scholarly journals A multi-model comparison of meteorological drivers of surface ozone over Europe

2018 ◽  
Author(s):  
Noelia Otero ◽  
Jana Sillmann ◽  
Kathleen A. Mar ◽  
Henning W. Rust ◽  
Sverre Solberg ◽  
...  
Keyword(s):  
Time Series ◽  
Air Quality ◽  
Relative Humidity ◽  
Surface Ozone ◽  
Meteorological Variables ◽  
Maximum Temperature ◽  
Quality Models ◽  
The Balkans ◽  
Ozone Concentrations ◽  
The Relationship

Abstract. The implementation of European emission abatement strategies has led to significant reduction in the emission of ozone precursors during the last decade. Ground level ozone is also influenced by meteorological factors such as temperature, which exhibit interannual variability, and are expected to change in the future. The impacts of climate change on air quality are usually investigated through air quality models that simulate interactions between emissions, meteorology and chemistry. Within a multi-model assessment, this study aims to better understand how air quality models represent the relationship between meteorological variables and surface ozone concentrations over Europe. A multiple linear regression (MLR) approach is applied to observed and modelled time series across ten European regions in springtime and summertime for the period of 2000–2010 for both models and observations. Overall, the air quality models are in better agreement with observations in summertime than in springtime, and particularly in certain regions, such as France, Mid-Europe or East-Europe, where local meteorological variables show a strong influence on surface ozone concentrations. Larger discrepancies are found for the southern regions, such as the Balkans, the Iberian Peninsula and the Mediterranean basin, especially in springtime. We show that the air quality models do not properly reproduce the sensitivity of surface ozone to some of the main meteorological drivers, such as maximum temperature, relative humidity and surface solar radiation. Specifically, all air quality models show more limitations to capture the strength of the relationship ozone-relative humidity detected in the observed time series in most of the regions, in both seasons. Here, we speculate that dry deposition schemes in the air quality models might play an essential role to capture this relationship. We further quantify the relationship between ozone and maximum temperature (mo3-T, climate penalty) in observations and air quality models. In summertime, most of the air quality models are able to reproduce reasonably well the observed climate penalty in certain regions such as France, Mid-Europe and North Italy. However, larger discrepancies are found in springtime, where air quality models tend to overestimate the magnitude of observed climate penalty.

scholarly journals A multi-model comparison of meteorological drivers of surface ozone over Europe

2018 ◽  
Vol 18 (16) ◽  
pp. 12269-12288 ◽  
Author(s):  
Noelia Otero ◽  
Jana Sillmann ◽  
Kathleen A. Mar ◽  
Henning W. Rust ◽  
Sverre Solberg ◽  
...  
Keyword(s):  
Time Series ◽  
Air Quality ◽  
Relative Humidity ◽  
Central Europe ◽  
Surface Ozone ◽  
Meteorological Variables ◽  
Maximum Temperature ◽  
Quality Models ◽  
Ozone Concentrations ◽  
The Relationship

Abstract. The implementation of European emission abatement strategies has led to a significant reduction in the emissions of ozone precursors during the last decade. Ground-level ozone is also influenced by meteorological factors such as temperature, which exhibit interannual variability and are expected to change in the future. The impacts of climate change on air quality are usually investigated through air-quality models that simulate interactions between emissions, meteorology and chemistry. Within a multi-model assessment, this study aims to better understand how air-quality models represent the relationship between meteorological variables and surface ozone concentrations over Europe. A multiple linear regression (MLR) approach is applied to observed and modelled time series across 10 European regions in springtime and summertime for the period of 2000–2010 for both models and observations. Overall, the air-quality models are in better agreement with observations in summertime than in springtime and particularly in certain regions, such as France, central Europe or eastern Europe, where local meteorological variables show a strong influence on surface ozone concentrations. Larger discrepancies are found for the southern regions, such as the Balkans, the Iberian Peninsula and the Mediterranean basin, especially in springtime. We show that the air-quality models do not properly reproduce the sensitivity of surface ozone to some of the main meteorological drivers, such as maximum temperature, relative humidity and surface solar radiation. Specifically, all air-quality models show more limitations in capturing the strength of the ozone–relative-humidity relationship detected in the observed time series in most of the regions, for both seasons. Here, we speculate that dry-deposition schemes in the air-quality models might play an essential role in capturing this relationship. We further quantify the relationship between ozone and maximum temperature (mo3−T, climate penalty) in observations and air-quality models. In summertime, most of the air-quality models are able to reproduce the observed climate penalty reasonably well in certain regions such as France, central Europe and northern Italy. However, larger discrepancies are found in springtime, where air-quality models tend to overestimate the magnitude of the observed climate penalty.

