scholarly journals Global source attribution of sulfate concentration and direct and indirect radiative forcing

2017 ◽  
Vol 17 (14) ◽  
pp. 8903-8922 ◽  
Author(s):  
Yang Yang ◽  
Hailong Wang ◽  
Steven J. Smith ◽  
Richard Easter ◽  
Po-Lun Ma ◽  
...  
Keyword(s):  
Southern Hemisphere ◽  
Northern Hemisphere ◽  
Radiative Forcing ◽  
Dimethyl Sulfide ◽  
Sulfur Source ◽  
Atmospheric Conditions ◽  
So2 Emissions ◽  
Near Surface ◽  
Indirect Radiative Forcing ◽  
Global Source

Abstract. The global source–receptor relationships of sulfate concentrations, and direct and indirect radiative forcing (DRF and IRF) from 16 regions/sectors for years 2010–2014 are examined in this study through utilizing a sulfur source-tagging capability implemented in the Community Earth System Model (CESM) with winds nudged to reanalysis data. Sulfate concentrations are mostly contributed by local emissions in regions with high emissions, while over regions with relatively low SO2 emissions, the near-surface sulfate concentrations are primarily attributed to non-local sources from long-range transport. Regional source efficiencies of sulfate concentrations are higher over regions with dry atmospheric conditions and less export, suggesting that lifetime of aerosols, together with regional export, is important in determining regional air quality. The simulated global total sulfate DRF is −0.42 W m−2, with −0.31 W m−2 contributed by anthropogenic sulfate and −0.11 W m−2 contributed by natural sulfate, relative to a state with no sulfur emissions. In the Southern Hemisphere tropics, dimethyl sulfide (DMS) contributes 17–84 % to the total DRF. East Asia has the largest contribution of 20–30 % over the Northern Hemisphere mid- and high latitudes. A 20 % perturbation of sulfate and its precursor emissions gives a sulfate incremental IRF of −0.44 W m−2. DMS has the largest contribution, explaining −0.23 W m−2 of the global sulfate incremental IRF. Incremental IRF over regions in the Southern Hemisphere with low background aerosols is more sensitive to emission perturbation than that over the polluted Northern Hemisphere.

scholarly journals Global source attribution of sulfate concentration, direct and indirect radiative forcing

2017 ◽  
Author(s):  
Yang Yang ◽  
Hailong Wang ◽  
Steven J. Smith ◽  
Richard Easter ◽  
Po-Lun Ma ◽  
...  
Keyword(s):  
Southeast Asia ◽  
East Asia ◽  
South Asia ◽  
Central Asia ◽  
Southern Hemisphere ◽  
North Africa ◽  
Radiative Forcing ◽  
Sulfate Concentration ◽  
Near Surface ◽  
Indirect Radiative Forcing

Abstract. The global source-receptor relationships of sulfate concentration, direct and indirect radiative forcing (DRF and IRF) from sixteen regions/sectors for years 2010–2014 are examined in this study through utilizing a sulfur source-tagging capability implemented in the Community Earth System Model (CESM) with winds nudged to reanalysis data. Sulfate concentrations are mostly contributed by local emissions in regions with high emissions, while over regions with relatively low SO2 emissions, the near-surface sulfate concentrations are primarily attributed to non-local sources from long-range transport. The export of SO2 and sulfate from Europe contributes 16–20 % of near-surface sulfate concentrations over North Africa, Russia/Belarus/Ukraine (RBU) region and Central Asia. Sources from the Middle East account for 15–24 % of sulfate over North Africa, Southern Africa and Central Asia in winter and autumn, and 19 % over South Asia in spring. Sources in RBU account for 21–42 % of sulfate concentrations over Central Asia. East Asia accounts for about 50 % of sulfate over Southeast Asia in winter and autumn, 15 % over RBU in summer, and 11 % over North America in spring. South Asia contributes to 11–24 % of sulfate over Southeast Asia in winter and spring. Regional source efficiencies of sulfate concentrations are higher over regions with dry atmospheric conditions and less export, suggesting that lifetime of aerosols, together with regional export, is important in determining regional air quality. The simulated global total sulfate DRF is −0.42 W m−2, with  0.31 W m−2 contributed by anthropogenic sulfate and −0.11 W m−2 contributed by natural sulfate, relative to a state with no sulfur emissions. In the Southern Hemisphere tropics, dimethyl sulfide (DMS) contributes 17–84 % to the total DRF. East Asia has the largest contribution of 20–30 % over the Northern Hemisphere mid- and high-latitudes. A 20 % perturbation of sulfate and its precursor emissions gives a sulfate incremental IRF of −0.44 W m−2. DMS has the largest contribution, explaining −0.23 W m−2 of the global sulfate incremental IRF. Incremental IRF over regions in the Southern Hemisphere with low background aerosols is more sensitive to emission perturbation than those over the polluted Northern Hemisphere.

