scholarly journals Comparison of Tar Samples from Reaction Zone and Outlet in Ex-Situ Underground Coal Gasification Experiment

Energies ◽  
2021 ◽  
Vol 14 (24) ◽  
pp. 8570
Author(s):  
Lele Feng ◽  
Maifan Dong ◽  
Yuxin Wu ◽  
Junping Gu
Keyword(s):  
Reaction Zone ◽  
Coal Gasification ◽  
Soot Formation ◽  
Temperature Drop ◽  
Experimental System ◽  
Pollution Source ◽  
Ex Situ ◽  
Underground Coal Gasification ◽  
Tar Cracking ◽  
Heavy Tar

Tar remaining in the gasification cavity during underground coal gasification (UCG) is an important pollution source, while the reported studies only focus on the tar behavior at the outlet. The present work aims to compare the tar properties from the reaction zone and the outlet, analyze the tar evolution during gasification, and discuss possible measures to control tar pollution. Tar was sampled with a self-developed equipment from an ex-situ underground coal gasification experimental system and analyzed by GC-MS. The gas composition, temperature, and PM10 were also compared for the reaction zone and the outlet. Compared with the tar from reaction zone, the tar from outlet has a smaller percentage of high boiling point content, PAHs, C, O, N, S, Cl, Si, and a larger percentage of H. The PAHs percentage in tar at the outlet in this work is closer to the field data than the lab data from literature, indicating the experimental system gives a good simulation of tar behavior in underground coal gasification. Condensation due to a fast temperature drop is one of the main reasons for PAHs decreasing. Tar cracking and soot formation also cause the decrease of heavy tar, proven by the light gas and particulate matter results.

scholarly journals Monitoring and evaluation of simulated underground coal gasification in an ex-situ experimental artificial coal seam system

2018 ◽  
Vol 223 ◽  
pp. 82-92 ◽  
Author(s):  
Fa-qiang Su ◽  
Akihiro Hamanaka ◽  
Ken-ichi Itakura ◽  
Wenyan Zhang ◽  
Gota Deguchi ◽  
...  
Keyword(s):  
Coal Seam ◽  
Coal Gasification ◽  
Monitoring And Evaluation ◽  
Ex Situ ◽  
Underground Coal Gasification

scholarly journals Chemometric Study of the Ex Situ Underground Coal Gasification Wastewater Experimental Data

2012 ◽  
Vol 223 (9) ◽  
pp. 5745-5758 ◽  
Author(s):  
Adam Smoliński ◽  
Krzysztof Stańczyk ◽  
Krzysztof Kapusta ◽  
Natalia Howaniec
Keyword(s):  
Experimental Data ◽  
Coal Gasification ◽  
Ex Situ ◽  
Underground Coal Gasification ◽  
Coal Gasification Wastewater

scholarly journals Regression Models Utilization to the Underground Temperature Determination at Coal Energy Conversion

Energies ◽  
2021 ◽  
Vol 14 (17) ◽  
pp. 5444
Author(s):  
Milan Durdán ◽  
Marta Benková ◽  
Marek Laciak ◽  
Ján Kačur ◽  
Patrik Flegner
Keyword(s):  
Coal Seam ◽  
Regression Model ◽  
Regression Models ◽  
Coal Gasification ◽  
Cavity Growth ◽  
Temperature Data ◽  
Ex Situ ◽  
Underground Coal Gasification ◽  
Gasification Process ◽  
Cavity Growth Rate

The underground coal gasification represents a technology capable of obtaining synthetic coal gas from hard-reached coal deposits and coal beds with tectonic faults. This technology is also less expensive than conventional coal mining. The cavity is formed in the coal seam by converting coal to synthetic gas during the underground coal gasification process. The cavity growth rate and the gasification queue’s moving velocity are affected by controllable variables, i.e., the operation pressure, the gasification agent, and the laboratory coal seam geometry. These variables can be continuously measured by standard measuring devices and techniques as opposed to the underground temperature. This paper researches the possibility of the regression models utilization for temperature data prediction for this reason. Several regression models were proposed that were differed in their structures, i.e., the number and type of selected controllable variables as independent variables. The goal was to find such a regression model structure, where the underground temperature is predicted with the greatest possible accuracy. The regression model structures’ proposal was realized on data obtained from two laboratory measurements realized in the ex situ reactor. The obtained temperature data can be used for visualization of the cavity growth in the gasified coal seam.

scholarly journals A COMPARATIVE STUDY OF DATA-DRIVEN MODELING METHODS FOR SOFT-SENSING IN UNDERGROUND COAL GASIFICATION

2019 ◽  
Vol 59 (4) ◽  
pp. 322-351
Author(s):  
Ján Kačur ◽  
Milan Durdán ◽  
Marek Laciak ◽  
Patrik Flegner
Keyword(s):  
Coal Gasification ◽  
Calorific Value ◽  
Multivariate Adaptive Regression Splines ◽  
Ex Situ ◽  
Gaussian Kernel ◽  
Support Vector ◽  
Underground Coal Gasification ◽  
Process Data ◽  
Adaptive Regression ◽  
Data Driven Modeling

