Moisture fluxes in the tropics dominated by deep convection up to near tropical tropopause levels

2021 ◽  
Author(s):  
Maximilien Bolot ◽  
Stephan Fueglistaler
Keyword(s):  
Large Scale ◽  
Deep Convection ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause ◽  
Convective Scale ◽  
Moisture Fluxes ◽  
Global Impacts ◽  
Observational Estimate ◽  
Cold Point ◽  
Open Question

<p>The role played by tropical storms in the tropical tropopause layer (TTL), the transitional layer regulating the flux into the stratosphere of trace gases affecting radiation and the ozone layer, has been a long-standing open question. Progress has been slow because of computational limitations and challenging conditions for measurements and most numerical studies have used simulations over limited domains whose results must be upscaled to the tropical surface to infer global impacts. We compute the first global observational estimate of the convective ice flux at near tropical tropopause levels by using spaceborne lidar measurements from CALIOP. The calculation uses a method to convert from lidar extinction to sedimenting ice flux and uses error propagation to provide margins of uncertainty. We show that, at any given level in the TTL, the sedimenting ice flux exceeds the inflow of vapor computed from ERA5 reanalysis, revealing additional ice transport and allowing to deduce the advective ice flux as a function of altitude. The contribution to this flux of large-scale motions (resolved by ERA5) is computed and the residual is hypothesized to represent the flux of ice on the convective scale. Results show without ambiguity that the upward ice flux in deep convection dominates moisture transport up to close to the level of the cold point tropopause.</p>

scholarly journals Hydration and dehydration at the tropical tropopause

2009 ◽  
Vol 9 (24) ◽  
pp. 9647-9660 ◽  
Author(s):  
C. Schiller ◽  
J.-U. Grooß ◽  
P. Konopka ◽  
F. Plöger ◽  
F. H. Silva dos Santos ◽  
...  
Keyword(s):  
Deep Convection ◽  
Transport And Transformation ◽  
Tropical Tropopause Layer ◽  
Mixing Ratios ◽  
Trajectory Calculations ◽  
Tropical Tropopause ◽  
Different Seasons ◽  
The Mean ◽  
Cold Point ◽  
Hydration And Dehydration

Abstract. High-resolution water measurements from three tropical airborne missions in Northern Australia, Southern Brazil and West Africa in different seasons are analysed to study the transport and transformation of water in the tropical tropopause layer (TTL) and its impact on the stratosphere. The mean profiles are quite different according to the season and location of the campaigns, with lowest mixing ratios below 2 ppmv at the cold point tropopause during the Australian mission in November/December and high TTL mixing ratios during the African measurements in August. We present backward trajectory calculations considering freeze-drying of the air to the minimum saturation mixing ratio and initialised with climatological satellite data. This trajectory-based reconstruction of water agrees well with the observed H2O average profiles and therefore demonstrates that the water vapour set point in the TTL is primarily determined by the Lagrangian saturation history. Deep convection was found to moisten the TTL, in several events even above the cold point up to 420 K potential temperatures. However, our study does not provide evidence for a larger impact of these highly-localised events on global scales.

scholarly journals The CO<sub>2</sub> tracer clock for the Tropical Tropopause Layer

2007 ◽  
Vol 7 (3) ◽  
pp. 6655-6685 ◽  
Author(s):  
S. Park ◽  
R. Jiménez ◽  
B. C. Daube ◽  
L. Pfister ◽  
T. J. Conway ◽  
...  
Keyword(s):  
Large Scale ◽  
Deep Convection ◽  
Potential Temperature ◽  
Co2 Concentration ◽  
Vertical Gradient ◽  
Warm Pool ◽  
Tropical Tropopause Layer ◽  
Ascent Rate ◽  
Tropical Tropopause ◽  
Validation Experiment

