Atmospheric aerosol scattering to mass ratio

1980 ◽  
Vol 58 (4) ◽  
pp. 549-553
Author(s):  
A. W. Harrison ◽  
Rosaline Pi
Keyword(s):  
Atmospheric Aerosol ◽  
Mass Concentration ◽  
Cascade Impactor ◽  
Scattering Coefficient ◽  
Mass Ratio ◽  
Aerosol Scattering ◽  
Combined Operation ◽  
Mass Size ◽  
Clean Air ◽  
Made In

The combined operation of a spectronephelometer and a cascade impactor has been used to study the ratio of differential scattering coefficient (at 550 nm) and mass concentration at mass concentrations of less than 40 µg m−3. Detailed analysis of the mass size distribution impactor data assumed to be near lognormal yielded values of the bulk density in the range 1 to 4 g cm−3. Measurements made in May–June 1978 and in November–December 1978 gave substantially the same results indicating no seasonal variation in either aerosol density or scattering coefficient to mass concentration ratio for mountain and continental background clean air.

scholarly journals Evaluation of Two Low-Cost Optical Particle Counters for the Measurement of Ambient Aerosol Scattering Coefficient and Ångström Exponent

Sensors ◽  
2020 ◽  
Vol 20 (9) ◽  
pp. 2617 ◽  
Author(s):  
Krzysztof M. Markowicz ◽  
Michał T. Chiliński
Keyword(s):  
Optical Properties ◽  
Correlation Coefficient ◽  
Mass Concentration ◽  
Low Cost ◽  
Pearson Correlation ◽  
Scattering Coefficient ◽  
Pearson Correlation Coefficient ◽  
Aerosol Optical Properties ◽  
Aerosol Scattering ◽  
Ångström Exponent

The aerosol scattering coefficient and Ångström exponent (AE) are important parameters in the understanding of aerosol optical properties and aerosol direct effect. These parameters are usually measured by a nephelometer network which is under-represented geographically; however, a rapid growth of air-pollution monitoring, using low-cost particle sensors, may extend observation networks. This paper presents the results of co-located measurements of aerosol optical properties, such as the aerosol scattering coefficient and the scattering AE, using low-cost sensors and using a scientific-grade polar Aurora 4000 nephelometer. A high Pearson correlation coefficient (0.94–0.96) between the low-cost particulate matter (PM) mass concentration and the aerosol scattering coefficient was found. For the PM10 mass concentration, the aerosol scattering coefficient relation is linear for the Dfrobot SEN0177 sensor and non-linear for the Alphasense OPC-N2 device. After regression analyses, both low-cost instruments provided the aerosol scattering coefficient with a similar mean square error difference (RMSE) of about 20 Mm−1, which corresponds to about 27% of the mean aerosol scattering coefficient. The relative uncertainty is independent of the pollution level. In addition, the ratio of aerosol number concentration between different bins showed a significant statistical (95% of confidence level) correlation with the scattering AE. For the SEN0177, the ratio of the particle number in bin 1 (radius of 0.15–0.25 µm) to bin 4 (radius of 1.25–2.5 µm) was a linear function of the scattering AE, with a Pearson correlation coefficient of 0.74. In the case of OPC-N2, the best correlation (r = 0.66) was found for the ratio between bin 1 (radius of 0.19–0.27 µm) and bin 2 (radius of 0.27–0.39 µm). Comparisons of an estimated scattering AE from a low-cost sensor with Aurora 4000 are given with the RMSE of 0.23–0.24, which corresponds to 16–19%. In addition, a three-year (2016–2019) observation by SEN0177 indicates that this sensor can be used to determine an annual cycle as well as a short-term variability.

scholarly journals Synthesis of Metal Organic Frameworks by Ball-Milling

Crystals ◽  
2020 ◽  
Vol 11 (1) ◽  
pp. 15
Author(s):  
Cheng-An Tao ◽  
Jian-Fang Wang
Keyword(s):  
Ball Milling ◽  
Large Scale ◽  
Raw Materials ◽  
Metal Organic Frameworks ◽  
Research Topic ◽  
Mass Ratio ◽  
Time Consumption ◽  
Metal Organic ◽  
Short Time ◽  
Made In

