scholarly journals Spatiotemporal variability and contribution of different aerosol types to the Aerosol Optical Depth over the Eastern Mediterranean

2016 ◽  
Author(s):  
Aristeidis K. Georgoulias ◽  
Georgia Alexandri ◽  
Konstantinos A. Kourtidis ◽  
Jos Lelieveld ◽  
Prodromos Zanis ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Eastern Mediterranean ◽  
Spatiotemporal Variability ◽  
Marine Aerosols ◽  
Anthropogenic Aerosols ◽  
Relative Contribution ◽  
Fine Mode ◽  
Natural Aerosols ◽  
Aerosol Types

Abstract. This study characterizes the spatiotemporal variability and relative contribution of different types of aerosols to the Aerosol Optical Depth (AOD) over the Eastern Mediterranean as derived from MODIS Terra (3/2000–12/2012) and Aqua (7/2002–12/2012) satellite instruments. For this purpose, a 0.1°×0.1° gridded MODIS dataset was compiled and validated against AERONET sunphotometric observations. The high spatial resolution and long temporal coverage of the dataset allows for the determination of local hot spots like megacities, medium sized cities, industrial zones, and power plant complexes, seasonal variabilities, and decadal averages. The average AOD at 550 nm (AOD550) for the entire region is ~ 0.22 ± 0.19 with maximum values in summer and seasonal variabilities that can be attributed to precipitation, photochemical production of secondary organic aerosols, transport of pollution and smoke from biomass burning in Central and Eastern Europe, and transport of dust from the Sahara Desert and the Middle East. The MODIS data were analyzed together with data from other satellite sensors, reanalysis projects and a chemistry-aerosol-transport model using an optimized algorithm tailored for the region and capable of estimating the contribution of different aerosol types to the total AOD550. The spatial and temporal variability of anthropogenic, dust and fine mode natural aerosols over land and anthropogenic, dust and marine aerosols over the sea is examined. The relative contribution of the different aerosol types to the total AOD550 exhibits a low/high seasonal variability over land/oceanic areas, respectively. Overall, anthropogenic aerosols, dust and fine mode natural aerosols account for ~ 51 %, ~ 34 % and ~ 15 % of the total AOD550 over land, while, anthropogenic aerosols, dust and marine aerosols account ~ 40 %, ~ 34 % and ~ 26 % of the total AOD550 over the sea, based on MODIS Terra and Aqua observations.

scholarly journals Spatiotemporal variability and contribution of different aerosol types to the aerosol optical depth over the Eastern Mediterranean

2016 ◽  
Vol 16 (21) ◽  
pp. 13853-13884 ◽  
Author(s):  
Aristeidis K. Georgoulias ◽  
Georgia Alexandri ◽  
Konstantinos A. Kourtidis ◽  
Jos Lelieveld ◽  
Prodromos Zanis ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Eastern Mediterranean ◽  
Spatiotemporal Variability ◽  
Marine Aerosols ◽  
Anthropogenic Aerosols ◽  
Relative Contribution ◽  
Fine Mode ◽  
Natural Aerosols ◽  
Aerosol Types

Abstract. This study characterizes the spatiotemporal variability and relative contribution of different types of aerosols to the aerosol optical depth (AOD) over the Eastern Mediterranean as derived from MODIS (Moderate Resolution Imaging Spectroradiometer) Terra (March 2000–December 2012) and Aqua (July 2002–December 2012) satellite instruments. For this purpose, a 0.1° × 0.1° gridded MODIS dataset was compiled and validated against sun photometric observations from the AErosol RObotic NETwork (AERONET). The high spatial resolution and long temporal coverage of the dataset allows for the determination of local hot spots like megacities, medium-sized cities, industrial zones and power plant complexes, seasonal variabilities and decadal averages. The average AOD at 550 nm (AOD550) for the entire region is ∼ 0.22 ± 0.19, with maximum values in summer and seasonal variabilities that can be attributed to precipitation, photochemical production of secondary organic aerosols, transport of pollution and smoke from biomass burning in central and eastern Europe and transport of dust from the Sahara and the Middle East. The MODIS data were analyzed together with data from other satellite sensors, reanalysis projects and a chemistry–aerosol-transport model using an optimized algorithm tailored for the region and capable of estimating the contribution of different aerosol types to the total AOD550. The spatial and temporal variability of anthropogenic, dust and fine-mode natural aerosols over land and anthropogenic, dust and marine aerosols over the sea is examined. The relative contribution of the different aerosol types to the total AOD550 exhibits a low/high seasonal variability over land/sea areas, respectively. Overall, anthropogenic aerosols, dust and fine-mode natural aerosols account for ∼ 51, ∼ 34 and ∼ 15 % of the total AOD550 over land, while, anthropogenic aerosols, dust and marine aerosols account ∼ 40, ∼ 34 and ∼ 26 % of the total AOD550 over the sea, based on MODIS Terra and Aqua observations.

