scholarly journals Marine aerosol properties over the Southern Ocean in relation to the wintertime meteorological conditions

2022 ◽  
Vol 22 (1) ◽  
pp. 119-137
Author(s):  
Manu Anna Thomas ◽  
Abhay Devasthale ◽  
Michael Kahnert
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Relative Humidity ◽  
Southern Ocean ◽  
Surface Wind ◽  
Ocean Surface ◽  
Meteorological Conditions ◽  
Sea Salt ◽  
Aerosol Backscatter ◽  
Aerosol Properties

Abstract. Given the vast expanse of oceans on our planet, marine aerosols (and sea salt in particular) play an important role in the climate system via multitude of direct and indirect effects. The efficacy of their net impact, however, depends strongly on the local meteorological conditions that influence their physical, optical and chemical properties. Understanding the coupling between aerosol properties and meteorological conditions is therefore important. It has been historically difficult to statistically quantify this coupling over larger oceanic areas due to the lack of suitable observations, leading to large uncertainties in the representation of aerosol processes in climate models. Perhaps no other region shows higher uncertainties in the representation of marine aerosols and their effects than the Southern Ocean. During winter the Southern Ocean boundary layer is dominated by sea salt emissions. Here, using 10 years of austral winter period (June, July and August, 2007–2016) space-based aerosol profiling by CALIOP-CALIPSO in combination with meteorological reanalysis data, we investigated the sensitivity of marine aerosol properties over the Southern Ocean (40–65∘ S) to various meteorological parameters, such as vertical relative humidity (RH), surface wind speed and sea surface temperature (SST) in terms of joint histograms. The sensitivity study is done for the climatological conditions and for the enhanced cyclonic and anticyclonic conditions in order to understand the impact of large-scale atmospheric circulation on the aerosol properties. We find a clear demarcation in the 532 nm aerosol backscatter and extinction at RH around 60 %, irrespective of the state of the atmosphere. The backscatter and extinction increase at higher relative humidity as a function of surface wind speed. This is mainly because of the water uptake by the wind-driven sea salt aerosols at high RH near the ocean surface resulting in an increase in size, which is confirmed by the decreased depolarization for the wet aerosols. An increase in aerosol backscatter and extinction is observed during the anticyclonic conditions compared to cyclonic conditions for the higher wind speeds and relative humidity, mainly due to aerosols being confined to the boundary layer, and their proximity to the ocean surface facilitates the growth of the particles. We further find a very weak dependency of aerosol backscatter on SSTs at lower wind speeds. However, when the winds are stronger than about 12 m s−1, the backscattering coefficient generally increases with SST. When aerosol properties are investigated in terms of aerosol verticality and in relation to meteorological parameters, it is seen that the aerosol backscatter values in the free troposphere (pressure <850 hPa) are much lower than in the boundary layer, irrespective of the RH and the three weather states. This indicates that the local emissions from the ocean surface make the dominant contribution to aerosol loads over the Southern Ocean. A clear separation of particulate depolarization is observed in the free and lower troposphere, more prominent in the climatological mean and the cyclonic states. For RH > 60 %, low depolarization values are noticeable in the lower troposphere, which is an indication of the dominance of water-coated and mostly spherical sea salt particles. For RH < 60 %, there are instances when the aerosol depolarization increases in the boundary layer; this is more prominent in the mean and anticyclonic cases, which can be associated with the presence of drier aerosol particles. Based on the joint histograms investigated here, we provide third-degree polynomials to obtain aerosol extinction and backscatter as a function of wind speed and relative humidity. Additionally, backscattering coefficient is also expressed jointly in terms of wind speed and sea surface temperature. Furthermore, depolarization is expressed as a function of relative humidity. These fitting functions would be useful to test and improve the parameterizations of sea salt aerosols in the climate models. We also note some limitations of our study. For example, interpreting the verticality of aerosol properties (especially depolarization) in relation to the meteorological conditions in the free and upper troposphere (pressure <850 hPa) was challenging. Furthermore, we do not see any direct evidence of sudden crystallization (efflorescence), deliquescence or hysteresis effects of the aerosols. Observing such effects will likely require a targeted investigation of individual cases considering tracer transport, rather than the statistical sensitivity study that entails temporally and geographically averaged large data sets.

scholarly journals Marine aerosol properties over the Southern Ocean in relation to the wintertime meteorological conditions

