scholarly journals Sunlight-absorbing aerosol amplifies the seasonal cycle in low cloud fraction over the southeast Atlantic

2021 ◽  
Author(s):  
Jianhao Zhang ◽  
Paquita Zuidema
Keyword(s):  
Boundary Layer ◽  
Seasonal Cycle ◽  
Large Scale ◽  
Cloud Fraction ◽  
Small Scale ◽  
Aerosol Cloud ◽  
Ascension Island ◽  
Tropospheric Aerosol ◽  
Low Cloud ◽  
Aerosol Cloud Interactions

Abstract. Many studies examining shortwave-absorbing aerosol-cloud interactions over the southeast Atlantic apply a seasonal averaging. This disregards a meteorology that raises the mean altitude of the smoke layer from July to October. This study details the month-by-month changes in cloud properties and the large-scale environment as a function of the biomass-burning aerosol loading at Ascension Island from July to October, based on measurements from Ascension Island (8º S, 14.5º W), satellite retrievals and reanalysis. In July and August, variability in the smoke loading predominantly occurs in the boundary layer. During both months, the low-cloud fraction is less and is increasingly cumuliform when more smoke is present, with the exception of a late morning boundary layer deepening that encourages a short-lived cloud development. The meteorology varies little, suggesting aerosol-cloud interactions consistent with a boundary-layer semi-direct effect can explain the cloudiness changes. September marks a transition month during which mid-latitude disturbances can intrude into the Atlantic subtropics, constraining the land-based anticyclonic circulation transporting free-tropospheric aerosol to closer to the coast. Stronger boundary layer winds help deepen, dry, and cool the boundary layer near the main stratocumulus deck compared to that on days with high smoke loadings, with stratocumulus reducing everywhere but at the northern deck edge. Longwave cooling rates generated by a sharp water vapor gradient at the aerosol layer top facilitates small-scale vertical mixing, and could help to maintain a better-mixed September free troposphere. The October meteorology is more singularly dependent on the strength of the free-tropospheric winds advecting aerosol offshore. Free-tropospheric aerosol is less, and moisture variability more, compared to September. Low-level clouds increase and are more stratiform, when the smoke loadings are higher. The increased free-tropospheric moisture can help sustain the clouds through reducing evaporative drying during cloud-top entrainment. Enhanced subsidence above the coastal upwelling region increasing cloud droplet number concentrations may further prolong cloud lifetime through microphysical interactions. Reduced subsidence underneath stronger free-tropospheric winds at Ascension supports slightly higher cloud tops during smokier conditions. Overall the monthly changes in the large-scale aerosol and moisture vertical structure act to amplify the seasonal cycle in low-cloud amount and morphology, raising a climate importance as cloudiness changes dominate changes in the top-of-atmosphere radiation budget.

scholarly journals Sunlight-absorbing aerosol amplifies the seasonal cycle in low-cloud fraction over the southeast Atlantic

2021 ◽  
Vol 21 (14) ◽  
pp. 11179-11199
Author(s):  
Jianhao Zhang ◽  
Paquita Zuidema
Keyword(s):  
Boundary Layer ◽  
Seasonal Cycle ◽  
Large Scale ◽  
Cloud Fraction ◽  
Small Scale ◽  
Free Troposphere ◽  
Aerosol Loading ◽  
Ascension Island ◽  
Tropospheric Aerosol ◽  
Low Cloud

