scholarly journals POLSTRACC: Airborne Experiment for Studying the Polar Stratosphere in a Changing Climate with the High Altitude and Long Range Research Aircraft (HALO)

2019 ◽  
Vol 100 (12) ◽  
pp. 2634-2664 ◽  
Author(s):  
Hermann Oelhaf ◽  
Björn-Martin Sinnhuber ◽  
Wolfgang Woiwode ◽  
Harald Bönisch ◽  
Heiko Bozem ◽  
...  
Keyword(s):  
Remote Sensing ◽  
High Altitude ◽  
Long Range ◽  
Potential Temperature ◽  
The Arctic ◽  
Ozone Loss ◽  
Changing Climate ◽  
Research Aircraft ◽  
Polar Stratosphere

Abstract The Polar Stratosphere in a Changing Climate (POLSTRACC) mission employed the German High Altitude and Long Range Research Aircraft (HALO). The payload comprised an innovative combination of remote sensing and in situ instruments. The in situ instruments provided high-resolution observations of cirrus and polar stratospheric clouds (PSCs), a large number of reactive and long-lived trace gases, and temperature at the aircraft level. Information above and underneath the aircraft level was achieved by remote sensing instruments as well as dropsondes. The mission took place from 8 December 2015 to 18 March 2016, covering the extremely cold late December to early February period and the time around the major warming in the beginning of March. In 18 scientific deployments, 156 flight hours were conducted, covering latitudes from 25° to 87°N and maximum altitudes of almost 15 km, and reaching potential temperature levels of up to 410 K. Highlights of results include 1) new aspects of transport and mixing in the Arctic upper troposphere–lower stratosphere (UTLS), 2) detailed analyses of special dynamical features such as tropopause folds, 3) observations of extended PSCs reaching sometimes down to HALO flight levels at 13–14 km, 4) observations of particulate NOy and vertical redistribution of gas-phase NOy in the lowermost stratosphere (LMS), 5) significant chlorine activation and deactivation in the LMS along with halogen source gas observations, and 6) the partitioning and budgets of reactive chlorine and bromine along with a detailed study of the efficiency of ClOx/BrOx ozone loss cycle. Finally, we quantify—based on our results—the ozone loss in the 2015/16 winter and address the question of how extraordinary this Arctic winter was.

scholarly journals Nitric acid trihydrate (NAT) formation at low NAT supersaturations

2004 ◽  
Vol 4 (6) ◽  
pp. 8579-8607 ◽  
Author(s):  
C. Voigt ◽  
H. Schlager ◽  
B. P. Luo ◽  
A. Dörnbrack ◽  
A. Roiger ◽  
...  
Keyword(s):  
Nitric Acid ◽  
High Altitude ◽  
Equilibrium Temperature ◽  
In Situ Measurements ◽  
The Arctic ◽  
Ozone Loss ◽  
Polar Stratospheric Cloud ◽  
Research Aircraft ◽  
Polar Ozone

Abstract. A polar stratospheric cloud (PSC) was observed on 6 February 2003 in the Arctic stratosphere by in-situ measurements onboard the high-altitude research aircraft Geophysica. Low number densities (~10−4 cm−3) of nitric acid (HNO3) containing particles – probably NAT – with diameters up to 6 µm were measured at altitudes between 18 and 20 km. These particles have the potential to grow further and to remove HNO3 from the stratosphere, thereby enhancing polar ozone loss. Interestingly, the NAT particles formed in less than a day at temperatures T>TNAT−3.5 K, just slightly below the NAT equilibrium temperature TNAT. This unique measurement of PSC formation at extremely low NAT saturation ratios (SNAT≤11) constrains current NAT nucleation theories. In particular, NAT formation on ice can for certain be excluded. Conversely, we suggest that meteoritic particles may be favorable candidates for triggering nucleation of NAT at the observed low number densities.

