scholarly journals Impact of Aerosol Vertical Distribution on Aerosol Optical Depth Retrieval from Passive Satellite Sensors

2020 ◽  
Vol 12 (9) ◽  
pp. 1524 ◽  
Author(s):  
Chong Li ◽  
Jing Li ◽  
Oleg Dubovik ◽  
Zhao-Cheng Zeng ◽  
Yuk L. Yung
Keyword(s):  
Vertical Distribution ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Vertical Profile ◽  
Retrieval Algorithm ◽  
Retrieval Error ◽  
Satellite Sensors ◽  
Absorbing Aerosols ◽  
The Impact ◽  
The Vertical Distribution

When retrieving Aerosol Optical Depth (AOD) from passive satellite sensors, the vertical distribution of aerosols usually needs to be assumed, potentially causing uncertainties in the retrievals. In this study, we use the Moderate Resolution Spectroradiometer (MODIS) and Visible Infrared Imaging Radiometer Suite (VIIRS) sensors as examples to investigate the impact of aerosol vertical distribution on AOD retrievals. A series of sensitivity experiments was conducted using radiative transfer models with different aerosol profiles and surface conditions. Assuming a 0.2 AOD, we found that the AOD retrieval error is the most sensitive to the vertical distribution of absorbing aerosols; a −1 km error in aerosol scale height can lead to a ~30% AOD retrieval error. Moreover, for this aerosol type, ignoring the existence of the boundary layer can further result in a ~10% AOD retrieval error. The differences in the vertical distribution of scattering and absorbing aerosols within the same column may also cause −15% (scattering aerosols above absorbing aerosols) to 15% (scattering aerosols below absorbing aerosols) errors. Surface reflectance also plays an important role in affecting the AOD retrieval error, with higher errors over brighter surfaces in general. The physical mechanism associated with the AOD retrieval errors is also discussed. Finally, by replacing the default exponential profile with the observed aerosol vertical profile by a micro-pulse lidar at the Beijing-PKU site in the VIIRS retrieval algorithm, the retrieved AOD shows a much better agreement with surface observations, with the correlation coefficient increased from 0.63 to 0.83 and bias decreased from 0.15 to 0.03. Our study highlights the importance of aerosol vertical profile assumption in satellite AOD retrievals, and indicates that considering more realistic profiles can help reduce the uncertainties.

Is aerosol optical depth a good metric to map dust properties? Lessons learned from AER-D

2020 ◽  
Author(s):  
Franco Marenco ◽  
Claire Ryder ◽  
Victor Estelles ◽  
Debbie O'Sullivan
Keyword(s):  
Remote Sensing ◽  
Particle Size ◽  
Vertical Distribution ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Field Experiments ◽  
Saharan Air Layer ◽  
Validation Experiment ◽  
Operational Models ◽  
The Vertical Distribution

<p>The main observable quantity used on a global scale to map aerosols is aerosol optical depth (AOD), from ground-based and satellite remote sensing. It is at the same time an optical property and a vertically integrated quantity, and it is commonly used as the main metric towards which to pull aerosol models, through data assimilation, verification, and tuning. Here we introduce a few reflections on how to better constrain our knowledge of the Saharan Air Layer and its associated mineral dust, following results from the AER-D campaign.</p><p>AER-D was a small field experiment in the Eastern Atlantic during August 2015, based on the opportunity given by the simultaneous ICE-D experiment. The purpose of AER-D was to investigate the physical properties of the Saharan Air Layer, and to assess and validate remote sensing and modelling products. The FAAM atmospheric research aircraft was used as a flying laboratory, and it carried a full set of instruments aimed at both in-situ sampling and remote sensing.</p><p>A broad distribution of particle sizes was consistently observed, with a significant giant mode up to 80 µm, generally larger than what was observed in previous experiments: we ascribe this to the set of instruments used, able to capture the full spectrum. We will discuss the representation of the particle size in operational models, and we will show that despite predicting an extinction coefficient of the correct order of magnitude, the particle size is generally underestimated. We will also discuss the implication of the giant particles for the ground-based remote sensing of columnar size-distributions from the SKYNET and AERONET networks (Sunphotometer Airborne Validation Experiment, which was a component of AER-D).</p><p>We will present the vertical structure of the Saharan Air Layer, and in particular one episode when the structure was very different than the one generally accepted in the conceptual model. Moreover, the comparison with the operational models showed that they can predict a correct aerosol optical depth (AOD, a vertically integrated quantity) despite missing the vertical distribution.</p><p>These findings lead to a series of reflections on how to better constrain our knowledge of the Saharan Air Layer and its representation in operational models. Size-resolved properties and the vertical distribution are essential companions of the global AOD observations commonly used operationally. We will also discuss objectives and ideas for future field experiments.</p>