2021 ◽  
Author(s):  
Manu Anna Thomas ◽  
Abhay Devasthale ◽  
Michael Kahnert
Keyword(s):  
Boundary Layer ◽  
Relative Humidity ◽  
Southern Ocean ◽  
Surface Wind ◽  
Lower Troposphere ◽  
Ocean Surface ◽  
Meteorological Conditions ◽  
Sea Salt ◽  
Aerosol Backscatter ◽  
Aerosol Properties

Abstract. Given the vast expanse of oceans on our planet, marine aerosols, and sea salt in particular, play an important role in the climate system via multitude of direct and indirect effects. The efficacy of their net impact however depends strongly on the local meteorological conditions that influence their physical, optical and chemical properties. Understanding the coupling between aerosol properties and meteorological conditions is therefore important. It has been historically difficult to statistically quantify this coupling over larger oceanic areas due to the lack of suitable observations, leading to large uncertainties in the representation of aerosol processes in climate models. Perhaps no other region shows higher uncertainties in the representation of marine aerosols and their effects than the Southern Ocean. During winter the Southern Ocean boundary layer is dominated by sea salt emissions. Here, using 10 years of austral winter period (June, July and August, 2007–2016) space based aerosol profiling by CALIOP-CALIPSO in combination with meteorological reanalysis data, we investigated the sensitivity of marine aerosol properties over the Southern Ocean (40S–65S) to various meteorological parameters, such as vertical relative humidity (RH), surface wind speed, and sea surface temperature (SST) in terms of joint histograms. The sensitivity study is done for the climatological conditions as well as for the enhanced cyclonic and anticyclonic conditions in order to understand the impact of large-scale atmospheric circulation on the aerosol properties. We find a clear demarcation in the 532 nm aerosol backscatter and extinction at RH around 60 %, irrespective of the state of the atmosphere. The backscatter and extinction increase at higher relative humidity as a function of surface wind speed. This is mainly because of the water uptake by the wind driven sea salt aerosols at high RH near the ocean surface resulting in an increase in size, which is confirmed by the decreased depolarization for the wet aerosols. An increase in aerosol backscatter and extinction is observed during the anticyclonic conditions compared to cyclonic conditions for the higher wind speeds and relative humidity, mainly due to aerosols being confined to the boundary layer and their proximity to the ocean surface facilitates the growth of the particles. We further find a very weak dependency of aerosol backscatter on SSTs at lower wind speeds. But when the winds are stronger than about 12 m/s, the backscattering coefficient generally increases with SST. When aerosol properties are investigated in terms of aerosol verticality and in relation to meteorological parameters, it is seen that the aerosol backscatter values in the free troposphere (pressure < 850 hPa) are much lower than in the boundary layer, irrespective of the RH and the three weather states. This indicates that the local emissions from the ocean surface make the dominant contribution to aerosol loads over the Southern Ocean. A clear separation of particulate depolarization is observed in the free and lower troposphere, more prominent in the climatological mean and the cyclonic states. For RH > 60 %, low depolarization values are noticeable in the lower troposphere, which is an indication of the dominance of water-coated, mostly spherical sea salt particles. For RH < 60 %, there are instances when the aerosol depolarization increases in the boundary layer, more prominently in the mean and anticyclonic cases which can be associated with the presence of drier aerosol particles. We also note some limitations of our study. For example, interpreting the verticality of aerosol properties (especially depolarization) in relation to the meteorological conditions in the free and upper troposphere (pressure < 850 hPa) was challenging. Furthermore, we do not see any direct evidence of sudden crystallization (efflorescence), deliquescence, or hysteresis effects of the aerosols. Observing such effects will likely require a targeted investigation of individual cases considering tracer transport, rather than the statistical sensitivity study that entails temporally and geographically averaged large data sets.

Ocean surface wind speed retrieval from C-band quad-polarized SAR measurements at optimal spatial resolution

2020 ◽  
Vol 12 (2) ◽  
pp. 155-164
Author(s):  
He Fang ◽  
William Perrie ◽  
Gaofeng Fan ◽  
Tao Xie ◽  
Jingsong Yang
Keyword(s):  
Wind Speed ◽  
Spatial Resolution ◽  
Surface Wind ◽  
Ocean Surface ◽  
Surface Wind Speed ◽  
Ocean Surface Wind

scholarly journals Evaluation of the AMPS Boundary Layer Simulations on the Ross Ice Shelf, Antarctica, with Unmanned Aircraft Observations

