Polarisation-dependent single-pulse ultrafast optical switching of an elementary ferromagnet

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely valuable stimuli for the all-optical magnetization reversal in ferrimagnetic and ferromagnetic alloys and multilayers, while this remains elusive in elementary ferromagnets. Here we demonstrate that a single laser pulse with sub-picosecond duration can lead to the reversal of the magnetization of bulk nickel, in tandem with the expected demagnetization. As revealed by realistic time-dependent electronic structure simulations, the central mechanism involves ultrafast light-induced torques that act on the magnetization. They are only effective if the laser pulse is circularly polarized on a plane that contains the initial orientation of the magnetization. We map the laser pulse parameter space enabling the magnetization switching and unveil rich intra-atomic orbital-dependent magnetization dynamics featuring transient inter-orbital non-collinear states. Our findings open further perspectives for the efficient implementation of optically-based spintronic devices.

Study of the Effect of Higher-order Dispersions on Photoionisation Induced by Ultrafast Laser Pulses Applying a Classical Theoretical Method

We investigated the effect of higher order dispersion on ultrafast photoionisation with Classical Trajectory Monte Carlo (CTMC) method for hydrogen and krypton atoms. In our calculations we used linearly polarised ultrashort 7 fs laser pulses, 6.5 × 1014 W/cm2 intensity, and a central wavelength of 800 nm. Our results show that electrons with the highest kinetic energies are obtained with transform limited (TL) pulses. The shaping of the pulses with negative second- third- or fourth- order dispersion results in higher ionisation yield and electron energies compared to pulses shaped with positive dispersion values. We have also investigated how the Carrier Envelope Phase (CEP) dependence of the ionisation is infuenced by dispersion. We calculated the left-right asymmetry as a function of energy and CEP for sodium atoms employing pulses of 4.5 fs, 800 nm central wavelength, and 4 × 1012 W/cm2 intensity. We found that the left-right asymmetry is more pronounced for pulses shaped with positive Group Delay Dispersion (GDD). It was also found that shaping a pulse with increasing amounts of GDD in absolute value blurs the CEP dependence, which is attributed to the increasing number of optical cycles.

Laser-assisted formation of luminescent domains in metal- or semiconductor-doped silicate and phosphate glasses

In this study, silicate and phosphate glasses doped with Ag or CdS were exposed to femtosecond laser pulses and photoluminescence properties of the laser-written domains were investigated. Laser writing in phosphate glass doped with CdS was found to induce very weak photoluminescence, while laser-written domains in silicate glass had a comparatively high photoluminescence intensity, that was assigned to the formation of the sulphur vacancies in the CdS nanocrystals precipitated under the ultrafast laser pulses. Observed photoluminescence bands in Ag-containing glasses we assigned to the formation of different silver nanospecies which provide photoluminescence bands with the maxima at 685 and 600 nm in Ag-doped silicate and phosphate glasses, respectively.

Soliton Generation in Negative Thermal Expansion Materials

Strain solitons have been observed statically in several 2D materials and dynamically in substrate materials using ultrafast laser pulses. The latter case relies on lattice relaxation in response to ultrafast heating in a light-absorbing transducer material, a process which is sensitive to the thermal expansion coefficient. Here we consider an unusual case where the sign of the thermal expansion coefficient is negative, a scenario which is experimentally feasible in light of rapid and recent advances in the discovery of negative thermal expansion materials. We present numerical solutions to a nonlinear differential equation which has been repeatedly demonstrated to quantitatively model experimental data and discuss the salient results using realistic parameters for material linear and nonlinear elasticity. The solitons that emerge from the initial value problem with negative and positive thermal expansion are qualitatively different in several ways. The new case of negative thermal expansion gives rise to a nearly-periodic soliton train with chirped profile and free of an isolated shock front. We suggest this unanticipated result may be realized experimentally and assess the potential for certain applications of this generic effect.

Large ultrafast-modulated Voigt effect in noncollinear antiferromagnet Mn3Sn

The time-resolved magneto-optical (MO) Voigt effect can be utilized to study the Néel order dynamics in antiferromagnetic (AFM) materials, but it has been limited for collinear AFM spin configuration. Here, we have demonstrated that in Mn3Sn with an inverse triangular spin structure, the quench of AFM order by ultrafast laser pulses can result in a large Voigt effect modulation. The modulated Voigt angle is significantly larger than the polarization rotation due to the crystal-structure related linear dichroism effect and the modulated MO Kerr angle arising from the ferroic ordering of cluster magnetic octupole. The AFM order quench time shows negligible change with increasing temperature approaching the Néel temperature (TN), in markedly contrast with the pronounced slowing-down demagnetization typically observed in conventional magnetic materials. This atypical behavior can be explained by the influence of weakened Dzyaloshinskii–Moriya interaction rather than the smaller exchange splitting on the diminished AFM order near TN. The temperature-insensitive ultrafast spin manipulation can pave the way for high-speed spintronic devices either working at a wide range of temperature or demanding spin switching near TN.

Tunable and Passively Mode-Locking Nd0.01:Gd0.89La0.1NbO4 Picosecond Laser

A high-quality Nd0.01:Gd0.89La0.1NbO4 (Nd:GLNO) crystal is grown by the Czochralski method, demonstrating wide absorption and fluorescence spectra and advantage for producing ultrafast laser pulses. In this paper, the tunable and passively mode-locking Nd:GLNO lasers are characterized for the first time. The tuning coverage is 34.87 nm ranging from 1058.05 to 1092.92 nm with a maximum output power of 4.6 W at 1065.29 nm. A stable continuous-wave (CW) passively mode-locking Nd:GLNO laser is achieved at 1065.26 nm, delivering a pulse width of 9.1 ps and a maximum CW mode-locking output power of 0.27 W.