Temporal patterns and trends of surface ozone concentrations over Portugal

2021 ◽  
Author(s):  
Carla Gama ◽  
Alexandra Monteiro ◽  
Myriam Lopes ◽  
Ana Isabel Miranda
Keyword(s):  
Air Quality ◽  
Iberian Peninsula ◽  
Human Health ◽  
Temporal Variability ◽  
Urban Areas ◽  
Surface Ozone ◽  
Quality Data ◽  
Ozone Concentrations ◽  
Long Term Study

<p>Tropospheric ozone (O<sub>3</sub>) is a critical pollutant over the Mediterranean countries, including Portugal, due to systematic exceedances to the thresholds for the protection of human health. Due to the location of Portugal, on the Atlantic coast at the south-west point of Europe, the observed O<sub>3</sub> concentrations are very much influenced not only by local and regional production but also by northern mid-latitudes background concentrations. Ozone trends in the Iberian Peninsula were previously analysed by Monteiro et al. (2012), based on 10-years of O<sub>3</sub> observations. Nevertheless, only two of the eleven background monitoring stations analysed in that study are located in Portugal and these two stations are located in Porto and Lisbon urban areas. Although during pollution events O<sub>3</sub> levels in urban areas may be high enough to affect human health, the highest concentrations are found in rural locations downwind from the urban and industrialized areas, rather than in cities. This happens because close to the sources (e.g., in urban areas) freshly emitted NO locally scavenges O<sub>3</sub>. A long-term study of the spatial and temporal variability and trends of the ozone concentrations over Portugal is missing, aiming to answer the following questions:</p><p>-           What is the temporal variability of ozone concentrations?</p><p>-           Which trends can we find in observations?</p><p>-           How were the ozone spring maxima concentrations affected by the COVID-19 lockdown during spring 2020?</p><p>In this presentation, these questions will be answered based on the statistical analysis of O<sub>3</sub> concentrations recorded within the national air quality monitoring network between 2005 and 2020 (16 years). The variability of the surface ozone concentrations over Portugal, on the timescales from diurnal to annual, will be presented and discussed, taking into account the physical and chemical processes that control that variability. Using the TheilSen function from the OpenAir package for R (Carslaw and Ropkins 2012), which quantifies monotonic trends and calculates the associated p-value through bootstrap simulations, O<sub>3</sub> concentration long-term trends will be estimated for the different regions and environments (e.g., rural, urban).  Moreover, taking advantage of the unique situation provided by the COVID-19 lockdown during spring 2020, when the government imposed mandatory confinement and citizens movement restriction, leading to a reduction in traffic-related atmospheric emissions, the role of these emissions on ozone levels during the spring period will be studied and presented.</p><p> </p><p>Carslaw and Ropkins, 2012. Openair—an R package for air quality data analysis. Environ. Model. Softw. 27-28,52-61. https://doi.org/10.1016/j.envsoft.2011.09.008</p><p>Monteiro et al., 2012. Trends in ozone concentrations in the Iberian Peninsula by quantile regression and clustering. Atmos. Environ. 56, 184-193. https://doi.org/10.1016/j.atmosenv.2012.03.069</p>

scholarly journals Turbulent transport, emissions and the role of compensating errors in chemical transport models

2014 ◽  
Vol 7 (3) ◽  
pp. 1001-1024 ◽  
Author(s):  
P. A. Makar ◽  
R. Nissen ◽  
A. Teakles ◽  
J. Zhang ◽  
Q. Zheng ◽  
...  
Keyword(s):  
Land Use ◽  
Time Series ◽  
Air Quality ◽  
Lower Limit ◽  
Turbulent Mixing ◽  
Turbulent Transport ◽  
Model Error ◽  
Quality Models ◽  
Regional Air Quality ◽  
Pm2.5 Emissions