2017 ◽  
Vol 56 (8) ◽  
pp. 2239-2258 ◽  
Author(s):  
Jonathan D. Wille ◽  
David H. Bromwich ◽  
John J. Cassano ◽  
Melissa A. Nigro ◽  
Marian E. Mateling ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Wind Speed ◽  
Relative Humidity ◽  
High Wind ◽  
Ice Shelf ◽  
High Wind Speed ◽  
Near Surface ◽  
Ross Ice Shelf ◽  
Low Cloud ◽  
The Antarctic

AbstractAccurately predicting moisture and stability in the Antarctic planetary boundary layer (PBL) is essential for low-cloud forecasts, especially when Antarctic forecasters often use relative humidity as a proxy for cloud cover. These forecasters typically rely on the Antarctic Mesoscale Prediction System (AMPS) Polar Weather Research and Forecasting (Polar WRF) Model for high-resolution forecasts. To complement the PBL observations from the 30-m Alexander Tall Tower! (ATT) on the Ross Ice Shelf as discussed in a recent paper by Wille and coworkers, a field campaign was conducted at the ATT site from 13 to 26 January 2014 using Small Unmanned Meteorological Observer (SUMO) aerial systems to collect PBL data. The 3-km-resolution AMPS forecast output is combined with the global European Centre for Medium-Range Weather Forecasts interim reanalysis (ERAI), SUMO flights, and ATT data to describe atmospheric conditions on the Ross Ice Shelf. The SUMO comparison showed that AMPS had an average 2–3 m s−1 high wind speed bias from the near surface to 600 m, which led to excessive mechanical mixing and reduced stability in the PBL. As discussed in previous Polar WRF studies, the Mellor–Yamada–Janjić PBL scheme is likely responsible for the high wind speed bias. The SUMO comparison also showed a near-surface 10–15-percentage-point dry relative humidity bias in AMPS that increased to a 25–30-percentage-point deficit from 200 to 400 m above the surface. A large dry bias at these critical heights for aircraft operations implies poor AMPS low-cloud forecasts. The ERAI showed that the katabatic flow from the Transantarctic Mountains is unrealistically dry in AMPS.

scholarly journals Deuterium excess in marine water vapor: Dependency on relative humidity and surface wind speed during evaporation

2014 ◽  
Vol 119 (2) ◽  
pp. 584-593 ◽  
Author(s):  
Marion Benetti ◽  
Gilles Reverdin ◽  
Catherine Pierre ◽  
Liliane Merlivat ◽  
Camille Risi ◽  
...  
Keyword(s):  
Water Vapor ◽  
Wind Speed ◽  
Relative Humidity ◽  
Surface Wind ◽  
Surface Wind Speed ◽  
Marine Water ◽  
Deuterium Excess

scholarly journals Estimating a relationship between aerosol optical thickness and surface wind speed over the ocean

2006 ◽  
Vol 6 (6) ◽  
pp. 11621-11651 ◽  
Author(s):  
P. Glantz ◽  
D. E. Nilsson ◽  
W. von Hoyningen-Huene
Keyword(s):  
Wind Speed ◽  
Optical Thickness ◽  
Surface Wind ◽  
Surface Wind Speed ◽  
Sea Salt ◽  
Aerosol Optical Thickness ◽  
Marine Aerosols ◽  
Hygroscopic Growth ◽  
The North ◽  
The North Pacific

Abstract. Retrieved aerosol optical thickness (AOT) based on data obtained by the Sea viewing Wide Field Sensor (SeaWiFS) is combined with surface wind speed, obtained at the European Centre for Medium-Range Weather Forecasts (ECMWFs), over the North Pacific for September 2001. In this study a cloud screening approach is introduced in an attempt to exclude pixels partly or fully covered by clouds. The relatively broad swath width for which the nadir looking SeaWiFS instrument scanned over the North Pacific means that the AOT can be estimated according to relatively large range of wind speeds for each of the scenes analyzed. The sensitivity in AOT due to sea salt and hygroscopic growth of the marine aerosols has also been investigated. The validation of the results is based on previous parameterization in combination with the environmental quantities wind speed, RH and boundary layer height (BLH), estimated at the ECMWF. In this study a factor of 2 higher mean AOT is obtained for a wind speed up to about 13 m s−1 for September 2001 over remote ocean areas. Furthermore, a factor of 2 higher AOT is more or less supported by the validation of the results. Approximately, 50% of the enhancement seems to be due to hygroscopic growth of the marine aerosols and the remaining part due to increase in the sea salt particle mass concentrations, caused by a wind driven water vapor and sea salt flux, respectively. Reasonable agreement occurs also between satellites retrieved aerosol optical thickness and AOT observed at several AERONET (Aerosol Robotic NETwork) ground-based remote sensing stations. Finally, possible reasons why relatively large standard deviations occur around the mean values of AOT estimated for a single scene are discussed.