scholarly journals Comparison of Columnar, Surface, and UAS Profiles of Absorbing Aerosol Optical Depth and Single-Scattering Albedo in South-East Poland

Atmosphere ◽  
2019 ◽  
Vol 10 (8) ◽  
pp. 446 ◽  
Author(s):  
Michał T. Chiliński ◽  
Krzysztof M. Markowicz ◽  
Olga Zawadzka ◽  
Iwona S. Stachlewska ◽  
Justyna Lisok ◽  
...  
Keyword(s):  
Absorption Coefficient ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Measurement Data ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Height Distribution ◽  
Vertical Profiles ◽  
Absorbing Aerosols ◽  
The Impact

The impact of absorbing aerosols on climate is complex, with their potential positive or negative forcing, depending on many factors, including their height distribution and reflective properties of the underlying background. Measurement data is very limited, due to insufficient remote sensing methods dedicated to the retrieval of their vertical distribution. Columnar values of absorbing aerosol optical depth (AAOD) and single scattering albedo (SSA) are retrieved by the Aerosol Robotic Network (AERONET). However, the number of available results is low due to sky condition and aerosol optical depth (AOD) limitation. Presented research describes results of field campaigns in Strzyżów (South-East Poland, Eastern Europe) dedicated to the comparison of the absorption coefficient and SSA measurements performed with on-ground in-situ devices (aethalomter, nephelometer), small unmanned aerial system (UAS) carrying micro-aethalometer, as well as with lidar/ceilometer. An important aspect is the comparison of measurement results with those delivered by AERONET. Correlation of absorption to scattering coefficients measured on ground (0.79) and correlation of extinction on ground to AOD measured by AERONET (0.77) was visibly higher than correlation between AOD and AAOD retrieved by AERONET (0.56). Columnar SSA was weakly correlated with ground SSA (higher values of columnar SSA), which were mainly explained by hygroscopic effects, increasing scattering coefficient in ambient (wet conditions), and partly high uncertainty of SSA retrieval. AAOD derived with the use of profiles from UAS up to PBL height, was estimated to contribute in average to 37% of the total AAOD. A method of AAOD estimation, in the whole troposphere, with use of measured vertical profiles of absorption coefficient and extinction coefficient profiles from lidars was proposed. AAOD measured with this method has poor correlation with AERONET data, however for some measurements, within PBL, AAOD was higher than reported by AERONET, suggesting potential underestimation in photometric measurement under particular conditions. Correlation of absorption coefficient in profile to on ground measurements decrease with altitude. Measurements of SSA from drones agree well with ground measurements and are lower than results from AERONET, which suggests a larger contribution of absorbing aerosols. As an alternative for AAOD estimation in case of lack of AERONET AAOD data simple models are proposed, which base on AOD scaling with SSA measured with different methods. Proposed solution increase potential of absorption coefficient measurements in vertical profiles and columns of the atmosphere. Presented solutions make measurements of absorption coefficients in vertical profiles more affordable and allow rough estimation of columnar values for the whole atmosphere.

scholarly journals Aerosol optical depth and fine-mode fraction retrieval over East Asia using multi-angular total and polarized remote sensing

2012 ◽  
Vol 5 (3) ◽  
pp. 501-516 ◽  
Author(s):  
T. Cheng ◽  
X. Gu ◽  
D. Xie ◽  
Z. Li ◽  
T. Yu ◽  
...  
Keyword(s):  
East Asia ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Lookup Table ◽  
Retrieval Algorithm ◽  
Spatial And Temporal Variability ◽  
Aerosol Retrieval ◽  
Fine Mode ◽  
Sun Photometer ◽  
The Impact