scholarly journals ML-CIRRUS: The Airborne Experiment on Natural Cirrus and Contrail Cirrus with the High-Altitude Long-Range Research Aircraft HALO

2017 ◽  
Vol 98 (2) ◽  
pp. 271-288 ◽  
Author(s):  
Christiane Voigt ◽  
Ulrich Schumann ◽  
Andreas Minikin ◽  
Ahmed Abdelmonem ◽  
Armin Afchine ◽  
...  
Keyword(s):  
Remote Sensing ◽  
High Altitude ◽  
Long Range ◽  
Prediction Models ◽  
Weather Prediction ◽  
Climate Impact ◽  
Jet Streams ◽  
Direct Observations ◽  
Research Aircraft

Abstract The Midlatitude Cirrus experiment (ML-CIRRUS) deployed the High Altitude and Long Range Research Aircraft (HALO) to obtain new insights into nucleation, life cycle, and climate impact of natural cirrus and aircraft-induced contrail cirrus. Direct observations of cirrus properties and their variability are still incomplete, currently limiting our understanding of the clouds’ impact on climate. Also, dynamical effects on clouds and feedbacks are not adequately represented in today’s weather prediction models. Here, we present the rationale, objectives, and selected scientific highlights of ML-CIRRUS using the G-550 aircraft of the German atmospheric science community. The first combined in situ–remote sensing cloud mission with HALO united state-of-the-art cloud probes, a lidar and novel ice residual, aerosol, trace gas, and radiation instrumentation. The aircraft observations were accompanied by remote sensing from satellite and ground and by numerical simulations. In spring 2014, HALO performed 16 flights above Europe with a focus on anthropogenic contrail cirrus and midlatitude cirrus induced by frontal systems including warm conveyor belts and other dynamical regimes (jet streams, mountain waves, and convection). Highlights from ML-CIRRUS include 1) new observations of microphysical and radiative cirrus properties and their variability in meteorological regimes typical for midlatitudes, 2) insights into occurrence of in situ–formed and lifted liquid-origin cirrus, 3) validation of cloud forecasts and satellite products, 4) assessment of contrail predictability, and 5) direct observations of contrail cirrus and their distinction from natural cirrus. Hence, ML-CIRRUS provides a comprehensive dataset on cirrus in the densely populated European midlatitudes with the scope to enhance our understanding of cirrus clouds and their role for climate and weather.

scholarly journals Nitric Acid Trihydrate (NAT) formation at low NAT supersaturation in Polar Stratospheric Clouds (PSCs)

2005 ◽  
Vol 5 (5) ◽  
pp. 1371-1380 ◽  
Author(s):  
C. Voigt ◽  
H. Schlager ◽  
B. P. Luo ◽  
A. Dörnbrack ◽  
A. Roiger ◽  
...  
Keyword(s):  
Nitric Acid ◽  
High Altitude ◽  
Equilibrium Temperature ◽  
In Situ Measurements ◽  
The Arctic ◽  
Polar Stratospheric Clouds ◽  
Research Aircraft ◽  
Stratospheric Clouds ◽  
Polar Ozone

Abstract. A PSC was detected on 6 February 2003 in the Arctic stratosphere by in-situ measurements onboard the high-altitude research aircraft Geophysica. Low number densities (~10-4cm-3) of small nitric acid (HNO3) containing particles (d<6µm) were observed at altitudes between 18 and 20km. Provided the temperatures remain below the NAT equilibrium temperature TNAT, these NAT particles have the potential to grow further and to remove HNO3 from the stratosphere, thereby enhancing polar ozone loss. Interestingly, the NAT particles formed in less than a day at temperatures just slightly below TNAT (T>TNAT-3.1K). This unique measurement of PSC formation at extremely low NAT saturation ratios (SNAT≤10) constrains current NAT nucleation theories. We suggest, that the NAT particles have formed heterogeneously, but for certain not on ice. Conversely, meteoritic particles may be favorable candidates for triggering NAT nucleation at the observed low number densities.

