DISPERSION OF THE QUASI-CONFINED OPTICAL PHONONS IN WURTZITE GaN/AlN MULTIPLE QUANTUM WELLS

2007 ◽  
Vol 21 (25) ◽  
pp. 4407-4418
Author(s):  
WEN DENG HUANG ◽  
SHU YI WEI ◽  
YA JIE REN ◽  
YA HUI WANG

Within the framework of the dielectric-continuum model and Loudon's uniaxial crystal model, the dispersions of the quasi-confined optical phonons in arbitrary wurtzite multiplelayer heterostructures are solved by using the transfer-matrix method. The dispersion relations of the quasi-confined phonons are investigated for GaN/AlN single QW and coupled QWs. The confinement of the quasi-confined phonons leads to a quantization of qz, j characterized by an integer m that defines the order of corresponding quasi-confined modes. The quasi-confined modes are more dispersive for decreasing m (i.e., for decreasing qz, j, the bands formed by the dispersion curves are narrower for higher order quasi-confined modes. The strain effect of QW structures has a clear influence on the dispersion behavior of the quasi-confined phonon modes and improves the frequency of the quasi-confined phonons.

2006 ◽  
Vol 20 (22) ◽  
pp. 1367-1381 ◽  
Author(s):  
WEN-DENG HUANG ◽  
SHU-YI WEI ◽  
YA-JIE REN

Within the framework of the dielectric-continuum model and Loudon's uniaxial crystal model, the equation of motion for p-polarization field in wurtzite multiplayer symmetry heterostructures are solved for the quasi-confined phonon (QC) modes. The polarization eigenvector, the dispersion relation, and the electron-QC interaction Fröhlich-like Hamiltonian are derived by using the transfer-matrix method. The analytical theory and formulas can be directly applied to the single quantum well (QW) and multiple quantum wells (QWs), and superlattices (SLs). The dispersion relations and the electron-QC coupling strength are investigated for a wurtzite GaN/Al 0.15 Ga 0.85 N single QW. The results show that there are infinite branches of the dispersion curve with definite symmetry with respect to the center of the QW structure. The confinement of the quasi-confined phonons in the QW leads to a quantization of qz,j characterized by an integer m that defines the order of corresponding quasi-confined modes. The QC modes are more dispersive for decreasing m. The QC modes display an interface behavior in the barrier and a confined behavior in the well. When q⊥ is small, the symmetric modes have more contribution to electron-QC interaction than the antisymmetric modes.


2006 ◽  
Vol 13 (01) ◽  
pp. 75-80 ◽  
Author(s):  
L. ZHANG

Under the dielectric continuum model and Loudon's uniaxial crystal model, the interface optical (IO) phonon modes in a quasi-one-dimensional (Q1D) wurtzite rectangular quantum wire are deduced and analyzed. Numerical calculation on a wurtzite GaN/AlN rectangular wurtzite quantum wire was performed. Results reveal that the dispersion frequencies of IO modes sensitively depend on the geometric structures of the Q1D wurtzite rectangular quantum wires. The degenerating behavior of the IO phonon modes in the Q1D wurtzite rectangular quantum wire has been clearly observed for small free wave number kz in z-direction. The limited frequency behaviors of IO modes have been analyzed deeply, and detailed comparisons with those in wurtzite planar quantum wells and cylindrical quantum wires are also done. Moreover, once the anisotropy of the wurtzite material has been ignored, the present theories can be naturally reduced to the situation of Q1D cubic rectangular quantum wire systems.


