Layering and vertical transport in sheared double-diffusive convection in the diffusive regime

A sequence of two- and three-dimensional simulations are conducted for the double-diffusive convection (DDC) flows in the diffusive regime subjected to an imposed shear. For a wide range of control parameters, and for sufficiently strong perturbation of the conductive initial state, staircase-like structures spontaneously develop, with relatively well-mixed layers separated by sharp interfaces of enhanced scalar gradient. Such staircases appear to be robust even in the presence of strong shear over very long times, with early-time coarsening of the observed layers. For the same set of control parameters, different asymptotic layered states, with markedly different vertical scalar fluxes, can arise for different initial perturbation structures. The imposed shear significantly spatio-temporally modifies the vertical transport of the various scalars. The flux ratio $\gamma ^*$ (i.e. the ratio between the density fluxes due to the total salt flux and the total heat flux) is found, at steady state, to be essentially equal to the square root of the ratio of the salt diffusivity to the thermal diffusivity, consistent with the physical model proposed by Linden & Shirtcliffe (J. Fluid Mech., vol. 87, 1978, pp. 417–432) and the variational arguments presented by Stern (J. Fluid Mech., vol. 114, 1982, pp. 105–121) for unsheared double-diffusive convection.

Crucial Role of Mesoscale Convective Systems in the Vertical Mass, Water and Energy Transports of the South Asian Summer Monsoon

Convective vertical transport is critical in the monsoonal overturning but the relative roles of different convective systems are not well understood. This study used a cloud classification and tracking technique to decompose a convection-permitting simulation of the South Asian summer monsoon (SASM) into sub-regimes of mesoscale convective system (MCS), non-MCS deep convection (non-MCS), congestus, and shallow convection/clear-sky. Isentropic analysis is adopted to quantify the contributions of different convective systems to the total SASM vertical mass, water, and energy transports. The results underscore the crucial roles of MCSs in the SASM vertical transports. Compared to non-MCSs, the total mass and energy transports by MCSs are at least 1.5 times stronger throughout the troposphere, with a larger contributing fraction from convective updrafts compared to upward motion in stratiform regions. Occurrence frequency of non-MCSs is around 40 times higher than that of MCSs. However, per instantaneous convection feature, the vertical transports and net MSE export by MCSs are about 70-100 and 58 times stronger than that of non-MCSs. While these differences are dominantly contributed by differences in the per-feature MCS and non-MCS area coverage, MCSs also show stronger transport intensities than non-MCSs over both ocean and land. Oceanic MCSs and non-MCSs show more obvious top-heavy structures than their inland counterparts, which are closely related to the widespread stratiform over ocean. Compared to the monsoon break phase, MCSs occur more frequently (~1.6 times) but their vertical transport intensity slightly weakens (by ~10%) during the active phases. These results are useful for understanding the SASM and advancing the energetic framework.

Reduced volatility of aerosols from surface emissions to the top of the planetary boundary layer

Aerosols from surface emission can be transported upwards through convective mixing in the planetary boundary layer (PBL), which subsequently interact with clouds, serving as important sources to nucleate droplets or ice particles. However, the evolution of aerosol composition during this vertical transport has yet to be explicitly understood. In this study, simultaneous measurements of detailed aerosol compositions were conducted at two sites, namely urban Beijing (50 m above sea level – a.s.l.) and Haituo mountain (1344 m a.s.l.) during wintertime, representing the anthropogenically polluted surface environment and the top of the PBL, respectively. The pollutants from surface emissions were observed to reach the mountain site on daily basis through daytime PBL convective mixing. From the surface to the top of PBL, we found efficient transport or formation of lower-volatility species (black carbon, sulfate, and low-volatile organic aerosol, OA); however, a notable reduction in semivolatile substances, such as the fractions of nitrate and semivolatile OA reduced by 74 % and 76 %, respectively, during the upward transport. This implies that the mass loss of these semivolatile species was driven by the evaporation process, which repartitioned the condensed semivolatile substances to the gas phase when aerosols were transported and exposed to a cleaner environment. In combination with the oxidation processes, these led to an enhanced oxidation state of OA at the top of the PBL compared to surface environment, with an increase of oxygen to carbon atomic ratio by 0.2. Such a reduction in aerosol volatility during vertical transport may be important in modifying its viscosity, nucleation activity, and atmospheric lifetime.