scholarly journals A High-Altitude Long-Range Aircraft Configured as a Cloud Observatory: The NARVAL Expeditions

2019 ◽  
Vol 100 (6) ◽  
pp. 1061-1077 ◽  
Author(s):  
Bjorn Stevens ◽  
Felix Ament ◽  
Sandrine Bony ◽  
Susanne Crewell ◽  
Florian Ewald ◽  
...  
Keyword(s):  
Remote Sensing ◽  
High Altitude ◽  
Long Range ◽  
Large Scale ◽  
Radiant Energy ◽  
Vertical Component ◽  
Field Studies ◽  
Meteorological Conditions ◽  
Research Aircraft ◽  
New Generation

AbstractA configuration of the High-Altitude Long-Range Research Aircraft (HALO) as a remote sensing cloud observatory is described, and its use is illustrated with results from the first and second Next-Generation Aircraft Remote Sensing for Validation (NARVAL) field studies. Measurements from the second NARVAL (NARVAL2) are used to highlight the ability of HALO, when configured in this fashion, to characterize not only the distribution of water condensate in the atmosphere, but also its impact on radiant energy transfer and the covarying large-scale meteorological conditions—including the large-scale velocity field and its vertical component. The NARVAL campaigns with HALO demonstrate the potential of airborne cloud observatories to address long-standing riddles in studies of the coupling between clouds and circulation and are helping to motivate a new generation of field studies.

scholarly journals Denitrification, dehydration and ozone loss during the Arctic winter 2015/2016

2017 ◽  
Author(s):  
Farahnaz Khosrawi ◽  
Oliver Kirner ◽  
Björn-Martin Sinnhuber ◽  
Sören Johansson ◽  
Michael Höpfner ◽  
...  
Keyword(s):  
Atmospheric Chemistry ◽  
Stratospheric Ozone ◽  
Satellite Observations ◽  
The Arctic ◽  
Cold Pool ◽  
Polar Stratospheric Clouds ◽  
Airborne Measurements ◽  
Ozone Loss ◽  
Polar Stratosphere ◽  
Stratospheric Clouds

Abstract. The Arctic winter 2015/2016 was one of the coldest stratospheric winters in recent years. A stable vortex formed by early December and the early winter was exceptionally cold. Cold pool temperatures dropped below the Nitric Acid Trihydrate (NAT) existence temperature of about 195 K, thus allowing Polar Stratospheric Clouds (PSCs) to form. The low temperatures in the polar stratosphere persisted until early March allowing chlorine activation and catalytic ozone destruction. Satellite observations indicate that sedimentation of PSC particles led to denitrification as well as dehydration of stratospheric layers. Model simulations of the Arctic winter 2015/2016 nudged toward European Center for Medium-Range Weather Forecasts (ECMWF) analyses data were performed with the atmospheric chemistry–climate model ECHAM5/MESSy Atmospheric Chemistry (EMAC) for the Polar Stratosphere in a Changing Climate (POLSTRACC) campaign. POLSTRACC is a High Altitude and LOng Range Research Aircraft (HALO) mission aimed at the investigation of the structure, composition and evolution of the Arctic Upper Troposphere and Lower Stratosphere (UTLS). The chemical and physical processes involved in Arctic stratospheric ozone depletion, transport and mixing processes in the UTLS at high latitudes, polar stratospheric clouds as well as cirrus clouds are investigated. In this study an overview of the chemistry and dynamics of the Arctic winter 2015/2016 as simulated with EMAC is given. Further, chemical-dynamical processes such as denitrification, dehydration and ozone loss during the Arctic winter 2015/2016 are investigated. Comparisons to satellite observations by the Aura Microwave Limb Sounder (Aura/MLS) as well as to airborne measurements with the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) performed on board of HALO during the POLSTRACC campaign show that the EMAC simulations are in fairly good agreement with observations. We derive a maximum polar stratospheric O3 loss of ~ 2 ppmv or 100 DU in terms of column in mid March. The stratosphere was denitrified by about 8 ppbv HNO3 and dehydrated by about 1 ppmv H2O in mid to end of February. While ozone loss was quite strong, but not as strong as in 2010/2011, denitrification and dehydration were so far the strongest observed in the Arctic stratosphere in the at least past 10 years.