Rapid cloud removal of dimethyl sulfide oxidation products limits SO2 and cloud condensation nuclei production in the marine atmosphere

2021 ◽  
Vol 118 (42) ◽  
pp. e2110472118
Author(s):  
Gordon A. Novak ◽  
Charles H. Fite ◽  
Christopher D. Holmes ◽  
Patrick R. Veres ◽  
J. Andrew Neuman ◽  
...  
Keyword(s):  
Radiative Forcing ◽  
Dimethyl Sulfide ◽  
Cloud Condensation Nuclei ◽  
Sulfide Oxidation ◽  
Radiation Balance ◽  
Marine Atmosphere ◽  
Condensation Nuclei ◽  
Near Surface ◽  
Loss Process ◽  
The Impact

Oceans emit large quantities of dimethyl sulfide (DMS) to the marine atmosphere. The oxidation of DMS leads to the formation and growth of cloud condensation nuclei (CCN) with consequent effects on Earth’s radiation balance and climate. The quantitative assessment of the impact of DMS emissions on CCN concentrations necessitates a detailed description of the oxidation of DMS in the presence of existing aerosol particles and clouds. In the unpolluted marine atmosphere, DMS is efficiently oxidized to hydroperoxymethyl thioformate (HPMTF), a stable intermediate in the chemical trajectory toward sulfur dioxide (SO2) and ultimately sulfate aerosol. Using direct airborne flux measurements, we demonstrate that the irreversible loss of HPMTF to clouds in the marine boundary layer determines the HPMTF lifetime (τHPMTF < 2 h) and terminates DMS oxidation to SO2. When accounting for HPMTF cloud loss in a global chemical transport model, we show that SO2 production from DMS is reduced by 35% globally and near-surface (0 to 3 km) SO2 concentrations over the ocean are lowered by 24%. This large, previously unconsidered loss process for volatile sulfur accelerates the timescale for the conversion of DMS to sulfate while limiting new particle formation in the marine atmosphere and changing the dynamics of aerosol growth. This loss process potentially reduces the spatial scale over which DMS emissions contribute to aerosol production and growth and weakens the link between DMS emission and marine CCN production with subsequent implications for cloud formation, radiative forcing, and climate.

scholarly journals Daily, Global, High-Resolution SST and Sea Ice Reanalysis for 1985–2007 Using the OSTIA System

2012 ◽  
Vol 25 (18) ◽  
pp. 6215-6232 ◽  
Author(s):  
Jonah Roberts-Jones ◽  
Emma Kathleen Fiedler ◽  
Matthew James Martin
Keyword(s):  
High Resolution ◽  
Sea Ice ◽  
Southern Hemisphere ◽  
Northern Hemisphere ◽  
Optimal Interpolation ◽  
In Situ Observation ◽  
High Latitudes ◽  
Sea Ice Concentration ◽  
Near Surface

Abstract A sea surface temperature (SST) and sea ice reanalysis has been produced at the Met Office based on the Operational SST and Sea Ice Analysis (OSTIA) system. The OSTIA reanalysis produces daily, high-resolution, global foundation SST and sea ice concentration fields from 1 January 1985 to 31 December 2007. The SST reanalysis uses reprocessed satellite and in situ observations that are assimilated using a multiscale optimal-interpolation-type scheme similar to that used in the near-real-time OSTIA system. Validation of the SST analysis using assimilated in situ observation-minus-background statistics shows that the accuracy of the analysis increases throughout the reanalysis period; the global root-mean-square difference is approximately 0.50 K by 2007. This approach to validation is supported in the recent period by results from comparisons with independent near-surface Argo data against which a global standard deviation error of 0.55 K was calculated. Assessment of the OSTIA reanalysis at high latitudes demonstrates that the SST and sea ice fields are more consistent with one another in the Southern Hemisphere than in the Northern Hemisphere. Comparison of the sea ice extents to those in a similar reanalysis shows OSTIA to have larger extents in the Northern Hemisphere, and the Southern Hemisphere extents are similar. The OSTIA reanalysis SSTs are shown to be regionally comparable with similar reanalyses, with the largest differences occurring at high latitudes in the summer hemisphere. Differences are observed around the ice edge and in regions with high SST gradients. The OSTIA reanalysis provides a valuable high-resolution addition to the satellite period SST data record that makes use of the (Advanced) Along-Track Scanning Radiometer [(A)ATSR] multimission data.

