Long-term changes in stratospheric water vapour and its implications for climate

2020 ◽  
Author(s):  
Michaela I. Hegglin
Keyword(s):  
Water Vapour ◽  
Radiative Forcing ◽  
Climate Model ◽  
Climate Data ◽  
Theoretical Understanding ◽  
Radiative Balance ◽  
Surface Climate ◽  
Long Term Changes ◽  
Stratospheric Water Vapour

<p>Water vapour is the most important natural greenhouse gas in the atmosphere and provides a positive feedback to the climate forcing from carbon dioxide. Water vapour is also the source of hydroxyl (OH) which controls the lifetime of shorter-lived pollutants and long-lived greenhouse gases. Despite the importance of water vapour to chemistry and the radiative balance of the atmosphere, its observed long-term changes in the stratosphere are not well understood, and may even conflict with the theoretical understanding of its drivers. </p><p>I here present a new climate data record of stratospheric water vapour developed within the ESA Water Vapour Climate Change Initiative and discuss recent changes in stratospheric water vapour concentrations in the light of earlier observational studies, modelling results from the SPARC Chemistry-Climate Model Initiative, and our theoretical understanding of its drivers. In addition, the radiative forcing of surface climate and inferred changes in the Brewer-Dobson Circulation will be highlighted. </p>

scholarly journals The role of methane in projections of 21st century stratospheric water vapour

2016 ◽  
Author(s):  
Laura Revell ◽  
Andrea Stenke ◽  
Eugene Rozanov ◽  
William Ball ◽  
Stefan Lossow ◽  
...  
Keyword(s):  
Water Vapour ◽  
Methane Oxidation ◽  
21St Century ◽  
Radiative Forcing ◽  
Lower Stratosphere ◽  
Climate Model ◽  
Radiative Balance ◽  
Canonical Representative ◽  
Cold Point ◽  
Stratospheric Water Vapour

Abstract. Stratospheric water vapour (SWV) is an important component of the Earth's atmosphere as it affects both radiative balance and the chemistry of the atmosphere. Key processes driving changes in SWV through the 21st century include dehydration of air masses transiting the cold-point tropopause (CPT) and methane oxidation. Increasing surface temperatures may strengthen the Brewer-Dobson circulation, such that more methane is transported into the stratosphere where it can be oxidised to SWV. We use a chemistry-climate model to simulate changes in SWV through the 21st century following the four canonical Representative Concentration Pathways (RCPs). Furthermore, we quantify the contribution that methane oxidation makes to SWV following each of the RCPs. The methane contribution to SWV maximises in the upper stratosphere, however modelled SWV trends are found to be driven predominantly by warming of the CPT and strengthening of the Brewer-Dobson circulation rather than by increasing methane oxidation. SWV changes by −5 % to 60 % (depending on the location in the atmosphere and emissions scenario) and increases in the lower stratosphere in all RCPs through the 21st century. Because the lower stratosphere is where water vapour radiative forcing maximises, SWV's influence on surface climate is also expected to increase through the 21st century.

scholarly journals The role of methane in projections of 21st century stratospheric water vapour

2016 ◽  
Vol 16 (20) ◽  
pp. 13067-13080 ◽  
Author(s):  
Laura E. Revell ◽  
Andrea Stenke ◽  
Eugene Rozanov ◽  
William Ball ◽  
Stefan Lossow ◽  
...  
Keyword(s):  
Water Vapour ◽  
Methane Oxidation ◽  
21St Century ◽  
Radiative Forcing ◽  
Lower Stratosphere ◽  
Climate Model ◽  
Radiative Balance ◽  
Canonical Representative ◽  
Cold Point ◽  
Stratospheric Water Vapour

Abstract. Stratospheric water vapour (SWV) is an important component of the Earth's atmosphere as it affects both radiative balance and the chemistry of the atmosphere. Key processes driving changes in SWV include dehydration of air masses transiting the cold-point tropopause (CPT) and methane oxidation. We use a chemistry–climate model to simulate changes in SWV through the 21st century following the four canonical representative concentration pathways (RCPs). Furthermore, we quantify the contribution that methane oxidation makes to SWV following each of the RCPs. Although the methane contribution to SWV maximizes in the upper stratosphere, modelled SWV trends are found to be driven predominantly by warming of the CPT rather than by increasing methane oxidation. SWV changes by −5 to 60 % (depending on the location in the atmosphere and emissions scenario) and increases in the lower stratosphere in all RCPs through the 21st century. Because the lower stratosphere is where water vapour radiative forcing maximizes, SWV's influence on surface climate is also expected to increase through the 21st century.

scholarly journals Effects of Strongly Enhanced Atmospheric Methane Concentrations in a Fully Coupled Chemistry-Climate Model