Abstract. Observations of CO2 were made in the upper troposphere and lower stratosphere in the deep tropics in order to determine the patterns of large-scale vertical transport and age of air in the Tropical Tropopause Layer (TTL). Flights aboard the NASA WB-57F aircraft over Central America and adjacent ocean areas took place in January and February, 2004 (Pre-AURA Validation Experiment, Pre-AVE) and 2006 (Costa Rice AVE, CR-AVE), and for the same flight dates of 2006, aboard the Proteus aircraft from the surface to 15 km over Darwin, Australia (Tropical Warm Pool International Cloud Experiment , TWP-ICE). The data demonstrate that the TTL is composed of two layers with distinctive features: (1) the lower TTL, 350–360 K (potential temperature (θ); approximately 12–14 km), is subject to inputs of convective outflows, as indicated by layers of variable CO2 concentrations, with air parcels of zero age distributed throughout the layer; (2) the upper TTL, from θ= ~360 K to ~390 K (14–18 km), ascends slowly and ages uniformly, as shown by a linear decline in CO2 mixing ratio tightly correlated with altitude, associated with increasing age. This division is confirmed by ensemble trajectory analysis. The CO2 concentration at the level of 360 K was 380.0(±0.2) ppmv, indistinguishable from surface site values in the Intertropical Convergence Zone (ITCZ) for the flight dates. Values declined with altitude to 379.2(±0.2) ppmv at 390 K, implying that air in the upper TTL monotonically ages while ascending. In combination with the winter slope of the CO2 seasonal cycle (+10.8±0.4 ppmv/yr), the vertical gradient of 0.78 (±0.09) ppmv gives a mean age of 26(±3) days for the air at 390 K and a mean ascent rate of 1.5(±0.3) mm s−1. The TTL near 360 K in the Southern Hemisphere over Australia is very close in CO2 composition to the TTL in the Northern Hemisphere over Costa Rica, with strong contrasts emerging at lower altitudes (<360 K). Both Pre-AVE and CR-AVE CO2 observed unexpected input from deep convection over Amazônia deep into the TTL. The CO2 data confirm the operation of a highly accurate tracer clock in the TTL that provides a direct measure of the ascent rate of the TTL and of the age of air entering the stratosphere.

scholarly journals The CO<sub>2</sub> tracer clock for the Tropical Tropopause Layer

2007 ◽  
Vol 7 (14) ◽  
pp. 3989-4000 ◽  
Author(s):  
S. Park ◽  
R. Jiménez ◽  
B. C. Daube ◽  
L. Pfister ◽  
T. J. Conway ◽  
...  
Keyword(s):  
Large Scale ◽  
Deep Convection ◽  
Potential Temperature ◽  
Co2 Concentration ◽  
Vertical Gradient ◽  
Warm Pool ◽  
Tropical Tropopause Layer ◽  
Ascent Rate ◽  
Tropical Tropopause ◽  
Validation Experiment

Abstract. Observations of CO2 were made in the upper troposphere and lower stratosphere in the deep tropics in order to determine the patterns of large-scale vertical transport and age of air in the Tropical Tropopause Layer (TTL). Flights aboard the NASA WB-57F aircraft over Central America and adjacent ocean areas took place in January and February, 2004 (Pre-AURA Validation Experiment, Pre-AVE) and 2006 (Costa Rice AVE, CR-AVE), and for the same flight dates of 2006, aboard the Proteus aircraft from the surface to 15 km over Darwin, Australia (Tropical Warm Pool International Cloud Experiment, TWP-ICE). The data demonstrate that the TTL is composed of two layers with distinctive features: (1) the lower TTL, 350–360 K (potential temperature(θ); approximately 12–14 km), is subject to inputs of convective outflows, as indicated by layers of variable CO2 concentrations, with air parcels of zero age distributed throughout the layer; (2) the upper TTL, from θ=~360 K to ~390 K (14–18 km), ascends slowly and ages uniformly, as shown by a linear decline in CO2 mixing ratio tightly correlated with altitude, associated with increasing age. This division is confirmed by ensemble trajectory analysis. The CO2 concentration at the level of 360 K was 380.0(±0.2) ppmv, indistinguishable from surface site values in the Intertropical Convergence Zone (ITCZ) for the flight dates. Values declined with altitude to 379.2(±0.2) ppmv at 390 K, implying that air in the upper TTL monotonically ages while ascending. In combination with the winter slope of the CO2 seasonal cycle (+10.8±0.4 ppmv/yr), the vertical gradient of –0.78 (±0.09) ppmv gives a mean age of 26(±3) days for the air at 390 K and a mean ascent rate of 1.5(±0.3) mm s−1. The TTL near 360 K in the Southern Hemisphere over Australia is very close in CO2 composition to the TTL in the Northern Hemisphere over Costa Rica, with strong contrasts emerging at lower altitudes (<360 K). Both Pre-AVE and CR-AVE CO2 observed unexpected input from deep convection over Amazônia deep into the TTL. The CO2 data confirm the operation of a highly accurate tracer clock in the TTL that provides a direct measure of the ascent rate of the TTL and of the age of air entering the stratosphere.

