scholarly journals How emissions uncertainty influences the distribution and radiative impacts of smoke from fires in North America

2019 ◽  
Author(s):  
Therese S. Carter ◽  
Colette L. Heald ◽  
Jose L. Jimenez ◽  
Pedro Campuzano-Jost ◽  
Yutaka Kondo ◽  
...  
Keyword(s):  
Air Quality ◽  
North America ◽  
Black Carbon ◽  
Dry Matter ◽  
Organic Aerosol ◽  
Carbonaceous Aerosol ◽  
Burned Area ◽  
Emission Inventories ◽  
Fire Emissions ◽  
Radiative Impacts

Abstract. Fires and the aerosols that they emit impact air quality, health, and climate, but the abundance and properties of carbonaceous aerosol (both black carbon and organic carbon) from biomass burning (BB) remain uncertain and poorly constrained. We aim to quantify the uncertainties associated with fire emissions and their air quality and radiative impacts from underlying dry matter consumed and emissions factors. To explore this, we compare model simulations from a global chemical transport model, GEOS-Chem, driven by a variety of fire emission inventories with surface and airborne observations of black carbon (BC) and organic aerosol (OA) concentrations and satellite-derived aerosol optical depth (AOD). We focus on two fire detection/burned area-based (FD/BA) inventories using burned area and active fire counts, respectively: the Global Fire Emissions Database version 4 (GFED4s) with small fires and the Fire INventory from NCAR version 1.5 (FINN1.5) and two fire radiative power (FRP)-based approaches: the Quick Fire Emission Dataset version 2.4 (QFED2.4) and the Global Fire Assimilation System version 1.2 (GFAS1.2). We show that, across the inventories, emissions of BB aerosol (BBA) differ by a factor of 4 to 7 over North America and that dry matter differences, not emissions factors, drive this spread. We find that simulations driven by QFED2.4 generally overestimate BC and, to a lesser extent, OA concentrations observations from two fire-influenced aircraft campaigns in North America (ARCTAS and DC3) and from the Interagency Monitoring of Protected Visual Environments (IMPROVE) network, while simulations driven by FINN1.5 substantially underestimate concentrations. The GFED4s and GFAS1.2-driven simulations provide the best agreement with OA and BC mass concentrations at the surface (IMPROVE), BC observed aloft (DC3 and ARCTAS), and AOD observed by MODIS over North America. We also show that a sensitivity simulation including an enhanced source of secondary organic aerosol (SOA) from fires based on the NOAA Fire Lab 2016 experiments produces substantial additional OA; however, the spread in the primary emissions estimates implies that this magnitude of SOA cannot be either confirmed or ruled out when comparing the simulations against the observations explored here. Given the substantial uncertainty in fire emissions, as represented by these four emission inventories, we find a sizeable range in BBA population-weighted exposure over Canada and the contiguous United States (0.5 to 1.6 µg m−3). We also show that the range in the estimated global direct radiative effect of carbonaceous aerosol from fires (−0.11 to −0.048 W m−2) is large and comparable to the direct radiative forcing of OA (−0.09 W m−2) estimated in AR5. Our analysis suggests that fire emissions uncertainty challenges our ability to accurately characterize the impact of smoke on air quality and climate.

scholarly journals How emissions uncertainty influences the distribution and radiative impacts of smoke from fires in North America

2020 ◽  
Vol 20 (4) ◽  
pp. 2073-2097 ◽  
Author(s):  
Therese S. Carter ◽  
Colette L. Heald ◽  
Jose L. Jimenez ◽  
Pedro Campuzano-Jost ◽  
Yutaka Kondo ◽  
...  
Keyword(s):  
Air Quality ◽  
North America ◽  
Black Carbon ◽  
Dry Matter ◽  
Organic Aerosol ◽  
Carbonaceous Aerosol ◽  
Burned Area ◽  
Emission Inventories ◽  
Fire Emissions ◽  
Radiative Impacts

