First Observation of Mercury Species on an Important Water Vapor Channel in the Southeast Tibetan Plateau

The Tibetan Plateau is generally considered to be a significantly clean area owing to its high altitude; however, the transport of atmospheric pollutants from the Indian subcontinent to the Tibetan Plateau has infected the Tibetan environments. Nyingchi is located at the end of an important water vapor channel. In this study, continuous monitoring of gaseous elemental mercury (GEM), gaseous oxidized mercury (GOM), and particle-bound mercury (PBM) was conducted in Nyingchi from March 30 to September 3, 2019, to study the influence of the Indian summer monsoon (ISM) on the origin, transport and behavior of mercury. The atmospheric Hg concentrations during the preceding Indian summer monsoon (PISM) period (1.20 ± 0.35 ng m−3, 13.5 ± 7.3 pg m−3, and 11.4 ± 4.8 pg m−3 for GEM, GOM, and PBM, respectively) were relatively higher than those during the ISM period (0.95 ± 0.21 ng m−3, 12.7 ± 14.3 pg m−3 and 8.8 ± 6.0 pg m−3). The average annual total gaseous mercury concentration in the Nyingchi region was obtained using a passive sampler as 1.12 ± 0.28 ng m−3. The GEM concentration showed that the sampling area was very clean. The GEM has several patterns of daily variation during different periods. Stable high GEM concentrations occur at night during PISM, which may be related to the nocturnal boundary layer. High values occurring in the late afternoon during the ISM may be related to long-range transport. The results of the trajectory model demonstrate that the sources of pollutants at Nyingchi are different under the control of different airflow fields. During westerly circulation, pollutants mainly originate from northeast India or Nepal. During the ISM period, the pollutants mainly originate from northeast India, or the Bay of Bengal, and the Indian Ocean. The strong precipitation and vegetation effects on Hg during the ISM resulted in low Hg concentrations transmitted to Nyingchi during this period. Further, principal component analysis showed that long-distance transport, local emissions, meteorological factors, and snowmelt factors are the main factors affecting the local Hg concentration in Nyingchi.

Relationships between Low-Level Jet and Low Visibility Associated with Precipitation, Air Pollution, and Fog in Tianjin

In this study, relationships between low-level jet (LLJ) and low visibility associated with precipitation, air pollution, and fog in Tianjin are investigated based on observational data from January to December, 2016. Statistical results show 55% of precipitation is accompanied by LLJ, and two causes responsible for the relatively high percentage are presented. The result of case analysis shows that some southwesterly LLJs are favorable for the formation of precipitation by transporting water vapor when the water vapor channel from the South China Sea or Bengal Bay to Bohai Rim region is established. Statistical results show 55% of pollution episodes (PEs) are accompanied by LLJs. When pollutions are observed in the southern industrial regions, nocturnal southwesterly LLJ, which can carry polluted air masses from polluted regions to Tianjin and induce turbulent mixing, can enhance surface PM2.5 concentration and is favorable for the formation of surface pollution at night. Nocturnal northerly or southeasterly LLJ leads to clear air masses mixing with polluted air masses and is favorable for increasing visibility. Contributions of southwesterly LLJs to the formation of fog and precipitation are similar, which both rely on establishing the water vapor channel despite occurrence heights of LLJs being different.

Development of on-site self-calibration and retrieval methods for sky-radiometer observations of precipitable water vapor

The Prede sky radiometer measures direct solar irradiance and the angular distribution of diffuse radiances at the ultraviolet, visible, and near-infrared wavelengths. These data are utilized for the remote sensing of aerosols, water vapor, ozone, and clouds, but the calibration constant, which is the sensor output current of the extraterrestrial solar irradiance at the mean distance between Earth and the Sun, is needed. The aerosol channels, which are the weak gas absorption wavelengths of 340, 380, 400, 500, 675, 870, and 1020 nm, can be calibrated by an on-site self-calibration method, the Improved Langley method. This on-site self-calibration method is useful for the continuous long-term observation of aerosol properties. However, the continuous long-term observation of precipitable water vapor (PWV) by the sky radiometer remains challenging because calibrating the water vapor absorption channel of 940 nm generally relies on the standard Langley (SL) method at limited observation sites (e.g., the Mauna Loa Observatory) and the transfer of the calibration constant by a side-by-side comparison with the reference sky radiometer calibrated by the SL method. In this study, we developed the SKYMAP algorithm, a new on-site method of self-calibrating the water vapor channel of the sky radiometer using diffuse radiances normalized by direct solar irradiance (normalized radiances). Because the sky radiometer measures direct solar irradiance and diffuse radiance using the same sensor, the normalization cancels the calibration constant included in the measurements. The SKYMAP algorithm consists of three steps. First, aerosol optical and microphysical properties are retrieved using direct solar irradiances and normalized radiances at aerosol channels. The aerosol optical properties at the water vapor channel are interpolated from those at aerosol channels. Second, PWV is retrieved using the angular distribution of the normalized radiances at the water vapor channel. Third, the calibration constant at the water vapor channel is estimated from the transmittance of PWV and aerosol optical properties. Intensive sensitivity tests of the SKYMAP algorithm using simulated data of the sky radiometer showed that the calibration constant is retrieved reasonably well for PWV<2 cm, which indicates that the SKYMAP algorithm can calibrate the water vapor channel on-site in dry conditions. Next, the SKYMAP algorithm was applied to actual measurements under the clear-sky and low-PWV (<2 cm) conditions at two sites, Tsukuba and Chiba, Japan, and the annual mean calibration constants at the two sites were determined. The SKYMAP-derived calibration constants were 10.1 % and 3.2 % lower, respectively, than those determined by a side-by-side comparison with the reference sky radiometer. After determining the calibration constant, we obtained PWV from the direct solar irradiances in both the dry and wet seasons. The retrieved PWV values corresponded well to those derived from a global-navigation-satellite-system–global-positioning-system receiver, a microwave radiometer, and an AERONET (Aerosol Robotic Network) sun–sky radiometer at both sites. The correlation coefficients were greater than 0.96. We calculated the bias errors and the root mean square errors by comparing PWV between the DSRAD (direct solar irradiance) algorithm and other instruments. The magnitude of the bias error and the root mean square error were <0.163 and <0.251 cm for PWV<3 cm, respectively. However, our method tended to underestimate PWV in the wet conditions, and the magnitude of the bias error and the root mean square error became large, <0.594 and <0.722 cm for PWV>3 cm, respectively. This problem was mainly due to the overestimation of the aerosol optical thickness before the retrieval of PWV. These results show that the SKYMAP algorithm enables us to observe PWV over the long term, based on its unique on-site self-calibration method.