2020 ◽  
Author(s):  
Laura Stecher ◽  
Franziska Winterstein ◽  
Martin Dameris ◽  
Patrick Jöckel ◽  
Michael Ponater ◽  
...  
Keyword(s):  
Hydroxyl Radical ◽  
Water Vapour ◽  
Climate Sensitivity ◽  
Radiative Forcing ◽  
Climate Model ◽  
Atmospheric Methane ◽  
Climate Feedbacks ◽  
Mixing Ratios ◽  
Radiative Impact ◽  
Stratospheric Water Vapour

Abstract. In a previous study the quasi-instantaneous chemical impacts (rapid adjustments) of strongly enhanced methane (CH4) mixing ratios have been analyzed. However, to quantify the influence of the respective slow climate feedbacks on the chemical composition it is necessary to include the radiation driven temperature feedback. Therefore, we perform sensitivity simulations with doubled and fivefold present-day (year 2010) CH4 mixing ratios with the chemistry-climate model EMAC and include in a novel set-up a mixed layer ocean model to account for tropospheric warming. We find that the slow climate feedbacks counteract the reduction of the hydroxyl radical in the troposphere, which is caused by the strongly enhanced CH4 mixing ratios. Thereby also the resulting prolongation of the tropospheric CH4 lifetime is weakened compared to the quasi-instantaneous response considered previously. Changes in the stratospheric circulation evolve clearly with the warming of the troposphere. The Brewer-Dobson circulation strengthens, affecting the response of trace gases, such as ozone, water vapour and CH4 in the stratosphere, and also causing stratospheric temperature changes. In the middle and upper stratosphere, the increase of stratospheric water vapour is reduced with respect to the quasi-instantaneous response. Weaker increases of the hydroxyl radical cause the chemical depletion of CH4 to be less strongly enhanced and thus the in situ source of stratospheric water vapour as well. However, in the lower stratosphere water vapour increases more strongly when tropospheric warming is accounted for enlarging its overall radiative impact. The response of the stratospheric adjusted temperatures driven by slow climate feedbacks is dominated by these increases of stratospheric water vapour, as well as strongly decreased ozone mixing ratios above the tropical tropopause, which result from enhanced tropical upwelling. While rapid radiative adjustments from ozone and stratospheric water vapour make an essential contribution to the effective CH4 radiative forcing, the radiative impact of the respective slow feedbacks is rather moderate. In line with this, the climate sensitivity from CH4 changes in this chemistry-climate model setup is not significantly different from the climate sensitivity in carbon dioxide-driven simulations, provided that the CH4 effective radiative forcing includes the rapid adjustments from ozone and stratospheric water vapour changes.

scholarly journals Slow feedbacks resulting from strongly enhanced atmospheric methane mixing ratios in a chemistry–climate model with mixed-layer ocean

2021 ◽  
Vol 21 (2) ◽  
pp. 731-754
Author(s):  
Laura Stecher ◽  
Franziska Winterstein ◽  
Martin Dameris ◽  
Patrick Jöckel ◽  
Michael Ponater ◽  
...  
Keyword(s):  
Water Vapour ◽  
Climate Sensitivity ◽  
Radiative Forcing ◽  
Climate Model ◽  
Climate Feedbacks ◽  
Mixing Ratios ◽  
Mixed Layer Ocean ◽  
Radiative Impact ◽  
Set Up ◽  
Stratospheric Water Vapour

Abstract. In a previous study the quasi-instantaneous chemical impacts (rapid adjustments) of strongly enhanced methane (CH4) mixing ratios have been analysed. However, to quantify the influence of the respective slow climate feedbacks on the chemical composition it is necessary to include the radiation-driven temperature feedback. Therefore, we perform sensitivity simulations with doubled and quintupled present-day (year 2010) CH4 mixing ratios with the chemistry–climate model EMAC (European Centre for Medium-Range Weather Forecasts, Hamburg version – Modular Earth Submodel System (ECHAM/MESSy) Atmospheric Chemistry) and include in a novel set-up a mixed-layer ocean model to account for tropospheric warming. Strong increases in CH4 lead to a reduction in the hydroxyl radical in the troposphere, thereby extending the CH4 lifetime. Slow climate feedbacks counteract this reduction in the hydroxyl radical through increases in tropospheric water vapour and ozone, thereby dampening the extension of CH4 lifetime in comparison with the quasi-instantaneous response. Changes in the stratospheric circulation evolve clearly with the warming of the troposphere. The Brewer–Dobson circulation strengthens, affecting the response of trace gases, such as ozone, water vapour and CH4 in the stratosphere, and also causing stratospheric temperature changes. In the middle and upper stratosphere, the increase in stratospheric water vapour is reduced with respect to the quasi-instantaneous response. We find that this difference cannot be explained by the response of the cold point and the associated water vapour entry values but by a weaker strengthening of the in situ source of water vapour through CH4 oxidation. However, in the lower stratosphere water vapour increases more strongly when tropospheric warming is accounted for, enlarging its overall radiative impact. The response of the stratosphere adjusted temperatures driven by slow climate feedbacks is dominated by these increases in stratospheric water vapour as well as strongly decreased ozone mixing ratios above the tropical tropopause, which result from enhanced tropical upwelling. While rapid radiative adjustments from ozone and stratospheric water vapour make an essential contribution to the effective CH4 radiative forcing, the radiative impact of the respective slow feedbacks is rather moderate. In line with this, the climate sensitivity from CH4 changes in this chemistry–climate model set-up is not significantly different from the climate sensitivity in carbon-dioxide-driven simulations, provided that the CH4 effective radiative forcing includes the rapid adjustments from ozone and stratospheric water vapour changes.