Abstract. Fires and the aerosols that they emit impact air quality, health, and climate, but the abundance and properties of carbonaceous aerosol (both black carbon and organic carbon) from biomass burning (BB) remain uncertain and poorly constrained. We aim to explore the uncertainties associated with fire emissions and their air quality and radiative impacts from underlying dry matter consumed and emissions factors. To investigate this, we compare model simulations from a global chemical transport model, GEOS-Chem, driven by a variety of fire emission inventories with surface and airborne observations of black carbon (BC) and organic aerosol (OA) concentrations and satellite-derived aerosol optical depth (AOD). We focus on two fire-detection-based and/or burned-area-based (FD-BA) inventories using burned area and active fire counts, respectively, i.e., the Global Fire Emissions Database version 4 (GFED4s) with small fires and the Fire INventory from NCAR version 1.5 (FINN1.5), and two fire radiative power (FRP)-based approaches, i.e., the Quick Fire Emission Dataset version 2.4 (QFED2.4) and the Global Fire Assimilation System version 1.2 (GFAS1.2). We show that, across the inventories, emissions of BB aerosol (BBA) differ by a factor of 4 to 7 over North America and that dry matter differences, not emissions factors, drive this spread. We find that simulations driven by QFED2.4 generally overestimate BC and, to a lesser extent, OA concentrations observations from two fire-influenced aircraft campaigns in North America (ARCTAS and DC3) and from the Interagency Monitoring of Protected Visual Environments (IMPROVE) network, while simulations driven by FINN1.5 substantially underestimate concentrations. The GFED4s and GFAS1.2-driven simulations provide the best agreement with OA and BC mass concentrations at the surface (IMPROVE), BC observed aloft (DC3 and ARCTAS), and AOD observed by MODIS over North America. We also show that a sensitivity simulation including an enhanced source of secondary organic aerosol (SOA) from fires, based on the NOAA Fire Lab 2016 experiments, produces substantial additional OA; however, the spread in the primary emissions estimates implies that this magnitude of SOA can be neither confirmed nor ruled out when comparing the simulations against the observations explored here. Given the substantial uncertainty in fire emissions, as represented by these four emission inventories, we find a sizeable range in 2012 annual BBA PM2.5 population-weighted exposure over Canada and the contiguous US (0.5 to 1.6 µg m−3). We also show that the range in the estimated global direct radiative effect of carbonaceous aerosol from fires (−0.11 to −0.048 W m−2) is large and comparable to the direct radiative forcing of OA (−0.09 W m−2) estimated in the Fifth Assessment Report (AR5) of the Intergovernmental Panel on Climate Change (IPCC). Our analysis suggests that fire emissions uncertainty challenges our ability to accurately characterize the impact of smoke on air quality and climate.

scholarly journals Global fire emissions estimates during 1997–2015

2017 ◽  
Author(s):  
Guido R. van der Werf ◽  
James T. Randerson ◽  
Louis Giglio ◽  
Thijs T. van Leeuwen ◽  
Yang Chen ◽  
...  
Keyword(s):  
North America ◽  
Fuel Consumption ◽  
Fire Severity ◽  
Emission Factors ◽  
Trace Gas ◽  
Burned Area ◽  
Biogeochemical Model ◽  
Fire Dynamics ◽  
Fire Emissions ◽  
Aerosol Emissions

