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2021 ◽  
Author(s):  
Liang Cai ◽  
Krishna M Kovur ◽  
Prashanthi Kovur ◽  
Carlo D. Montemagno

We report the design, fabrication and quantitative performance analysis of a low-cost, flexible carbon nanotube (CNT) network-based deoxyribonucleic acid (DNA) sensor. These sensors comprise an array of ink-jet printed silver (Ag) electrodes on a transparent polyethylene terephthalate (PET) flexible substrate, where a CNT network acts as a sensing layer. The DNA hybridization is studied by immobilizing single-stranded DNA (ssDNA) probes on the CNT surface; these probes recognize their complementary DNA target. Further, we have carried out a quantitative performance analysis of the flexible CNT biosensors using the analytic hierarchy process (AHP). We have identified various influencing factors and sub-factors (performance indicators), and quantified the performance of the flexible CNT biosensors in different measured states (before bending, during bending and after bending). Additionally, the noise and other external factors contributing to the measured real signal have been quantified. The interpretation of the overall outcome will enable the improvement of the performance of flexible biosensors fabricated through large-scale manufacturing for possible commercialization.


Author(s):  
Zolile Wiseman Dlamini ◽  
Sreedevi Vallabhapurapu ◽  
Olamide Abiodun Daramola ◽  
Potlaki Foster Tseki ◽  
Rui Werner Macedo Krause ◽  
...  

In this paper, we report on the resistive switching (RS) and conduction mechanisms in devices consisting of CdTe/CdSe core–shell quantum dots embedded chitosan composites active layer. Two devices with active layers sandwiched between (1) Al and Ag, and (2) ITO and Ag electrodes were studied. Both devices exhibited bipolar memory behavior with [Formula: see text] V and [Formula: see text][Formula: see text]V, for the Al-based device, while [Formula: see text] V and [Formula: see text][Formula: see text]V were observed for the ITO-based device, enabling both devices to be operated at low powers. However, the switching mechanisms of both devices were different, i.e., RS in Al device was attributed to conductive bridge mechanism, while space-charge-limited driven conduction filament attributed the switching mechanism of the ITO device. Additionally, the Al-based device showed long retention ([Formula: see text][Formula: see text]s) and a reasonable large ([Formula: see text]) ON/OFF ratio. Additionally, for this device, we also observed sweeping cycle-induced reversal of voltage polarity of the [Formula: see text] and [Formula: see text]. In contrast, we observed that increasing sweeping cycles resulted in an exponential decrease of the OFF-state resistance of the ITO-based device.


2021 ◽  
Vol 2086 (1) ◽  
pp. 012043
Author(s):  
V A Vorontsov ◽  
D A Antonov ◽  
A V Kruglov ◽  
I N Antonov ◽  
M E Shenina ◽  
...  

Abstract We report on an experimental study of resistive switching (RS) of individual dislocations in Ag/Ge/Si(001) memristors by combined grazing incidence ion sputtering of the Ag electrodes and application of Conductive Atomic Force Microscopy to provide an electrical contact to individual Ag-filled dislocations in the Ge layer. Two types of RS were observed corresponding to two different RS mechanisms: (i) drift of Ag+ ions inside the dislocation cores and (ii) RedOx reactions in residual GeO x in the etch pits on the Ge layer surface.


Polymers ◽  
2021 ◽  
Vol 13 (22) ◽  
pp. 4020
Author(s):  
Chung-Yueh Shih ◽  
Jian-Zhi Huang ◽  
Mei-Hsin Chen ◽  
Cheng-Che Hsu ◽  
Chih-I Wu ◽  
...  

A bathocuproine (BCP) layer is typically used as the hole-blocking layer in p-i-n-structure perovskite solar cells (PSCs) between PC61BM and Ag electrodes. Before evaporating the Ag, we used a low-temperature (<40 °C) atmospheric-pressure dielectric barrier discharge jet (DBDjet) to treat the BCP with different scan rates. The main purpose of this was to change the contact resistance between the BCP layer and the Ag electrodes through surface modification using a DBDjet. The best power conversion efficiency (PCE) of 13.11% was achieved at a DBDjet scan rate of 2 cm/s. The He DBDjet treatment introduced nitrogen to form C-N bonds and create pits on the BCP layer. This deteriorated the interface between the BCP and the follow-up deposited-Ag top electrode. Compared to the device without the plasma treatment on the BCP layer, the He DBDjet treatment on the BCP layer reduced photocurrent hysteresis but deteriorated the fill factor and the efficiency of the PSCs.


