scholarly journals Benchmark PhotoIonization Cross-Sections of Neutral Scandium from the Ground and Excited States

Atoms ◽  
2021 ◽  
Vol 9 (4) ◽  
pp. 83
Author(s):  
Swaraj S. Tayal ◽  
Oleg Zatsarinny

The B-spline R-matrix method has been used to investigate cross-sections for photoionization of neutral scandium from the ground and excited states in the energy region from the 3d and 4s valence electron ionization thresholds to 25 eV. The initial bound states of Sc and the final residual Sc+ ionic states have been accurately calculated by combining the multiconfiguration Hartree-Fock method with the frozen-core close-coupling approach. The lowest 20 bound states of Sc I belonging to the ground 3d4s2 and excited 3d24s, 3d24p, 3d4s4p, 4s24p, and 3d3 configurations have been considered as initial states. The 81 LS final ionic states of Sc+ belonging to the terms of 3p63d2, 3p63d4l (l = 0–3), 3p63d5l (l = 0–3), 3p63d6s, 3p64s2, 3p64s4l (l = 0–3), 3p64s5l (l = 0–1), and 3p64p2 configurations have been included in the final-state close-coupling expansion. The cross-sections are dominated by complicated resonance structures in the low energy region converging to several Sc+ ionic thresholds. The inclusion of all these final ionic states has been noted to significantly impact the near-threshold resonance structures and background cross-sections. The important scattering channels for leaving the residual ion in various final states have been identified, and the 3d electron ionization channels have been noted to dominate the cross-sections at higher photon energies.

Atoms ◽  
2020 ◽  
Vol 8 (3) ◽  
pp. 51
Author(s):  
Oleg Zatsarinny ◽  
Swaraj Tayal

Partial and total photoionization cross sections of iron-peak elements are important for the determination of abundances in late-type stars and nebular objects. We have investigated photoionization of neutral chromium from the ground and excited states in the low energy region from the first ionization threshold at 6.77 eV to 30 eV. Accurate descriptions of the initial bound states of Cr I and the final residual Cr II ionic states have been obtained in the multiconfiguration Hartree-Fock method together with adjustable configuration expansions and term-dependent non-orthogonal orbitals. The B-spline R-matrix method has been used for the calculation of photoionization cross sections. The 194 LS final ionic states of Cr II 3d44s, 3d34s2, 3d5, 3d44p, and 3d34s4p principal configurations have been included in the close-coupling expansion. The inclusion of all terms of these configurations has significant impact on the near-threshold resonance structures as well as on the nonresonant background cross sections. Total photoionization cross sections from the ground 3d54sa7S and excited 3d54sa5S, 3d44s2a5D, 3d54pz5P, and 3d44s4py5P states of Cr I have been compared with other available R-matrix calculation to estimate the likely uncertainties in photoionization cross sections. We analyzed the partial photoionization cross sections for leaving the residual ion in various states to identify the important scattering channels, and noted that 3d electron ionization channel becomes dominant at higher energies.


A crossed beams method has been used to measure the cross section for the production of He + (2 S ) by electrons incident upon He + (1 S ) in the energy range from threshold to 750 eV. The cross section was measured in arbitrary units with an accuracy of ± 5 % and at the higher energies its energy dependence is in close agreement with that calculated by means of the plane-wave Born approximation. Consequently the cross section has been normalized to the plane-wave Born cross section at energies between 435 and 750 eV to obtain the absolute magnitude. An independent estimate of the absolute magnitude was made to with in ± 30 % using only the experimental parameters, and the absolute cross sections given by the two methods agree within the experimental uncertainties. The normalized cross section is compared with cross sections given by the close-coupling approximation and various Coulomb-Born approximations. At the lower energies the normalized cross section is considerably smaller than any of the theoretical values, but the measurements are consistent with the existence of a finite cross section at threshold if the energy spread of the electron beam is taken in to account.


1968 ◽  
Vol 23 (7) ◽  
pp. 970-978
Author(s):  
H. Schlumbohm

Measurements of the photoemission caused by collisions of ground level He+- and Ne+-ions with Ar- and Kr-atoms have shown several multipletts of Ar II and Kr II within the investigated wavelength range of 3500 to 5500 A. At a high rate the charge transfer processes occur into excited states of Ar* and Kr*. The reactions are endothermic with a deficit of internal energy between 6 and 19 eV.The cross sections measured for several chosen transitions start at characteristic threshold energies between 10 and 25 eV. Above the threshold the cross sections rise slowly with increasing energy when Ne* is the colliding ion and very fast for He+. Above 50 to 100 eV the cross sections show nearly constant values. — The minimum kinetic energy values are calculated, which can just fill up the deficits of internal energy, and are shown to be equal to the measured threshold energies. Thus it follows that the pseudo-crossing of the potential energy curves of the quasimolecules occurs at an energy value equal to the asymptotic level of the above curve.