Abstract. Climate, land use, and other anthropogenic and natural drivers have the potential to influence fire dynamics in many regions. To develop a mechanistic understanding of the changing role of these drivers and their impact on atmospheric composition, long term fire records are needed that fuse information from different satellite and in-situ data streams. Here we describe the fourth version of the Global Fire Emissions Database (GFED) and quantify global fire emissions patterns during 1997–2015. The modeling system, based on the Carnegie-Ames-Stanford-Approach (CASA) biogeochemical model, has several modifications from the previous version and uses higher quality input datasets. Significant upgrades include: 1) new burned area estimates with contributions from small fires, 2) a revised fuel consumption parameterization optimized using field observations, 3) modifications that improve the representation of fuel consumption in frequently burning landscapes, and 4) fire severity estimates that better represent continental differences in burning processes across boreal regions of North America and Eurasia. The new version has a higher spatial resolution (0.25°) and uses a different set of emission factors that separately resolves trace gas and aerosol emissions from temperate and boreal forest ecosystems. Global mean carbon emissions using the burned area dataset with small fires (GFED4s) were 2.2 x 1015 grams carbon per year (Pg C yr-1) during 1997–2015, with a maximum in 1997 (3.0 Pg C yr-1) and minimum in 2013 (1.8 Pg C yr-1). These estimates were 11 % higher than our previous estimates (GFED3) during 1997–2011, when the two datasets overlapped. This increase was the result of a substantial increase in burned area (37 %), mostly due to the inclusion of small fires, and a modest decrease in mean fuel consumption (–19 %) to better match estimates from field studies, primarily in savannas and grasslands. For trace gas and aerosol emissions, differences between GFED4s and GFED3 were often larger due to the use of revised emission factors. If small fire burned area was excluded (GFED4 without the "s" for small fires), average emissions were 1.5 Pg C yr-1. The addition of small fires had the largest impact on emissions in temperate North America, Central America, Europe, and temperate Asia. Our improved dataset provides an internally consistent set of burned area and emissions that may contribute to a better understanding of multi-decadal changes in fire dynamics and their impact on the Earth System. GFED data is available from http://www.globalfiredata.org.

scholarly journals Fog scavenging of organic and inorganic aerosol in the Po Valley

2014 ◽  
Vol 14 (4) ◽  
pp. 4787-4826 ◽  
Author(s):  
S. Gilardoni ◽  
P. Massoli ◽  
L. Giulianelli ◽  
M. Rinaldi ◽  
M. Paglione ◽  
...  
Keyword(s):  
Chemical Composition ◽  
Black Carbon ◽  
Functional Group ◽  
Group Composition ◽  
Organic Aerosol ◽  
Water Soluble ◽  
Carbonaceous Aerosol ◽  
Model Description ◽  
Po Valley ◽  
Scavenging Efficiency

Abstract. The interaction of aerosol with atmospheric water affects the processing and wet removal of atmospheric particles. Understanding such interaction is mandatory to improve model description of aerosol lifetime and ageing. We analyzed the aerosol-water interaction at high relative humidity during fog events in the Po Valley, in the framework of the ARPA-ER Supersite project. For the first time in this area, the changes in particle chemical composition caused by fog are discussed along with changes in particle microphysics. During the experiment, 14 fog events were observed. The average mass scavenging efficiency was 70% for nitrate, 68% for ammonium, 61% for sulfate, 50% for organics, and 39% for black carbon. After fog formation, the interstitial aerosol was dominated by particles smaller than 200 nm Dva (vacuum aerodynamic diameter) and enriched in carbonaceous aerosol, mainly black carbon and water insoluble organic aerosol (WIOA). For each fog event, the size segregated scavenging efficiency of nitrate and organic aerosol (OA) was calculated by comparing chemical species size distribution before and after fog formation. For both nitrate and OA, the size segregated scavenging efficiency followed a sigmoidal curve, with values close to zero below 100 nm Dva and close to 1 above 700 nm Dva. OA was able to affect scavenging efficiency of nitrate in particles smaller than 300 nm Dva. A linear correlation between nitrate scavenging and particle hygroscopicity (κ) was observed, indicating that 44–51% of the variability of nitrate scavenging in smaller particles (below 300 nm Dva) was explained by changes in particle chemical composition. The size segregated scavenging curves of OA followed those of nitrate, suggesting that organic scavenging was controlled by mixing with water-soluble species. In particular, functional group composition and OA elemental analysis indicated that more oxidized OA was scavenged more efficiently than less oxidized OA. Nevertheless, the small variability of organic functional group composition during the experiment did not allow us to discriminate the effect of different organic functionalities on OA scavenging.

scholarly journals Global fire emissions estimates during 1997–2016

2017 ◽  
Vol 9 (2) ◽  
pp. 697-720 ◽  
Author(s):  
Guido R. van der Werf ◽  
James T. Randerson ◽  
Louis Giglio ◽  
Thijs T. van Leeuwen ◽  
Yang Chen ◽  
...  
Keyword(s):  
North America ◽  
Fuel Consumption ◽  
Fire Severity ◽  
Emission Factors ◽  
Trace Gas ◽  
Burned Area ◽  
Biogeochemical Model ◽  
Fire Dynamics ◽  
Fire Emissions ◽  
Aerosol Emissions

