Black carbon aerosol reductions during COVID-19 confinement quantified by aircraft measurements over Europe

The abrupt reduction in human activities during the first lockdown of the COVID-19 pandemic created unprecedented atmospheric conditions. To quantify the changes in lower tropospheric air pollution, we conducted the BLUESKY aircraft campaign and measured vertical profiles of black carbon (BC) aerosol particles over Western and Southern Europe in May and June 2020. We compared the results to similar measurements of the EMeRGe EU campaign performed in July 2017 and found that the BC mass concentrations (MBC) were reduced by about 47 %. For BC particle number concentrations, we found comparable reductions. Based on EMAC chemistry-transport model simulations, we find differences in meteorological conditions and flight patterns responsible for about 7 % of the reductions in MBC, whereas 40 % can be attributed to reduced anthropogenic emissions. Our results reflect the strong and immediate positive effect of changes in human activities on air quality and the atmospheric role of BC aerosols as a major air pollutant and climate forcing agent in the Anthropocene.

A probabilistic framework for quantifying the role of anthropogenic climate change in marine-terminating glacier retreats

Many marine-terminating outlet glaciers have retreated rapidly in recent decades, but these changes have not been formally attributed to anthropogenic climate change. A key challenge for such an attribution assessment is that if glacier termini are sufficiently perturbed from bathymetric highs, ice-dynamic feedbacks can cause rapid retreat even without further climate forcing. In the presence of internal climate variability, attribution thus depends on understanding whether (or how frequently) these rapid retreats could be triggered by climatic noise alone. Our simulations with idealized glaciers show that in a noisy climate, rapid retreat is a stochastic phenomenon. We therefore propose a probabilistic approach to attribution and present a framework for analysis that uses ensembles of many simulations with independent realizations of random climate variability. Synthetic experiments show that century-scale climate trends substantially increase the likelihood of rapid glacier retreat. This effect depends on the timescales over which ice dynamics integrate forcing. For a population of synthetic glaciers with different topographies, we find that external trends increase the number of large retreats triggered within the population, offering a metric for regional attribution. Our analyses suggest that formal attribution studies are tractable and should be further pursued to clarify the human role in recent ice-sheet change. We emphasize that early-industrial-era constraints on glacier and climate state are likely to be crucial for such studies.

Modeled and observed properties related to the direct aerosol radiative effect of biomass burning aerosol over the southeastern Atlantic

Biomass burning smoke is advected over the southeastern Atlantic Ocean between July and October of each year. This smoke plume overlies and mixes into a region of persistent low marine clouds. Model calculations of climate forcing by this plume vary significantly in both magnitude and sign. NASA EVS-2 (Earth Venture Suborbital-2) ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) had deployments for field campaigns off the west coast of Africa in 3 consecutive years (September 2016, August 2017, and October 2018) with the goal of better characterizing this plume as a function of the monthly evolution by measuring the parameters necessary to calculate the direct aerosol radiative effect. Here, this dataset and satellite retrievals of cloud properties are used to test the representation of the smoke plume and the underlying cloud layer in two regional models (WRF-CAM5 and CNRM-ALADIN) and two global models (GEOS and UM-UKCA). The focus is on the comparisons of those aerosol and cloud properties that are the primary determinants of the direct aerosol radiative effect and on the vertical distribution of the plume and its properties. The representativeness of the observations to monthly averages are tested for each field campaign, with the sampled mean aerosol light extinction generally found to be within 20 % of the monthly mean at plume altitudes. When compared to the observations, in all models, the simulated plume is too vertically diffuse and has smaller vertical gradients, and in two of the models (GEOS and UM-UKCA), the plume core is displaced lower than in the observations. Plume carbon monoxide, black carbon, and organic aerosol masses indicate underestimates in modeled plume concentrations, leading, in general, to underestimates in mid-visible aerosol extinction and optical depth. Biases in mid-visible single scatter albedo are both positive and negative across the models. Observed vertical gradients in single scatter albedo are not captured by the models, but the models do capture the coarse temporal evolution, correctly simulating higher values in October (2018) than in August (2017) and September (2016). Uncertainties in the measured absorption Ångstrom exponent were large but propagate into a negligible (<4 %) uncertainty in integrated solar absorption by the aerosol and, therefore, in the aerosol direct radiative effect. Model biases in cloud fraction, and, therefore, the scene albedo below the plume, vary significantly across the four models. The optical thickness of clouds is, on average, well simulated in the WRF-CAM5 and ALADIN models in the stratocumulus region and is underestimated in the GEOS model; UM-UKCA simulates cloud optical thickness that is significantly too high. Overall, the study demonstrates the utility of repeated, semi-random sampling across multiple years that can give insights into model biases and how these biases affect modeled climate forcing. The combined impact of these aerosol and cloud biases on the direct aerosol radiative effect (DARE) is estimated using a first-order approximation for a subset of five comparison grid boxes. A significant finding is that the observed grid box average aerosol and cloud properties yield a positive (warming) aerosol direct radiative effect for all five grid boxes, whereas DARE using the grid-box-averaged modeled properties ranges from much larger positive values to small, negative values. It is shown quantitatively how model biases can offset each other, so that model improvements that reduce biases in only one property (e.g., single scatter albedo but not cloud fraction) would lead to even greater biases in DARE. Across the models, biases in aerosol extinction and in cloud fraction and optical depth contribute the largest biases in DARE, with aerosol single scatter albedo also making a significant contribution.

