scholarly journals Sensitivity of transatlantic dust transport to chemical aging and related atmospheric processes

2017 ◽  
Vol 17 (6) ◽  
pp. 3799-3821 ◽  
Author(s):  
Mohamed Abdelkader ◽  
Swen Metzger ◽  
Benedikt Steil ◽  
Klaus Klingmüller ◽  
Holger Tost ◽  
...  
Keyword(s):  
Atlantic Ocean ◽  
Wet Deposition ◽  
Dust Emission ◽  
Dust Particles ◽  
Emission Flux ◽  
Dust Transport ◽  
Chemical Aging ◽  
Calcium Cation ◽  
Convection Schemes ◽  
The Impact

Abstract. We present a sensitivity study on transatlantic dust transport, a process which has many implications for the atmosphere, the ocean and the climate. We investigate the impact of key processes that control the dust outflow, i.e., the emission flux, convection schemes and the chemical aging of mineral dust, by using the EMAC model following Abdelkader et al. (2015). To characterize the dust outflow over the Atlantic Ocean, we distinguish two geographic zones: (i) dust interactions within the Intertropical Convergence Zone (ITCZ), or the dust–ITCZ interaction zone (DIZ), and (ii) the adjacent dust transport over the Atlantic Ocean (DTA) zone. In the latter zone, the dust loading shows a steep and linear gradient westward over the Atlantic Ocean since particle sedimentation is the dominant removal process, whereas in the DIZ zone aerosol–cloud interactions, wet deposition and scavenging processes determine the extent of the dust outflow. Generally, the EMAC simulated dust compares well with CALIPSO observations; however, our reference model configuration tends to overestimate the dust extinction at a lower elevation and underestimates it at a higher elevation. The aerosol optical depth (AOD) over the Caribbean responds to the dust emission flux only when the emitted dust mass is significantly increased over the source region in Africa by a factor of 10. These findings point to the dominant role of dust removal (especially wet deposition) in transatlantic dust transport. Experiments with different convection schemes have indeed revealed that the transatlantic dust transport is more sensitive to the convection scheme than to the dust emission flux parameterization. To study the impact of dust chemical aging, we focus on a major dust outflow in July 2009. We use the calcium cation as a proxy for the overall chemical reactive dust fraction and consider the uptake of major inorganic acids (i.e., H2SO4, HNO3 and HCl) and their anions, i.e., sulfate (SO42−), bisulfate (HSO4−), nitrate (NO3−) and chloride (Cl−), on the surface of mineral particles. The subsequent neutralization reactions with the calcium cation form various salt compounds that cause the uptake of water vapor from the atmosphere, i.e., through the chemical aging of dust particles leading to an increase of 0.15 in the AOD under subsaturated conditions (July 2009 monthly mean). As a result of the radiative feedback on surface winds, dust emissions increased regionally. On the other hand, the aged dust particles, compared to the non-aged particles, are more efficiently removed by both wet and dry deposition due to the increased hygroscopicity and particle size (mainly due to water uptake). The enhanced removal of aged particles decreases the dust burden and lifetime, which indirectly reduces the dust AOD by 0.05 (monthly mean). Both processes can be significant (major dust outflow, July 2009), but the net effect depends on the region and level of dust chemical aging.

scholarly journals Chemical aging of atmospheric mineral dust during transatlantic transport

2016 ◽  
Author(s):  
Mohamed Abdelkader ◽  
Swen Metzger ◽  
Benedikt Steil ◽  
Klaus Klingmüller ◽  
Holger Tost ◽  
...  
Keyword(s):  
Atlantic Ocean ◽  
Direct Effect ◽  
Dust Particles ◽  
Hygroscopic Growth ◽  
Aging Effects ◽  
Particle Sedimentation ◽  
Inter Tropical Convergence Zone ◽  
Dust Transport ◽  
Dust Fraction ◽  
The Impact