Correction: Tabata, T., et al. Recalibration of over 35 Years of Infrared and Water Vapor Channel Radiances of the JMA Geostationary Satellites. Remote Sens. 2019, 11, 1189

The authors wish to make the following corrections to this paper [...]

Development of on-site self-calibration and retrieval methods for sky-radiometer observations of precipitable water vapor

The Prede sky-radiometer, whose aerosol channels are calibrated by on-site measurements (the Improved Langley method), has been used for continuous long-term observation of aerosol properties. However, continuous long-term observation of precipitable water vapor (PWV) by sky-radiometer remain challenge, because the water vapor channel is generally calibrated by the standard Langley method at limited observation sites (e.g., the Mauna Loa Observatory). In this study, we developed SKYMAP, a new onsite self-calibration method for the water vapor channel of the Prede sky-radiometer using diffuse radiances normalized by direct solar irradiance. The SKYMAP algorithm consists of three steps. First, aerosol optical and microphysical properties are retrieved using direct solar irradiances and the normalized diffuse radiances at aerosol channels. The aerosol optical properties at the water vapor channel are interpolated from those at aerosol channels. Second, the transmittance of PWV is retrieved using the diffuse radiance normalized to the direct solar irradiance at the water vapor channel, which does not need the calibration constant. Third, the calibration constant at the water vapor channel is estimated from the transmittance of PWV and aerosol optical properties. Intensive sensitivity tests of SKYMAP using simulated data of the sky-radiometer showed that the calibration constant is retrieved reasonably well for PWV < 2 cm, indicating that SKYMAP can calibrate the water vapor channel on-site in dry conditions. Then SKYMAP was applied to actual measurements in the dry season at two sites (Tsukuba and Chiba, Japan). Because the SKYMAP algorithm is useful for clear-sky and low PWV (< 2 cm) conditions, the water vapor channel was calibrated for the dry season. After determining the calibration constant, PWV is able to be retrieved using direct solar irradiances for the whole year. The retrieved PWV values correspond well to those derived from a Global Navigation Satellite System (GNSS)/Global Positioning System (GPS) receiver, a microwave radiometer, and a AERONET sun-sky radiometer at both sites (correlation coefficient γ > 0.96), indicating that the Prede sky-radiometer provides both aerosol and PWV data based on its unique on-site calibration methods.

Observations of Gravity Waves with High-Pass Filtering in the New Generation of Geostationary Imagers and Their Relation to Aircraft Turbulence

This paper introduces a method of image filtering for viewing gravity waves in satellite imagery, which is particularly timely to the advent of the next-generation Advanced Himawari Imager (AHI) and the Advanced Baseline Imager (ABI). Applying a “high pass” filter to the upper-troposphere water vapor channel reveals sub-Kelvin-degree variations in brightness temperature that depict an abundance of gravity wave activity at the AHI/ABI sensitivity. Three examples demonstrate that this high-pass product can be exploited in a forecasting setting to identify possible varieties of turbulence-prone gravity waves that either 1) move roughly orthogonally to the apparent background flow or 2) produce interference as separate wave packets pass through the same location.

Diffuse sunlight based calibration of the water vapor channel in the upc raman lidar

A method for determining the calibration factor of the water vapor channel of a Raman lidar, based on zenith measurements of diffuse sunlight and on assumptions regarding some system parameters and Raman scattering models, has been applied to the lidar system of Universitat Politècnica de Catalunya (UPC; Technical University of Catalonia, Spain). Results will be analyzed in terms of stability and comparison with typical methods relying on simultaneous radiosonde measurements.