Comparative study of construction of divergence of wind field based on OLR data obtained from – polar orbiting and geostationary satellites

An assessment of Outgoing longwave radiation data obtained from polar orbiting and geostationary satellites is made to see which one, is more convenient and useful for the construction of divergence of the wind field for regional models. The availability of OLR data from TIROS-N (polar orbiting) and GOES-IO (geostationary) satellites during 1979 made it possible to assess and explore a statistical relationship among the OLR data and divergence of the wind field at 850 and 2°9 hPa. constructed from the analysls of the Global Experiment data sets. This study reveals a very strong relationship between these fields in the region of deep convective activity and this relationship has also been found to be stronger for geostationary satellite than polar orbiting satellite. The use or this relationship especially over data-sparse tropical oceanic regions for NWP models is suggested.

Phosgene distribution derived from MIPAS ESA v8 data: intercomparisons and trends

The Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) measured the middle-infrared limb emission spectrum of the atmosphere from 2002 to 2012 on board ENVISAT, a polar-orbiting satellite. Recently, the European Space Agency (ESA) completed the final reprocessing of MIPAS measurements, using version 8 of the level 1 and level 2 processors, which include more accurate models, processing strategies, and auxiliary data. The list of retrieved gases has been extended, and it now includes a number of new species with weak emission features in the MIPAS spectral range. The new retrieved trace species include carbonyl chloride (COCl2), also called phosgene. Due to its toxicity, its use has been reduced over the years; however, it is still used by chemical industries for several applications. Besides its direct injection in the troposphere, stratospheric phosgene is mainly produced from the photolysis of CCl4, a molecule present in the atmosphere because of human activity. Since phosgene has a long stratospheric lifetime, it must be carefully monitored as it is involved in the ozone destruction cycles, especially over the winter polar regions. In this paper we exploit the ESA MIPAS version 8 data in order to discuss the phosgene distribution, variability, and trends in the middle and lower stratosphere and in the upper troposphere. The zonal averages show that phosgene volume mixing ratio is larger in the stratosphere, with a peak of 40 pptv (parts per trillion by volume) between 50 and 30 hPa at equatorial latitudes, while at middle and polar latitudes it varies from 10 to 25 pptv. A moderate seasonal variability is observed in polar regions, mostly between 80 and 50 hPa. The comparison of MIPAS–ENVISAT COCl2 v8 profiles with the ones retrieved from MIPAS balloon and ACE-FTS (Atmospheric Chemistry Experiment – Fourier Transform Spectrometer) measurements highlights a negative bias of about 2 pptv, mainly in polar and mid-latitude regions. Part of this bias is attributed to the fact that the ESA level 2 v8 processor uses an updated spectroscopic database. For the trend computation, a fixed pressure grid is used to interpolate the phosgene profiles, and, for each pressure level, VMR (volume mixing ratio) monthly averages are computed in pre-defined 10∘ wide latitude bins. Then, for each latitudinal bin and pressure level, a regression model has been fitted to the resulting time series in order to derive the atmospheric trends. We find that the phosgene trends are different in the two hemispheres. The analysis shows that the stratosphere of the Northern Hemisphere is characterized by a negative trend of about −7 pptv per decade, while in the Southern Hemisphere phosgene mixing ratios increase with a rate of the order of +4 pptv per decade. This behavior resembles the stratospheric trend of CCl4, which is the main stratospheric source of COCl2. In the upper troposphere a positive trend is found in both hemispheres.

EUNADICS-AV early warning system dedicated to supporting aviation in the case of a crisis from natural airborne hazards and radionuclide clouds