Abstract. Transatlantic dust transport has many implications for the atmosphere, ocean and climate. We present a modeling study on the impact of the key processes (dust emissions flux, convection and dust aging parameterizations) that control the transatlantic dust transport. Typically, the Inter-Tropical Convergence Zone (ITCZ) acts as a barrier for the meridional dust transport. To characterize the dust outflow over the Atlantic Ocean, we address two regional phenomena: (i) dust interactions with the ITCZ (DIZ) and (ii) the adjacent dust transport over the Atlantic Ocean (DTA). In the DTA zone, the dust loading shows a steep and linear gradient westward over the Atlantic Ocean where particle sedimentation is the dominant removal process, whereas in the DIZ zone cloud interactions and wet deposition predominate. To study the different impacts of aging, we present two case studies that exclude condensation and coagulation, and include dust aging at various levels of complexity. For dust aging, we consider the uptake of inorganic acids on the surface of mineral particles that form salt compounds. Calcium, used as a proxy for the overall chemically reactive dust fraction, drives the dust-related neutralization reactions leading to higher dust aerosol optical depth (AOD). The aged dust particles are transferred to the soluble aerosol modes in the model and are mixed with other species that originate from anthropogenic and natural sources. The neutralization products (salts) take up water vapor from the atmosphere and increase the dust AOD under subsaturated conditions. We define the "direct effect of dust aging" to refer to the increase in AOD as a result of hygroscopic growth. On the other hand, the aged dust is more efficiently removed (wet and dry) because of the increase in particle size and hygroscopicity. This more efficient removal reduces the dust AOD over the DIZ zone. We define this as the "indirect effect of dust aging", complementary to the direct effect that is dominant in the DTA zone. Distinction of the two aging effects helps develop insight into the regional importance of dust–air-pollution interactions.

scholarly journals Implementation of dust emission and chemistry into the Community Multiscale Air Quality modeling system and initial application to an Asian dust storm episode

2012 ◽  
Vol 12 (21) ◽  
pp. 10209-10237 ◽  
Author(s):  
K. Wang ◽  
Y. Zhang ◽  
A. Nenes ◽  
C. Fountoukis
Keyword(s):  
Air Quality ◽  
Dust Storm ◽  
Dust Emission ◽  
Forecast Model ◽  
Heterogeneous Reactions ◽  
Dust Particles ◽  
Aerodynamic Diameter ◽  
Dust Emissions ◽  
New Model ◽  
The Impact

Abstract. The US Environmental Protection Agency's (EPA) Community Multiscale Air Quality (CMAQ) modeling system version 4.7 is further developed to enhance its capability in simulating the photochemical cycles in the presence of dust particles. The new model treatments implemented in CMAQ v4.7 in this work include two online dust emission schemes (i.e., the Zender and Westphal schemes), nine dust-related heterogeneous reactions, an updated aerosol inorganic thermodynamic module ISORROPIA II with an explicit treatment of crustal species, and the interface between ISORROPIA II and the new dust treatments. The resulting improved CMAQ (referred to as CMAQ-Dust), offline-coupled with the Weather Research and Forecast model (WRF), is applied to the April 2001 dust storm episode over the trans-Pacific domain to examine the impact of new model treatments and understand associated uncertainties. WRF/CMAQ-Dust produces reasonable spatial distribution of dust emissions and captures the dust outbreak events, with the total dust emissions of ~111 and 223 Tg when using the Zender scheme with an erodible fraction of 0.5 and 1.0, respectively. The model system can reproduce well observed meteorological and chemical concentrations, with significant improvements for suspended particulate matter (PM), PM with aerodynamic diameter of 10 μm, and aerosol optical depth than the default CMAQ v4.7. The sensitivity studies show that the inclusion of crustal species reduces the concentration of PM with aerodynamic diameter of 2.5 μm (PM2.5) over polluted areas. The heterogeneous chemistry occurring on dust particles acts as a sink for some species (e.g., as a lower limit estimate, reducing O3 by up to 3.8 ppb (~9%) and SO2 by up to 0.3 ppb (~27%)) and as a source for some others (e.g., increasing fine-mode SO42− by up to 1.1 μg m−3 (~12%) and PM2.5 by up to 1.4 μg m−3 (~3%)) over the domain. The long-range transport of Asian pollutants can enhance the surface concentrations of gases by up to 3% and aerosol species by up to 20% in the Western US.