Strateole-2: High-resolution observations of the tropical tropopause layer with long-duration balloons

2021 ◽  
Author(s):  
Albert Hertzog ◽  
Riwal Plougonven ◽  
Keyword(s):  
Water Vapor ◽  
High Resolution ◽  
Lower Stratosphere ◽  
Deep Convection ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause ◽  
Long Duration ◽  
First Results ◽  
Seychelles Islands ◽  
Cold Point

&lt;p&gt;Strateole-2 is a project aimed at studying the coupling between the troposphere and the stratosphere in the deep tropics. The project originality pertains to the use of long-duration ballons, which can fly for several months at 18 or 20 km altitude. The first Strateole-2 campaign took place from November 2019 to February 2020: 8 balloons with various instrumental configurations were released in the lower stratosphere from Seychelles Islands, in the Indian Ocean.&lt;br&gt;This first campaign was primarily devoted to testing all systems (balloons, gondolas, and instruments) developed for the project, and was very successful: the balloons flew for 85 days onaverage over the whole tropical band, and most instruments performed nominally. In-situ meteorological measurements performed every 30-s on each flight provide a unique description of gravity-wave activity in the tropics and its relation to deep convection. The first observations of aerosols and water vapor onboard long-duration balloons were also achieved, which e.g. highlighted the tape recorder signal in the tropical lower stratosphere. Very innovative instruments also premiered during the campaign: RACHuTS, a light reeled payload, for instance performed 50 high-resolution vertical profiles of temperature, aerosols and water vapor down to 2km below the balloon, crossing several times the cold-point tropopause. ROC collected hundreds of temperature profiles down to the middle troposphere through GPS radio-occultations. Last, one balloon also carried a nadir-pointing backscatter lidar, which has described the underlying convection at unprecedented temporal resolution. An overview of the flights and first results will be presented.&lt;br&gt;Two forthcoming balloon campaigns are planned within Strateole-2, in 2021-22 and 2024-25. Each will release 20 balloons.&amp;#160;&lt;/p&gt;

scholarly journals Hydration and dehydration at the tropical tropopause

2009 ◽  
Vol 9 (4) ◽  
pp. 17495-17529 ◽  
Author(s):  
C. Schiller ◽  
J.-U. Grooß ◽  
P. Konopka ◽  
F. Plöger ◽  
F. H. Silva dos Santos ◽  
...  
Keyword(s):  
Deep Convection ◽  
Transport And Transformation ◽  
Tropical Tropopause Layer ◽  
Mixing Ratios ◽  
Trajectory Calculations ◽  
Tropical Tropopause ◽  
Different Seasons ◽  
The Mean ◽  
Cold Point ◽  
Hydration And Dehydration

Abstract. High-resolution water measurements from three tropical airborne missions in Northern Australia, Southern Brazil and West Africa in different seasons are analysed to study the transport and transformation of water in the tropical tropopause layer (TTL) and its impact on the stratosphere. The mean profiles are quite different according to the season and location of the campaigns, with lowest mixing ratios below 2 ppmv at the cold point tropopause during the Australian mission in November/December and high TTL mixing ratios during the African measurements in August. We present backward trajectory calculations considering freeze-drying of the air to the minimum saturation mixing ratio and initialised with climatological satellite data. This trajectory-based reconstruction of water agrees well with the observed H2O average profiles and therefore demonstrates that the water vapour set point in the TTL is primarily determined by the Lagrangian saturation history. Deep convection was found to moisten the TTL, in several events even above the cold point up to 420 K potential temperatures. However, our study does not provide evidence for a larger impact of these highly-localised events on global scales.