Abstract. The mean altitude of the smoke loading over the southeast Atlantic moves from the boundary layer in July to the free troposphere by October. This study details the month-by-month changes in cloud properties and the large-scale environment as a function of the biomass burning aerosol loading at Ascension Island (8∘ S, 14.5∘ W) from July to October, based on island measurements, satellite retrievals, and reanalysis. In July and August, the smoke loading predominantly varies within the boundary layer. During both months, the low-cloud fraction is less and is increasingly cumuliform when more smoke is present, with the exception of a late morning boundary layer deepening that encourages a short-lived cloud development. The meteorology varies little, suggesting aerosol–cloud interactions explain the cloudiness changes. September marks a transition month during which midlatitude disturbances can intrude into the Atlantic subtropics, constraining the free tropospheric aerosol closer to the African coast. Stronger boundary layer winds on cleaner days help deepen, dry, and cool much of the marine boundary layer compared to that on days with high smoke loadings, with stratocumulus reducing everywhere but at the northern deck edge. The September free troposphere is better mixed on smoky days compared to October. Longwave cooling rates, generated by a sharp water vapor gradient at the aerosol layer top, encourage a small-scale vertical mixing that could help maintain the well-mixed smoky September free troposphere. The October meteorology primarily varies as a function of the strength of the free tropospheric winds advecting aerosol offshore. The free tropospheric aerosol loading is less than in September, and the moisture variability is greater. Low-level clouds increase and are more stratiform in October when the smoke loadings are higher. The increased free tropospheric moisture can help sustain the clouds through a reduction in evaporative drying during cloud-top entrainment. Enhanced subsidence above the coastal upwelling region, increasing cloud droplet number concentrations, may further prolong cloud lifetime through microphysical interactions. Reduced subsidence underneath stronger free tropospheric winds at Ascension Island supports slightly higher cloud tops during smokier conditions. Overall, the monthly changes in the large-scale aerosol and moisture vertical structure act to amplify the seasonal cycle in low-cloud amount and morphology. This is climatically important, as cloudiness changes dominate changes in the top-of-atmosphere radiation budget.

scholarly journals Building a cloud in the Southeast Atlantic: Understanding low-cloud controls based on satellite observations with machine learning

2018 ◽  
Author(s):  
Julia Fuchs ◽  
Jan Cermak ◽  
Hendrik Andersen
Keyword(s):  
Machine Learning ◽  
Large Scale ◽  
Cloud Droplet ◽  
Reanalysis Data ◽  
Cloud Fraction ◽  
Effective Radius ◽  
Gradient Boosting ◽  
Tropospheric Temperature ◽  
Aerosol Cloud ◽  
Low Cloud

Abstract. Understanding the processes that determine low-cloud properties and aerosol–cloud interactions (ACI) is crucial for the estimation of their radiative effects. However, the covariation of meteorology and aerosols complicates the determination of cloud-relevant influences and the quantification of the aerosol–cloud relation. This study identifies and analyzes sensitivities of cloud fraction and cloud droplet effective radius to their meteorological and aerosol environment in the atmospherically stable Southeast Atlantic during the biomass-burning season. The effect of geophysical parameters on clouds is investigated based on a machine learning technique, gradient boosting regression trees (GBRTs), using a combination of satellite and reanalysis data as well as trajectory modeling of air-mass origins. A comprehensive, multivariate analysis of important drivers of cloud occurrence and properties is performed and evaluated. The statistical model reveals marked subregional differences of relevant drivers and processes determining low clouds in the Southeast Atlantic. Cloud fraction is sensitive to changes of lower tropospheric stability in the oceanic, southwestern subregion, while in the northeastern subregion it is governed mostly by surface winds. In the pristine, oceanic subregion large-scale dynamics and aerosols seem to be more important for changes of cloud droplet effective radius than in the polluted, near-shore subregion, where free tropospheric temperature is more relevant. This study suggests the necessity to consider distinct ACI regimes in cloud studies in the Southeast Atlantic.

scholarly journals Ultra-clean and smoky marine boundary layers frequently occur in the same season over the southeast Atlantic

2019 ◽  
Author(s):  
Sam Pennypacker ◽  
Michael Diamond ◽  
Robert Wood
Keyword(s):  
Boundary Layer ◽  
Boundary Layers ◽  
Liquid Water ◽  
Large Scale ◽  
Marine Boundary Layer ◽  
Median Surface ◽  
Liquid Water Path ◽  
Water Path ◽  
Aerosol Cloud ◽  
Ascension Island