scholarly journals Convective distribution of dust over the Arabian Peninsula: the impact of model resolution

2019 ◽  
Author(s):  
Jennie Bukowski ◽  
Susan C. van den Heever
Keyword(s):  
Arabian Peninsula ◽  
Dust Emission ◽  
Dust Storms ◽  
Radiation Budget ◽  
Grid Spacing ◽  
Heating Rates ◽  
Dust Transport ◽  
Order Of Magnitude ◽  
The Impact ◽  
Cumulus Parameterizations

Abstract. Along the coasts of the Arabian Peninsula, convective dust storms are a considerable source of mineral dust to the atmosphere. Reliable predictions of convective dust events are necessary to determine their effects on air quality, visibility, and the radiation budget. In this study, the Weather Research and Forecasting Model coupled with Chemistry (WRF-Chem) is used to simulate a 2016 summertime dust event over the Arabian Peninsula and examine the variability in dust fields and associated vertical transport due to the choice of convective parameterization and explicit versus parameterized convection. Simulations are run at 45 km and 15 km grid spacing with multiple cumulus parameterizations, and are compared to a 3 km simulation that permits explicit convective processes. Five separate cumulus parameterizations at 15 km grid spacing were tested to quantify the spread across different parameterizations. Finally, the impact these variations have on radiation, specifically aerosol heating rates is also investigated. On average, in these simulations the explicit case produces higher quantities of dust than the parameterized cases in terms of dust uplift potential, vertical dust concentrations, and vertical dust fluxes. Major drivers of this discrepancy between the simulations stem from the explicit case exhibiting higher surface windspeeds during convective activity, lower dust emission wind threshold velocities due to drier soil, and more frequent, stronger vertical velocities which transport dust aloft and increase the atmospheric lifetime of these particles. For aerosol heating rates in the lowest levels, the shortwave effect prevails in the explicit case with a net cooling effect, whereas a longwave net warming effect is present in the parameterized cases. The spread in dust concentrations across cumulus parameterizations at the same grid resolution (15 km) is an order of magnitude lower than the impact of moving from parameterized to explicit convection. We conclude that tuning dust emissions in coarse resolution simulations can only improve the results to first-order and cannot fully rectify the discrepancies originating from disparities in the representation of convective dust transport.

scholarly journals Implementation of dust emission and chemistry into the Community Multiscale Air Quality modeling system and initial application to an Asian dust storm episode

2012 ◽  
Vol 12 (5) ◽  
pp. 13457-13514 ◽  
Author(s):  
K. Wang ◽  
Y. Zhang ◽  
A. Nenes ◽  
C. Fountoukis
Keyword(s):  
Air Quality ◽  
Dust Storm ◽  
Dust Emission ◽  
Heterogeneous Reactions ◽  
Dust Particles ◽  
Aerodynamic Diameter ◽  
Dust Emissions ◽  
New Model ◽  
The Us ◽  
The Impact

Abstract. The US Environmental Protection Agency (EPA)'s Community Multiscale Air Quality (CMAQ) modeling system version 4.7 is further developed to enhance its capability in simulating the photochemical cycles in the presence of dust particles. The new model treatments implemented in CMAQ v4.7 in this work include two online-dust emission schemes, nine dust-related heterogeneous reactions, an updated aerosol inorganic thermodynamic module ISORROPIA II with an explicit treatment of crustal species, and the interface between ISORROPIA II and the new dust treatments. The resulting improved CMAQ (referred to as CMAQ-Dust), offline-coupled with the Weather Research and Forecast model (WRF), are applied to the April 2001 dust storm episode over the trans-Pacific domain to examine the impact of new model treatments and understand associated uncertainties. WRF/CMAQ-Dust produces reasonable spatial distribution of dust emissions and captures the dust outbreak events, with the total dust emissions of ∼111 and 223 Tg when the erodible fraction is assumed to be 0.5 and 1.0, respectively, for the April 2001 episode. The model system can reproduce well observed meteorological and chemical concentrations, with significant improvements for suspended particulate matter (PM), PM with aerodynamic diameter of 10 μm and aerosol optical depth than default CMAQ v4.7. The sensitivity studies show that the inclusion of crustal species reduces the concentration of PM with aerodynamic diameter of 2.5 μm (PM2.5) over polluted areas. The heterogeneous chemistry occurring on dust particles acts as a sink for some species (e.g., as a lower limit estimate, O3 by up to 3.8 ppb (∼9%) and SO2 by up to 0.3 ppb (∼27%)) and as a source for some others (e.g., fine-mode SO42− by up to 1.1 μg m−3 (∼12%) and PM2.5 by up to 1.4 μg m−3 (∼3%) over the domain. The long-range transport of Asian pollutants can enhance the background concentrations of gases by up to 3% and aerosol species by up to 20% in the US.

