Matrix effects in white-beam X-ray fluorescence holography

2015 ◽  
Vol 48 (2) ◽  
pp. 542-549 ◽  
Author(s):  
D. T. Dul ◽  
P. Korecki

Recently, it has been shown that atomic structure determination with X-ray fluorescence holography (XFH) can be hindered by matrix effects,i.e.beam attenuation and indirect excitation. The analysis was limited to the monochromatic regime. In this work, the description of matrix effects is extended to the polychromatic case. It is shown that matrix effects affect the element sensitivity of white-beam XFH by introducing distortions in the holographic signal which may lead to spurious maxima in the reconstructed image. For high energies of the X-ray beam it is found that the effect of beam attenuation is very weak and indirect excitation mainly contributes to the distortions. A correction for matrix effects is proposed in the high-energy range, which allows one to remove the distortions and retrieve pure element-sensitive information. Numerical model calculations are performed to visualize the reduction of element sensitivity and its implications on local structure imaging.

2016 ◽  
Vol 230 (4) ◽  
Author(s):  
Dawid Tadeusz Dul ◽  
Paweł Korecki

AbstractThe influence of matrix effects i.e. beam attenuation (BA) and indirect excitation (IE) on local structure imaging with multiple-energy x-ray fluorescence holography is studied using computer simulations. An analytic formalism is developed which allows for the description of BA and IE when the thickness of the sample is arbitrary. It is shown that beyond the thin-sample approximation, in specific cases, the measured holograms cannot be treated as entirely element sensitive. Consequently, it is demonstrated that due to the reduction of element sensitivity, spurious maxima can arise in the holographic reconstruction which can be misinterpreted as atomic images. The proposed formalism allows one to analyse BA and IE and to correct for them. It opens way for quantitative interpretation of x-ray fluorescence holograms.


2020 ◽  
Vol 497 (3) ◽  
pp. 2553-2561
Author(s):  
Felicia Krauß ◽  
Emily Calamari ◽  
Azadeh Keivani ◽  
Alexis Coleiro ◽  
Phil A Evans ◽  
...  

ABSTRACT High-energy neutrinos are a promising tool for identifying astrophysical sources of high and ultra-high energy cosmic rays (UHECRs). Prospects of detecting neutrinos at high energies (≳TeV) from blazars have been boosted after the recent association of IceCube-170922A and TXS 0506+056. We investigate the high-energy neutrino, IceCube-190331A, a high-energy starting event (HESE) with a high likelihood of being astrophysical in origin. We initiated a Swift/XRT and UVOT tiling mosaic of the neutrino localization and followed up with ATCA radio observations, compiling a multiwavelength spectral energy distribution (SED) for the most likely source of origin. NuSTAR observations of the neutrino location and a nearby X-ray source were also performed. We find two promising counterpart in the 90 per cent confidence localization region and identify the brightest as the most likely counterpart. However, no Fermi/LAT γ-ray source and no prompt Swift/BAT source is consistent with the neutrino event. At this point, it is unclear whether any of the counterparts produced IceCube-190331A. We note that the Helix Nebula is also consistent with the position of the neutrino event and we calculate that associated particle acceleration processes cannot produce the required energies to generate a high-energy HESE neutrino.


2011 ◽  
Vol 178-179 ◽  
pp. 360-365 ◽  
Author(s):  
Alexander Gröschel ◽  
Johannes Will ◽  
Christoph Bergmann ◽  
Hannes Grillenberger ◽  
Stefan Eichler ◽  
...  

A defocused Laue diffractometer setup operating with the white beam of a high energy X-ray tube has been used for a topographic visualization of structural defects in semiconductor wafers. The laboratory white beam X-ray topograph of a Czochralski Si wafer with oxygen precipitates grown in an annealing process is compared to a μPCD image. Further, the dislocation network in a VGF GaAs wafer is studied under thermal annealing up to 1140°C and the in-situ capability of the setup is demonstrated.


2008 ◽  
Vol 86 (1) ◽  
pp. 267-276 ◽  
Author(s):  
A S Safronova ◽  
V L Kantsyrev ◽  
P Neill ◽  
U I Safronova ◽  
D A Fedin ◽  
...  

The results from the last six years of X-ray spectroscopy and spectropolarimetry of high-energy density Z-pinch plasmas complemented by experiments with the electron beam ion trap (EBIT) at the Lawrence Livermore National Laboratory (LLNL) are presented. The two topics discussed are the development of M-shell X-ray W spectroscopic diagnostics and K-shell Ti spectropolarimetry of Z-pinch plasmas. The main focus is on radiation from a specific load configuration called an “X-pinch”. In this work the study of X-pinches with tungsten wires combined with wires from other, lower Z materials is reported. Utilizing data produced with the LLNL EBIT at different energies of the electron beam the theoretical prediction of line positions and intensity of M-shell W spectra were tested and calibrated. Polarization-sensitive X-pinch experiments at the University of Nevada, Reno (UNR) provide experimental evidence for the existence of strong electron beams in Ti and Mo X-pinch plasmas and motivate the development of X-ray spectropolarimetry of Z-pinch plasmas. This diagnostic is based on the measurement of spectra recorded simultaneously by two spectrometers with different sensitivity to the linear polarization of the observed lines and compared with theoretical models of polarization-dependent spectra. Polarization-dependent K-shell spectra from Ti X-pinches are presented and compared with model calculations and with spectra generated by a quasi-Maxwellian electron beam at the LLNL EBIT-II electron beam ion trap.PACS Nos.: 32.30.Rj, 52.58.Lq, 52.70.La