Abstract. We study forty-one days with daily median surface accumulation mode aerosol particle concentrations below 50 cm−3 (ultra-clean conditions) observed at Ascension Island (7.9° S, 14.4° W) between June 2016 and October 2017 as part of the Layered Atlantic Smoke Interactions with Clouds (LASIC) campaign. Interestingly, these days occur during a period of great relevance for aerosol-cloud-radiation interactions, the southeast Atlantic (SEATL) biomass-burning season (approximately June–October). That means that these critical months can feature both the highest surface aerosol numbers, from smoke intrusion into the marine boundary layer, as well as the lowest. While carbon monoxide and refractory black carbon concentrations on ultra-clean days do not approach those on days with heavy smoke, they also frequently exceed background concentrations calculated in the non-burning season from December 2016–April 2017. This is evidence that even what become ultra-clean boundary layers can make contact with and entrain from an overlying SEATL smoke layer before undergoing a process of rapid aerosol removal. Because many ultra-clean and polluted boundary layers observed at Ascension Island follow similar isobaric back-trajectories, the variability in this entrainment is likely closely tied to the variability in the overlying smoke rather than large-scale horizontal circulation through the boundary layer. Finally, surface drizzle rates, frequencies and accumulation – as well as retrievals of liquid water path – all consistently tend toward higher values on ultra-clean days. This implicates enhanced coalescence scavenging in low clouds as the key driver of ultra-clean events in the southeast Atlantic marine boundary layer. These enhancements occur against and are likely mediated by the backdrop of a seasonal increase in daily mean cloud fraction and daily median liquid water path over ASI, peaking in September and October in both LASIC years. Therefore the seasonality in ultra-clean day occurrence seems directly linked to the seasonality in SEATL cloud properties. These results highlight the importance of two-way aerosol-cloud interactions in the region.

scholarly journals Building a cloud in the southeast Atlantic: understanding low-cloud controls based on satellite observations with machine learning

2018 ◽  
Vol 18 (22) ◽  
pp. 16537-16552 ◽  
Author(s):  
Julia Fuchs ◽  
Jan Cermak ◽  
Hendrik Andersen
Keyword(s):  
Machine Learning ◽  
Large Scale ◽  
Cloud Droplet ◽  
Cloud Fraction ◽  
Effective Radius ◽  
Gradient Boosting ◽  
Tropospheric Temperature ◽  
Data Set ◽  
Aerosol Cloud ◽  
Low Cloud

Abstract. Understanding the processes that determine low-cloud properties and aerosol–cloud interactions (ACIs) is crucial for the estimation of their radiative effects. However, the covariation of meteorology and aerosols complicates the determination of cloud-relevant influences and the quantification of the aerosol–cloud relation. This study identifies and analyzes sensitivities of cloud fraction and cloud droplet effective radius to their meteorological and aerosol environment in the atmospherically stable southeast Atlantic during the biomass-burning season based on an 8-day-averaged data set. The effect of geophysical parameters on clouds is investigated based on a machine learning technique, gradient boosting regression trees (GBRTs), using a combination of satellite and reanalysis data as well as trajectory modeling of air-mass origins. A comprehensive, multivariate analysis of important drivers of cloud occurrence and properties is performed and evaluated. The statistical model reveals marked subregional differences of relevant drivers and processes determining low clouds in the southeast Atlantic. Cloud fraction is sensitive to changes of lower tropospheric stability in the oceanic, southwestern subregion, while in the northeastern subregion it is governed mostly by surface winds. In the pristine, oceanic subregion large-scale dynamics and aerosols seem to be more important for changes of cloud droplet effective radius than in the polluted, near-shore subregion, where free tropospheric temperature is more relevant. This study suggests the necessity to consider distinct ACI regimes in cloud studies in the southeast Atlantic.

scholarly journals Global and regional modeling of clouds and aerosols in the marine boundary layer during VOCALS: the VOCA Intercomparison

2014 ◽  
Vol 14 (5) ◽  
pp. 6537-6587 ◽  
Author(s):  
M. C. Wyant ◽  
C. S. Bretherton ◽  
R. Wood ◽  
G. R. Carmichael ◽  
A. Clarke ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Marine Boundary Layer ◽  
Quantitative Estimation ◽  
Cloud Droplet ◽  
South American ◽  
Aerosol Cloud ◽  
Low Cloud ◽  
Forecast Models ◽  
Low Cloud Cover ◽  
Aerosol Cloud Interactions

