepared from the measurements carried out. These radiation maps are essential tools to know the radioactive background of an area, especially useful to assess artificial radioactive deposits produced after a nuclear accident or incident.

scholarly journals Development of CarbonTracker Europe-CH<sub>4</sub> – Part 2: global methane emission estimates and their evaluation for 2000–2012

2016 ◽  
Author(s):  
Aki Tsuruta ◽  
Tuula Aalto ◽  
Leif Backman ◽  
Janne Hakkarainen ◽  
Ingrid T. van der Laan-Luijkx ◽  
...  
Keyword(s):  
North American ◽  
Transport Model ◽  
Vertical Mixing ◽  
Total Carbon ◽  
In Situ Observation ◽  
Convection Scheme ◽  
Temperate Region ◽  
Northern Latitude ◽  
The North

Abstract. Gobal methane emissions were estimated for 2000–2012 using the CarbonTracker Europe-CH4 (CTE-CH4) data assimilation system. In CTE-CH4, the anthropogenic and biosphere emissions of CH4 are simultaneously constrained by global atmospheric in-situ methane mole fraction observations. We use three configurations developed in Tsuruta et al. (2016) to assess the sensitivity of the CH4 flux estimates to (a) the number of unknown flux scaling factors to be optimized which in turn depends on the choice of underlying land-ecosystem map, and (b) on the parametrization of vertical mixing in the 30 atmospheric transport model TM5. The posterior emission estimates were evaluated by comparing simulations to surface in-situ observation sites, to profile observations made by aircraft, to dry air total column-averaged mole fractions (XCH4) observations from the Total Carbon Column Observing Network (TCCON), and to XCH4 retrievals from the Greenhouse gases Observing SATellite (GOSAT). Our estimated posterior mean global total emissions during 2000–2012 are 516 ± 51 Tg CH4 yr−1, and emission estimates during 2007–2012 are 18 Tg CH4 yr−1 greater than those from 2001–2006, mainly driven by an 35 increase in emissions from the south America temperate region, the Asia temperate region and Asia tropics. The sensitivity of the flux estimates to the underlying ecosystem map was large for the Asia temperate region and Australia, but not significant in the northern latitude regions, i.e. the north American boreal region, the north American temperate region and Europe. Instead, the posterior estimates for the northern latitude regions show larger sensitivity to the choice of convection scheme in TM5. The Gregory et al. (2000) mixing scheme with faster interhemispheric exchange leads to higher estimated CH4 emissions at northern latitudes, and lower emissions in southern latitudes, compared to the estimates using Tiedtke (1989) convection scheme. Our evaluation with non-assimilated observations showed that posterior mole fractions were better matched with the 5 observations when Gregory et al. (2000) convection scheme was used.

Lifetime Management of EDF PWR Pressure Vessels and Pipings

2004 ◽  
Author(s):  
F. Hedin ◽  
J. C. Legendre
Keyword(s):  
Nuclear Power ◽  
Power Plants ◽  
Cost Benefit Analysis ◽  
Cost Benefit ◽  
Pressure Vessels ◽  
Destructive Testing ◽  
Key Points ◽  
Cast Stainless Steel ◽  
Non Destructive

Lifetime management of EDF PWR vessels and pipings are one of the main technical key points of safety and competitivness. This paper describes the EDF global approach in this field, which is applied to the nuclear fleet i.e 58 nuclear power plants, and particularly to the first 34 three loops, as far as lifetime is concerned: • operating procedures and routine maintenance, special maintenance and ten years safety reassessment, • engineering analysis, based on feed back experience, scientific knowledge, degradations mechanisms, causes and consequences management, • operating loadings decrease, • complementary deterministic and cost-benefit analysis, • fit for service justifications, • anticipation strategy to prepare future, based on Non Destructive Testing investigations, ability to repair and/or to replace components, in situ expertises, ... Some examples are given: lifetime management of reactor vessels heads and bottom penetrations of pressure vessels, fit for service of cast stainless steel primary pipings, primary nozzles and auxiliary pipings special maintenance.

scholarly journals Using ship-borne observations of methane isotopic ratio in the Arctic Ocean to understand methane sources in the Arctic