scholarly journals Inorganic bromine in the marine boundary layer: a critical review

2003 ◽  
Vol 3 (3) ◽  
pp. 2963-3050 ◽  
Author(s):  
R. Sander ◽  
W. C. Keene ◽  
A. A. P. Pszenny ◽  
R. Arimoto ◽  
G. P. Ayers ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Gas Phase ◽  
Marine Boundary Layer ◽  
Sea Water ◽  
Ocean Surface ◽  
Sea Salt ◽  
Future Research ◽  
Laboratory Studies ◽  
Model Calculations ◽  
Sea Salt Aerosol

Abstract. The cycling of inorganic bromine in the marine boundary layer (mbl) has received increased attention in recent years. Bromide, a constituent of sea water, is injected into the atmosphere in association with sea-salt aerosol by breaking waves on the ocean surface. Measurements reveal that supermicrometer sea-salt aerosol is depleted in bromine by about 50% relative to conservative tracers, whereas marine submicrometer aerosol is often enriched in bromine. Model calculations, laboratory studies, and field observations strongly suggest that these depletions reflect the chemical transformation of particulate bromide to reactive inorganic gases that influence the processing of ozone and other important constituents of marine air. However, currently available techniques cannot reliably quantify many \\chem{Br}-containing compounds at ambient concentrations and, consequently, our understanding of inorganic Br cycling over the oceans and its global significance are uncertain. To provide a more coherent framework for future research, we have reviewed measurements in marine aerosol, the gas phase, and in rain. We also summarize sources and sinks, as well as model and laboratory studies of chemical transformations. The focus is on inorganic bromine over the open oceans, excluding the polar regions. The generation of sea-salt aerosol at the ocean surface is the major tropospheric source producing about 6.2 Tg/a of bromide. The transport of  Br from continents (as mineral aerosol, and as products from biomass-burning and fossil-fuel combustion) can be of local importance. Transport of degradation products of long-lived Br-containing compounds from the stratosphere and other sources contribute lesser amounts. Available evidence suggests that, following aerosol acidification, sea-salt bromide reacts to form Br2 and BrCl that volatilize to the gas phase and photolyze in daylight to produce atomic Br and Cl. Subsequent transformations can destroy tropospheric ozone, oxidize dimethylsulfide (DMS) and hydrocarbons in the gas phase and S(IV) in aerosol solutions, and thereby potentially influence climate. The diurnal cycle of gas-phase \\Br and the corresponding particulate Br deficits are correlated. Higher values of Br in the gas phase during daytime are consistent with expectations based on photochemistry. Mechanisms that explain the widely reported accumulation of particulate Br in submicrometer aerosols are not yet understood. We expect that the importance of inorganic Br cycling will vary in the future as a function of both increasing acidification of the atmosphere (through anthropogenic emissions) and climate changes. The latter affects bromine cycling via meteorological factors including global wind fields (and the associated production of sea-salt aerosol), temperature, and relative humidity.

scholarly journals Analysis of simultaneous aerosol and ocean glint retrieval using multi-angle observations

2020 ◽  
Author(s):  
Kirk Knobelspiesse ◽  
Amir Ibrahim ◽  
Bryan Franz ◽  
Sean Bailey ◽  
Robert Levy ◽  
...  
Keyword(s):  
Optical Properties ◽  
Wind Speed ◽  
Radiative Transfer ◽  
Size Distribution ◽  
Atmospheric Correction ◽  
Surface Wind ◽  
Ocean Surface ◽  
True Value ◽  
Aerosol State ◽  
The Impact