Abstract. A diverse collection of models are used to simulate the marine boundary layer in the Southeast Pacific region during the period of the October–November 2008 VOCALS REx field campaign. Regional models simulate the period continuously in boundary-forced free-running mode, while global forecast models and GCMs are run in forecast mode. The models are compared to extensive observations along a line at 20° S extending westward from the South American coast. Most of the models simulate cloud and aerosol characteristics and gradients across the region that are recognizably similar to observations, despite the complex interaction of processes involved in the problem, many of which are parameterized or poorly resolved. Some models simulate the regional low cloud cover well, though many models underestimate MBL depth near the coast. Most models qualitatively simulate the observed offshore gradients of SO2, sulfate aerosol, CCN concentration in the MBL, and the related gradient in cloud droplet concentrations, but there are large quantitative intermodel differences in both means and gradients of these quantities. Most models underestimate large CCN (at 0.1% supersaturation) in the MBL and free troposphere. The GCMs also have difficulty simulating coastal gradients in CCN and cloud droplet number concentration. The overall performance of the models demonstrates their potential utility in simulating aerosol-cloud interactions in the MBL, though quantitative estimation of aerosol-cloud interactions and aerosol indirect effects of MBL clouds with these models remains uncertain.

scholarly journals Significant underestimation of radiative forcing by aerosol–cloud interactions derived from satellite-based methods

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Hailing Jia ◽  
Xiaoyan Ma ◽  
Fangqun Yu ◽  
Johannes Quaas
Keyword(s):  
Radiative Forcing ◽  
Cloud Fraction ◽  
Future Climate Change ◽  
Satellite Measurements ◽  
Aerosol Cloud ◽  
Fine Mode ◽  
Sampling Biases ◽  
Aerosol Cloud Interactions ◽  
Significant Underestimation ◽  
Weak Satellite

AbstractSatellite-based estimates of radiative forcing by aerosol–cloud interactions (RFaci) are consistently smaller than those from global models, hampering accurate projections of future climate change. Here we show that the discrepancy can be substantially reduced by correcting sampling biases induced by inherent limitations of satellite measurements, which tend to artificially discard the clouds with high cloud fraction. Those missed clouds exert a stronger cooling effect, and are more sensitive to aerosol perturbations. By accounting for the sampling biases, the magnitude of RFaci (from −0.38 to −0.59 W m−2) increases by 55 % globally (133 % over land and 33 % over ocean). Notably, the RFaci further increases to −1.09 W m−2 when switching total aerosol optical depth (AOD) to fine-mode AOD that is a better proxy for CCN than AOD. In contrast to previous weak satellite-based RFaci, the improved one substantially increases (especially over land), resolving a major difference with models.

Pressure gradient effects on the large-scale structure of turbulent boundary layers

2013 ◽  
Vol 715 ◽  
pp. 477-498 ◽  
Author(s):  
Zambri Harun ◽  
Jason P. Monty ◽  
Romain Mathis ◽  
Ivan Marusic
Keyword(s):  
Boundary Layer ◽  
Reynolds Number ◽  
Pressure Gradient ◽  
Boundary Layers ◽  
Amplitude Modulation ◽  
Large Scale ◽  
Outer Region ◽  
Adverse Pressure Gradient ◽  
Turbulent Boundary Layers ◽  
Small Scale

AbstractResearch into high-Reynolds-number turbulent boundary layers in recent years has brought about a renewed interest in the larger-scale structures. It is now known that these structures emerge more prominently in the outer region not only due to increased Reynolds number (Metzger & Klewicki, Phys. Fluids, vol. 13(3), 2001, pp. 692–701; Hutchins & Marusic, J. Fluid Mech., vol. 579, 2007, pp. 1–28), but also when a boundary layer is exposed to an adverse pressure gradient (Bradshaw, J. Fluid Mech., vol. 29, 1967, pp. 625–645; Lee & Sung, J. Fluid Mech., vol. 639, 2009, pp. 101–131). The latter case has not received as much attention in the literature. As such, this work investigates the modification of the large-scale features of boundary layers subjected to zero, adverse and favourable pressure gradients. It is first shown that the mean velocities, turbulence intensities and turbulence production are significantly different in the outer region across the three cases. Spectral and scale decomposition analyses confirm that the large scales are more energized throughout the entire adverse pressure gradient boundary layer, especially in the outer region. Although more energetic, there is a similar spectral distribution of energy in the wake region, implying the geometrical structure of the outer layer remains universal in all cases. Comparisons are also made of the amplitude modulation of small scales by the large-scale motions for the three pressure gradient cases. The wall-normal location of the zero-crossing of small-scale amplitude modulation is found to increase with increasing pressure gradient, yet this location continues to coincide with the large-scale energetic peak wall-normal location (as has been observed in zero pressure gradient boundary layers). The amplitude modulation effect is found to increase as pressure gradient is increased from favourable to adverse.