scholarly journals Retrieval of the Fine-Mode Aerosol Optical Depth over East China Using a Grouped Residual Error Sorting (GRES) Method from Multi-Angle and Polarized Satellite Data

2018 ◽  
Vol 10 (11) ◽  
pp. 1838 ◽  
Author(s):  
Yang Zhang ◽  
Zhengqiang Li ◽  
Zhihong Liu ◽  
Juan Zhang ◽  
Lili Qie ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Residual Error ◽  
East China ◽  
Anthropogenic Aerosols ◽  
Aerosol Model ◽  
Retrieval Accuracy ◽  
Aerosol Loading ◽  
Fine Mode ◽  
Fine Mode Aerosol

The fine-mode aerosol optical depth (AODf) is an important parameter for the environment and climate change study, which mainly represents the anthropogenic aerosols component. The Polarization and Anisotropy of Reflectances for Atmospheric Science coupled with Observations from a Lidar (PARASOL) instrument can detect polarized signal from multi-angle observation and the polarized signal mainly comes from the radiation contribution of the fine-mode aerosols, which provides an opportunity to obtain AODf directly. However, the currently operational algorithm of Laboratoire d’Optique Atmosphérique (LOA) has a poor AODf retrieval accuracy over East China on high aerosol loading days. This study focused on solving this issue and proposed a grouped residual error sorting (GRES) method to determine the optimal aerosol model in AODf retrieval using the traditional look-up table (LUT) approach and then the AODf retrieval accuracy over East China was improved. The comparisons between the GRES retrieved and the Aerosol Robotic Network (AERONET) ground-based AODf at Beijing, Xianghe, Taihu and Hong_Kong_PolyU sites produced high correlation coefficients (r) of 0.900, 0.933, 0.957 and 0.968, respectively. The comparisons of the GRES retrieved AODf and PARASOL AODf product with those of the AERONET observations produced a mean absolute error (MAE) of 0.054 versus 0.104 on high aerosol loading days (AERONET mean AODf at 865 nm = 0.283). An application using the GRES method for total AOD (AODt) retrieval also showed a good expandability for multi-angle aerosol retrieval of this method.

scholarly journals High temporal resolution estimates of columnar aerosol microphysical parameters from spectrum of aerosol optical depth by linear estimation: application to long-term AERONET and star-photometry measurements

2015 ◽  
Vol 8 (8) ◽  
pp. 3117-3133 ◽  
Author(s):  
D. Pérez-Ramírez ◽  
I. Veselovskii ◽  
D. N. Whiteman ◽  
A. Suvorina ◽  
M. Korenskiy ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Temporal Resolution ◽  
High Temporal Resolution ◽  
Linear Estimation ◽  
Night Time ◽  
Microphysical Properties ◽  
Fine Mode ◽  
Using Data ◽  
Aerosol Types

Abstract. This work deals with the applicability of the linear estimation technique (LE) to invert spectral measurements of aerosol optical depth (AOD) provided by AERONET CIMEL sun photometers. The inversion of particle properties using only direct-sun AODs allows the evaluation of parameters such as effective radius (reff) and columnar volume aerosol content (V) with significantly better temporal resolution than the operational AERONET algorithm which requires both direct sun and sky radiance measurements. Sensitivity studies performed demonstrate that the constraints on the range of the inversion are very important to minimize the uncertainties, and therefore estimates of reff can be obtained with uncertainties less than 30 % and of V with uncertainties below 40 %. The LE technique is applied to data acquired at five AERONET sites influenced by different aerosol types and the retrievals are compared with the results of the operational AERONET code. Good agreement between the two techniques is obtained when the fine mode predominates, while for coarse mode cases the LE results systematically underestimate both reff and V. The highest differences are found for cases where no mode predominates. To minimize these biases, correction functions are developed using the multi-year database of observations at selected sites, where the AERONET retrieval is used as the reference. The derived corrections are tested using data from 18 other AERONET stations offering a range of aerosol types. After correction, the LE retrievals provide better agreement with AERONET for all the sites considered. Finally, the LE approach developed here is applied to AERONET and star-photometry measurements in the city of Granada (Spain) to obtain day-to-night time evolution of columnar aerosol microphysical properties.