Abstract. The balance between turbulent transport and emissions is a key issue in understanding the formation of O3 and particulate matter with diameters less than 2.5 μm (PM2.5). Discrepancies between observed and simulated concentrations for these species have, in the past, been ascribed to insufficient turbulent mixing, particularly for atmospherically stable environments. This assumption may be simplistic – turbulent mixing deficiencies may explain only part of these discrepancies, and as turbulence parameterizations are improved, the timing of primary PM2.5 emissions may play a much more significant role in the further reduction of model error. In a study of these issues, two regional air-quality models, the Community Multi-scale Air Quality model (CMAQ, version 4.6) and A Unified Regional Air-quality Modelling System (AURAMS, version 1.4.2), were compared to observations for a domain in north-western North America. The air-quality models made use of the same emissions inventory, emissions processing system, meteorological driving model, and model domain, map projection and horizontal grid, eliminating these factors as potential sources of discrepancies between model predictions. The initial statistical comparison between the models and monitoring network data showed that AURAMS' O3 simulations outperformed those of this version of CMAQ4.6, while CMAQ4.6 outperformed AURAMS for most PM2.5 statistical measures. A process analysis of the models revealed that many of the differences between the models' results could be attributed to the strength of turbulent diffusion, via the choice of an a priori lower limit in the magnitude of vertical diffusion coefficients, with AURAMS using 0.1 m2 s−1 and CMAQ4.6 using 1.0 m2 s−1. The use of the larger CMAQ4.6 value for the lower limit of vertical diffusivity within AURAMS resulted in a similar performance for the two models (with AURAMS also showing improved PM2.5, yet degraded O3, and a similar time series as CMAQ4.6). The differences between model results were most noticeable at night, when the higher minimum turbulent diffusivity resulted in an erroneous secondary peak in predicted night-time O3. A spatially invariant and relatively high lower limit in diffusivity could not reduce errors in both O3 and PM2.5 fields, implying that other factors aside from the strength of turbulence might be responsible for the PM2.5 over-predictions. Further investigation showed that the magnitude, timing and spatial allocation of area source emissions could result in improvements to PM2.5 performance with minimal O3 performance degradation. AURAMS was then used to investigate a land-use-dependant lower limit in diffusivity of 1.0 m2 s−1 in urban regions, linearly scaling to 0.01 m2s−1 in rural areas, as employed in CMAQ5.0.1. This strategy was found to significantly improve mean statistics for PM2.5 throughout the day and mean O3 statistics at night, while significantly degrading (halving) midday PM2.5 correlation coefficients and slope of observed to model simulations. Time series of domain-wide model error statistics aggregated by local hour were shown to be a useful tool for performance analysis, with significant variations in performance occurring at different hours of the day. The use of the land-use-dependant lower limit in diffusivity was also shown to reduce the model's sensitivity to the temporal allocation of its emissions inputs. The modelling scenarios suggest that while turbulence plays a key role in O3 and PM2.5 formation in urban regions, and in their downwind transport, the spatial and temporal allocation of primary PM2.5 emissions also has a potentially significant impact on PM2.5 concentration levels. The results show the complex nature of the interactions between turbulence and emissions, and the potential of the strength of the former to mask the impact of changes in the latter.

scholarly journals Spatio-temporal of surface ozone (O3) variations at urban and suburban sites in Sarawak region of Malaysia

2021 ◽  
Vol 880 (1) ◽  
pp. 012004
Author(s):  
H Mahidin ◽  
M T Latif ◽  
A Hamdan ◽  
J Salleh ◽  
D Dominick ◽  
...  
Keyword(s):  
Air Quality ◽  
Surface Ozone ◽  
Ambient Air ◽  
Quality Standard ◽  
Transportation Systems ◽  
Pollutant Emissions ◽  
Daily Maximum ◽  
Spatio Temporal ◽  
Ambient Air Quality Standard ◽  
The Relationship