scholarly journals The Appearance of a “Fresh” Surface on 596 Scheila as a Consequence of the 2010 Impact Event

2022 ◽  
Vol 924 (1) ◽  
pp. L9
Author(s):  
Sunao Hasegawa ◽  
Michaël Marsset ◽  
Francesca E. DeMeo ◽  
Schelte J. Bus ◽  
Masateru Ishiguro ◽  
...  
Keyword(s):  
Near Infrared ◽  
Dust Emission ◽  
Interplanetary Dust ◽  
Dust Particles ◽  
Impact Event ◽  
Main Belt ◽  
Interplanetary Dust Particles ◽  
Slope Change ◽  
The Impact ◽  
Fresh Surface

Abstract Dust emission was detected on main-belt asteroid 596 Scheila in 2010 December and was attributed to the collision of a few-tens-of-meters projectile on the surface of the asteroid. In such an impact, the ejected material from the collided body is expected to mainly come from its fresh, unweathered subsurface. Therefore, it is expected that the surface of 596 was partially or entirely refreshed during the 2010 impact. By combining spectra of 596 from the literature and our own observations, we show that the 2010 impact event resulted in a significant slope change in the near-infrared (0.8–2.5 μm) spectrum of the asteroid, from moderately red (T type) before the impact to red (D type) after the impact. This provides evidence that red carbonaceous asteroids become less red with time due to space weathering, in agreement with predictions derived from laboratory experiments on the primitive Tagish Lake meteorite, which is spectrally similar to 596. This discovery provides the very first telescopic confirmation of the expected weathering trend of asteroids spectrally analog to Tagish Lake and/or anhydrous chondritic porous interplanetary dust particles. Our results also suggest that the population of implanted objects from the outer solar system is much larger than previously estimated in the main belt, but many of these objects are hidden below their space-weathered surfaces.

scholarly journals Mass deposition fluxes of Saharan mineral dust to the tropical northeast Atlantic Ocean: an intercomparison of methods

2012 ◽  
Vol 12 (12) ◽  
pp. 33025-33081 ◽  
Author(s):  
N. Niedermeier ◽  
A. Held ◽  
T. Müller ◽  
B. Heinold ◽  
K. Schepanski ◽  
...  
Keyword(s):  
Atlantic Ocean ◽  
Mineral Dust ◽  
Sonic Anemometer ◽  
Dust Emission ◽  
Deposition Flux ◽  
Deposition Fluxes ◽  
Dust Transport ◽  
Northeast Atlantic ◽  
Average Value ◽  
Northeast Atlantic Ocean