scholarly journals Model study of the cross-tropopause transport of biomass burning pollution

2007 ◽  
Vol 7 (14) ◽  
pp. 3713-3736 ◽  
Author(s):  
B. N. Duncan ◽  
S. E. Strahan ◽  
Y. Yoshida ◽  
S. D. Steenrod ◽  
N. Livesey
Keyword(s):  
Biomass Burning ◽  
El Niño ◽  
Fossil Fuels ◽  
Extreme Event ◽  
El Nino ◽  
Deep Convection ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause ◽  
El Niño Event ◽  
The Impact

Abstract. We present a modeling study of the troposphere-to-stratosphere transport (TST) of pollution from major biomass burning regions to the tropical upper troposphere and lower stratosphere (UT/LS). TST occurs predominately through 1) slow ascent in the tropical tropopause layer (TTL) to the LS and 2) quasi-horizontal exchange to the lowermost stratosphere (LMS). We show that biomass burning pollution regularly and significantly impacts the composition of the TTL, LS, and LMS. Carbon monoxide (CO) in the LS in our simulation and data from the Aura Microwave Limb Sounder (MLS) shows an annual oscillation in its composition that results from the interaction of an annual oscillation in slow ascent from the TTL to the LS and seasonal variations in sources, including a semi-annual oscillation in CO from biomass burning. The impacts of CO sources that peak when ascent is seasonally low are damped (e.g. Southern Hemisphere biomass burning) and vice-versa for sources that peak when ascent is seasonally high (e.g. extra-tropical fossil fuels). Interannual variation of CO in the UT/LS is caused primarily by year-to-year variations in biomass burning and the locations of deep convection. During our study period, 1994–1998, we find that the highest concentrations of CO in the UT/LS occurred during the strong 1997–1998 El Niño event for two reasons: i. tropical deep convection shifted to the eastern Pacific Ocean, closer to South American and African CO sources, and ii. emissions from Indonesian biomass burning were higher. This extreme event can be seen as an upper bound on the impact of biomass burning pollution on the UT/LS. We estimate that the 1997 Indonesian wildfires increased CO in the entire TTL and tropical LS (>60 mb) by more than 40% and 10%, respectively, for several months. Zonal mean ozone increased and the hydroxyl radical decreased by as much as 20%, increasing the lifetimes and, subsequently TST, of trace gases. Our results indicate that the impact of biomass burning pollution on the UT/LS is likely greatest during an El Niño event due to favorable dynamics and historically higher burning rates.

scholarly journals Cold trap dehydration in the Tropical Tropopause Layer characterized by SOWER chilled-mirror hygrometer network data in the Tropical Pacific

2012 ◽  
Vol 12 (9) ◽  
pp. 25833-25885 ◽  
Author(s):  
F. Hasebe ◽  
Y. Inai ◽  
M. Shiotani ◽  
M. Fujiwara ◽  
H. Vömel ◽  
...  
Keyword(s):  
Ice Nucleation ◽  
Tropical Pacific ◽  
Cold Trap ◽  
Mixing Ratio ◽  
Back Trajectories ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause ◽  
Scatter Plots ◽  
Cold Point ◽  
The Tropical Pacific

Abstract. A network of balloon-born radiosonde observations employing chilled-mirror hygrometers for water and electrochemical concentration cells for ozone has been operated since late 1990s in the Tropical Pacific trying to capture the progress of dehydration for the air parcels advected horizontally in the Tropical Tropopause Layer (TTL). The analyses of this dataset are made on isentropes taking advantage of the conservative properties of tracers in adiabatic motion. The existence of ice particles is diagnosed by lidars simultaneously operated with sonde flights. Characteristics of the TTL dehydration are presented on the basis of individual soundings and statistical features. Supersaturations close to 80% in the relative humidity with respect to ice (RHice) have been observed in subvisible cirrus clouds located near the cold point tropopause at extremely low temperatures around 180 K. Further observational evidence is needed to confirm the credibility of such high values of RHice. The progress of TTL dehydration is reflected in isentropic scatter plots between the sonde-observed mixing ratio (OMR) and the minimum saturation mixing ratio (SMRmin) along the back trajectories associated with the observed air mass. The supersaturation exceeding the critical value of the homogeneous ice nucleation (OMR > 1.6 × SMRmin) is frequently observed on 360 and 365 K surfaces indicating that the cold trap dehydration is under progress in the TTL. The near correspondence between the two (OMR ~ SMRmin) on 380 K on the other hand implies that this surface is not significantly cold for the advected air parcels to be dehydrated. Above 380 K, the cold trap dehydration would scarcely function while some moistening in turn occurs before the air parcels reach the lowermost stratosphere at around 400 K where OMR is generally smaller than SMRmin.