2021 ◽  
Author(s):  
Zolile Wiseman Dlamini ◽  
Sreedevi Vallabhapurapu ◽  
Tebogo Sfiso Mahule ◽  
Shuying Wu ◽  
Vijaya Srinivasu Vallabhapur

Abstract Resistive switching in MoS2 embedded PVP composite-based ReRAM with Al and Ag electrodes is reported. A cost-free drop cast method was used to deposit active layers consisting of 30 wt%, 40 wt%, and 70 wt% of MoS2 in PVP. Each system exhibited unique electroforming and switching mode. Asymmetrical bipolar resistive switching occurring only in the positive voltage bias, a typical bipolar resistive switching and a typical ‘O-type’ resistive switching were observed for the 30 wt%, 40 wt%, and 70 wt% systems, respectively. Furthermore, injection of charge carriers at the electrode/active layer interface and electrochemical metalization mechanisms drove the formation of a nanoscale conductive filament in the device A and B. On the other hand, we attributed the conduction mechanism of device C to hopping conduction. Our results demonstrate the behaviour of MoS2 embedded PVP composite-based ReRAM has a strong dependence on the amount of MoS2 and that both the switching and conduction mechanism can be exploited by controlling the amount of MoS2 in the composite.


2021 ◽  
Author(s):  
Liang Cai ◽  
Krishna M Kovur ◽  
Prashanthi Kovur ◽  
Carlo D. Montemagno

We report the design, fabrication and quantitative performance analysis of a low-cost, flexible carbon nanotube (CNT) network-based deoxyribonucleic acid (DNA) sensor. These sensors comprise an array of ink-jet printed silver (Ag) electrodes on a transparent polyethylene terephthalate (PET) flexible substrate, where a CNT network acts as a sensing layer. The DNA hybridization is studied by immobilizing single-stranded DNA (ssDNA) probes on the CNT surface; these probes recognize their complementary DNA target. Further, we have carried out a quantitative performance analysis of the flexible CNT biosensors using the analytic hierarchy process (AHP). We have identified various influencing factors and sub-factors (performance indicators), and quantified the performance of the flexible CNT biosensors in different measured states (before bending, during bending and after bending). Additionally, the noise and other external factors contributing to the measured real signal have been quantified. The interpretation of the overall outcome will enable the improvement of the performance of flexible biosensors fabricated through large-scale manufacturing for possible commercialization.


2021 ◽  
Author(s):  
Liang Cai ◽  
Krishna M Kovur ◽  
Prashanthi Kovur ◽  
Carlo D. Montemagno

We report the design, fabrication and quantitative performance analysis of a low-cost, flexible carbon nanotube (CNT) network-based deoxyribonucleic acid (DNA) sensor. These sensors comprise an array of ink-jet printed silver (Ag) electrodes on a transparent polyethylene terephthalate (PET) flexible substrate, where a CNT network acts as a sensing layer. The DNA hybridization is studied by immobilizing single-stranded DNA (ssDNA) probes on the CNT surface; these probes recognize their complementary DNA target. Further, we have carried out a quantitative performance analysis of the flexible CNT biosensors using the analytic hierarchy process (AHP). We have identified various influencing factors and sub-factors (performance indicators), and quantified the performance of the flexible CNT biosensors in different measured states (before bending, during bending and after bending). Additionally, the noise and other external factors contributing to the measured real signal have been quantified. The interpretation of the overall outcome will enable the improvement of the performance of flexible biosensors fabricated through large-scale manufacturing for possible commercialization.


2021 ◽  
Author(s):  
Liang Cai ◽  
Krishna M Kovur ◽  
Prashanthi Kovur ◽  
Carlo D. Montemagno

We report the design, fabrication and quantitative performance analysis of a low-cost, flexible carbon nanotube (CNT) network-based deoxyribonucleic acid (DNA) sensor. These sensors comprise an array of ink-jet printed silver (Ag) electrodes on a transparent polyethylene terephthalate (PET) flexible substrate, where a CNT network acts as a sensing layer. The DNA hybridization is studied by immobilizing single-stranded DNA (ssDNA) probes on the CNT surface; these probes recognize their complementary DNA target. Further, we have carried out a quantitative performance analysis of the flexible CNT biosensors using the analytic hierarchy process (AHP). We have identified various influencing factors and sub-factors (performance indicators), and quantified the performance of the flexible CNT biosensors in different measured states (before bending, during bending and after bending). Additionally, the noise and other external factors contributing to the measured real signal have been quantified. The interpretation of the overall outcome will enable the improvement of the performance of flexible biosensors fabricated through large-scale manufacturing for possible commercialization.


Energies ◽  
2021 ◽  
Vol 14 (18) ◽  
pp. 5837
Author(s):  
Jiaxin Guo ◽  
Ziming Bu ◽  
Shuo Han ◽  
Yanyu Deng ◽  
Chunyu Liu ◽  
...  

The continuous thin film of silver (Ag) film is important for semitransparent electrodes in polymer solar cells, while the Ag atoms form as non-continuous below a critical thickness. Here, semitransparent inverted polymer solar cells were fabricated using thermally evaporated Ag/germanium (Ge)/Ag as highly transparent electrodes. An ultra-thin Ge film was introduced to modify the growth mode of Ag. The dependence of the device performance and the thickness of the outer Ag film was investigated. Ag/Ge/Ag electrodes exhibited excellent optical and electrical properties, which were proved by the transmittance and reflectance spectra. A champion efficiency of 5.1% was achieved with an open-circuit voltage level of 0.703 V, a short current density of 11.63 mA/cm2, and a fill factor of 63%. The average visible transmittance (300–800 nm) of devices with Ag/Ge/Ag was calculated as 25%.


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