Abstract. The aim of this study is to determine the mass deposition flux of mineral dust to the tropical northeast Atlantic Ocean at the Cape Verde Atmospheric Observatory (CVAO) on the island Sao Vicente for January 2009. Five different methods were applied to estimate the deposition flux, using different meteorological and microphysical measurements, remote sensing, and regional dust transport simulations. The set of observations comprises micrometeorological measurements with an ultra-sonic anemometer and profile measurements using 2-D anemometers at two different heights, and microphysical measurements of the size-resolved mass concentrations of mineral dust. In addition, the total mass concentration of mineral dust was derived from absorption photometer observations and passive sampling. The regional dust model COSMO-MUSCAT was used for simulations of dust emission and transport, including dry and wet deposition processes. The four observation-based methods yield a monthly average deposition flux of mineral dust of 12–29 ng m−2 s−1. The simulation results come close to the upper range of the measurements with an average value of 47 ng m−2 s−1. It is shown, that the mass deposition flux of mineral dust obtained by the combination of micrometeorological (ultra-sonic anemometer) and microphysical measurements (particle mass size distribution of mineral dust) is within 5% to modeled mass deposition fluxes when the mineral dust is relatively homogenously distributed over the investigated area.

scholarly journals Sensitivity of the WRF-Chem (V3.6.1) model to different dust emission parametrisation: assessment in the broader Mediterranean region

2017 ◽  
Vol 10 (8) ◽  
pp. 2925-2945 ◽  
Author(s):  
Emmanouil Flaounas ◽  
Vassiliki Kotroni ◽  
Konstantinos Lagouvardos ◽  
Martina Klose ◽  
Cyrille Flamant ◽  
...  
Keyword(s):  
North Africa ◽  
Eastern Mediterranean ◽  
Dust Emission ◽  
Model Performance ◽  
Dust Particles ◽  
Dust Transport ◽  
Dust Emissions ◽  
Extinction Coefficients ◽  
Airborne Measurements ◽  
Model Aerosol

Abstract. In this study we aim to assess the WRF-Chem model capacity to reproduce dust transport over the eastern Mediterranean. For this reason, we compare the model aerosol optical depth (AOD) outputs to observations, focusing on three key regions: North Africa, the Arabian Peninsula and the eastern Mediterranean. Three sets of four simulations have been performed for the 6-month period of spring and summer 2011. Each simulation set uses a different dust emission parametrisation and for each parametrisation, the dust emissions are multiplied with various coefficients in order to tune the model performance. Our assessment approach is performed across different spatial and temporal scales using AOD observations from satellites and ground-based stations, as well as from airborne measurements of aerosol extinction coefficients over the Sahara. Assessment over the entire domain and simulation period shows that the model presents temporal and spatial variability similar to observed AODs, regardless of the applied dust emission parametrisation. On the other hand, when focusing on specific regions, the model skill varies significantly. Tuning the model performance by applying a coefficient to dust emissions may reduce the model AOD bias over a region, but may increase it in other regions. In particular, the model was shown to realistically reproduce the major dust transport events over the eastern Mediterranean, but failed to capture the regional background AOD. Further comparison of the model simulations to airborne measurements of vertical profiles of extinction coefficients over North Africa suggests that the model realistically reproduces the total atmospheric column AOD. Finally, we discuss the model results in two sensitivity tests, where we included finer dust particles (less than 1 µm) and changed accordingly the dust bins' mass fraction.

Impact of surface roughness on dust occurrence frequency over arid regions

2021 ◽  
Author(s):  
Martina Klose ◽  
Carlos Pérez García-Pando ◽  
Paul Ginoux ◽  
Ron L. Miller
Keyword(s):  
Surface Roughness ◽  
Spatial Patterns ◽  
Arid Regions ◽  
Transport Model ◽  
Dust Emission ◽  
Occurrence Frequency ◽  
Dust Transport ◽  
Drag Partition ◽  
The Impact ◽  
Semi Arid

<p>Soil dust aerosol created by wind erosion of arid and semi-arid surfaces dominates climate effects over large areas of the Earth. To represent the dust cycle, Global Earth System Models (ESMs) typically prescribe preferential dust sources phenomenologically using empirical source scaling functions. While this approach has helped to compensate for a lack or inaccuracy of soil and surface input data to models, it potentially limits progress in the representation of the global dust cycle, because such strong empirical constraints make models less sensitive to parameters known to affect dust emission, and thus potentially insensitive to changes in climate. Here we investigate the link between surface roughness due to non-erodible elements such as vegetation, pebbles and rocks, and the spatial patterns of dust activity. Using two different satellite-based methods to represent roughness within an atmospheric dust transport model, we evaluate the impact of surface roughness on the spatial distribution of dust optical depth occurrence frequency observed from satellite by both reducing the atmospheric momentum available for particle entrainment and protecting the surface from dust emission. We test the variability of our results across conceptually different parameterizations of dust emission and drag partition. Our results suggest that the spatial patterns of dust activity are largely determined by surface roughness, not only in semi-arid, but also in arid regions, where green vegetation is sparse or absent. </p>