scholarly journals Ozonesonde profiles from the West Pacific Warm Pool

2015 ◽  
Vol 15 (12) ◽  
pp. 16655-16696 ◽  
Author(s):  
R. Newton ◽  
G. Vaughan ◽  
H. M. A. Ricketts ◽  
L. L. Pan ◽  
A. J. Weinheimer ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Ozone Concentration ◽  
Deep Convection ◽  
Warm Pool ◽  
Atmospheric Composition ◽  
Measured Signal ◽  
Background Current ◽  
West Pacific ◽  
Tropical Tropopause Layer ◽  
Tropical Tropopause

Abstract. We present a series of ozonesonde profiles measured from Manus Island, Papua New Guinea, during February 2014. The experiment formed a part of a wider airborne campaign involving three aircraft based in Guam, to characterise the atmospheric composition above the tropical West Pacific in unprecedented detail. Thirty-nine ozonesondes were launched between 2 and 25 February, of which 34 gave good ozone profiles. Particular attention was paid to measuring the background current of the ozonesonde before launch, as this can amount to half the measured signal in the tropical tropopause layer (TTL). An unexpected contamination event affected these measurements and required a departure from standard operating procedures for the ozonesondes. Comparison with aircraft measurements allows validation of the measured ozone profiles and confirms that for well-characterized sondes (background current <50 nA) a constant background current should be assumed throughout the profile, equal to the minimum value measured during preparation just before launch. From this set of 34 ozonesondes, the minimum reproducible ozone concentration measured in the TTL was 12–13 ppbv; no examples of near-zero ozone concentration as reported by other recent papers were measured. The lowest ozone concentrations coincided with outflow from extensive deep convection to the east of Manus, consistent with uplift of ozone-poor air from the boundary layer. However, these minima were lower than the ozone concentration measured through most of the boundary layer, and were matched only by measurements at the surface in Manus.

scholarly journals Ultrathin Tropical Tropopause Clouds (UTTCs): I. Cloud morphology and occurrence

2003 ◽  
Vol 3 (4) ◽  
pp. 1083-1091 ◽  
Author(s):  
Th. Peter ◽  
B. P. Luo ◽  
M. Wirth ◽  
C. Kiemle ◽  
H. Flentje ◽  
...  
Keyword(s):  
Gas Phase ◽  
Large Scale ◽  
Lower Stratosphere ◽  
Western Indian Ocean ◽  
Ice Crystals ◽  
Mixing Ratio ◽  
Efficient Point ◽  
Tropical Tropopause ◽  
Cold Point

Abstract. Subvisible cirrus clouds (SVCs) may contribute to dehydration close to the tropical tropopause. The higher and colder SVCs and the larger their ice crystals, the more likely they represent the last efficient point of contact of the gas phase with the ice phase and, hence, the last dehydrating step, before the air enters the stratosphere. The first simultaneous in situ and remote sensing measurements of SVCs were taken during the APE-THESEO campaign in the western Indian ocean in February/March 1999. The observed clouds, termed Ultrathin Tropical Tropopause Clouds (UTTCs), belong to the geometrically and optically thinnest large-scale clouds in the Earth's atmosphere. Individual UTTCs may exist for many hours as an only 200--300 m thick cloud layer just a few hundred meters below the tropical cold point tropopause, covering up to 105 km2. With temperatures as low as 181 K these clouds are prime representatives for defining the water mixing ratio of air entering the lower stratosphere.

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