Buoyancy effects on large-scale motions in convective atmospheric boundary layers: implications for modulation of near-wall processes

2018 ◽  
Vol 856 ◽  
pp. 135-168 ◽  
Author(s):  
S. T. Salesky ◽  
W. Anderson
Keyword(s):  
Boundary Layer ◽  
Velocity Field ◽  
Boundary Layers ◽  
Vertical Velocity ◽  
Amplitude Modulation ◽  
Large Scale ◽  
Streamwise Velocity ◽  
Small Scale ◽  
Convective Conditions ◽  
Wide Range

A number of recent studies have demonstrated the existence of so-called large- and very-large-scale motions (LSM, VLSM) that occur in the logarithmic region of inertia-dominated wall-bounded turbulent flows. These regions exhibit significant streamwise coherence, and have been shown to modulate the amplitude and frequency of small-scale inner-layer fluctuations in smooth-wall turbulent boundary layers. In contrast, the extent to which analogous modulation occurs in inertia-dominated flows subjected to convective thermal stratification (low Richardson number) and Coriolis forcing (low Rossby number), has not been considered. And yet, these parameter values encompass a wide range of important environmental flows. In this article, we present evidence of amplitude modulation (AM) phenomena in the unstably stratified (i.e. convective) atmospheric boundary layer, and link changes in AM to changes in the topology of coherent structures with increasing instability. We perform a suite of large eddy simulations spanning weakly ($-z_{i}/L=3.1$) to highly convective ($-z_{i}/L=1082$) conditions (where$-z_{i}/L$is the bulk stability parameter formed from the boundary-layer depth$z_{i}$and the Obukhov length $L$) to investigate how AM is affected by buoyancy. Results demonstrate that as unstable stratification increases, the inclination angle of surface layer structures (as determined from the two-point correlation of streamwise velocity) increases from$\unicode[STIX]{x1D6FE}\approx 15^{\circ }$for weakly convective conditions to nearly vertical for highly convective conditions. As$-z_{i}/L$increases, LSMs in the streamwise velocity field transition from long, linear updrafts (or horizontal convective rolls) to open cellular patterns, analogous to turbulent Rayleigh–Bénard convection. These changes in the instantaneous velocity field are accompanied by a shift in the outer peak in the streamwise and vertical velocity spectra to smaller dimensionless wavelengths until the energy is concentrated at a single peak. The decoupling procedure proposed by Mathiset al.(J. Fluid Mech., vol. 628, 2009a, pp. 311–337) is used to investigate the extent to which amplitude modulation of small-scale turbulence occurs due to large-scale streamwise and vertical velocity fluctuations. As the spatial attributes of flow structures change from streamwise to vertically dominated, modulation by the large-scale streamwise velocity decreases monotonically. However, the modulating influence of the large-scale vertical velocity remains significant across the stability range considered. We report, finally, that amplitude modulation correlations are insensitive to the computational mesh resolution for flows forced by shear, buoyancy and Coriolis accelerations.

scholarly journals Implementation of aerosol–cloud interactions in the regional atmosphere–aerosol model COSMO-MUSCAT(5.0) and evaluation using satellite data

2017 ◽  
Vol 10 (6) ◽  
pp. 2231-2246 ◽  
Author(s):  
Sudhakar Dipu ◽  
Johannes Quaas ◽  
Ralf Wolke ◽  
Jens Stoll ◽  
Andreas Mühlbauer ◽  
...  
Keyword(s):  
Satellite Data ◽  
Transport Model ◽  
Cloud Condensation Nuclei ◽  
Cloud Droplet ◽  
Atmospheric Model ◽  
Horizontal Resolution ◽  
Small Scale ◽  
Aerosol Model ◽  
Aerosol Cloud ◽  
Aerosol Cloud Interactions