2006 ◽  
Vol 20 (05) ◽  
pp. 559-578 ◽  
Author(s):  
LI ZHANG ◽  
JUN-JIE SHI

Under the dielectric continuum model and Loudon's uniaxial crystal model, by adopting the transfer matrix method, the dispersion properties of the interface optical (IO) and surface optical (SO) phonon modes and their couplings with electrons in multi-layer coupling wurtzite quantum wells (QWs) are deduced and analyzed via the method of electrostatic potential expanding. Numerical calculations on a freestanding symmetrical wurtzite QW and an asymmetrical wurtzite QW have been performed. Results reveal that, in general, there are four branches of IO and two branches of SO phonon modes in the systems. The dispersions of these IO and SO phonon modes are obvious only when the free two-dimensional phonon wave number ktparallel to the heterostructure interfaces is small. The degenerating behavior for these phonon modes has been clearly observed for small kt. When ktis relatively large, with the increase in kt, the frequencies of the IO and SO phonon modes converge to some definite limiting frequencies in corresponding wurtzite single planar heterostructure. This feature have been analyzed in depth from the mathematical and physical viewpoints. The calculations of electron-phonon coupling function show that, the electrostatic potential distribution of the IO and SO mode in freestanding symmetrical wurtzite QW is either symmetrical or is antisymmetrical; but that in freestanding asymmetrical wurtzite QW is neither symmetrical nor is antisymmetric. The calculation also shows that the SO modes and the short wavelength phonon modes play a more important role in the electron-phonon interaction.


2005 ◽  
Vol 12 (03) ◽  
pp. 433-442
Author(s):  
LI ZHANG ◽  
SONG GAO ◽  
JUN-JIE SHI

Within the framework of the dielectric continuum model and Loudon's uniaxial crystal model, the properties of frequency dispersion of the interface optical (IO) phonon modes and the coupling functions of electron–IO-phonon interaction in an asymmetrical wurtzite quantum well (QW) are deduced and analyzed via the method of electrostatic potential expansion. Numerical results reveal that in general, there are four branches of IO phonon modes in the systems. The dispersions of the four branches of IO phonon modes are obvious only when the free wavenumber ktin xy plane is small. The degenerating behavior of all the four branches of IO phonon modes in the asymmetric wurtzite QWs has been clearly observed for small kt. When ktis relatively large, with the increase of kt, the frequencies of the IO phonon modes converge to the four definite limiting frequencies in the corresponding wurtzite single planar heterostructure. This feature is obviously different from that in symmetric wurtzite QW, and the mathematical and physical reasons have been analyzed in depth. The calculations of electron–phonon coupling function show that the electrostatic distribution of the IO modes is neither symmetrical nor antisymmetrical, and the high-frequency IO phonon branches and the short-wavelength IO phonon modes play a more important role in the electron–phonon interaction.


1998 ◽  
Vol 09 (01) ◽  
pp. 281-312 ◽  
Author(s):  
M. DUTTA ◽  
M. A. STROSCIO ◽  
K. W. KIM

As device dimensions in electronic and optoelectronic devices are reduced, the characteristics and interactions of dimensionally-confined longitudinal-optical (LO) and acoustic phonons deviate substantially from those of bulk semiconductors. Furthermore, as würtzite materials are applied increasingly in electronic and optoelectronic devices it becomes more important to understand the phonon modes in such systems. This account emphasizes the properties of bulk optical phonons in würtzite structures, the properties of LO-phonon modes and acoustic-phonon modes arising in polar-semiconductor quantum wells, superlattices, quantum wires and quantum dots, with a variety of cross sectional geometries and, lastly, the properties of optical phonons in würtzite materials as predicted by the dielectric continuum model. Emphasis is placed on the dielectric continuum and elastic continuum models of bulk, confined and interface phonons. This article emphasizes device applications of confined phonons in GaAs-based systems and provides a brief discussion of carrier-LO-phonon interactions in bulk würtzite structures. This account also includes discussions on the use of metal-semiconductor heterointerfaces to reduce scattering and on the role of phonons in Fröhlich, deformation and piezoelectric interactions in electronic and optoelectronic structures; specific device applications high-lighted here include quantum cascade lasers, mesoscopic devices, thermoelectric devices and optically-pumped resonant intersubband lasers.