The purpose of the EUNADICS-AV (European Natural Airborne Disaster Information and Coordination System for Aviation) prototype early warning system (EWS) is to develop the combined use of harmonised data products from satellite, ground-based and in situ instruments to produce alerts of airborne hazards (volcanic, dust, smoke and radionuclide clouds), satisfying the requirement of aviation air traffic management (ATM) stakeholders (https://cordis.europa.eu/project/id/723986, last access: 5 November 2021). The alert products developed by the EUNADICS-AV EWS, i.e. near-real-time (NRT) observations, email notifications and netCDF (Network Common Data Form) alert data products (called NCAP files), have shown significant interest in using selective detection of natural airborne hazards from polar-orbiting satellites. The combination of several sensors inside a single global system demonstrates the advantage of using a triggered approach to obtain selective detection from observations, which cannot initially discriminate the different aerosol types. Satellite products from hyperspectral ultraviolet–visible (UV–vis) and infrared (IR) sensors (e.g. TROPOMI – TROPOspheric Monitoring Instrument – and IASI – Infrared Atmospheric Sounding Interferometer) and a broadband geostationary imager (Spinning Enhanced Visible and InfraRed Imager; SEVIRI) and retrievals from ground-based networks (e.g. EARLINET – European Aerosol Research Lidar Network, E-PROFILE and the regional network from volcano observatories) are combined by our system to create tailored alert products (e.g. selective ash detection, SO2 column and plume height, dust cloud, and smoke from wildfires). A total of 23 different alert products are implemented, using 1 geostationary and 13 polar-orbiting satellite platforms, 3 external existing service, and 2 EU and 2 regional ground-based networks. This allows for the identification and the tracking of extreme events. The EUNADICS-AV EWS has also shown the need to implement a future relay of radiological data (gamma dose rate and radionuclides concentrations in ground-level air) in the case of a nuclear accident. This highlights the interest of operating early warnings with the use of a homogenised dataset. For the four types of airborne hazard, the EUNADICS-AV EWS has demonstrated its capability to provide NRT alert data products to trigger data assimilation and dispersion modelling providing forecasts and inverse modelling for source term estimate. Not all of our alert data products (NCAP files) are publicly disseminated. Access to our alert products is currently restricted to key users (i.e. Volcanic Ash Advisory Centres, national meteorological services, the World Meteorological Organization, governments, volcano observatories and research collaborators), as these are considered pre-decisional products. On the other hand, thanks to the EUNADICS-AV–SACS (Support to Aviation Control Service) web interface (https://sacs.aeronomie.be, last access: 5 November 2021), the main part of the satellite observations used by the EUNADICS-AV EWS is shown in NRT, with public email notification of volcanic emission and delivery of tailored images and NCAP files. All of the ATM stakeholders (e.g. pilots, airlines and passengers) can access these alert products through this free channel.

Capability of Airline Jets as an Observation Platform for Noctilucent Clouds at Middle Latitudes

The exact occurrence frequency of noctilucent clouds (NLCs) in middle latitudes is significant information because it is thought to be sensitive to long-term atmospheric change. We conducted NLC observation from airline jets in the Northern Hemisphere during the summer 2019 to evaluate the effectiveness of NLC observation from airborne platforms. By cooperating with the Japanese airline All Nippon Airways (ANA), imaging observations of NLCs were conducted on 13 flights from Jun 8 to Jul 12. As a result of careful analysis, 8 of these 13 flights were found to successfully detect NLCs from middle latitudes (lower than 55°N) during their cruising phase. Based on the results of these test observations, it is shown that an airline jet is a powerful tool to continuously monitor the occurrence frequency of NLCs at midlatitudes which is generally difficult with a polar orbiting satellite due to sparse sampling in both temporal and spatial domain. The advantages and merits of NLC observation from jets over satellite observation from a point of view of imaging geometry is also presented.

An Observational Study of Aerosols and Tropical Cyclones over the Eastern Atlantic Ocean Basin for Recent Hurricane Seasons

The aerosol vertical distribution in the tropical cyclone (TC) main development region (MDR) during the recent active hurricane seasons (2015–2018) was investigated using observations from NASA’s Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) Satellite. The Total Attenuated Backscatter (TAB) at 532 nm was measured by the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP Lidar) onboard CALIPSO which is a polar orbiting satellite that evaluates the role clouds and atmospheric aerosols play in Earth’s weather, climate and air quality. The TAB was used to illustrate the dispersion and magnitude of the aerosol vertical distribution in the TC-genesis region. A combination of extinction quality flag, cloud fraction, and cloud-aerosol discrimination (CAD) scores were used to filter out the impact of clouds. To better describe the qualitative and quantitative difference of aerosol along the paths of African Easterly Waves (AEWs), the MDR was further divided into two domains from 18° W to 30° W (Domain 1) and 30° W to 45° W (Domain 2), respectively. The distribution of average aerosol concentration from the time of active cyclogenesis was compared and quantified between each case. The resulting observations suggest that there are two distinct layers of aerosols in the vertical profile, a near surface layer from 0.5–1.75 km and an upper layer at 1.75–5 km in altitude. A quantification of the total aerosol concentration values indicate domain 2 cases were associated with higher aerosol concentrations than domain 1 cases. The environmental variables such as sea surface temperature (SST), vertical windshear (VWS), and relative humidity (RH) tended to be favorable for genesis to occur. Among all cases in this study, the results suggested tropical cyclone genesis and further development occurred under dust-loaded conditions while the environmental variables were favorable, indicating that dust aerosols may not play a significant role in inhibiting the genesis process of TCs.