Abstract. The regional atmospheric model Consortium for Small-scale Modeling (COSMO) coupled to the Multi-Scale Chemistry Aerosol Transport model (MUSCAT) is extended in this work to represent aerosol–cloud interactions. Previously, only one-way interactions (scavenging of aerosol and in-cloud chemistry) and aerosol–radiation interactions were included in this model. The new version allows for a microphysical aerosol effect on clouds. For this, we use the optional two-moment cloud microphysical scheme in COSMO and the online-computed aerosol information for cloud condensation nuclei concentrations (Cccn), replacing the constant Cccn profile. In the radiation scheme, we have implemented a droplet-size-dependent cloud optical depth, allowing now for aerosol–cloud–radiation interactions. To evaluate the models with satellite data, the Cloud Feedback Model Intercomparison Project Observation Simulator Package (COSP) has been implemented. A case study has been carried out to understand the effects of the modifications, where the modified modeling system is applied over the European domain with a horizontal resolution of 0.25°  ×  0.25°. To reduce the complexity in aerosol–cloud interactions, only warm-phase clouds are considered. We found that the online-coupled aerosol introduces significant changes for some cloud microphysical properties. The cloud effective radius shows an increase of 9.5 %, and the cloud droplet number concentration is reduced by 21.5 %.

scholarly journals Magnetosheath-cusp interface

2004 ◽  
Vol 22 (1) ◽  
pp. 183-212 ◽  
Author(s):  
S. Savin ◽  
L. Zelenyi ◽  
S. Romanov ◽  
I. Sandahl ◽  
J. Pickett ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Solar Wind ◽  
Magnetic Fields ◽  
Large Scale ◽  
Traditional Approach ◽  
Qualitative Difference ◽  
Small Scale ◽  
Nonlinear Phenomena ◽  
Solar Wind Interaction ◽  
Linear Superposition

Abstract. We advance the achievements of Interball-1 and other contemporary missions in exploration of the magnetosheath-cusp interface. Extensive discussion of published results is accompanied by presentation of new data from a case study and a comparison of those data within the broader context of three-year magnetopause (MP) crossings by Interball-1. Multi-spacecraft boundary layer studies reveal that in ∼80% of the cases the interaction of the magnetosheath (MSH) flow with the high latitude MP produces a layer containing strong nonlinear turbulence, called the turbulent boundary layer (TBL). The TBL contains wave trains with flows at approximately the Alfvén speed along field lines and "diamagnetic bubbles" with small magnetic fields inside. A comparison of the multi-point measurements obtained on 29 May 1996 with a global MHD model indicates that three types of populating processes should be operative: large-scale (∼few RE) anti-parallel merging at sites remote from the cusp; medium-scale (few thousandkm) local TBL-merging of fields that are anti-parallel on average; small-scale (few hundredkm) bursty reconnection of fluctuating magnetic fields, representing a continuous mechanism for MSH plasma inflow into the magnetosphere, which could dominate in quasi-steady cases. The lowest frequency (∼1–2mHz) TBL fluctuations are traced throughout the magnetosheath from the post-bow shock region up to the inner magnetopause border. The resonance of these fluctuations with dayside flux tubes might provide an effective correlative link for the entire dayside region of the solar wind interaction with the magnetopause and cusp ionosphere. The TBL disturbances are characterized by kinked, double-sloped wave power spectra and, most probably, three-wave cascading. Both elliptical polarization and nearly Alfvénic phase velocities with characteristic dispersion indicate the kinetic Alfvénic nature of the TBL waves. The three-wave phase coupling could effectively support the self-organization of the TBL plasma by means of coherent resonant-like structures. The estimated characteristic scale of the "resonator" is of the order of the TBL dimension over the cusps. Inverse cascades of kinetic Alfvén waves are proposed for forming the larger scale "organizing" structures, which in turn synchronize all nonlinear cascades within the TBL in a self-consistent manner. This infers a qualitative difference from the traditional approach, wherein the MSH/cusp interaction is regarded as a linear superposition of magnetospheric responses on the solar wind or MSH disturbances. Key words. Magnetospheric physics (magnetopause, cusp, and boundary layers) – Space plasma physics (turbulence; nonlinear phenomena)

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