Study of the Effect of Higher-order Dispersions on Photoionisation Induced by Ultrafast Laser Pulses Applying a Classical Theoretical Method

We investigated the effect of higher order dispersion on ultrafast photoionisation with Classical Trajectory Monte Carlo (CTMC) method for hydrogen and krypton atoms. In our calculations we used linearly polarised ultrashort 7 fs laser pulses, 6.5 × 1014 W/cm2 intensity, and a central wavelength of 800 nm. Our results show that electrons with the highest kinetic energies are obtained with transform limited (TL) pulses. The shaping of the pulses with negative second- third- or fourth- order dispersion results in higher ionisation yield and electron energies compared to pulses shaped with positive dispersion values. We have also investigated how the Carrier Envelope Phase (CEP) dependence of the ionisation is infuenced by dispersion. We calculated the left-right asymmetry as a function of energy and CEP for sodium atoms employing pulses of 4.5 fs, 800 nm central wavelength, and 4 × 1012 W/cm2 intensity. We found that the left-right asymmetry is more pronounced for pulses shaped with positive Group Delay Dispersion (GDD). It was also found that shaping a pulse with increasing amounts of GDD in absolute value blurs the CEP dependence, which is attributed to the increasing number of optical cycles.

State-selective charge exchange cross sections in Be$$^{4+} -\hbox {H}(2\textit{lm})$$ collision based on the classical trajectory Monte Carlo method

A three-body classical trajectory Monte Carlo method is used to calculate the nl state-selective charge exchange cross sections in $$\hbox {Be}^{\mathrm {4+}}+$$ Be 4 + + H(2lm) collisions in the energy range between 10 and 200 keV/amu. We present partial cross sections for charge exchange into $$\hbox {Be}^{\mathrm {3+}}$$ Be 3 + (nl) $$(\textit{nl} = 2s, 2p, 3s, 3p, 3d, 4s, 4p, 4d, 4f)$$ ( nl = 2 s , 2 p , 3 s , 3 p , 3 d , 4 s , 4 p , 4 d , 4 f ) states as a function of impact energy. Our results are compared with the previous classical and quantum-mechanical results. We show that the classical treatment can able to describe reasonably well the charge exchange cross sections. Graphic abstract

Wavelength-Dependent Features of Photoelectron Spectra from Nanotip Photoemission

If a metal nanotip is irradiated with the light of a wavelength much larger than the nanotip’s radius of curvature, optical near-fields become excited. These fields are responsible for distinct strong-field electron dynamics, due to both the field enhancement and spatial localization. By classical trajectory, Monte Carlo (CTMC) simulation, and the integration of the time-dependent Schrödinger equation (TDSE), we find that the photoelectron spectra for nanotip strong-field photoemission, irradiated by mid-infrared laser pulses, present distinctive wavelength-dependent features, especially in the mid- to high-electron energy regions, which are different from the well known ones. By extracting the electron trajectories from the CTMC simulation, we investigate these particular wavelength-dependent features. Our theoretical results contribute to understanding the photoemission and electron dynamics at nanostructures, and pave new pathways for designing high-energy nanometer-sized ultrafast electron sources.

Ionization Cross Sections in the Collision between Two Ground State Hydrogen Atoms at Low Energies

The interaction between two ground state hydrogen atoms in a collision was studied using the four-body classical trajectory Monte Carlo method. We present the total cross sections for the dominant channels, namely for the single ionization of the target, the ionization of the projectile, resulting from pure ionization, and also from the electron transfer (capture or loss) processes. We also present cross sections for the complete break of the system, resulting in the final channel for four free particles. The calculations were carried out at low energies, relevant to the interest of fusion research. We present our cross sections in the projectile energy range between 2.0 keV and 100 keV and compare them with previously obtained theoretical and experimental results.

Interaction of Be4+ and Ground State Hydrogen Atom—Classical Treatment of the Collision

The interaction between Be4+ and hydrogen atom is studied using the three-body classical trajectory Monte Carlo method (CTMC) and the quasiclassical trajectory Monte Carlo method of Kirschbaum and Wilets (QTMC-KW). We present total cross sections for target ionization, target excitation, and charge exchange to the projectile bound states. Calculations are carried out in the projectile energy range between 10 and 1000 keV/au, relevant to the interest of fusion research when the target hydrogen atom is in the ground state. Our results are compared with previous theoretical results. We found that the classical treatment describes reasonably well the cross sections for various final channels. Moreover, we show that the calculations by the QTMC-KW model significantly improve the obtained cross sections.