On the Radiative Impact of Biomass-Burning Aerosols in the Arctic: The August 2017 Case Study

Boreal fires have increased during the last years and are projected to become more intense and frequent as a consequence of climate change. Wildfires produce a wide range of effects on the Arctic climate and ecosystem, and understanding these effects is crucial for predicting the future evolution of the Arctic region. This study focuses on the impact of the long-range transport of biomass-burning aerosol into the atmosphere and the corresponding radiative perturbation in the shortwave frequency range. As a case study, we investigate an intense biomass-burning (BB) event which took place in summer 2017 in Canada and subsequent northeastward transport of gases and particles in the plume leading to exceptionally high values (0.86) of Aerosol Optical Depth (AOD) at 500 nm measured in northwestern Greenland on 21 August 2017. This work characterizes the BB plume measured at the Thule High Arctic Atmospheric Observatory (THAAO; 76.53∘N, 68.74∘W) in August 2017 by assessing the associated shortwave aerosol direct radiative impact over the THAAO and extending this evaluation over the broader region (60∘N–80∘N, 110∘W–0∘E). The radiative transfer simulations with MODTRAN6.0 estimated an aerosol heating rate of up to 0.5 K/day in the upper aerosol layer (8–12 km). The direct aerosol radiative effect (ARE) vertical profile shows a maximum negative value of −45.4 Wm−2 for a 78∘ solar zenith angle above THAAO at 3 km altitude. A cumulative surface ARE of −127.5 TW is estimated to have occurred on 21 August 2017 over a portion (∼3.1×106 km2) of the considered domain (60∘N–80∘N, 110∘W–0∘E). ARE regional mean daily values over the same portion of the domain vary between −65 and −25 Wm−2. Although this is a limited temporal event, this effect can have significant influence on the Arctic radiative budget, especially in the anticipated scenario of increasing wildfires.

Aerosol radiative impact during the summer 2019 heatwave produced partly by an inter-continental Saharan dust outbreak – Part 1: Short-wave dust direct radiative effect

The short-wave (SW) direct radiative effect (DRE) during the summer 2019 heatwave produced partly by a moderate, long-lasting Saharan dust outbreak over Europe is analysed in this study. Two European sites (periods) are considered: Barcelona, Spain (23–30 June), and Leipzig, Germany (29 and 30 June), 1350 km apart from each other. Major data are obtained from AERONET and polarised Micro-Pulse Lidar (P-MPL) observations. Modelling is used to describe the different dust pathways, as observed at both sites. The coarse dust (Dc) and fine dust (Df) components (with total dust, DD = Dc + Df) are identified in the profiles of the total particle backscatter coefficient using the POLIPHON (POlarisation LIdar PHOtometer Networking) method in synergy with P-MPL measurements. This information is used to calculate the relative mass loading and the centre-of-mass height, as well as the contribution of each dust mode to the total dust DRE. Several aspects of the ageing of dust are put forward. The mean dust optical depth and its Df/DD ratios are, respectively, 0.153 and 24 % in Barcelona and 0.039 and 38 % in Leipzig; this Df increase in Leipzig is attributed to a longer dust transport path in comparison to Barcelona. The dust produced a cooling effect on the surface with a mean daily DRE of −9.1 and −2.5 W m−2, respectively, in Barcelona and Leipzig, but the Df/DD DRE ratio is larger for Leipzig (52 %) than for Barcelona (37 %). Cooling is also observed at the top of the atmosphere (TOA), although less intense than on the surface. However, the Df/DD DRE ratio at the TOA is even higher (45 % and 60 %, respectively, in Barcelona and Leipzig) than on the surface. Despite the predominance of Dc particles under dusty conditions, the SW radiative impact of Df particles can be comparable to, even higher than, that induced by the Dc ones. In particular, the Df/DD DRE ratio in Barcelona increases by +2.4 % d−1 (surface) and +2.9 % d−1 (TOA) during the dusty period. This study is completed by a second paper about the long-wave and net radiative effects. These results are especially relevant for the next ESA EarthCARE mission (planned in 2022) as it is devoted to aerosol–cloud–radiation interaction research.

Introduction to the Special Issue “Radiative Transfer in the Earth Atmosphere”

This Special Issue aims at addressing the recent developments towards improving our understanding of the diverse radiative impact of different types of aerosols and clouds [...]

Characterisation and surface radiative impact of Arctic low clouds from the IAOOS field experiment

The Ice, Atmosphere, Arctic Ocean Observing System (IAOOS) field experiment took place from 2014 to 2019. Over this period, more than 20 instrumented buoys were deployed at the North Pole. Once locked into the ice, the buoys drifted for periods of a month to more than a year. Some of these buoys were equipped with 808 nm wavelength lidars which acquired a total of 1777 profiles over the course of the campaign. This IAOOS lidar dataset is exploited to establish a novel statistic of cloud cover and of the geometrical and optical characteristics of the lowest cloud layer. The average cloud frequency from April to December over the course of the campaign was 75 %. Cloud occurrence frequencies were above 85 % from May to October. Single layers are thickest in October/November and thinnest in the summer. Meanwhile, their optical depth is maximum in October. On the whole, the cloud base height is very low, with the great majority of first layer bases beneath 120 m. In April and October, surface temperatures are markedly warmer when the IAOOS profile contains at least one low cloud than when it does not. This temperature difference is statistically insignificant in the summer months. Indeed, summer clouds have a shortwave cooling effect which can reach −60 W m−2 and balance out their longwave warming effect.