scholarly journals Simulation of denitrification and ozone loss for the Arctic winter 2002/2003

2005 ◽  
Vol 5 (6) ◽  
pp. 1437-1448 ◽  
Author(s):  
J.-U. Grooß ◽  
G. Günther ◽  
R. Müller ◽  
P. Konopka ◽  
S. Bausch ◽  
...  
Keyword(s):  
Inorganic Nitrogen ◽  
Potential Temperature ◽  
Three Dimensional ◽  
Lagrangian Model ◽  
The Arctic ◽  
Particle Nucleation ◽  
Ozone Loss ◽  
Dimensional Version ◽  
Total Inorganic Nitrogen ◽  
Catalytic Cycles

Abstract. We present simulations with the Chemical Lagrangian Model of the Stratosphere (CLaMS) for the Arctic winter 2002/2003. We integrated a Lagrangian denitrification scheme into the three-dimensional version of CLaMS that calculates the growth and sedimentation of nitric acid trihydrate (NAT) particles along individual particle trajectories. From those, we derive the HNO3 downward flux resulting from different particle nucleation assumptions. The simulation results show a clear vertical redistribution of total inorganic nitrogen ( ), with a maximum vortex average permanent removal of over 5ppb in late December between 500 and 550K and a corresponding increase of of over 2ppb below about 450K. The simulated vertical redistribution of is compared with balloon observations by MkIV and in-situ observations from the high altitude aircraft Geophysica. Assuming a globally uniform NAT particle nucleation rate of 7.8x10-6cm-3h-1 in the model, the observed denitrification is well reproduced. In the investigated winter 2002/2003, the denitrification has only moderate impact (≤14%) on the simulated vortex average ozone loss of about 1.1ppm near the 460K level. At higher altitudes, above 600K potential temperature, the simulations show significant ozone depletion through -catalytic cycles due to the unusual early exposure of vortex air to sunlight.

scholarly journals HAMP – the microwave package on the High Altitude and LOng range research aircraft HALO

2014 ◽  
Vol 7 (5) ◽  
pp. 4623-4657
Author(s):  
M. Mech ◽  
E. Orlandi ◽  
S. Crewell ◽  
F. Ament ◽  
L. Hirsch ◽  
...  
Keyword(s):  
High Altitude ◽  
Long Range ◽  
Microwave Remote Sensing ◽  
Passive Microwave ◽  
Lower Atmosphere ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Model Calculations ◽  
Cloud Radar ◽  
Research Aircraft

Abstract. An advanced package of microwave remote sensing instrumentation has been developed for the operation on the new German High Altitude LOng range research aircraft (HALO). The HALO Microwave Package, HAMP, consists of two nadir looking instruments: a cloud radar at 36 GHz and a suite of passive microwave radiometers with 26 frequencies in different bands between 22.24 and 183.31 ± 12.5 GHz. We present a description of HAMP's instrumentation together with an illustration of its potential. To demonstrate this potential synthetic measurements for the implemented passive microwave frequencies and the cloud radar based on cloud resolving and radiative transfer model calculations were performed. These illustrate the advantage of HAMP's chosen frequency coverage, which allows for improved detection of hydrometeors both via the emission and scattering of radiation. Regression algorithms compare HAMP retrieval with standard satellite instruments from polar orbiters and show its advantages particularly for the lower atmosphere with a reduced root mean square error by 5 and 15% for temperature and humidity, respectively. HAMP's main advantage is the high spatial resolution of about 1 km which is illustrated by first measurements from test flights. Together these qualities make it an exciting tool for gaining better understanding of cloud processes, testing retrieval algorithms, defining future satellite instrument specifications, and validating platforms after they have been placed in orbit.