Abstract. Climate, land use, and other anthropogenic and natural drivers have the potential to influence fire dynamics in many regions. To develop a mechanistic understanding of the changing role of these drivers and their impact on atmospheric composition, long-term fire records are needed that fuse information from different satellite and in situ data streams. Here we describe the fourth version of the Global Fire Emissions Database (GFED) and quantify global fire emissions patterns during 1997–2016. The modeling system, based on the Carnegie–Ames–Stanford Approach (CASA) biogeochemical model, has several modifications from the previous version and uses higher quality input datasets. Significant upgrades include (1) new burned area estimates with contributions from small fires, (2) a revised fuel consumption parameterization optimized using field observations, (3) modifications that improve the representation of fuel consumption in frequently burning landscapes, and (4) fire severity estimates that better represent continental differences in burning processes across boreal regions of North America and Eurasia. The new version has a higher spatial resolution (0.25°) and uses a different set of emission factors that separately resolves trace gas and aerosol emissions from temperate and boreal forest ecosystems. Global mean carbon emissions using the burned area dataset with small fires (GFED4s) were 2.2  ×  1015 grams of carbon per year (Pg C yr−1) during 1997–2016, with a maximum in 1997 (3.0 Pg C yr−1) and minimum in 2013 (1.8 Pg C yr−1). These estimates were 11 % higher than our previous estimates (GFED3) during 1997–2011, when the two datasets overlapped. This net increase was the result of a substantial increase in burned area (37 %), mostly due to the inclusion of small fires, and a modest decrease in mean fuel consumption (−19 %) to better match estimates from field studies, primarily in savannas and grasslands. For trace gas and aerosol emissions, differences between GFED4s and GFED3 were often larger due to the use of revised emission factors. If small fire burned area was excluded (GFED4 without the s for small fires), average emissions were 1.5 Pg C yr−1. The addition of small fires had the largest impact on emissions in temperate North America, Central America, Europe, and temperate Asia. This small fire layer carries substantial uncertainties; improving these estimates will require use of new burned area products derived from high-resolution satellite imagery. Our revised dataset provides an internally consistent set of burned area and emissions that may contribute to a better understanding of multi-decadal changes in fire dynamics and their impact on the Earth system. GFED data are available from http://www.globalfiredata.org.

scholarly journals Modelling of organic aerosols over Europe (2002–2007) using a volatility basis set (VBS) framework: application of different assumptions regarding the formation of secondary organic aerosol

2012 ◽  
Vol 12 (18) ◽  
pp. 8499-8527 ◽  
Author(s):  
R. Bergström ◽  
H. A. C. Denier van der Gon ◽  
A. S. H. Prévôt ◽  
K. E. Yttri ◽  
D. Simpson
Keyword(s):  
Secondary Organic Aerosol ◽  
Transport Model ◽  
Organic Aerosol ◽  
Basis Set ◽  
Emission Inventories ◽  
Chemical Transport Model ◽  
Wood Combustion ◽  
Fire Emissions ◽  
Model Studies ◽  
Primary Emissions

Abstract. A new organic aerosol module has been implemented into the EMEP chemical transport model. Four different volatility basis set (VBS) schemes have been tested in long-term simulations for Europe, covering the six years 2002–2007. Different assumptions regarding partitioning of primary organic aerosol and aging of primary semi-volatile and intermediate volatility organic carbon (S/IVOC) species and secondary organic aerosol (SOA) have been explored. Model results are compared to filter measurements, aerosol mass spectrometry (AMS) data and source apportionment studies, as well as to other model studies. The present study indicates that many different sources contribute significantly to organic aerosol in Europe. Biogenic and anthropogenic SOA, residential wood combustion and vegetation fire emissions may all contribute more than 10% each over substantial parts of Europe. This study shows smaller contributions from biogenic SOA to organic aerosol in Europe than earlier work, but relatively greater anthropogenic SOA. Simple VBS based organic aerosol models can give reasonably good results for summer conditions but more observational studies are needed to constrain the VBS parameterisations and to help improve emission inventories. The volatility distribution of primary emissions is one important issue for further work. Emissions of volatile organic compounds from biogenic sources are also highly uncertain and need further validation. We can not reproduce winter levels of organic aerosol in Europe, and there are many indications that the present emission inventories substantially underestimate emissions from residential wood combustion in large parts of Europe.

