Microfluidic salt precipitation: implications for geological CO2 storage

Lab on a Chip ◽  
2020 ◽  
Vol 20 (20) ◽  
pp. 3806-3814
Author(s):  
Tsai-Hsing Martin Ho ◽  
Peichun Amy Tsai

Novel microfluidic visualizations reveal the simultaneous dynamics of salt nucleation and fluid drying rates while mimicking carbon capture and storage processes.

Energies ◽  
2021 ◽  
Vol 14 (6) ◽  
pp. 1557
Author(s):  
Amine Tadjer ◽  
Reidar B. Bratvold

Carbon capture and storage (CCS) has been increasingly looking like a promising strategy to reduce CO2 emissions and meet the Paris agreement’s climate target. To ensure that CCS is safe and successful, an efficient monitoring program that will prevent storage reservoir leakage and drinking water contamination in groundwater aquifers must be implemented. However, geologic CO2 sequestration (GCS) sites are not completely certain about the geological properties, which makes it difficult to predict the behavior of the injected gases, CO2 brine leakage rates through wellbores, and CO2 plume migration. Significant effort is required to observe how CO2 behaves in reservoirs. A key question is: Will the CO2 injection and storage behave as expected, and can we anticipate leakages? History matching of reservoir models can mitigate uncertainty towards a predictive strategy. It could prove challenging to develop a set of history matching models that preserve geological realism. A new Bayesian evidential learning (BEL) protocol for uncertainty quantification was released through literature, as an alternative to the model-space inversion in the history-matching approach. Consequently, an ensemble of previous geological models was developed using a prior distribution’s Monte Carlo simulation, followed by direct forecasting (DF) for joint uncertainty quantification. The goal of this work is to use prior models to identify a statistical relationship between data prediction, ensemble models, and data variables, without any explicit model inversion. The paper also introduces a new DF implementation using an ensemble smoother and shows that the new implementation can make the computation more robust than the standard method. The Utsira saline aquifer west of Norway is used to exemplify BEL’s ability to predict the CO2 mass and leakages and improve decision support regarding CO2 storage projects.


1969 ◽  
Vol 17 ◽  
pp. 13-16 ◽  
Author(s):  
Peter Frykman ◽  
Lars Henrik Nielsen ◽  
Thomas Vangkilde-Pedersen

Carbon capture and storage (CCS) is increasingly considered to be a tool that can significantly reduce the emission of CO2. It is viewed as a technology that can contribute to a substantial, global reduction of emitted CO2 within the timeframe that seems available for mitigating the effects of present and continued emission. In order to develop the CCS method the European Union (EU) has supported research programmes for more than a decade, which focus on capture techniques, transport and geological storage. The results of the numerous research projects on geological storage are summarised in a comprehensive best practice manual outlining guidelines for storage in saline aquifers (Chadwick et al. 2008). A detailed directive for geological storage is under implementation (European Commission 2009), and the EU has furthermore established a programme for supporting the development of more than ten large-scale demonstration plants throughout Europe. Geological investigations show that suitable storage sites are present in most European countries. In Denmark initial investigations conducted by the Geological Survey of Denmark and Greenland and private companies indicate that there is significant storage potential at several locations in the subsurface.


Energies ◽  
2020 ◽  
Vol 13 (23) ◽  
pp. 6456
Author(s):  
Ewa Knapik ◽  
Katarzyna Chruszcz-Lipska

Worldwide experiences related to geological CO2 storage show that the process of the injection of carbon dioxide into depleted oil reservoirs (CCS-EOR, Carbon Capture and Storage—Enhanced Oil Recovery) is highly profitable. The injection of CO2 will allow an increasing recovery factor (thus increasing CCS process profitability) and revitalize mature reservoirs, which may lead to oil spills due to pressure buildups. In Poland, such a solution has not yet been implemented in the industry. This work provides additional data for analysis of the possibility of the CCS-EOR method’s implementation for three potential clusters of Polish oil reservoirs located at a short distance one from another. The aim of the work was to examine the properties of reservoir fluids for these selected oil reservoirs in order to assure a better understanding of the physicochemical phenomena that accompany the gas injection process. The chemical composition of oils was determined by gas chromatography. All tested oils represent a medium black oil type with the density ranging from 795 to 843 g/L and the viscosity at 313 K, varying from 1.95 to 5.04 mm/s. The content of heavier components C25+ is up to 17 wt. %. CO2–oil MMP (Minimum Miscibility Pressure) was calculated in a CHEMCAD simulator using the Soave–Redlich–Kwong equation of state (SRK EoS). The oil composition was defined as a mixture of n-alkanes. Relatively low MMP values (ca. 8.3 MPa for all tested oils at 313 K) indicate a high potential of the EOR method, and make this geological CO2 storage form more attractive to the industry. For reservoir brines, the content of the main ions was experimentally measured and CO2 solubility under reservoir conditions was calculated. The reservoir brines showed a significant variation in properties with total dissolved solids contents varying from 17.5 to 378 g/L. CO2 solubility in brines depends on reservoir conditions and brine chemistry. The highest calculated CO2 solubility is 1.79 mol/kg, which suggest possible CO2 storage in aquifers.


2020 ◽  
Vol 52 (1) ◽  
pp. 163-171 ◽  
Author(s):  
Jon G. Gluyas ◽  
Usman Bagudu

AbstractThe Endurance, four-way, dip-closed structure in UK Blocks 42/25 and 43/21 occurs over a salt swell diapir and within Triassic and younger strata. The Lower Triassic Bunter Sandstone Formation reservoir within the structure was tested twice for natural gas (in 1970 and 1990) but both wells were dry. The reservoir is both thick and high quality and, as such, an excellent candidate site for subsurface CO2 storage.In 2013 a consortium led by National Grid Carbon drilled an appraisal well on the structure and undertook an injection test ahead of a planned development of Endurance as the first bespoke storage site on the UK Continental Shelf with an expected injection rate of 2.68 × 106 t of dense phase CO2 each year for 20 years. The site was not developed following the UK Government's removal of financial support for carbon capture and storage (CCS) demonstration projects, but it is hoped with the recent March 2020 Budget that government support for CCS may now be back on track.