Underground coal gasification (UCG) is a technological process, which converts solid coal into a gas in the underground, using injected gasification agents. In the UCG process, a lot of process variables can be measurable with common measuring devices, but there are variables that cannot be measured so easily, e.g., the temperature deep underground. It is also necessary to know the future impact of different control variables on the syngas calorific value in order to support a predictive control. This paper examines the possibility of utilizing Neural Networks, Multivariate Adaptive Regression Splines and Support Vector Regression in order to estimate the UCG process data, i.e., syngas calorific value and underground temperature. It was found that, during the training with the UCG data, the SVR and Gaussian kernel achieved the best results, but, during the prediction, the best result was obtained by the piecewise-cubic type of the MARS model. The analysis was performed on data obtained during an experimental UCG with an ex-situ reactor.

scholarly journals Modelling Test of Autothermal Gasification Process Using CFD

2017 ◽  
Vol 62 (2) ◽  
pp. 253-268
Author(s):  
Tomasz Janoszek ◽  
Krzysztof Stańczyk ◽  
Adam Smoliński
Keyword(s):  
Numerical Model ◽  
Coal Gasification ◽  
Energy Transport ◽  
Fluid Dynamic ◽  
Fixed Bed ◽  
Complex Model ◽  
Ex Situ ◽  
Underground Coal Gasification ◽  
Gasification Process ◽  
Physical And Chemical

AbstractThere are many complex physical and chemical processes, which take place among the most notable are the chemical reactions, mass and energy transport, and phase transitions. The process itself takes place in a block of coal, which properties are variable and not always easy to determine in the whole volume. The complexity of the phenomena results in the need for a construction of a complex model in order to study the process on the basis of simulation. In the present study attempts to develop a numerical model of the fixed bed coal gasification process in homogeneous solid block with a given geometry were mode. On the basis of analysis and description of the underground coal gasification simulated in the ex-situ experiment, a numerical model of the coal gasification process was developed. The model was implemented with the use of computational fluid dynamic CFD methods. Simulations were conducted using commercial numerical CFD code and the results were verified with the experimental data.

Ex Situ UCG Model Experiments with Oxygen Enriched Air in an Artificial Coal Seam

2017 ◽  
Vol 737 ◽  
pp. 379-384
Author(s):  
Fa Qiang Su ◽  
Ken-ichi Itakura ◽  
Akihiro Hamanaka ◽  
Gota Deguchi ◽  
Kohki Sato ◽  
...  
Keyword(s):  
Coal Seam ◽  
Coal Gasification ◽  
Calorific Value ◽  
Close Correlation ◽  
Gas Production ◽  
Ex Situ ◽  
Underground Coal Gasification ◽  
Coal Consumption ◽  
Gas Leakage ◽  
Gasification Reaction

Underground Coal Gasification (UCG) demands precise evaluation of the combustion area in the coal seam. Especially, the monitoring of fracture activity in the coal seam and around rock is important not only for efficient gas production but also for estimation of subsidence and gas leakage to the surface. For this objective, laboratory experiments were conducted using the simulated UCG models. This paper also investigated gas energy for coal consumption, the production gas quantity and heat value, the application of oxygen element balance in the gasification reaction process, and the gas composition obtained in this study. During burning of the coal, temperatures inside the coal, contents of product gases and acoustic emission (AE) activities were monitored successively under the control of feeding gas (air/oxygen and steam) flow rate. Comparison of the temperature variation and accumulated AE event curves revealed a close correlation between them. The local change of temperature inside the coal induced fractures with AE. The AE activity was related closely to the local changes of temperature inside the model. The evaluation of gas energy recovery calculated from the obtained product gas provided a fair evaluation for the coal consumed, and the quantity of gas product and calorific value obtained from the UCG process.

Experimental results of underground coal gasification of Turkish lignite in an ex-situ reactor

Fuel ◽  
2017 ◽  
Vol 203 ◽  
pp. 997-1006 ◽  
Author(s):  
Mesut Gur ◽  
Nurdil Eskin ◽  
Hasancan Okutan ◽  
Ahmet Arısoy ◽  
Erhan Böke ◽  
...  
Keyword(s):  
Coal Gasification ◽  
Experimental Results ◽  
Ex Situ ◽  
Underground Coal Gasification

scholarly journals An ex Situ Underground Coal Gasification Experiment with a Siderite Interlayer. Course of the Process, Production Gas, Temperatures and Energy Efficiency

2020 ◽  
Author(s):  
Marian Wiatowski ◽  
Krzysztof Kapusta ◽  
Jacek Nowak ◽  
Marcin Szyja ◽  
Wioleta Basa
Keyword(s):  
Energy Efficiency ◽  
High Temperature ◽  
Flow Rate ◽  
Coal Gasification ◽  
High Energy ◽  
Ex Situ ◽  
Hard Coal ◽  
Underground Coal Gasification ◽  
Gasification Process ◽  
Process Gas

Abstract A 72-hour ex situ hard coal gasification test in one large block of coal was carried out. The gasifying agent was oxygen with a constant flow rate of 4.5 Nm3/h. The surroundings of coal were simulated with wet sand with 11% moisture content. A 2-cm interlayer of siderite was placed in the horizontal cut of the coal block. As a result of this process, gas with an average flow rate of 12.46 Nm3/h was produced. No direct influence of siderite on the gasification process was observed; however, measurements of CO2 content in the siderite interlayer before and after the process allowed to determine the location of high-temperature zones in the reactor. The greatest influence on the efficiency of the gasification process was exerted by water contained in wet sand. At the high temperature that prevailed in the reactor, this water evaporated and reacted with the incandescent coal, producing hydrogen and carbon monoxide. This reaction contributed to the relatively high calorific value of the resulting process gas, averaging 9.41 MJ/kmol, and to the high energy efficiency of the whole gasification process, which amounted to approximately 70%.

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