scholarly journals The impact of monthly variation of the Pacific-North America (PNA) teleconnection pattern on wintertime surface-layer aerosol concentrations in the United States

2015 ◽  
Vol 15 (22) ◽  
pp. 33209-33251
Author(s):  
J. Feng ◽  
H. Liao ◽  
J. Li
Keyword(s):  
United States ◽  
Surface Layer ◽  
Air Quality ◽  
North America ◽  
Organic Carbon ◽  
Black Carbon ◽  
The United States ◽  
Monthly Variation ◽  
The Pacific ◽  
The Us

Abstract. The Pacific-North America teleconnection (PNA) is the leading general circulation pattern in the troposphere over the region of North Pacific to North America during wintertime. This study examined the impacts of monthly variation of the PNA phase (positive or negative phase) on wintertime surface-layer aerosol concentrations in the US by analyzing observations during 1999–2013 from the Air Quality System of Environmental Protection Agency (EPA-AQS) and the model results for 1986–2006 from the global three-dimensional Goddard Earth Observing System (GEOS) chemical transport model (GEOS-Chem). The composite analyses on the EPA-AQS observations over 1999–2003 showed that the average concentrations of PM2.5, sulfate, nitrate, ammonium, organic carbon, and black carbon aerosols over the US were higher in the PNA positive phases than in the PNA negative phases by 1.4 μg m−3 (12.7 %), 0.1 μg m−3 (6.4 %), 0.3 μg m−3 (39.1 %), 0.2 μg m−3 (22.8 %), 0.8 μg m−3 (21.3 %), and 0.2 μg m−3 (34.1 %), respectively. The simulated geographical patterns of the differences in concentrations of all aerosol species between the PNA positive and negative phases were similar to observations. Based on the GEOS-Chem simulation driven by the assimilated meteorological fields, the PNA-induced variation in planetary boundary layer height was found to be the most dominant meteorological factor that influenced the concentrations of PM2.5, sulfate, ammonium, organic carbon, and black carbon, and the PNA-induced variation in temperature was the most important parameter that influenced nitrate aerosol. Results from this work have important implications for understanding and prediction of air quality in the United States.

scholarly journals Connecting smoke plumes to sources using Hazard Mapping System (HMS) smoke and fire location data over North America

2018 ◽  
Vol 18 (3) ◽  
pp. 1745-1761 ◽  
Author(s):  
Steven J. Brey ◽  
Mark Ruminski ◽  
Samuel A. Atwood ◽  
Emily V. Fischer
Keyword(s):  
United States ◽  
Air Quality ◽  
North America ◽  
Fire Severity ◽  
Information Service ◽  
Hazard Mapping ◽  
Fire Emissions ◽  
The North ◽  
Mapping System ◽  
Smoke Plumes

Abstract. Fires represent an air quality challenge because they are large, dynamic and transient sources of particulate matter and ozone precursors. Transported smoke can deteriorate air quality over large regions. Fire severity and frequency are likely to increase in the future, exacerbating an existing problem. Using the National Environmental Satellite, Data, and Information Service (NESDIS) Hazard Mapping System (HMS) smoke data for North America for the period 2007 to 2014, we examine a subset of fires that are confirmed to have produced sufficient smoke to warrant the initiation of a U.S. National Weather Service smoke forecast. We find that gridded HMS-analyzed fires are well correlated (r= 0.84) with emissions from the Global Fire Emissions Inventory Database 4s (GFED4s). We define a new metric, smoke hours, by linking observed smoke plumes to active fires using ensembles of forward trajectories. This work shows that the Southwest, Northwest, and Northwest Territories initiate the most air quality forecasts and produce more smoke than any other North American region by measure of the number of HYSPLIT points analyzed, the duration of those HYSPLIT points, and the total number of smoke hours produced. The average number of days with smoke plumes overhead is largest over the north-central United States. Only Alaska, the Northwest, the Southwest, and Southeast United States regions produce the majority of smoke plumes observed over their own borders. This work moves a new dataset from a daily operational setting to a research context, and it demonstrates how changes to the frequency or intensity of fires in the western United States could impact other regions.