1977 ◽  
Vol 55 (23) ◽  
pp. 2113-2120 ◽  
Author(s):  
G. Goulard ◽  
R. Roy ◽  
R. J. Slobodrian

Excited states of 12C between 29 and 34 MeV are studied through the 3He + 9Be and d + 10B reactions leading to three α particles in the final state. Correlated energy spectra are analyzed with a two-stage process and new information is given about the studied excited energy region.


1978 ◽  
Vol 56 (5) ◽  
pp. 565-570 ◽  
Author(s):  
V. S. Kulhar ◽  
C. S. Shastry

The two state approximation method for the study of the rearrangement collisions is applied to the process of positronium formation in excited states for positron–hydrogen charge exchange collisions. Differential and integrated cross sections are computed for positronium formation in 2S, 2P, and 3S excited states. The results obtained in the energy region 2 to 10 Ry are compared with positronium formation cross sections in ground state. Total positronium formation cross sections including the contributions of capture into all the higher excited states of positronium are also computed in the first Born approximation and the two state approximation in the energy region considered.


1999 ◽  
Vol 52 (3) ◽  
pp. 603
Author(s):  
Dmitry V. Fursa

We have used the nonrelativistic convergent close-coupling (CCC) method to investigate electron scattering from the ground (6s2)1S state and excited (6s6p)1 Po1 and (6s5d)1,3De2 states of barium. For the scattering from the barium ground state, we have found very good agreement with measurements of (6s6p)1 Po1 apparent cross sections at all energies. Similarly, good agreement is found for differential cross sections for elastic scattering and (6s6p)1 Po and (6s5d)1 De2 excitations and with the (6s6p)1 Po1 state electron{photon angular correlations. For the scattering from excited states of barium we have found good agreement with elastic (6s6p)1 Po1 scattering and the (6s5d)1De2 → (6s6p)1 Po1 transition for both differential cross sections and electron–photon angular correlations.


2020 ◽  
Vol 29 (08) ◽  
pp. 2050056
Author(s):  
E. M. Darwish ◽  
H. M. Al-Ghamdi

Incoherent [Formula: see text]-photoproduction on the deuteron is investigated for photon energies near threshold with particular focus on beam-target double spin asymmetries. The analysis is based on a [Formula: see text] reaction model in which realistic elementary amplitudes for [Formula: see text], [Formula: see text] and [Formula: see text] are incorporated. Numerical results on all possible beam-target double spin asymmetries of the differential and total cross-sections in the photon energy region near threshold are presented. Effects of [Formula: see text] and [Formula: see text] final-state interactions are investigated and their roles are found to be important.


1995 ◽  
Vol 09 (25) ◽  
pp. 3269-3301 ◽  
Author(s):  
M. SCHULZ

Theoretical and experimental studies on double excitation in proton–helium collisions are reviewed. Two theoretical approaches, which are common in the treatment of atomic collision processes, are described: perturbative approaches and the close coupling method. Experimentally, double excitation has mainly been studied by spectroscopy of the autoionized electrons emitted by the decay of the doubly excited states and by projectile energy-loss spectroscopy. The results emerging from the theoretical and experimental studies include the following points: first, the coupling of the doubly excited states to the continuum is very important in the electron spectra leading to pronounced interference effects. Second, double excitation mechanisms involving the electron–electron interaction are dominant except for low projectile energies. Third, interference effects between various double excitation mechanisms appear to be insignificant in the cross-sections differential in the electron emission angle, but might be important under certain conditions in the cross-sections differential in the projectile scattering angle.


2014 ◽  
Vol 31 ◽  
pp. 1460304
Author(s):  
Chengping Shen ◽  

My report consists of two parts: (1). Using samples of 102 million ϒ(1S) and 158 million ϒ(2S) events at Belle, we study 17 exclusive hadronic decays of these two bottomonium resonances to some Vector-Pseudoscalar (VP), Vector-Tensor (VT) and Axial-vector-Pseudoscalar (AP) processes and their final states. Branching fractions are measured for all the processes. The ratios of the branching fractions of ϒ(2S) and ϒ(1S) decays into the same final state are used to test a perturbative QCD (pQCD) prediction for OZI-suppressed bottomonium decays. (2). Using data samples of 89 fb-1, 703 fb-1, and 121 fb-1 collected at center-of-mass (CMS) energies 10.52, 10.58, and 10.876 GeV, respectively, we measure the cross sections of e+e- → ωπ0, [Formula: see text], and [Formula: see text]. The energy dependence of the cross sections is presented.


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