Ground-based Remote Sensing of Cirrus Clouds

Cirrus ◽  
2002 ◽  
Author(s):  
Kenneth Sassen ◽  
Gerald Mace
Keyword(s):  
Remote Sensing ◽  
Multispectral Imaging ◽  
Cirrus Clouds ◽  
Radiative Energy ◽  
Radiation Balance ◽  
Cirrus Cloud ◽  
Microphysical Properties ◽  
Research Aircraft ◽  
Cloud Modeling

Cirrus clouds have only recently been recognized as having a significant influence on weather and climate through their impact on the radiative energy budget of the atmosphere. In addition, the unique difficulties presented by the study of cirrus put them on the “back burner” of atmospheric research for much of the twentieth century. Foremost, because they inhabit the frigid upper troposphere, their inaccessibility has hampered intensive research. Other factors have included a lack of in situ instrumentation to effectively sample the clouds and environment, and basic uncertainties in the underlying physics of ice cloud formation, growth, and maintenance. Cloud systems that produced precipitation, severe weather, or hazards to aviation were deemed more worthy of research support until the mid- 1980s. Beginning at this time, however, major field research programs such as the First ISCCP (International Satellite Cloud Climatology Program) Regional Experiment (FIRE; Cox et al. 1987), International Cirrus Experiment (ICE; Raschke et al. 1990), Experimental Cloud Lidar Pilot Study (ECLIPS; Platt et al. 1994), and the Atmospheric Radiation Measurement (ARM) Program (Stokes and Schwartz 1994) have concentrated on cirrus cloud research, relying heavily on ground-based remote sensing observations combined with research aircraft. What has caused this change in research emphasis is an appreciation for the potentially significant role that cirrus play in maintaining the radiation balance of the earth-atmosphere system (Liou 1986). As climate change issues were treated more seriously, it was recognized that the effects, or feedbacks, of extensive high-level ice clouds in response to global warming could be pivotal. This fortunately came at a time when new generations of meteorological instrumentation were becoming available. Beginning in the early 1970s, major advancements were made in the fields of numerical cloud modeling and cloud measurements using aircraft probes, satellite multispectral imaging, and remote sensing with lidar, short-wavelength radar, and radiometers, all greatly facilitating cirrus research. Each of these experimental approaches have their advantages and drawbacks, and it should also be noted that a successful cloud modeling effort relies on field data for establishing boundary conditions and providing case studies for validation. Although the technologies created for in situ aircraft measurements can clearly provide unique knowledge of cirrus cloud thermodynamic and microphysical properties (Dowling and Radke 1990), available probes may suffer from limitations in their response to the wide range of cirrus particles and actually sample a rather small volume of cloud during any mission.

scholarly journals Current systematic carbon-cycle observations and the need for implementing a policy-relevant carbon observing system

2014 ◽  
Vol 11 (13) ◽  
pp. 3547-3602 ◽  
Author(s):  
P. Ciais ◽  
A. J. Dolman ◽  
A. Bombelli ◽  
R. Duren ◽  
A. Peregon ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Carbon Cycle ◽  
Fossil Fuel ◽  
The Arctic ◽  
Observation System ◽  
Observation Data ◽  
Current State ◽  
Spatial Coverage