Abstract. Since early 2000, NASA's Multi-angle Imaging SpectroRadiometer (MISR) instrument has been performing remote sensing retrievals of aerosol optical properties from the polar orbiting Terra spacecraft. A noteworthy aspect of MISR observations over the ocean is that, for much of the Earth, some of the multi-angle views have contributions from solar reflection by the ocean surface (glint, or glitter), while others do not. Aerosol retrieval algorithms often discard these glint influenced observations because they can overwhelm the signal and are difficult to predict without knowledge of the (wind speed driven) ocean surface roughness. However, theoretical studies have shown that multi-angle observations of a location at geometries with and without reflected sun glint can be a rich source of information, sufficient to support simultaneous retrieval of both the aerosol state and the wind speed at the ocean surface. We are in the early stages of creating such an algorithm. In this manuscript, we describe our assessment of the appropriate level of parameterization for simultaneous aerosol and ocean surface property retrievals using sun glint. For this purpose, we use Generalized Nonlinear Retrieval Analysis (GENRA), an information content assessment (ICA) technique employing Bayesian inference, and simulations from the Ahmad-Fraser iterative radiative transfer code. We find that four parameters are suitable: aerosol optical depth (τ), particle size distribution (expressed as the fine mode fraction f of small particles in a bimodal size distribution), surface wind speed (w), and relative humidity (r, to define the aerosol water content and complex refractive index). None of these parameters define ocean optical properties, as we found that the aerosol state could be retrieved with the nine MISR near-infrared views alone, where the ocean body is black in the open ocean. We also found that retrieval capability varies with observation geometry, and that as τ increases so does the ability to determine aerosol intensive optical properties (r and f, while it decreases for w). Increases in wind speed decrease the ability to determine the true value of that parameter, but have minimal impact on retrieval of aerosol properties. We explored the benefit of excluding the two most extreme MISR view angles for which radiative transfer with the plane parallel approximation is less certain, but found no advantage in doing so. Finally, the impact of treating wind speed as a scalar parameter, rather than as a two parameter directional wind, was tested. While the simpler scalar model does contribute to overall aerosol uncertainty, it is not sufficiently large to justify the addition of another dimension to parameter space. An algorithm designed upon these principles is in development. It will be used to perform an atmospheric correction with MISR for coincident ocean color (OC) observations by the Moderate Resolution Imaging Spectroradiometer (MODIS) instrument, also on the NASA Terra spacecraft. Unlike MISR, MODIS is a single view angle instrument, but it has a more complete set of spectral channels ideal for determination of ocean optical properties. The atmospheric correction of MODIS OC data can therefore benefit from MISR aerosol retrievals. Furthermore, higher spatial resolution data from coincident MISR observations may also improve glint screening.

scholarly journals Evaluation of the Ocean Surface Wind Speed Change following the Super Typhoon from Space-Borne GNSS-Reflectometry

2020 ◽  
Vol 12 (12) ◽  
pp. 2034 ◽  
Author(s):  
Hongsu Liu ◽  
Shuanggen Jin ◽  
Qingyun Yan
Keyword(s):  
Wind Speed ◽  
Correlation Coefficient ◽  
Surface Wind ◽  
Ocean Surface ◽  
Surface Wind Speed ◽  
Wind Speeds ◽  
Mean Error ◽  
Super Typhoon ◽  
The Mean ◽  
Ocean Surface Wind

Ocean surface wind speed is an essential parameter for typhoon monitoring and forecasting. However, traditional satellite and buoy observations are difficult to monitor the typhoon due to high cost and low temporal-spatial resolution. With the development of spaceborne GNSS-R technology, the cyclone global navigation satellite system (CYGNSS) with eight satellites in low-earth orbit provides an opportunity to measure the ocean surface wind speed of typhoons. Though observations are made at the extremely efficient spatial and temporal resolution, its accuracy and reliability are unclear in an actual super typhoon case. In this study, the wind speed variations over the life cycle of the 2018 Typhoon Mangkhut from CYGNSS observations were evaluated and compared with European Centre for Medium-Range Weather Forecasts (ECMWF) Re-Analysis-5 (ERA-5). The results show that the overall root-mean-square error (RMSE) of CYGNSS versus ECMWF was 4.12 m/s, the mean error was 1.36 m/s, and the correlation coefficient was 0.96. For wind speeds lower and greater than 15 m/s, the RMSE of CYGNSS versus ECMWF were 1.02 and 4.36 m/s, the mean errors were 0.05 and 1.61 m/s, the correlation coefficients were 0.91 and 0.90, and the average relative errors were 9.8% and 11.6%, respectively. When the typhoon reached a strong typhoon or super typhoon, the RMSE of CYGNSS with respect to ERA-5 from ECMWF was 5.07 m/s; the mean error was 3.57 m/s; the correlation coefficient was 0.52 and the average relative error was 11.0%. The CYGNSS estimation had higher precision for wind speeds below 15 m/s, but degraded when the wind speed was above 15 m/s.

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