Metal-organic frameworks (MOFs) have been used in adsorption, separation, catalysis, sensing, photo/electro/magnetics, and biomedical fields because of their unique periodic pore structure and excellent properties and have become a hot research topic in recent years. Ball milling is a method of small pollution, short time-consumption, and large-scale synthesis of MOFs. In recent years, many important advances have been made. In this paper, the influencing factors of MOFs synthesized by grinding were reviewed systematically from four aspects: auxiliary additives, metal sources, organic linkers, and reaction specific conditions (such as frequency, reaction time, and mass ratio of ball and raw materials). The prospect for the future development of the synthesis of MOFs by grinding was proposed.

scholarly journals Ultrafine Aerosol Particle Sizer Based on Piezoresistive Microcantilever Resonators with Integrated Air-Flow Channel

Sensors ◽  
2021 ◽  
Vol 21 (11) ◽  
pp. 3731
Author(s):  
Maik Bertke ◽  
Ina Kirsch ◽  
Erik Uhde ◽  
Erwin Peiner
Keyword(s):  
Mass Concentration ◽  
Limit Of Detection ◽  
A Priori ◽  
Micro Electro Mechanical System ◽  
Single Chip ◽  
Air Stream ◽  
Mems Technology ◽  
Clean Air ◽  
Particle Sizer ◽  
Ultrafine Aerosol

To monitor airborne nano-sized particles (NPs), a single-chip differential mobility particle sizer (DMPS) based on resonant micro cantilevers in defined micro-fluidic channels (µFCs) is introduced. A size bin of the positive-charged fraction of particles herein is separated from the air stream by aligning their trajectories onto the cantilever under the action of a perpendicular electrostatic field of variable strength. We use previously described µFCs and piezoresistive micro cantilevers (PMCs) of 16 ng mass fabricated using micro electro mechanical system (MEMS) technology, which offer a limit of detection of captured particle mass of 0.26 pg and a minimum detectable particulate mass concentration in air of 0.75 µg/m3. Mobility sizing in 4 bins of a nebulized carbon aerosol NPs is demonstrated based on finite element modelling (FEM) combined with a-priori knowledge of particle charge state. Good agreement of better than 14% of mass concentration is observed in a chamber test for the novel MEMS-DMPS vs. a simultaneously operated standard fast mobility particle sizer (FMPS) as reference instrument. Refreshing of polluted cantilevers is feasible without de-mounting the sensor chip from its package by multiply purging them alternately in acetone steam and clean air.

scholarly journals Tropospheric aerosol scattering and absorption over Central Europe: a closure study for the dry particle state

2013 ◽  
Vol 13 (10) ◽  
pp. 27811-27854 ◽  
Author(s):  
N. Ma ◽  
W. Birmili ◽  
T. Müller ◽  
T. Tuch ◽  
Y. F. Cheng ◽  
...  
Keyword(s):  
Optical Properties ◽  
Direct Measurement ◽  
Radiative Forcing ◽  
Control Measure ◽  
Atmospheric Stability ◽  
Scattering Coefficient ◽  
Particle State ◽  
Air Mass ◽  
Aerosol Scattering ◽  
Tropospheric Aerosol

Abstract. This work analyses optical properties of the dry tropospheric aerosol measured at the regional GAW observation site Melpitz in East Germany. For a continuous observation period between 2007 and 2010, we provide representative values of the dry-state scattering coefficient, the hemispheric backscattering coefficient, the absorption coefficient, single scattering albedo, and the Ångström exponent. Besides the direct measurement, the aerosol scattering coefficient was alternatively computed from experimental particle number size distributions using a Mie code. Within pre-defined limits, a closure could be achieved with the direct measurement. The achievement of closure implies that such calculations can be used as a high-level quality control measure for data sets involving multiple instrumentation. All dry optical properties showed significant annual variations, which were attributed to corresponding variations in the regional emission fluxes, the intensity of secondary particle formation, and the mixed layer height. Air mass classification showed that atmospheric stability is a major factor influencing the dry aerosol properties at the GAW station. In the cold season, temperature inversions limit the volume available for atmospheric mixing, so that the aerosol optical properties near the ground proved quite sensitive to the geographical origin of the air mass. In the warm season, when the atmosphere is usually well-mixed during day-time, considerably less variability was observed for the optical properties between different air masses. This work provides, on the basis of quality-checked in-situ measurements, a first step towards a climatological assessment of direct aerosol radiative forcing in the region under study.

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