scholarly journals Emissions from village cookstoves in Haryana, India and their potential impacts on air quality

2018 ◽  
Author(s):  
Lauren T. Fleming ◽  
Robert Weltman ◽  
Ankit Yadav ◽  
Rufus D. Edwards ◽  
Narendra K. Arora ◽  
...  
Keyword(s):  
Air Quality ◽  
Fine Particulate Matter ◽  
Organic Aerosol ◽  
Rural India ◽  
Aerosol Formation ◽  
Fire Emissions ◽  
Flame Ionization ◽  
Fine Particulate ◽  
Volatile Organic ◽  
The Relationship

Abstract. Air quality in rural India is impacted by residential cooking and heating with biomass fuels. In this study, emissions of CO, CO2, and 76 volatile organic compounds (VOCs) and fine particulate matter (PM2.5) were quantified to better understand the relationship between cook fire emissions and ambient ozone and secondary organic aerosol formation. Cooking was carried out by a local cook and traditional dishes were prepared on locally built chulha or angithi cookstoves using brushwood or dung fuels. Cook fire emissions were collected throughout the cooking event in a Kynar bag (VOCs) and on PTFE filters (PM2.5). Gas samples were transferred from a Kynar bag to previously evacuated stainless steel canisters and analyzed using gas chromatography coupled to flame ionization, electron capture, and mass spectrometry detectors. Filter samples were weighed to calculate PM2.5 emission factors. Dung fuels and angithi cookstoves resulted in significantly higher emissions of most VOCs (p 

scholarly journals The 2018 fire season in North America as seen by TROPOMI: aerosol layer height intercomparisons and evaluation of model-derived plume heights

2020 ◽  
Vol 13 (3) ◽  
pp. 1427-1445 ◽  
Author(s):  
Debora Griffin ◽  
Christopher Sioris ◽  
Jack Chen ◽  
Nolan Dickson ◽  
Andrew Kovachik ◽  
...  
Keyword(s):  
Air Quality ◽  
North America ◽  
Measurement Techniques ◽  
Fire Season ◽  
Orthogonal Polarization ◽  
Potential Game ◽  
Aerosol Layer ◽  
Plume Height ◽  
Layer Height ◽  
Fire Emissions

Abstract. Before the launch of the TROPOspheric Monitoring Instrument (TROPOMI), only two other satellite instruments were able to observe aerosol plume heights globally, the Multi-angle Imaging SpectroRadiometer (MISR) and Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). The TROPOMI aerosol layer height is a potential game changer, since it has daily global coverage, and the aerosol layer height retrieval is available in near real time. The aerosol layer height can be useful for aviation and air quality alerts, as well as for improving air quality forecasting related to wildfires. Here, TROPOMI's aerosol layer height product is evaluated with MISR and CALIOP observations for wildfire plumes in North America for the 2018 fire season (June to August). Further, observing system simulation experiments were performed to interpret the fundamental differences between the different products. The results show that MISR and TROPOMI are, in theory, very close for aerosol profiles with single plumes. For more complex profiles with multiple plumes, however, different plume heights are retrieved; the MISR plume height represents the top layer, and the plume height retrieved with TROPOMI tends to have an average altitude of several plume layers. The comparison between TROPOMI and MISR plume heights shows that, on average, the TROPOMI aerosol layer heights are lower, by approximately 600 m, compared to MISR, which is likely due to the different measurement techniques. From the comparison to CALIOP, our results show that the TROPOMI aerosol layer height is more accurate over dark surfaces, for thicker plumes, and plumes between approximately 1 and 4.5 km. MISR and TROPOMI are further used to evaluate the plume height of Environment and Climate Change Canada's operational forecasting system FireWork with fire plume injection height estimates from the Canadian Forest Fire Emissions Prediction System (CFFEPS). The modelled plume heights are similar compared to the satellite observations but tend to be slightly higher with average differences of 270–580 and 60–320 m compared to TROPOMI and MISR, respectively.

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