Author(s):  
А.Ю. Маслов ◽  
О.В. Прошина

Abstract The specific features of the interaction of charged particles with polar optical phonons have been studied theoretically for quantum wells with the barriers that are asymmetric in their dielectric properties. It is shown that the interaction with interface phonon modes makes the greatest contribution in narrow quantum wells. The parameters of the electron-phonon interaction were found for the cases of different values of the phonon frequencies in the barrier materials. It turned out that a significant (by almost an order of magnitude) change in the parameters of the electron-phonon interaction can occur in such structures. This makes it possible, in principle, to trace the transition from weak to strong interactions in quantum wells of the same type but with different compositions of barrier materials. The conditions are found under which an enhancement of the electron-phonon interaction is possible in an asymmetric structure in comparison with a symmetric one with the barriers of the same composition.


1995 ◽  
Vol 51 (24) ◽  
pp. 17728-17739 ◽  
Author(s):  
A. J. Shields ◽  
M. P. Chamberlain ◽  
M. Cardona ◽  
K. Eberl

Author(s):  
Mohamed Boumaza

We report on hole polar optical phonon scattering processes in thin GaAs/AlxGa1-xAs quantum wells grown in various crystallographic directions, such as [001], [110]. Using the dielectric continuum model we focus on how the different scattering processes of holes with interface phonon modes depend on the initial hole energy. In our work, we use the Luttinger-Kohn (LK) 6×6 k.p Hamiltonian with the envelope function approximation, from which we compute numerically the electronic structure of holes for a thin quantum well sustaining only one bound state for each type of hole. Due to mixing between the heavy, light, and split off bands, hole subbands exhibit strong nonparabolicity and important warping that have their word to say on physical properties. Detailed and extensive calculations that the rates for intra-subband scattering processes differ significantly from those of bulk GaAs because of quantization and reduced dimensionality. Moreover, the study of scattering as a function of hole energy shows that the trend of the scattering rates is governed mostly by i) overlap integrals and ii) the density of the final states to which the hole scatters. The influence of warping, in the hole energy dispersion, on the phonon scattering rates is also explored and found to be important when the initial hole energy is high. Our calculations show evidence of strong anisotropy in the scattering rates especially for processes involving the heavy hole subband, which anisotropy is in fact quite important and far from being negligible. However, strain effect can reduce scattering rates.


2020 ◽  
Vol 20 (7) ◽  
pp. 4444-4449
Author(s):  
Jeung Hun Park ◽  
Richard S. Kim ◽  
Se-Jeong Park ◽  
Choong-Heui Chung

We report the systematic investigation of the surface optical phonon modes in Au-catalyzed GaAs nanowires grown on an Au pre-patterned GaAs(111)B substrate using μ-Raman spectroscopy. We employed electron-beam dose rate as a control parameter during the substrate patterning step for adjusting the nanowire base diameter and coverage, which are independent from the nanowire growth conditions. We have experimentally studied the effect of the fill factor and average diameter on the surface optical phonon modes and explained the red-shift and broadening of the surface optical phonon frequencies by employing the dielectric continuum model. The surface optical phonon mode shift is exhibited to be sensitive to fill factor, rather than base diameter. The decrease in the average diameter from 280 nm to 180 nm results in the asymmetric broadening and red-shift of the surface optical phonon frequency (~1.83 cm−1) but the theoretical calculation from the isolated single nanowire-based dielectric continuum model cannot solely explain the behaviors of the surface optical phonon mode. In contrast, the change in the fill factor from 0.01 to 0.83 results in a shift of the surface optical phonon frequency (~6.5 cm−1) from the GaAs bulk value. The red-shift and asymmetric broadening of the surface optical phonons, in an agreement with the Maxwell-Garnett approximation, are consequences of dipolar interaction of randomly aligned neighboring nanowires and the polar nature of GaAs nanowire bundles. This work suggests the pre-patterning parameter dependent surface optical phonon characteristics of GaAs nanowire bundles which are of great importance in the nondestructive characterization of low-dimensional opto-electronic materials and devices.


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