Value-added by high-resolution regional simulations of climate-relevant aerosol properties
Abstract. Despite recent advances in global Earth System Models (ESMs), the current global mean aerosol direct and indirect radiative effects remain uncertain, as does their future role in climate forcing and regional manifestations. Reasons for this uncertainty include the high spatio-temporal variability of aerosol populations. Thus, limited area (regional) models applied at higher resolution over specific regions of interest are generally expected to "add value", i.e. improve the fidelity of the physical-dynamical-chemical processes that induce extreme events and dictate climate forcing, via more realistic representation of spatio-temporal variability. However, added value is not inevitable, and there remains a need to optimize use of numerical resources, and to quantify the impact on simulation fidelity that derives from increased resolution. Here we quantify the value added by enhanced spatial resolution in simulations of the drivers of aerosol direct radiative forcing by applying the Weather Research and Forecasting model with coupled Chemistry (WRF-Chem) over eastern North America at different resolutions. Using Brier Skill Scores and other statistical metrics it is shown that enhanced resolution (from 60 to 12 km) improves model performance for all of the meteorological parameters and gas phase concentrations considered, in addition to both mean and extreme Aerosol Optical Depth (AOD) in three wavelengths in the visible relative to satellite observations, principally via increase of potential skill. Some of the enhanced model performance for AOD appears to be attributable to improved simulation of specific humidity and the resulting impact on aerosol hygroscopic growth/hysteresis.