The Challenge of Non-Stationary Feedbacks in Modeling the Response of Debris-Covered Glaciers to Climate Forcing

Ongoing changes in mountain glaciers affect local water resources, hazard potential and global sea level. An increasing proportion of remaining mountain glaciers are affected by the presence of a surface cover of rock debris, and the response of these debris-covered glaciers to climate forcing is different to that of glaciers without a debris cover. Here we take a back-to-basics look at the fundamental terms that control the processes of debris evolution at the glacier surface, to illustrate how the trajectory of debris cover development is partially decoupled from prevailing climate conditions, and that the development of a debris cover over time should prevent the glacier from achieving steady state. We discuss the approaches and limitations of how this has been treated in existing modeling efforts and propose that “surrogate world” numerical representations of debris-covered glaciers would facilitate the development of well-validated parameterizations of surface debris cover that can be used in regional and global glacier models. Finally, we highlight some key research targets that would need to be addressed in order to enable a full representation of debris-covered glacier system response to climate forcing.

The blue suns of 1831: was the eruption of Ferdinandea, near Sicily, one of the largest volcanic climate forcing events of the nineteenth century?

One of the largest climate forcing eruptions of the nineteenth century was, until recently, believed to have taken place at the Babuyan Claro volcano, in the Philippines, in 1831. However, a recent investigation found no reliable evidence of such an eruption, suggesting that the 1831 eruption must have taken place elsewhere. We here present our newly compiled dataset of reported observations of a blue, purple and green sun in August 1831, which we use to reconstruct the transport of a stratospheric aerosol plume from that eruption. The source of the aerosol plume is identified as the eruption of Ferdinandea, which took place about 50 km off the south-west coast of Sicily (37.1∘ N, 12.7∘ E), in July and August 1831. The modest magnitude of this eruption, assigned a volcanic explosivity index (VEI) of 3, has commonly caused it to be discounted or overlooked when identifying the likely source of the stratospheric sulfate aerosol in 1831. It is proposed, however, that convective instability in the troposphere contributed to aerosol reaching the stratosphere and that the aerosol load was enhanced by addition of a sedimentary sulfur component to the volcanic plume. Thus, one of the largest climate forcing volcanic eruptions of the nineteenth century would effectively have been hiding in plain sight, arguably “lowering the bar” for the types of eruptions capable of having a substantial climate forcing impact. Prior estimates of the mass of stratospheric sulfate aerosol responsible for the 1831 Greenland ice core sulfate deposition peaks which have assumed a source eruption at a low-latitude site will, therefore, have been overstated. The example presented in this paper serves as a useful reminder that VEI values were not intended to be reliably correlated with eruption sulfur yields unless supplemented with compositional analyses. It also underlines that eye-witness accounts of historical geophysical events should not be neglected as a source of valuable scientific data.

Rice straw open burning: emissions, effects and multiple benefitsof non-burning alternatives

Rice is one of the most important staple foods not just to people in Asia, but around the world. To meet domestic and export demands, farmers in Southeast Asia (SEA) grow 2-3 crop cycles per year, which leaves only a short period for land preparation. Field open burning of rice straw has been widely practiced to quickly clear the surface biomass for the next crop planting. However, this uncontrolled open combustion of rice straw releases large amounts of toxic air pollutants including key conventional pollutants along with carcinogenic compounds like dioxins, polycyclic aromatic hydrocarbons, and benzene, as well as major climate forcing agents. Emissions from rice straw open burning (RSOB) have been shown to significantly elevate ambient levels of PM2.5 and surface ozone in adjacent urban areas. During the dry season, when stagnant meteorological conditions are prevalent, intensive open burning activities further intensify haze episodes. Rice straw, however, is a valuable resource that should be recovered and not disposed of by open burning. Indeed, several non-open burning alternatives are available that would bring in multiple benefits to air quality, climate, health, and economy. For example, the production of rice straw fuel pellets for cooking in clean gasifier cookstoves is one promising option. For the successful elimination of RSOB in SEA, technology development along with formulation and implementation of appropriate policies should be in place to mobilise active participation from all stakeholders.

Permafrost thaw driven changes in hydrology and vegetation cover increase trace gas emissions and climate forcing in Stordalen Mire from 1970 to 2014

Permafrost thaw increases active layer thickness, changes landscape hydrology and influences vegetation species composition. These changes alter belowground microbial and geochemical processes, affecting production, consumption and net emission rates of climate forcing trace gases. Net carbon dioxide (CO 2 ) and methane (CH 4 ) fluxes determine the radiative forcing contribution from these climate-sensitive ecosystems. Permafrost peatlands may be a mosaic of dry frozen hummocks, semi-thawed or perched sphagnum dominated areas, wet permafrost-free sedge dominated sites and open water ponds. We revisited estimates of climate forcing made for 1970 and 2000 for Stordalen Mire in northern Sweden and found the trend of increasing forcing continued into 2014. The Mire continued to transition from dry permafrost to sedge and open water areas, increasing by 100% and 35%, respectively, over the 45-year period, causing the net radiative forcing of Stordalen Mire to shift from negative to positive. This trend is driven by transitioning vegetation community composition, improved estimates of annual CO 2 and CH 4 exchange and a 22% increase in the IPCC's 100-year global warming potential (GWP_100) value for CH 4 . These results indicate that discontinuous permafrost ecosystems, while still remaining a net overall sink of C, can become a positive feedback to climate change on decadal timescales. This article is part of a discussion meeting issue ‘Rising methane: is warming feeding warming? (part 2)’.