Why does the climate response to greenhouse warming and greenhouse cooling differ? 

2021 ◽  
Author(s):  
Jennifer Kay ◽  
Jason Chalmers
Keyword(s):  
Carbon Dioxide ◽  
Radiative Forcing ◽  
Climate Model ◽  
Temperature Response ◽  
Greenhouse Warming ◽  
Climate Response ◽  
Cloud Feedbacks ◽  
Surface Climate ◽  
Carbon Dioxide Concentrations ◽  
Radiative Feedbacks

<p>While the long-standing quest to constrain equilibrium climate sensitivity has resulted in intense scrutiny of the processes controlling idealized greenhouse warming, the processes controlling idealized greenhouse cooling have received less attention. Here, differences in the climate response to increased and decreased carbon dioxide concentrations are assessed in state-of-the-art fully coupled climate model experiments. One hundred and fifty years after an imposed instantaneous forcing change, surface global warming from a carbon dioxide doubling (abrupt-2xCO2, 2.43 K) is larger than the surface global cooling from a carbon dioxide halving (abrupt-0p5xCO2, 1.97 K). Both forcing and feedback differences explain these climate response differences. Multiple approaches show the radiative forcing for a carbon dioxide doubling is ~10% larger than for a carbon dioxide halving. In addition, radiative feedbacks are less negative in the doubling experiments than in the halving experiments. Specifically, less negative tropical shortwave cloud feedbacks and more positive subtropical cloud feedbacks lead to more greenhouse 2xCO2 warming than 0.5xCO2 greenhouse cooling. Motivated to directly isolate the influence of cloud feedbacks on these experiments, additional abrupt-2xCO2 and abrupt-0p5xCO2 experiments with disabled cloud-climate feedbacks were run. Comparison of these “cloud-locked” simulations with the original “cloud active” simulations shows cloud feedbacks help explain the nonlinear global surface temperature response to greenhouse warming and greenhouse cooling. Overall, these results demonstrate that both radiative forcing and radiative feedbacks are needed to explain differences in the surface climate response to increased and decreased carbon dioxide concentrations.</p>

scholarly journals Simulation of the isotopic composition of stratospheric water vapour – Part 1: Description and evaluation of the EMAC model

2015 ◽  
Vol 15 (10) ◽  
pp. 5537-5555 ◽  
Author(s):  
R. Eichinger ◽  
P. Jöckel ◽  
S. Brinkop ◽  
M. Werner ◽  
S. Lossow
Keyword(s):  
Isotopic Composition ◽  
Water Vapour ◽  
General Circulation ◽  
Climate Model ◽  
Hydrological Cycle ◽  
Circulation Model ◽  
Isotope Ratios ◽  
Physical Fractionation ◽  
Water Isotopologues ◽  
Stratospheric Water Vapour

Abstract. This modelling study aims at an improved understanding of the processes that determine the water vapour budget in the stratosphere by means of the investigation of water isotope ratios. An additional (and separate from the actual) hydrological cycle has been introduced into the chemistry–climate model EMAC, including the water isotopologues HDO and H218O and their physical fractionation processes. Additionally an explicit computation of the contribution of methane oxidation to H2O and HDO has been incorporated. The model expansions allow detailed analyses of water vapour and its isotope ratio with respect to deuterium throughout the stratosphere and in the transition region to the troposphere. In order to assure the correct representation of the water isotopologues in the model's hydrological cycle, the expanded system has been evaluated in several steps. The physical fractionation effects have been evaluated by comparison of the simulated isotopic composition of precipitation with measurements from a ground-based network (GNIP) and with the results from the isotopologue-enabled general circulation model ECHAM5-wiso. The model's representation of the chemical HDO precursor CH3D in the stratosphere has been confirmed by a comparison with chemical transport models (1-D, CHEM2D) and measurements from radiosonde flights. Finally, the simulated stratospheric HDO and the isotopic composition of water vapour have been evaluated, with respect to retrievals from three different satellite instruments (MIPAS, ACE-FTS, SMR). Discrepancies in stratospheric water vapour isotope ratios between two of the three satellite retrievals can now partly be explained.