scholarly journals High temporal resolution estimates of columnar aerosol microphysical parameters from spectrum of aerosol optical depth by Linear Estimation: application to long-term AERONET and Star-photometry measurements

2015 ◽  
Vol 8 (3) ◽  
pp. 2331-2378
Author(s):  
D. Pérez-Ramírez ◽  
I. Veselovskii ◽  
D. N. Whiteman ◽  
A. Suvorina ◽  
M. Korenskiy ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Temporal Resolution ◽  
High Temporal Resolution ◽  
Linear Estimation ◽  
Night Time ◽  
Microphysical Properties ◽  
Fine Mode ◽  
Using Data ◽  
Aerosol Types

Abstract. This work deals with the applicability of the Linear Estimation technique (LE) to invert spectral measurements of aerosol optical depth (AOD) provided by AERONET CIMEL sun-photometers. The inversion of particle properties using only direct sun AODs allows the evaluation of parameters such as effective radius (reff) and columnar volume aerosol content (V) with significantly better temporal resolution than the operational AERONET algorithm which requires both direct sun and sky radiance measurements. Sensitivity studies performed demonstrate that the constraints on the range of the inversion are very important to minimize the uncertainties, and therefore estimates of reff can be obtained with uncertainties less than 30% and of V with uncertainties below 40%. The LE technique is applied to data acquired at five AERONET sites influenced by different aerosol types and the retrievals are compared with the results of the operational AERONET code. Good agreement between the two techniques is obtained when the fine mode predominates, while for coarse mode cases the LE results systematically underestimate both reff and V. The highest differences are found for cases where no mode predominates. To minimize these biases, correction functions are developed using the multi-year database of observations at selected sites, where the AERONET retrieval is used as the reference. The derived corrections are tested using data from 18 other AERONET stations offering a range of aerosol types. After correction, the LE retrievals provide better agreement with AERONET for all the sites considered. Finally, the LE approach developed here is applied to AERONET and star-photometry measurements at the city of Granada (Spain) to obtain day-to-night time-evolution of columnar aerosol microphysical properties.

scholarly journals Airborne observation during KORUS-AQ show aerosol optical depth are more spatially self-consistent than aerosol intensive properties

2022 ◽  
Author(s):  
Samuel E. LeBlanc ◽  
Michal Segal-Rozenhaimer ◽  
Jens Redemann ◽  
Connor J. Flynn ◽  
Roy R. Johnson ◽  
...  
Keyword(s):  
Air Quality ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Temporal Variability ◽  
Spatial Scales ◽  
Aerosol Emission ◽  
Fine Mode ◽  
Predominant Factor ◽  
Spatio Temporal ◽  
Microphysical Processes