scholarly journals The Effects of the Spatial Distribution of Direct Anthropogenic Aerosols Radiative Forcing on Atmospheric Circulation

2018 ◽  
Vol 31 (17) ◽  
pp. 7129-7145 ◽  
Author(s):  
Rei Chemke ◽  
Guy Dagan
Keyword(s):  
Spatial Distribution ◽  
Atmospheric Circulation ◽  
Southern Hemisphere ◽  
Northern Hemisphere ◽  
Radiative Forcing ◽  
General Circulation ◽  
Circulation Model ◽  
Hadley Cell ◽  
Global Circulation Model ◽  
Anthropogenic Aerosols

The large uncertainty in estimating the global aerosol radiative forcing (ARF) is one of the major challenges the climate community faces for climate projection. While the global-mean ARF may affect global quantities such as surface temperature, its spatial distribution may result in local thermodynamical and, thus, dynamical changes. Future changes in aerosol emissions distribution could further modulate the atmospheric circulation. Here, the effects of the spatial distribution of the direct anthropogenic ARF are studied using an idealized global circulation model, forced by a range of estimated-ARF amplitudes, based on the Copernicus Atmosphere Monitoring Service data. The spatial distribution of the estimated-ARF is globally decomposed, and the effects of the different modes on the circulation are studied. The most dominant spatial distribution feature is the cooling of the Northern Hemisphere in comparison to the Southern Hemisphere. This induces a negative meridional temperature gradient around the equator, which modulates the mean fields in the tropics. The ITCZ weakens and shifts southward, and the Northern (Southern) Hemisphere Hadley cell strengthens (weakens). The localization of the ARF in the Northern Hemisphere midlatitudes shifts the subtropical jet poleward and strengthens both the eddy-driven jet and Ferrel cell, because of the weakening of high-latitude eddy fluxes. Finally, the larger aerosol concentration in Asia compared to North America results in an equatorial superrotating jet. Understanding the effects of the different modes on the general circulation may help elucidate the circulation’s future response to the projected changes in ARF distribution.

Alpha-Effect, Current and Kinetic Helicities for Magnetically Driven Turbulence, and Solar Dynamo

2000 ◽  
Vol 179 ◽  
pp. 387-388
Author(s):  
Gaetano Belvedere ◽  
V. V. Pipin ◽  
G. Rüdiger
Keyword(s):  
Southern Hemisphere ◽  
Northern Hemisphere ◽  
Convection Zone ◽  
Solar Surface ◽  
Momentum Transport ◽  
Angular Momentum Transport ◽  
Magnetic Buoyancy ◽  
Alpha Effect ◽  
Current Helicity

Extended AbstractRecent numerical simulations lead to the result that turbulence is much more magnetically driven than believed. In particular the role ofmagnetic buoyancyappears quite important for the generation ofα-effect and angular momentum transport (Brandenburg &amp; Schmitt 1998). We present results obtained for a turbulence field driven by a (given) Lorentz force in a non-stratified but rotating convection zone. The main result confirms the numerical findings of Brandenburg &amp; Schmitt that in the northern hemisphere theα-effect and the kinetic helicityℋkin= 〈u′ · rotu′〉 are positive (and negative in the northern hemisphere), this being just opposite to what occurs for the current helicityℋcurr= 〈j′ ·B′〉, which is negative in the northern hemisphere (and positive in the southern hemisphere). There has been an increasing number of papers presenting observations of current helicity at the solar surface, all showing that it isnegativein the northern hemisphere and positive in the southern hemisphere (see Rüdigeret al. 2000, also for a review).