scholarly journals Microscale dynamics between dust and microorganisms in alpine snowpack

2021 ◽  
Author(s):  
Alison Thurston ◽  
Zoe Courville ◽  
Lauren Farnsworth ◽  
Ross Lieblappen ◽  
Shelby Rosten ◽  
...  
Keyword(s):  
Mechanical Properties ◽  
Dust Particles ◽  
Dust Deposition ◽  
Dust Transport ◽  
Source Regions ◽  
Chemical Signatures ◽  
Scale Properties ◽  
Bacteria And Fungi ◽  
The Impact ◽  
Snow Samples

Dust particles carry microbial and chemical signatures from source regions to deposition regions. Dust and its occupying microorganisms are incorporated into, and can alter, snowpack physical properties including snow structure and resultant radiative and mechanical properties that in turn affect larger-scale properties, including surrounding hydrology and maneuverability. Microorganisms attached to deposited dust maintain genetic evidence of source substrates and can be potentially used as bio-sensors. The objective of this study was to investigate the impact of dust-associated microbial deposition on snowpack and microstructure. As part of this effort, we characterized the microbial communities deposited through dust transport, examined dust provenance, and identified the microscale location and fate of dust within a changing snow matrix. We found dust characteristics varied with deposition event and that dust particles were generally embedded in the snow grains, with a small fraction of the dust particles residing on the exterior of the snow matrix. Dust deposition appears to retard expected late season snow grain growth. Both bacteria and fungi were identified in the collected snow samples.

scholarly journals The global dust cycle and uncertainty in CMIP5 (Coupled Model Intercomparison Project phase 5) models

2020 ◽  
Vol 20 (17) ◽  
pp. 10401-10425
Author(s):  
Chenglai Wu ◽  
Zhaohui Lin ◽  
Xiaohong Liu
Keyword(s):  
Wet Deposition ◽  
Climate Models ◽  
Dust Emission ◽  
Coupled Model ◽  
Dust Particles ◽  
Earth System ◽  
Model Intercomparison ◽  
Dust Deposition ◽  
The Earth ◽  
Intercomparison Project

Abstract. The dust cycle is an important component of the Earth system and has been implemented in climate models and Earth system models (ESMs). An assessment of the dust cycle in these models is vital to address their strengths and weaknesses in simulating dust aerosol and its interactions with the Earth system and enhance the future model developments. This study presents a comprehensive evaluation of the global dust cycle in 15 models participating in the fifth phase of the Coupled Model Intercomparison Project (CMIP5). The various models are compared with each other and with an aerosol reanalysis as well as station observations. The results show that the global dust emission in these models varies by a factor of 4–5 for the same size range. The models generally agree with each other and observations in reproducing the “dust belt”, which extends from North Africa, the Middle East, Central and South Asia to East Asia, although they differ greatly in the spatial extent of this dust belt. The models also differ in other dust source regions such as North America and Australia. We suggest that the coupling of dust emission with dynamic vegetation can enlarge the range of simulated dust emission. For the removal process, all the models estimate that wet deposition is smaller than dry deposition and wet deposition accounts for 12 %–39 % of total deposition. The models also estimate that most (77 %–91 %) dust particles are deposited onto continents and 9 %–23 % of dust particles are deposited into oceans. Compared to the observations, most models reproduce the dust deposition and dust concentrations within a factor of 10 at most stations, but larger biases by more than a factor of 10 are also noted at specific regions and for certain models. These results highlight the need for further improvements of the dust cycle especially on dust emission in climate models.

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