Abstract. A globally integrated carbon observation and analysis system is needed to improve the fundamental understanding of the global carbon cycle, to improve our ability to project future changes, and to verify the effectiveness of policies aiming to reduce greenhouse gas emissions and increase carbon sequestration. Building an integrated carbon observation system requires transformational advances from the existing sparse, exploratory framework towards a dense, robust, and sustained system in all components: anthropogenic emissions, the atmosphere, the ocean, and the terrestrial biosphere. The paper is addressed to scientists, policymakers, and funding agencies who need to have a global picture of the current state of the (diverse) carbon observations. We identify the current state of carbon observations, and the needs and notional requirements for a global integrated carbon observation system that can be built in the next decade. A key conclusion is the substantial expansion of the ground-based observation networks required to reach the high spatial resolution for CO2 and CH4 fluxes, and for carbon stocks for addressing policy-relevant objectives, and attributing flux changes to underlying processes in each region. In order to establish flux and stock diagnostics over areas such as the southern oceans, tropical forests, and the Arctic, in situ observations will have to be complemented with remote-sensing measurements. Remote sensing offers the advantage of dense spatial coverage and frequent revisit. A key challenge is to bring remote-sensing measurements to a level of long-term consistency and accuracy so that they can be efficiently combined in models to reduce uncertainties, in synergy with ground-based data. Bringing tight observational constraints on fossil fuel and land use change emissions will be the biggest challenge for deployment of a policy-relevant integrated carbon observation system. This will require in situ and remotely sensed data at much higher resolution and density than currently achieved for natural fluxes, although over a small land area (cities, industrial sites, power plants), as well as the inclusion of fossil fuel CO2 proxy measurements such as radiocarbon in CO2 and carbon-fuel combustion tracers. Additionally, a policy-relevant carbon monitoring system should also provide mechanisms for reconciling regional top-down (atmosphere-based) and bottom-up (surface-based) flux estimates across the range of spatial and temporal scales relevant to mitigation policies. In addition, uncertainties for each observation data-stream should be assessed. The success of the system will rely on long-term commitments to monitoring, on improved international collaboration to fill gaps in the current observations, on sustained efforts to improve access to the different data streams and make databases interoperable, and on the calibration of each component of the system to agreed-upon international scales.

scholarly journals Empirical Relationships between Remote-Sensing Reflectance and Selected Inherent Optical Properties in Nordic Sea Surface Waters for the MODIS and OLCI Ocean Colour Sensors

2020 ◽  
Vol 12 (17) ◽  
pp. 2774
Author(s):  
Marta Konik ◽  
Piotr Kowalczuk ◽  
Monika Zabłocka ◽  
Anna Makarewicz ◽  
Justyna Meler ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Large Scale ◽  
Field Work ◽  
The Arctic ◽  
Significant Shift ◽  
Form Complex ◽  
Water Properties ◽  
Remote Sensing Reflectance ◽  
Phytoplankton Communities

The Nordic Seas and the Fram Strait regions are a melting pot of a number of water masses characterized by distinct optical water properties. The warm Atlantic Waters transported from the south and the Arctic Waters from the north, combined with the melt waters contributing to the Polar Waters, mediate the dynamic changes of the year-to-year large-scale circulation patterns in the area, which often form complex frontal zones. In the last decade, moreover, a significant shift in phytoplankton phenology in the area has been observed, with a certain northward expansion of temperate phytoplankton communities into the Arctic Ocean which could lead to a deterioration in the performance of remote sensing algorithms. In this research, we exploited the capability of the satellite sensors to monitor those inter-annual changes at basin scales. We propose locally adjusted algorithms for retrieving chlorophyll a concentrations Chla, absorption by particles ap at 443 and 670 nm, and total absorption atot at 443 and 670 nm developed on the basis of intensive field work conducted in 2013–2015. Measured in situ hyper spectral remote sensing reflectance has been used to reconstruct the MODIS and OLCI spectral channels for which the proposed algorithms have been adapted. We obtained MNB ≤ 0.5% for ap(670) and ≤3% for atot(670) and Chla. RMS was ≤30% for most of the retrieved optical water properties except ap(443) and Chla. The mean monthly mosaics of ap(443) computed on the basis of the proposed algorithm were used for reconstructing the spatial and temporal changes of the phytoplankton biomass in 2013–2015. The results corresponded very well with in situ measurements.

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