Abstract Sarawak Region of Malaysia is currently experiencing a high demand for capital needs such as transformation forest to plantations, economic development, and improving transportation systems. Those land cover changes will increase primary pollutant emissions and trigger surface O3 formation. Surface O3 is a secondary pollutant and a significant greenhouse gas contributing to climate change and declining air quality. In this study, variations in surface O3 concentrations at urban and suburban sites in Sarawak were explored using the Malaysian Department of Environment data spanning a two-year cycle (2018-2019). The primary aim of this study is to ascertain the variation of surface O3 concentrations reported at four monitoring stations in Sarawak, namely Kuching (SQ1) (Urban), Sibu (SQ2) (Suburban), Bintulu (SQ3) (Suburban), and Miri (SQ4) (Suburban). The study also analysed the relationship between O3 distribution and nitrogen oxides (NO and NO2). The findings showed that O3 concentrations observed in the region during the study period were lower than the maximum permissible value of 100 ppbv suggested by the Malaysian Ambient Air Quality Standard (2020). SQ4 (Miri) at suburban sites recorded the highest average surface O3 concentrations with an hourly average and daily maximum O3 concentration of 15.7 and 89.5 ppbv, respectively. Temperatures, UV exposure, and wind speed all impact the concentration of surface O3 in Sarawak. In all stations, concentrations of O3 were inversely linked with NO, NO2, and relative humidity (RH). This research will assist the relevant agency in forecast, monitor, and mitigate the level of O3 in the ambient environment, especially in the Sarawak Region.

scholarly journals Impacts of changes in land use and land cover on atmospheric chemistry and air quality over the 21st century

2011 ◽  
Vol 11 (5) ◽  
pp. 15469-15495 ◽  
Author(s):  
S. Wu ◽  
L. J. Mickley ◽  
J. O. Kaplan ◽  
D. J. Jacob
Keyword(s):  
Land Use ◽  
Air Quality ◽  
Land Use Change ◽  
Land Cover ◽  
21St Century ◽  
Secondary Organic Aerosols ◽  
Surface Ozone ◽  
Organic Aerosols ◽  
Ozone Concentrations ◽  
Anthropogenic Land Use

Abstract. The effects of future land use and land cover change on the chemical composition of the atmosphere and air quality are largely unknown. To investigate the potential effects associated with future changes in vegetation driven by atmospheric CO2 concentrations, climate, and anthropogenic land use over the 21st century, we performed a series of model experiments combining a general circulation model with a dynamic global vegetation model and an atmospheric chemical-transport model. Our results indicate that climate- and CO2-induced changes in vegetation composition and density could lead to decreases in summer afternoon surface ozone of up to 10 ppb over large areas of the northern mid-latitudes. This is largely driven by the substantial increases in ozone dry deposition associated with changes in the composition of temperate and boreal forests where conifer forests are replaced by those dominated by broadleaf tree types, as well as a CO2-driven increase in vegetation density. Climate-driven vegetation changes over the period 2000–2100 lead to general increases in isoprene emissions, globally by 15 % in 2050 and 36 % in 2100. These increases in isoprene emissions result in decreases in surface ozone concentrations where the NOx levels are low, such as in remote tropical rainforests. However, over polluted regions, such as the northeastern United States, ozone concentrations are calculated to increase with higher isoprene emissions in the future. Increases in biogenic emissions also lead to higher concentrations of secondary organic aerosols, which increase globally by 10 % in 2050 and 20 % in 2100. Surface concentrations of secondary organic aerosols are calculated to increase by up to 1 μg m−3 for large areas in Eurasia. When we use a scenario of future anthropogenic land use change, we find less increase in global isoprene emissions due to replacement of higher-emitting forests by lower-emitting cropland. The global atmospheric burden of secondary organic aerosols changes little by 2100 when we account for future land use change, but both secondary organic aerosols and ozone show large regional changes at the surface.

scholarly journals Assessment of the Relationship between Cerebrospinal Meningitis and Climate Variables in Kaduna State, Nigeria