Abstract. Aerosol particles can be emitted, transported, removed, or transformed, leading to aerosol variability at scales impacting the climate (days to years and over hundreds of kilometers) or the air quality (hours to days and from meters to hundreds of kilometers). We present the temporal and spatial scales of changes in AOD (Aerosol Optical Depth), and aerosol size (using Angstrom Exponent; AE, and Fine-Mode-Fraction; FMF) over Korea during the 2016 KORUS-AQ (KORea-US Air Quality) atmospheric experiment. We use measurements and retrievals of aerosol optical properties from airborne instruments for remote sensing (4STAR; Spectrometers for Sky-Scanning Sun Tracking Atmospheric Research) and in situ (LARGE; NASA Langley Aerosol Research Group Experiment) on board the NASA DC-8, geostationary satellite (GOCI; Geostationary Ocean Color Imager; Yonsei aerosol retrieval (YAER) version 2) and reanalysis (MERRA-2; Modern-Era Retrospective Analysis for Research and Applications, version 2). Measurements from 4STAR when flying below 500 m, show an average AOD at 501 nm of 0.43 and an average AE of 1.15 with large standard deviation (0.32 and 0.26 for AOD and AE respectively) likely due to mixing of different aerosol types (fine and coarse mode). The majority of AODs due to fine mode aerosol is observed at altitudes lower than 2 km. Even though there are large variations, for 18 out of the 20 flight days, the column AOD measurements by 4STAR along the NASA DC-8 flight trajectories matches the south-Korean regional average derived from GOCI. We also observed that, contrary to prevalent understanding, AE and FMF are more spatially variable than AOD during KORUS-AQ, even when accounting for potential sampling biases by using Monte Carlo resampling. Averaging between measurements and model for the entire KORUS-AQ period, a reduction in correlation by 15 % is 65.0 km for AOD and shorter at 22.7 km for AE. While there are observational and model differences, the predominant factor influencing spatial-temporal homogeneity is the meteorological period. High spatio-temporal variability occur during the dynamic period (25–31 May), and low spatio-temporal variability occur during blocking Rex pattern (01–07 June). The changes in spatial variability scales between AOD and FMF/AE, while inter-related, indicate that microphysical processes that impact mostly the dominant aerosol size, like aerosol particle formation, growth, and coagulation, vary at shorter scales than the aerosol concentration processes that mostly impact AOD, like aerosol emission, transport, and removal.

scholarly journals Assessment of tropospheric CALIPSO Version 4.2 aerosol types over the ocean using independent CALIPSO-SODA lidar ratios

2021 ◽  
Author(s):  
Zhujun Li ◽  
David Painemal ◽  
Gregory Schuster ◽  
Marian Clayton ◽  
Richard Ferrare ◽  
...  
Keyword(s):  
Optical Depth ◽  
Classification Scheme ◽  
Signal To Noise Ratio ◽  
Open Ocean ◽  
African Continent ◽  
Marine Aerosols ◽  
Lidar Ratio ◽  
Aerosol Plume ◽  
Aerosol Types ◽  
Aerosol Type

Abstract. We assess the CALIPSO Version 4.2 (V4) aerosol typing and assigned lidar ratios over ocean using aerosol optical depth (AOD) retrievals from the Synergized Optical Depth of Aerosols (SODA) algorithm and retrieved columnar lidar ratio estimated by combining SODA AOD and CALIPSO attenuated backscatter (CALIPSO-SODA). Six aerosol types – clean marine, dusty marine, dust, polluted continental/smoke, polluted dust, and elevated smoke – are characterized using CALIPSO-SODA over ocean and the results are compared against the prescribed V4 lidar ratios, when only one aerosol type is present in the atmospheric column. For samples detected at 5-km or 20-km spatial resolutions and having AOD > 0.05, the CALIPSO-SODA lidar ratios are significantly different between different aerosol types, and are consistent with the type-specific values assigned in V4 to within 10 sr (except for polluted continental/smoke). This implies that the CALIPSO classification scheme generally categorizes aerosols correctly. We find remarkable daytime/nighttime regional agreement for clean marine aerosol over the open ocean (CALIPSO-SODA = 20–25 sr, V4 = 23 sr), elevated smoke over the southeast Atlantic (CALIPSO-SODA = 65–75 sr, V4 = 70 sr), and dust over the subtropical Atlantic adjacent to the African continent (CALIPSO-SODA = 40–50 sr, V4 = 44 sr). In contrast, daytime polluted continental/smoke lidar ratio is more than 20 sr smaller than the constant V4 vaue for that type, attributed in part to the challenge of classifying tenuous aerosol with low signal-to-noise ratio. Dust over most of the Atlantic Ocean features CALIPSO-SODA lidar ratios less than 40 sr, possibly suggesting the presence of dust mixed with marine aerosols or lidar ratio values that depend on source and evolution of the aerosol plume. The new dusty marine type introduced in V4 features similar magnitudes and spatial distribution as its clean marine counterpart with lidar ratio differences of less than 3 sr, and nearly identical values over the open ocean, implying that some modification of the classification scheme for the marine subtypes is warranted.