The Hemispheric Sign Rule of Current Helicity during the Rising Phase of Cycle 23

2000 ◽  
Vol 179 ◽  
pp. 303-306
Author(s):  
S. D. Bao ◽  
G. X. Ai ◽  
H. Q. Zhang
Keyword(s):  
Solar Cycle ◽  
Southern Hemisphere ◽  
Northern Hemisphere ◽  
Active Regions ◽  
Hemispheric Preference ◽  
Current Helicity

AbstractWe compute the signs of two different current helicity parameters (i.e., αbestandHc) for 87 active regions during the rise of cycle 23. The results indicate that 59% of the active regions in the northern hemisphere have negative αbestand 65% in the southern hemisphere have positive. This is consistent with that of the cycle 22. However, the helicity parameterHcshows a weaker opposite hemispheric preference in the new solar cycle. Possible reasons are discussed.

scholarly journals Improved estimates of preindustrial biomass burning reduce the magnitude of aerosol climate forcing in the Southern Hemisphere

2021 ◽  
Vol 7 (22) ◽  
pp. eabc1379
Author(s):  
Pengfei Liu ◽  
Jed O. Kaplan ◽  
Loretta J. Mickley ◽  
Yang Li ◽  
Nathan J. Chellman ◽  
...  
Keyword(s):  
Southern Hemisphere ◽  
Radiative Forcing ◽  
Ice Core ◽  
Ice Cores ◽  
Terrestrial Ecosystems ◽  
Rapid Expansion ◽  
Past Century ◽  
Fire Emissions ◽  
The Past ◽  
Fire Activity

Fire plays a pivotal role in shaping terrestrial ecosystems and the chemical composition of the atmosphere and thus influences Earth’s climate. The trend and magnitude of fire activity over the past few centuries are controversial, which hinders understanding of preindustrial to present-day aerosol radiative forcing. Here, we present evidence from records of 14 Antarctic ice cores and 1 central Andean ice core, suggesting that historical fire activity in the Southern Hemisphere (SH) exceeded present-day levels. To understand this observation, we use a global fire model to show that overall SH fire emissions could have declined by 30% over the 20th century, possibly because of the rapid expansion of land use for agriculture and animal production in middle to high latitudes. Radiative forcing calculations suggest that the decreasing trend in SH fire emissions over the past century largely compensates for the cooling effect of increasing aerosols from fossil fuel and biofuel sources.

scholarly journals First results of low frequency electromagnetic wave detector of TC-2/Double Star program

2005 ◽  
Vol 23 (8) ◽  
pp. 2803-2811 ◽  
Author(s):  
J. B. Cao ◽  
Z. X. Liu ◽  
J. Y. Yang ◽  
C. X. Yian ◽  
Z. G. Wang ◽  
...  
Keyword(s):  
Electromagnetic Wave ◽  
Southern Hemisphere ◽  
Northern Hemisphere ◽  
Geomagnetic Storms ◽  
Low Frequency ◽  
Wave Detector ◽  
Ion Cyclotron Waves ◽  
Satellite Platform ◽  
Ion Cyclotron ◽  
First Results

Abstract. LFEW is a low frequency electromagnetic wave detector mounted on TC-2, which can measure the magnetic fluctuation of low frequency electromagnetic waves. The frequency range is 8 Hz to 10 kHz. LFEW comprises a boom-mounted, three-axis search coil magnetometer, a preamplifier and an electronics box that houses a Digital Spectrum Analyzer. LFEW was calibrated at Chambon-la-Forêt in France. The ground calibration results show that the performance of LFEW is similar to that of STAFF on TC-1. The first results of LFEW show that it works normally on board, and that the AC magnetic interference of the satellite platform is very small. In the plasmasphere, LFEW observed the ion cyclotron waves. During the geomagnetic storm on 8 November 2004, LFEW observed a wave burst associated with the oxygen ion cyclotron waves. This observation shows that during geomagnetic storms, the oxygen ions are very active in the inner magnetosphere. Outside the plasmasphere, LFEW observed the chorus on 3 November 2004. LFEW also observed the plasmaspheric hiss and mid-latitude hiss both in the Southern Hemisphere and Northern Hemisphere on 8 November 2004. The hiss in the Southern Hemisphere may be the reflected waves of the hiss in the Northern Hemisphere.

Sign in / Sign up

Export Citation Format

Share Document