2021 ◽  
pp. 33-41
Author(s):  
Joyce Imara Nchom ◽  
A. S. Abubakar ◽  
F. O. Arimoro ◽  
B. Y. Mohammed
Keyword(s):  
Relative Humidity ◽  
Air Temperature ◽  
Linear Trend ◽  
Pearson Correlation ◽  
Maximum Temperature ◽  
Data Set ◽  
International Research Institute ◽  
Wind Speed Maximum ◽  
Weather Parameters ◽  
The Relationship

This study examines the relationship between Meningitis and weather parameters (air temperature, maximum temperature, relative humidity, and rainfall) in Kaduna state, Nigeria on a weekly basis from 2007–2019. Meningitis data was acquired weekly from Nigeria Centre for Disease Control (NCDC), Bureau of Statistics and weather parameters were sourced from daily satellite data set National Oceanic and Atmospheric Administration (NOAA), International Research Institute for Climate and Society (IRI). The daily data were aggregated weekly to suit the study. The data were analysed using linear trend and Pearson correlation for relationship. The linear trend results revealed a weekly decline in Cerebro Spinal Meningitis (CSM), wind speed, maximum and air temperature and an increase in relative humidity and rainfall. Generally, results reveal that the most important explanatory weather variables influencing CSM amongst the five (5) are the weekly maximum temperature and air temperature with a positive correlation of 0.768 and 0.773. This study recommends that keen interest be placed on temperature as they play an essential role in the transmission of this disease and most times aggravate the patients' condition.

scholarly journals SEASONAL AND INTERANNUAL PATTERN OF METEOROLOGICAL VARIABLES IN CUIABÁ, MATO GROSSO STATE, BRAZIL

2015 ◽  
Vol 33 (3) ◽  
pp. 477 ◽  
Author(s):  
Nadja Gomes Machado ◽  
Marcelo Sacardi Biudes ◽  
Carlos Alexandre Santos Querino ◽  
Victor Hugo De Morais Danelichen ◽  
Maísa Caldas Souza Velasque
Keyword(s):  
Wind Speed ◽  
Relative Humidity ◽  
Meteorological Data ◽  
Seasonal Pattern ◽  
Global Radiation ◽  
Meteorological Variables ◽  
Maximum Temperature ◽  
Wet Season ◽  
Agricultural Producers ◽  
Mato Grosso

ABSTRACT. Cuiab´a is located on the border of the Pantanal and Cerrado, in Mato Grosso State, which is recognized as one of the biggest agricultural producers of Brazil. The use of natural resources in a sustainable manner requires knowledge of the regional meteorological variables. Thus, the objective of this study was to characterize the seasonal and interannual pattern of meteorological variables in Cuiab´a. The meteorological data from 1961 to 2011 were provided by the Instituto Nacional de Meteorologia (INMET – National Institute of Meteorology). The results have shown interannual and seasonal variations of precipitation, solar radiation, air temperature and relative humidity, and wind speed and direction, establishing two main distinct seasons (rainy and dry). On average, 89% of the rainfall occurred in the wet season. The annual average values of daily global radiation, mean, minimum and maximum temperature and relative humidity were 15.6 MJ m–2 y–1, 27.9◦C, 23.0◦C, 30.0◦C and 71.6%, respectively. Themaximum temperature and the wind speed had no seasonal pattern. The wind speed average decreased in the NWdirectionand increased in the S direction.Keywords: meteorological variables, climatology, ENSO. RESUMO. Cuiabá está localizado na fronteira do Pantanal com o Cerrado, no Mato Grosso, que é reconhecido como um dos maiores produtores agrícolas do Brasil. A utilização dos recursos naturais de forma sustentável requer o conhecimento das variáveis meteorológicas em escala regional. Assim, o objetivo deste estudo foi caracterizar o padrão sazonal e interanual das variáveis meteorológicas em Cuiabá. Os dados meteorológicos de 1961 a 2011 foram fornecidos pelo Instituto Nacional de Meteorologia (INMET). Os resultados mostraram variações interanuais e sazonais de precipitação, radiação solar, temperatura e umidade relativa do ar e velocidade e direção do vento, estabelecendo duas principais estações distintas (chuvosa e seca). Em média, 89% da precipitação ocorreu na estação chuvosa. Os valores médios anuais de radiação diária global, temperatura do ar média, mínima e máxima e umidade relativa do ar foram 15,6 MJ m–2 y–1, 27,9◦C, 23,0◦C, 30,0◦C e 71,6%, respectivamente. A temperatura máxima e a velocidade do vento não tiveram padrão sazonal. A velocidade média do vento diminuiu na direção NW e aumentou na direção S.Palavras-chave: variáveis meteorológicas, climatologia, ENOS.