2018 ◽  
Vol 14 (S342) ◽  
pp. 176-179
Author(s):  
Giulia Migliori

AbstractObservations at high-energies are important to define the first stages of the evolution of extragalactic radio sources and to characterize the interstellar medium of their host galaxies. In some of the X-ray-observed Compact Symmetric Objects (CSOs, among the youngest and most compact radio galaxies), we measured values of the total hydrogen column densities large enough to slow or prevent the radio source growth. The γ-ray window has the potential to constrain the non-thermal contribution of jets and lobes to the total high-energy emission. However, so far, young radio sources remain elusive in γ-rays, with only a handful of detections (or candidates) reported by Fermi. I present our γ-ray study of the CSO PKS 1718–649, and draw comparison with the restarted, γ-ray detected, radio galaxy 3C 84.


2015 ◽  
Vol 1792 ◽  
Author(s):  
Stephen Babalola ◽  
Samuel Uba ◽  
Anwar Hossain ◽  
Giuseppe Camarda ◽  
Ralph James ◽  
...  

ABSTRACTCZT is a semiconductor material that promises to be a good candidate for uncooled gamma radiation detectors. However, to date, we are yet to overcome the technological difficulties in production of large size, defect-free CZT crystals. The most common problem is accumulation of Tellurium precipitates as microscopic inclusions. These inclusions influence the charge collection through charge trapping and electric field distortion. We employed high energy transmission X-ray diffraction techniques to study the quality of the CdZnTe crystals grown by Bridgman Technique. Crystallinity and defects within two different growth set-ups, i.e. with and without choked seeding, were compared by imaging the crystal orientation topography with white beam X-ray diffraction topography (WBXDT). The X-ray diffraction topography results show high correlation with large-area infrared transmission images of the crystals. Grain boundaries that are highly decorated with Te inclusions are observed. Characteristic Te inclusion arrangements as a result of growth conditions are discussed. We also measured the electronic properties of the detectors fabricated from ingots grown using two Bridgman processes, and observed a reduction in electrical resistivity of choked-seeding-grown CdZnTe crystals. Our results show that although choked seeding technique holds a promise in the realization of high quality mono-crystalline CdZnTe, current growth parameters must be improved to obtain defect-free crystals. These results are helpful to attain optimal seeding process for Bridgman-growth of large single crystals of CdZnTe.


2008 ◽  
Author(s):  
S. Y. Zhang ◽  
W. Vorster ◽  
T. S. Jun ◽  
X. Song ◽  
M. Golshan ◽  
...  

Author(s):  
Phil Uttley ◽  
Roland den Hartog ◽  
Cosimo Bambi ◽  
Didier Barret ◽  
Stefano Bianchi ◽  
...  

AbstractWe propose the development of X-ray interferometry (XRI), to reveal the Universe at high energies with ultra-high spatial resolution. With baselines which can be accommodated on a single spacecraft, XRI can reach 100 μ as resolution at 10 Å (1.2 keV) and 20 μ as at 2 Å (6 keV), enabling imaging and imaging-spectroscopy of (for example) X-ray coronae of nearby accreting supermassive black holes (SMBH) and the SMBH ‘shadow’; SMBH accretion flows and outflows; X-ray binary winds and orbits; stellar coronae within $\sim $ ∼ 100 pc and many exoplanets which transit across them. For sufficiently luminous sources XRI will resolve sub-pc scales across the entire observable Universe, revealing accreting binary SMBHs and enabling trigonometric measurements of the Hubble constant with X-ray light echoes from quasars or explosive transients. A multi-spacecraft ‘constellation’ interferometer would resolve well below 1 μ as, enabling SMBH event horizons to be resolved in many active galaxies and the detailed study of the effects of strong field gravity on the dynamics and emission from accreting gas close to the black hole.


2017 ◽  
Vol 3 (3) ◽  
pp. 3-14
Author(s):  
Виктор Гречнев ◽  
Victor Grechnev ◽  
Валентин Киселев ◽  
Valentin Kiselev ◽  
Наталия Мешалкина ◽  
...  

We analyze the relations between various combinations of peak fluxes and fluences of solar microwave bursts at 35 GHz recorded with the Nobeyama Radio Polarimeters during 1990–2015, and corresponding parameters of proton enhancements with E>100 MeV exceeding 0.1 pfu registered by GOES monitors in near-Earth environment. The highest correlation has been found between the microwave and proton fluences. This fact reflects a dependence of the total number of protons on the total duration of the acceleration process. In the events with strong flares, the correlation coefficients of proton fluences with microwave and soft X-ray fluences are higher than those with speeds of coronal mass ejections. The results indicate a statistically larger contribution of flare processes to acceleration of high-energy protons. Acceleration by shock waves seems to be less important at high energies in events associated with strong flares, although its contribution probably prevails in weaker events. The probability of a detectable proton enhancement was found to directly depend on the peak flux and duration of the microwave burst, that can be used for diagnostics of proton enhancements based on microwave observations.


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