scholarly journals Key drivers of ozone change and its radiative forcing over the 21st century

2018 ◽  
Vol 18 (9) ◽  
pp. 6121-6139 ◽  
Author(s):  
Fernando Iglesias-Suarez ◽  
Douglas E. Kinnison ◽  
Alexandru Rap ◽  
Amanda C. Maycock ◽  
Oliver Wild ◽  
...  
Keyword(s):  
Climate Change ◽  
21St Century ◽  
Radiative Forcing ◽  
Climate Model ◽  
Stratospheric Ozone ◽  
Atmospheric Composition ◽  
Climate Conditions ◽  
Radiative Balance ◽  
Radiative Forcings ◽  
Year 2000

Abstract. Over the 21st century changes in both tropospheric and stratospheric ozone are likely to have important consequences for the Earth's radiative balance. In this study, we investigate the radiative forcing from future ozone changes using the Community Earth System Model (CESM1), with the Whole Atmosphere Community Climate Model (WACCM), and including fully coupled radiation and chemistry schemes. Using year 2100 conditions from the Representative Concentration Pathway 8.5 (RCP8.5) scenario, we quantify the individual contributions to ozone radiative forcing of (1) climate change, (2) reduced concentrations of ozone depleting substances (ODSs), and (3) methane increases. We calculate future ozone radiative forcings and their standard error (SE; associated with inter-annual variability of ozone) relative to year 2000 of (1) 33 ± 104 m Wm−2, (2) 163 ± 109 m Wm−2, and (3) 238 ± 113 m Wm−2 due to climate change, ODSs, and methane, respectively. Our best estimate of net ozone forcing in this set of simulations is 430 ± 130 m Wm−2 relative to year 2000 and 760 ± 230 m Wm−2 relative to year 1750, with the 95 % confidence interval given by ±30 %. We find that the overall long-term tropospheric ozone forcing from methane chemistry–climate feedbacks related to OH and methane lifetime is relatively small (46 m Wm−2). Ozone radiative forcing associated with climate change and stratospheric ozone recovery are robust with regard to background climate conditions, even though the ozone response is sensitive to both changes in atmospheric composition and climate. Changes in stratospheric-produced ozone account for ∼ 50 % of the overall radiative forcing for the 2000–2100 period in this set of simulations, highlighting the key role of the stratosphere in determining future ozone radiative forcing.

scholarly journals Radiative forcing due to stratospheric water vapour from CH4oxidation

2007 ◽  
Vol 34 (1) ◽  
Author(s):  
Gunnar Myhre ◽  
Jørgen S. Nilsen ◽  
Line Gulstad ◽  
Keith P. Shine ◽  
Bjørg Rognerud ◽  
...  
Keyword(s):  
Water Vapour ◽  
Radiative Forcing ◽  
Stratospheric Water Vapour

scholarly journals A statistics-based reconstruction of high-resolution global terrestrial climate for the last 800,000 years

2021 ◽  
Vol 8 (1) ◽  
Author(s):  
Mario Krapp ◽  
Robert M. Beyer ◽  
Stephen L. Edmundson ◽  
Paul J. Valdes ◽  
Andrea Manica
Keyword(s):  
Net Primary Productivity ◽  
Climate Model ◽  
Global Climate ◽  
Computational Cost ◽  
Climate Data ◽  
Land Type ◽  
Research Areas ◽  
Climate Simulations ◽  
Bioclimatic Variables

AbstractCurated global climate data have been generated from climate model outputs for the last 120,000 years, whereas reconstructions going back even further have been lacking due to the high computational cost of climate simulations. Here, we present a statistically-derived global terrestrial climate dataset for every 1,000 years of the last 800,000 years. It is based on a set of linear regressions between 72 existing HadCM3 climate simulations of the last 120,000 years and external forcings consisting of CO2, orbital parameters, and land type. The estimated climatologies were interpolated to 0.5° resolution and bias-corrected using present-day climate. The data compare well with the original HadCM3 simulations and with long-term proxy records. Our dataset includes monthly temperature, precipitation, cloud cover, and 17 bioclimatic variables. In addition, we derived net primary productivity and global biome distributions using the BIOME4 vegetation model. The data are a relevant source for different research areas, such as archaeology or ecology, to study the long-term effect of glacial-interglacial climate cycles for periods beyond the last 120,000 years.

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