Phosgene distribution derived from MIPAS ESA v8 data: intercomparisons and trends

The Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) measured the middle-infrared limb emission spectrum of the atmosphere from 2002 to 2012 on board ENVISAT, a polar-orbiting satellite. Recently, the European Space Agency (ESA) completed the final reprocessing of MIPAS measurements, using Version 8 of the Level 1 and Level 2 processors, which include more accurate models, processing strategies and auxiliary data. The list of retrieved gases has been extended, it now includes a number of new species with weak emission features in the MIPAS spectral range. The new retrieved trace species include carbonyl chloride (COCl2), also called phosgene. Due to its toxicity, its use has been reduced over the years, however it is still used by chemical industries for sevaeral applications. Besides its direct injection in the troposphere, stratospheric phosgene is mainly produced from the photolysis of CCl4, a molecule present in the atmosphere because of human activity. Since phosgene has a long stratospheric lifetime, it must be carefully monitored as it is involved in the ozone destruction cycles, especially over the winter polar regions. In this paper we exploit the ESA MIPAS Version 8 data in order to discuss the phosgene distribution, variability and trends in the middle and lower stratosphere and in the upper troposphere. The zonal averages show that phosgene volume mixing ratio is larger in the stratosphere, with a peak of 40 pptv between 50 and 30 hPa at equatorial latitudes, while at middle and polar latitudes it varies from 10 to 25 pptv. A moderate seasonal variability is observed in polar regions, mostly between 80 and 50 hPa. The comparison of MIPAS/ENVISAT COCl2 v.8 profiles with the ones retrieved from MIPAS/balloon and ACE-FTS measurements highlights a negative bias of about 2 pptv, mainly in polar and mid-latitude regions. Part of this bias is attributed to the fact that the ESA Level 2 v.8 processor uses an updated spectroscopic database. For the trend computation, a fixed pressure grid is used to interpolate the phosgene profiles and, for each pressure level, VMR monthly averages are computed in pre-defined 10°-wide latitude bins. Then, for each latitudinal bin and pressure level, a regression model has been fitted to the resulting time-series in order to derive the atmospheric trends. We find that the phosgene trends are different in the two hemispheres. The analysis shows that the stratosphere of the Northern Hemisphere is characterised by a negative trend, of about −7 pptv/decade, while in the Southern Hemisphere phosgene mixing ratios increase with a rate of the order of +4 pptv/decade. In the upper troposphere a positive trend is found in both hemispheres.

Retrieval of High Temporal Resolution Aerosol Optical Depth Using the GOCI Remote Sensing Data

High temporal resolution aerosol optical depth (AOD) products are very important for the studies of atmospheric environment and climate change. Geostationary Ocean Color Imager (GOCI) is a suitable data source for AOD retrieval, as it can monitor hourly aerosol changes and make up for the low temporal resolution deficiency of polar orbiting satellite. In this study, we proposed an algorithm for retrieving high temporal resolution AOD using GOCI data and then applied the algorithm in the Yangtze River Delta, a typical region suffering severe air pollution issues. Based on Moderate-resolution Imaging Spectroradiometer (MODIS) surface reflectance determined by MODIS V5.2 algorithm and MODIS Bidirectional Reflectance Distribution Function (BRDF) data, after spectral conversion between MODIS and GOCI, the GOCI surface reflectance at different solar angles were obtained and used to retrieve AOD. Five indicators including correlation coefficient (R), significant level of the correlation (p value), mean absolute error (MAE), mean relative error (MRE) and root mean square error (RMSE) were employed to analyze the errors between the Aerosol Robotic Network (AERONET) observed AOD and the GOCI retrieved AOD. The results showed that the GOCI AOD retrieved by the continental aerosol look-up table was consistent with the AERONET AOD (R > 0.7, p ≤ 0.05). The highest R value of Taihu Station and Xuzhou CUMT Station are both 0.84 (8:30 a.m.); the minimum RMSE at Taihu and Xuzhou-CUMT stations were 0.2077 (11:30 a.m.) and 0.1937 (10:30 a.m.), respectively. Moreover, the results suggested that the greater the solar angle of the GOCI sensor, the higher the AOD retrieval accuracy, while the retrieved AOD at noon exhibited the largest error as assessed by MAE and MRE. We concluded that the inaccurate estimation of surface reflectance was the root cause of the retrieval errors. This study has implications in providing a deep understanding of the effects of solar angle changes on retrieving AOD using GOCI.