Stratospheric residence time and the lifetime of volcanic aerosol

<p>The cumulative radiative impact of major volcanic eruptions depends strongly on the length of time volcanic sulfate aerosol remains in the stratosphere. Observations of aerosol from recent eruptions have been used to suggest that residence time depends on the latitude of the volcanic eruption, with tropical eruptions producing aerosol loading that persists longer than that from extratropical eruptions. However, the limited number of eruptions observed make it difficult to disentangle the roles of latitude and injection height in controlling aerosol lifetime. Here we use satellite observations and model experiments to explore the relationship between eruption latitude, injection height and resulting residence time of stratospheric aerosol. We find that contrary to earlier interpretations of observations, the residence time of aerosol from major tropical eruptions like Pinatubo (1991) is on the order of 24 months. Model results suggest that the residence time is greatly sensitive to the height of the sulfur injection, especially within the lowest few kilometers of the stratosphere. As injection heights and latitudes are unknown for the majority of eruptions over the common era, we estimate the impact of this uncertainty on volcanic aerosol forcing reconstructions. </p>

Variability of the aerosol content in the tropical lower stratosphere from 2013 to 2019 as influenced by moderate volcanic eruptions

<p>The cumulative impacts of frequent moderate-magnitude eruptions on stratospheric aerosols were identified among the factors in recent decadal climate trends. Moderate volcanic eruptions are a recurrent source of sulfur dioxide (SO2) in the Upper Troposphere and Lower Stratosphere (UTLS) region and the resulting formation of sulfuric acid aerosol particles from the SO2 emitted provides sites for chemical reactions leading to enhancement of stratospheric optical depth (SAOD) and ozone depletion. Modelling properly the volcanic aerosol content and its evolution in this region is important for radiative impact issues. In this work, we explore the variability of the tropical UTLS aerosol content between 2013 and 2019, a period which was particularly impacted by moderate tropical and mid-latitude volcanic eruptions. For that purpose, space-borne observations from OMPS (version 2, datasets from GES DISC), and IASI, together with simulations by the Whole Atmosphere Community Climate Model (WACCM) coupled with the Community Aerosol and Radiation Model for Atmospheres (CARMA), are used. Different model sensitive experiments, particularly for the injection altitude and timing, have been conducted to evaluate how the model captures the aerosol plume in terms of content, optical and microphysical properties, transport and residence time. We find that the decay of the Calbuco and Kelud plumes observed by OMPS version 2 is well reproduced by the model. Comparisons with unique datasets in the tropical southern hemisphere from the NDACC Maïdo observatory (Reunion Island, France, 20.5°S, 55.5°E) show good agreement between the lidar SAOD observations and WACCM-CARMA SAOD simulations although we observe a difference in the altitude of the maximum aerosol concentration between the model and the in situ profile after Calbuco eruption in April 2015. A particular focus is also made on recent eruptions like Raikoke, Ambae and Ulawun. The plume of the Ambae volcano (15°S, 167°E) which erupted in July 2018 is shown to propagate to the northern hemisphere with some influence until summer 2019 in the Asian monsoon region. For the year 2019, we investigate how the Ulawun (5°S, 151°E; ~0.14 Tg of SO2) tropical eruption and the Raikoke mid-latitude eruption (48°N, 153°E; ~1.5Tg of SO2), have influenced the aerosol burden in the tropics.</p>

Slow feedbacks resulting from strongly enhanced atmospheric methane mixing ratios in a chemistry–climate model with mixed-layer ocean

In a previous study the quasi-instantaneous chemical impacts (rapid adjustments) of strongly enhanced methane (CH4) mixing ratios have been analysed. However, to quantify the influence of the respective slow climate feedbacks on the chemical composition it is necessary to include the radiation-driven temperature feedback. Therefore, we perform sensitivity simulations with doubled and quintupled present-day (year 2010) CH4 mixing ratios with the chemistry–climate model EMAC (European Centre for Medium-Range Weather Forecasts, Hamburg version – Modular Earth Submodel System (ECHAM/MESSy) Atmospheric Chemistry) and include in a novel set-up a mixed-layer ocean model to account for tropospheric warming. Strong increases in CH4 lead to a reduction in the hydroxyl radical in the troposphere, thereby extending the CH4 lifetime. Slow climate feedbacks counteract this reduction in the hydroxyl radical through increases in tropospheric water vapour and ozone, thereby dampening the extension of CH4 lifetime in comparison with the quasi-instantaneous response. Changes in the stratospheric circulation evolve clearly with the warming of the troposphere. The Brewer–Dobson circulation strengthens, affecting the response of trace gases, such as ozone, water vapour and CH4 in the stratosphere, and also causing stratospheric temperature changes. In the middle and upper stratosphere, the increase in stratospheric water vapour is reduced with respect to the quasi-instantaneous response. We find that this difference cannot be explained by the response of the cold point and the associated water vapour entry values but by a weaker strengthening of the in situ source of water vapour through CH4 oxidation. However, in the lower stratosphere water vapour increases more strongly when tropospheric warming is accounted for, enlarging its overall radiative impact. The response of the stratosphere adjusted temperatures driven by slow climate feedbacks is dominated by these increases in stratospheric water vapour as well as strongly decreased ozone mixing ratios above the tropical tropopause, which result from enhanced tropical upwelling. While rapid radiative adjustments from ozone and stratospheric water vapour make an essential contribution to the effective CH4 radiative forcing, the radiative impact of the respective slow feedbacks is rather moderate. In line with this, the climate sensitivity from CH4 changes in this chemistry–climate model set-up is not significantly different from the climate sensitivity in carbon-dioxide-driven simulations, provided that the CH4 effective radiative forcing includes the rapid adjustments from ozone and stratospheric water vapour changes.