A vertical transport window of water vapor in the troposphere over the Tibetan Plateau with implication for global change

By using the multi-source data of meteorology over recent decades, this study discovered a summertime “hollow wet pool” in the troposphere with a center of high water vapor over Asian water tower (AWT) on the Tibetan Plateau (TP), where is featured by a vertical transport “window” in the troposphere. The water vapor transport in the upper troposphere extends from the vertical transport window over the TP with the significant connections among the Arctic, Antarctic and TP regions, highlighting an effect of TP’s vertical transport window of tropospheric vapor in the “hollow wet pool” on global change. The vertical transport window was built by the AWT’s thermal forcing in associated with the dynamic effect of the TP’s “hollow heat island”. Our study improve the understanding on the vapor transport over the TP with an important implication to global change.

The modification of turbulent thermal wind balance by non-traditional effects

The meridional component of the earth's rotation is often neglected in geophysical contexts. This is referred to as the ‘traditional approximation’ and is justified by the typically small vertical velocity and aspect ratio of such problems. Ocean fronts are regions of strong horizontal buoyancy gradient and are associated with strong vertical transport of tracers and nutrients. Given these comparatively large vertical velocities, non-traditional rotation may play a role in governing frontal dynamics. Here the effects of non-traditional rotation on a front in turbulent thermal wind balance are considered using an asymptotic approach. Solutions are presented for a general horizontal buoyancy profile and examined in the simple case of a straight front. Non-traditional effects are found to depend strongly on the direction of the front and may lead to the generation of jets and the modification of the frontal circulation and vertical transport.

Vehicle-induced turbulence and atmospheric pollution

Theoretical models of the Earth's atmosphere adhere to an underlying concept of flow driven by radiative transfer and the nature of the surface over which the flow is taking place: heat from the sun and/or anthropogenic sources are the sole sources of energy driving atmospheric constituent transport. However, another source of energy is prevalent in the human environment at the very local scale – the transfer of kinetic energy from moving vehicles to the atmosphere. We show that this source of energy, due to being co-located with combustion emissions, can influence their vertical distribution to the extent of having a significant influence on lower-troposphere pollutant concentrations throughout North America. The effect of vehicle-induced turbulence on freshly emitted chemicals remains notable even when taking into account more complex urban radiative transfer-driven turbulence theories at high resolution. We have designed a parameterization to account for the at-source vertical transport of freshly emitted pollutants from mobile emissions resulting from vehicle-induced turbulence, in analogy to sub-grid-scale parameterizations for plume rise emissions from large stacks. This parameterization allows vehicle-induced turbulence to be represented at the scales inherent in 3D chemical transport models, allowing this process to be represented over larger regions than is currently feasible with large eddy simulation models. Including this sub-grid-scale parameterization for the vertical transport of emitted pollutants due to vehicle-induced turbulence in a 3D chemical transport model of the atmosphere reduces pre-existing North American nitrogen dioxide biases by a factor of 8 and improves most model performance scores for nitrogen dioxide, particulate matter, and ozone (for example, reductions in root mean square errors of 20 %, 9 %, and 0.5 %, respectively).

Influence of the Saharan Air Layer on Hurricane Nadine (2012). Part I: Observations from the Hurricane and Severe Storm Sentinel (HS3) Investigation and Modeling Results

This study uses a model with aerosol-cloud-radiation coupling to examine the impact of Saharan dust and other aerosols on Hurricane Nadine (2012). In order to study aerosol direct (radiation) and indirect (cloud microphysics) effects from individual, as well as all aerosol species, eight different NU-WRF simulations were conducted. In several simulations, aerosols led to storm strengthening, followed by weakening relative to the Ctrl simulation. This variability of the aerosol impact may be related to whether aerosols are ingested into clouds within the outer rainbands or the eyewall. Upper tropospheric aerosol concentrations indicate vertical transport of all aerosol types in the outer bands but only vertical transport of sea salt in the inner core. The results suggest that aerosols, particularly sea salt, may have contributed to a stronger initial intensification, but that aerosols ingestion into the outer bands at later times may have weakened the storm in the longer term. In most aerosol experiments, aerosols led to a reduction in cloud and precipitation hydrometeors, the exception being the dust-only case that produced periods of enhanced hydrometeor growth. The Saharan Air Layer (SAL) also impacted Nadine by causing a region of strong easterlies impinging on the eastern side of the storm. At the leading edge of these easterlies, cool and dry air near the top of the SAL was being ingested into the outer-band convection. This midlevel low equivalent-potential-temperature air gradually lowered toward the surface and eventually contributed to significant cold pool activity in the eastern rain band and in the northeast quadrant of the storm. Such enhanced downdraft activity could have led to weakening of the storm, but it is not presently possible to quantify this impact.