scholarly journals Using the OMI Aerosol Index and Absorption Aerosol Optical Depth to evaluate the NASA MERRA Aerosol Reanalysis

2014 ◽  
Vol 14 (23) ◽  
pp. 32177-32231 ◽  
Author(s):  
V. Buchard ◽  
A. M. da Silva ◽  
P. R. Colarco ◽  
A. Darmenov ◽  
C. A. Randles ◽  
...  
Keyword(s):  
Optical Properties ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Biomass Burning ◽  
Saharan Dust ◽  
Aerosol Layer ◽  
Anthropogenic Aerosols ◽  
Aerosol Absorption ◽  
Modis Aod ◽  
Aerosol Index

Abstract. A radiative transfer interface has been developed to simulate the UV Aerosol Index (AI) from the NASA Goddard Earth Observing System version 5 (GEOS-5) aerosol assimilated fields. The purpose of this work is to use the AI and Aerosol Absorption Optical Depth (AAOD) derived from the Ozone Monitoring Instrument (OMI) measurements as independent validation for the Modern Era Retrospective analysis for Research and Applications Aerosol Reanalysis (MERRAero). MERRAero is based on a version of the GEOS-5 model that is radiatively coupled to the Goddard Chemistry, Aerosol, Radiation, and Transport (GOCART) aerosol module and includes assimilation of Aerosol Optical Depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor. Since AI is dependent on aerosol concentration, optical properties and altitude of the aerosol layer, we make use of complementary observations to fully diagnose the model, including AOD from the Multi-angle Imaging SpectroRadiometer (MISR), aerosol retrievals from the Aerosol Robotic Network (AERONET) and attenuated backscatter coefficients from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) mission to ascertain potential misplacement of plume height by the model. By sampling dust, biomass burning and pollution events in 2007 we have compared model produced AI and AAOD with the corresponding OMI products, identifying regions where the model representation of absorbing aerosols was deficient. As a result of this study over the Saharan dust region, we have obtained a new set of dust aerosol optical properties that retains consistency with the MODIS AOD data that were assimilated, while resulting in better agreement with aerosol absorption measurements from OMI. The analysis conducted over the South African and South American biomass burning regions indicates that revising the spectrally-dependent aerosol absorption properties in the near-UV region improves the modeled-observed AI comparisons. Finally, during a period where the Asian region was mainly dominated by anthropogenic aerosols, we have performed a qualitative analysis in which the specification of anthropogenic emissions in GEOS-5 is adjusted to provide insight into discrepancies observed in AI comparisons.

scholarly journals The potential of elastic and polarization lidars to retrieve extinction profiles

2020 ◽  
Vol 13 (2) ◽  
pp. 893-905 ◽  
Author(s):  
Elina Giannakaki ◽  
Panos Kokkalis ◽  
Eleni Marinou ◽  
Nikolaos S. Bartsotas ◽  
Vassilis Amiridis ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Dust Particles ◽  
Depolarization Ratio ◽  
Lidar System ◽  
Lidar Measurements ◽  
Lidar Ratio ◽  
Linear Depolarization Ratio ◽  
Aerosol Types ◽  
532 Nm

Abstract. A new method, called ElEx (elastic extinction), is proposed for the estimation of extinction coefficient lidar profiles using only the information provided by the elastic and polarization channels of a lidar system. The method is applicable to lidar measurements both during daytime and nighttime under well-defined aerosol mixtures. ElEx uses the particle backscatter profiles at 532 nm and the vertically resolved particle linear depolarization ratio measurements at the same wavelength. The particle linear depolarization ratio and the lidar ratio values of pure aerosol types are also taken from literature. The total extinction profile is then estimated and compared well with Raman retrievals. In this study, ElEx was applied in an aerosol mixture of marine and dust particles at Finokalia station during the CHARADMExp campaign. Any difference between ElEx and Raman extinction profiles indicates that the nondust component could be probably attributed to polluted marine or polluted continental aerosols. Comparison with sun photometer aerosol optical depth observations is performed as well during daytime. Differences in the total aerosol optical depth are varying between 1.2 % and 72 %, and these differences are attributed to the limited ability of the lidar to correctly represent the aerosol optical properties in the near range due to the overlap problem.

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