Fengyun-3D/MERSI-II Cloud Thermodynamic Phase Determination Using a Machine-Learning Approach

Global cloud thermodynamic phase (CP) is normally derived from polar-orbiting satellite imaging data with high spatial resolution. However, constraining conditions and empirical thresholds used in the MODIS (Moderate Resolution Imaging Spectroradiometer) CP algorithm are closely associated with spectral properties of the MODIS infrared (IR) spectral bands, with obvious deviations and incompatibility induced when the algorithm is applied to data from other similar space-based sensors. To reduce the algorithm dependence on spectral properties and empirical thresholds for CP retrieval, a machine learning (ML)-based methodology was developed for retrieving CP data from China’s new-generation polar-orbiting satellite, FY-3D/MERSI-II (Fengyun-3D/Moderate Resolution Spectral Imager-II). Five machine learning algorithms were used, namely, k-nearest-neighbor (KNN), support vector machine (SVM), random forest (RF), Stacking and gradient boosting decision tree (GBDT). The RF algorithm gave the best performance. One year of EOS (Earth Observation System) MODIS CP products (July 2018 to June 2019) were used as reference labels to train the relationship between MODIS CP (MYD06 IR) and six IR bands of MERSI-II. CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization), MODIS, and FY-3D/MERSI-II CP products were used together for cross-validation. Results indicate strong spatial consistency between ML-based MERSI-II and MODIS CP products. The hit rate (HR) of random forest (RF) CP product could reach 0.85 compared with MYD06 IR CP products. In addition, when compared with the operational FY-3D/MERSI CP product, the RF-based CP product had higher HRs. Using the CALIOP cloud product as an independent reference, the liquid-phase accuracy of the RF CP product was higher than that of operational FY-3D/MERSI-II and MYD06 IR CP products. This study aimed to establish a robust algorithm for deriving FY-3D/MERSI-II CP climate data record (CDR) for research and applications.

EUNADICS early warning system dedicated to support aviation in case of crisis from natural airborne hazard and radionuclide cloud

The purpose of the EUNADICS prototype Early Warning System (EWS) is to proceed the combined use of harmonise data products from satellite, ground-based and in situ instruments to produce alerts of airborne hazard (volcanic, dust, smoke and radionuclide clouds), satisfying the requirement of ATM stakeholders (www.eunadics.eu). The alert products developed by EUNADICS EWS (i.e. NRT observations, email notifications and NetCDF Alert data Products, called NCAP) have shown shows the significant interest in using selective detection of natural airborne hazards from polar orbiting satellite. The combination of several sensors inside a single global system demonstrates the advantage of using a triggered approach to obtain selective detection from observations, which cannot initially discriminate the different aerosol types. Satellite products from hyperspectral UV and IR sensors (e.g. TROPOMI, IASI) and broadband geostationary imager (SEVIRI), and retrievals from ground-based networks (e.g. EARLINET, E-PROFILE and the regional network from volcanic observatories), are combined by our system to create tailored alert products (e.g. selective ash detection, SO2 column and plume height, dust cloud and smoke from wildfires). A total of 23 different alert products are implemented, using 1 geostationary and 12 polar orbiting satellite platforms, 3 external existing service, 2 EU and 2 regional ground-based networks. This allows the identification and the traceability of extreme events. EUNADICS EWS has also shown the interest to proceed a future relay of radiological data (gamma dose rate and radionuclides concentrations in ground-level air) in case of nuclear accident, highlighting the capability of operating early warnings with the use of homogenised dataset. For the four types of airborne hazard, EUNADICS EWS has demonstrated its capability to provide NRT alert data products to trigger data assimilation and dispersion modelling providing forecasts, and inverse modelling for source term estimate. All our alert data products (NCAP files) are not publicly disseminated. Access to our alert products is currently restricted to key users (i.e. Volcanic Ash Advisory Centres, National Meteorological Services, World Meteorological Organization, governments, volcanic observatories and research collaborators), as these are considered pre-decisional products. On the other hand, thanks to the SACS/EUNADICS web interface (https://sacs.aeronomie.be), the main part of the satellite observations used by EUNADICS EWS, are shown in NRT, with public email notification of volcanic emission and delivery of tailored images and NCAP files. All the ATM stakeholders (e.g. VAACs, NMSs, WMOs, Airlines and Pilots) can access and benefit of these alert products through this free channel.