2019 ◽  
Vol 8 (6) ◽  
pp. e12861023 ◽  
Author(s):  
Pedro Junior Zucatelli ◽  
Ana Paula Meneguelo ◽  
Gisele de Lorena Diniz Chaves ◽  
Gisele de Lorena Diniz Chaves ◽  
Marielce de Cassia Ribeiro Tosta

The integrity of natural systems is already at risk because of climate change caused by the intense emissions of greenhouse gases in the atmosphere. The goal of geological carbon sequestration is to capture, transport and store CO2 in appropriate geological formations. In this review, we address the geological environments conducive to the application of CCS projects (Carbon Capture and Storage), the phases that make up these projects, and their associated investment and operating costs. Furthermore it is presented the calculations of the estimated financial profitability of different types of projects in Brazil. Using mathematical models, it can be concluded that the Roncador field presents higher gross revenue when the amount of extra oil that can be retrieved is 9.3% (US$ 48.55 billions approximately in 2018). Additional calculations show that the Paraná saline aquifer has the highest gross revenue (US$ 6.90 trillions in 2018) when compared to the Solimões (US$ 3.76 trillions approximately in 2018) and Santos saline aquifers (US$ 2.21 trillions approximately in 2018) if a CCS project were to be employed. Therefore, the proposed Carbon Capture and Storage method in this study is an important scientific contribution for reliable large-scale CO2 storage in Brazil.


2019 ◽  
Vol 59 (2) ◽  
pp. 565
Author(s):  
Aaron De Fina ◽  
Marc Chable ◽  
Cameron Wills

The CO2CRC Otway Project continues to demonstrate that carbon capture and storage is a viable option for CO2 mitigation. The CO2CRC Otway Project is Australia’s first CO2 demonstration project, with two projects completed, involving geological storage of some 80000 tonnes of CO2 over the past 10 years. The project was initially authorised for a single stage with a finite life, but the growing requirements of the global carbon capture and storage community required further research on carbon capture and storage technologies and behaviour (via Stages 2 and 3), and so the project was extended. CO2CRC has undertaken 360-degree stakeholder engagement processes throughout the project, regularly consulting with regulators, governments, industry, partners, researchers and the community. This has been especially important as the project changed, operating in a niche space between Victorian environment, petroleum and water Acts. This process has allowed CO2CRC to contribute to alignment efforts within regulatory bodies, to enhance regulations to cover project activities, ensuring best practices are documented and observed to the satisfaction of the regulators and wider community. The Otway Basin in south-west Victoria is a region not immune to broader community concerns regarding the oil and gas and other industries. The surrounding area is predominately dairy farming, with locals relying heavily on the aquifers beneath their land. Although such a backdrop suggests potentially high levels of concern and scrutiny, especially when projects necessitate drilling or other invasive activities, the project has maintained strong local stakeholder engagement and support due to ongoing implementation and evaluation of the stakeholder management processes.


Author(s):  
Nediljka Gaurina-Medjimurec ◽  
Borivoje Pasic

Geologic storage is the component of Carbon Capture and Storage (CCS) in which the carbon dioxide (CO2) is disposed in the appropriate underground formation. To successfully inject CO2 into the subsurface to mitigate greenhouse gases in the atmosphere, the CO2 must to be trapped in the subsurface and must not be allowed to leak to the surface or to potable water sources above the injection zone. For the purposes of risk assessment, a priority is to evaluate what would happen if CO2 migrated unexpectedly through the confining unit(s), potentially resulting in undesirable impacts on a variety of potential receptors. One of the main risks identified in geological CO2 storage is the potential for CO2 leakage through or along wells. To avoid leakage from the injection wells, the integrity of the wells must be maintained during the injection period and for as long as free CO2 exists in the injection zone.


2013 ◽  
Vol 4 (2) ◽  
pp. 237-251 ◽  
Author(s):  
K. Becker ◽  
V. Wulfmeyer ◽  
T. Berger ◽  
J. Gebel ◽  
W. Münch

Abstract. We present a comprehensive, interdisciplinary project which demonstrates that large-scale plantations of Jatropha curcas – if established in hot, dry coastal areas around the world – could capture 17–25 t of carbon dioxide per hectare per year from the atmosphere (over a 20 yr period). Based on recent farming results it is confirmed that the Jatropha curcas plant is well adapted to harsh environments and is capable of growing alone or in combination with other tree and shrub species with minimal irrigation in hot deserts where rain occurs only sporadically. Our investigations indicate that there is sufficient unused and marginal land for the widespread cultivation of Jatropha curcas to have a significant impact on atmospheric CO2 levels at least for several decades. In a system in which desalinated seawater is used for irrigation and for delivery of mineral nutrients, the sequestration costs were estimated to range from 42–63 EUR per tonne CO2. This result makes carbon farming a technology that is competitive with carbon capture and storage (CCS). In addition, high-resolution simulations using an advanced land-surface–atmosphere model indicate that a 10 000 km2 plantation could produce a reduction in mean surface temperature and an onset or increase in rain and dew fall at a regional level. In such areas, plant growth and CO2 storage could continue until permanent woodland or forest had been established. In other areas, salinization of the soil may limit plant growth to 2–3 decades whereupon irrigation could be ceased and the captured carbon stored as woody biomass.


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