scholarly journals Explicit Modeling of Meteorological Explanatory Variables in Short-Term Forecasting of Maximum Ozone Concentrations via a Multiple Regression Time Series Framework

Atmosphere ◽  
2020 ◽  
Vol 11 (12) ◽  
pp. 1304
Author(s):  
Sigfrido Iglesias-Gonzalez ◽  
Maria E. Huertas-Bolanos ◽  
Ivan Y. Hernandez-Paniagua ◽  
Alberto Mendoza
Keyword(s):  
Time Series ◽  
Air Quality ◽  
Multiple Regression ◽  
Urban Areas ◽  
Moving Average ◽  
Time Series Forecasting ◽  
Air Pollutant ◽  
Short Term ◽  
Ozone Level ◽  
Ozone Concentrations

Statistical time series forecasting is a useful tool for predicting air pollutant concentrations in urban areas, especially in emerging economies, where the capacity to implement comprehensive air quality models is limited. In this study, a general multiple regression with seasonal autoregressive moving average errors model was estimated and implemented to forecast maximum ozone concentrations with a short time resolution: overnight, morning, afternoon and evening. In contrast to a number of short-term air quality time series forecasting applications, the model was designed to explicitly include the effects of meteorological variables on the ozone level as exogenous variables. As the application location, the model was constructed with data from five monitoring stations in the Monterrey Metropolitan Area of Mexico. The results show that, together with structural stochastic components, meteorological parameters have a significant contribution for obtaining reliable forecasts. The resulting model is an interpretable, useful and easily implementable model for forecasting ozone maxima. Moreover, it proved to be consistent with the general dynamics of ozone formation and provides a suitable platform for forecasting, showing similar or better performance compared to models in other existing studies.

scholarly journals Investigation of Climate Change Anomaly by Using Nonparametric Test for Navsari District of South Gujarat

2021 ◽  
Vol 9 (3) ◽  
pp. 266-275
Author(s):  
Neeraj Kumar ◽  
Keyword(s):  
Climate Change ◽  
Time Series ◽  
Relative Humidity ◽  
Nonparametric Test ◽  
Maximum Temperature ◽  
Rainfall Trend ◽  
Regression Slope ◽  
Sunshine Hours ◽  
Increasing Trend ◽  
Daily Sunshine

Navsari district of rainfall was shows highest increasing rainfall trend obtained September and negative January, July, October, November and December. The regression slope of the yearly time series is about 12.35 mm/36 years. Maximum temperature shows the highest increasing trend in month October, followed by December and August. The month highest decreasing trend was noticed that January, followed by February and July. The regression slope of the yearly time series is about 0.025°C/36 years. Minimum temperature highest values of the slope (0.109°C/36 year) with high value of regression Slope of determination (0.111°C), the annual Kendall’s tau statistic (0.492°C/36 year), the Kendall Score (310). All the month January to December shows increasing trend. The highest increasing trend found that November, followed by March and July, respectively. This finding shows that all the month shows increasing trend with the range between 0.308°C to 0.390°C. In case of RH-I the highest increasing trend shows September, followed by April and June. Similarly decreasing trend was found that January, followed by February and October, respectively. Relative humidity-II increasing trend was found only at the September month 0.084%, the increasing trend was detected in January to August and October to December, respectively. The strongest trend in the Bright sunshine hour’s decline of all month’s average daily sunshine hours was for the Navsari district. No significant trends were detected in all months and seasons for all weather elements. A similar trend was found in Sen’s slope and regression slope all the months for all the weather elements.

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