2019 ◽  
Author(s):  
Antoine Berchet ◽  
Isabelle Pison ◽  
Patrick M. Crill ◽  
Brett Thornton ◽  
Philippe Bousquet ◽  
...  
Keyword(s):  
Arctic Ocean ◽  
Large Scale ◽  
Transport Model ◽  
Isotopic Ratio ◽  
The Arctic ◽  
Isotopic Ratios ◽  
Air Masses ◽  
Remote Areas ◽  
The Arctic Ocean

Abstract. Due to the large variety and heterogeneity of sources in remote areas hard to document, the Arctic regional methane budget remain very uncertain. In situ campaigns provide valuable data sets to reduce these uncertainties. Here we analyse data from the SWERUS-C3 campaign, on-board the icebreaker Oden, that took place during summer 2014 in the Arctic Ocean along the Northern Siberian and Alaskan shores. Total concentrations of methane, as well as isotopic ratios were measured continuously during this campaign for 35 days in July and August 2014. Using a chemistry-transport model, we link observed concentrations and isotopic ratios to regional emissions and hemispheric transport structures. A simple inversion system helped constraining source signatures from wetlands in Siberia and Alaska and oceanic sources, as well as the isotopic composition of lower stratosphere air masses. The variation in the signature of low stratosphere air masses, due to strongly fractionating chemical reactions in the stratosphere, was suggested to explain a large share of the observed variability in isotopic ratios. These points at required efforts to better simulate large scale transport and chemistry patterns to use isotopic data in remote areas. It is found that constant and homogeneous source signatures for each type of emission in the region (mostly wetlands and oil and gas industry) is not compatible with the strong synoptic isotopic signal observed in the Arctic. A regional gradient in source signatures is highlighted between Siberian and Alaskan wetlands, the later ones having a lighter signatures than the first ones. Arctic continental shelf sources are suggested to be a mixture of methane from a dominant thermogenic origin and a secondary biogenic one, consistent with previous in-situ isotopic analysis of seepage along the Siberian shores.

scholarly journals Spatiotemporal patterns of the fossil-fuel CO<sub>2</sub> signal in central Europe: Results from a high-resolution atmospheric transport model

2017 ◽  
Author(s):  
Yu Liu ◽  
Nicolas Gruber ◽  
Dominik Brunner
Keyword(s):  
High Resolution ◽  
Central Europe ◽  
Western Europe ◽  
Fossil Fuel ◽  
Transport Model ◽  
Atmospheric Transport ◽  
Temporal Variations ◽  
Atmospheric Co2 ◽  
Fuel Component ◽  
Atmospheric Transport Model

Abstract. The emission of CO2 from the burning of fossil fuel is a prime determinant of variations in atmospheric CO2. Here, we simulate this fossil fuel signal together with the natural and background components with a regional high-resolution atmospheric transport model for central and southern Europe considering separately the emissions from different sectors and countries on the basis of emission inventories and hourly emission time functions. The simulated variations in atmospheric CO2 agree very well with observation-based estimates, although the observed variance is slightly underestimated, particularly for the fossil fuel component. Despite relatively rapid atmospheric mixing, the simulated fossil fuel signal reveals distinct annual mean structures deep into the troposphere reflecting the spatially dense aggregation of most emissions. The fossil fuel signal accounts for more than half of the total (fossil fuel + biospheric + background) temporal variations in atmospheric CO2 in most areas of northern and western central Europe, with the largest variations occurring on diurnal timescales owing to the combination of diurnal variations in emissions and atmospheric mixing/transport out of the surface layer. Their co-variance leads to a fossil-fuel diurnal rectifier effect with a magnitude as large as 9 ppm compared to a case with time-constant emissions. The spatial pattern of CO2 from the different sectors largely reflects the distribution and relative magnitude of the corresponding emissions, with power plant emissions leaving the most distinguished mark. An exception is southern and western Europe, where the emissions from the transportation sector dominate the fossil fuel signal. Most of the fossil fuel CO2 remains within the country responsible for the emission, although in smaller countries, up to 80 % of the fossil fuel signal can come from abroad. A fossil fuel emission reduction of 30 % is clearly detectable for a surface-based observing system for atmospheric CO2, while it is beyond the edge of detectability for the current generation of satellites with the exception of a few hotspot sites. Changes in variability in atmospheric CO2 might open an additional door for the monitoring and verification of changes in fossil fuel emissions, primarily for surface based systems.

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