Abstract. A new aerosol retrieval algorithm using multi-angular total and polarized measurements is presented. The algorithm retrieves aerosol optical depth (AOD), fine-mode fraction (FMF) for studying the impact of aerosol on climate change. The retrieval algorithm is based on a lookup table (LUT) method, which assumes that one fine and one coarse lognormal aerosol modes can be combined with proper weightings to represent the ambient aerosol properties. To reduce the ambiguity in retrieval algorithm, the key characteristics of aerosol model over East Asia are constrained using the cluster analysis technique based on the AERONET sun-photometer observation over East Asia, and the fine and coarse modes are not fixed but can vary. A mixing model of bare soil and green vegetation spectra and the Nadal and Breon model for the bidirectional polarized reflectance factor (BPDF) were used to simulate total and polarized surface reflectance of East Asia. By applying the present algorithm to POLDER measurements, three different aerosol cases of clear, polluted and dust are analyzed to test the algorithm. The comparison of retrieved aerosol optical depth (AOD) and fine-mode fraction (FMF) with those of AERONET sun-photometer observations show reliable results. Preliminary validation is encouraging. Using the new aerosol retrieval algorithm for multi-angular total and polarized measurements, the spatial and temporal variability of anthropogenic aerosol optical properties over East Asia, which were observed during a heavy polluted event, were analyzed. Exceptionally high values of aerosol optical depth contributed by fine mode of up to 0.5 (at 0.865 μm), and high values of fine-mode fraction of up to 0.9, were observed in this case study.

scholarly journals Aerosol optical depth and fine-mode fraction retrieval over East Asia using multi-angular total and polarized remote sensing

2011 ◽  
Vol 4 (5) ◽  
pp. 5689-5716
Author(s):  
T. Cheng ◽  
X. Gu ◽  
D. Xie ◽  
Z. Li ◽  
T. Yu ◽  
...  
Keyword(s):  
East Asia ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Lookup Table ◽  
Retrieval Algorithm ◽  
Spatial And Temporal Variability ◽  
Aerosol Retrieval ◽  
Fine Mode ◽  
Sun Photometer ◽  
The Impact

Abstract. A new aerosol retrieval algorithm using multi-angular total and polarized measurements is presented. The algorithm retrieves aerosol optical depth (AOD), fine-mode fraction (FMF) for studying the impact of aerosol on climate change. The retrieval algorithm is based on a lookup table (LUT) method, which assumes that one fine and one coarse lognormal aerosol modes can be combined with proper weightings to represent the ambient aerosol properties. To reduce the ambiguity in retrieval algorithm, the key characteristics of aerosol model over East Asia are constrained using the cluster analysis technique based on the AERONET sun-photometer observation over East Asia. A mixing model of bare soil and green vegetation spectra and the Nadal and Breon model for the bidirectional polarized reflectance factor (BPDF) were used to simulate total and polarized surface reflectance of East Asia. By applying the present algorithm to POLDER measurements, three different aerosol cases of clear, polluted and dust are analyzed to test the algorithm. The comparison of retrieved aerosol optical depth (AOD) and fine-mode fraction (FMF) with those of AERONET sun-photometer observations show reliable results. Preliminary validation is encouraging. Using the new aerosol retrieval algorithm for multi-angular total and polarized measurements, the spatial and temporal variability of anthropogenic aerosol optical properties over East Asia, which were observed during a heavy polluted event, were analyzed. Exceptionally high values of aerosol optical depth contributed by fine mode of up to 0.5 (at 0.865 μm), and high values of fine-mode fraction of up to 0.9, were observed in this case study.

Retrieval of aerosol single scattering albedo using joint satellite and surface visibility measurements

2020 ◽  
Author(s):  
Jing Li ◽  
Yueming Dong
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Radiative Forcing ◽  
Optical Parameter ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Retrieval Algorithm ◽  
Extensive Coverage ◽  
Satellite Sensors ◽  
Aerosol Radiative

<p>Aerosol single scattering albedo is a critical optical parameter that determines aerosol radiative effect. However, most existing passive satellite sensors such as MODIS and VIIRS only measures the intensity of reflected solar radiation and can only retrieve aerosol optical depth, while aerosol single scattering albedo needs to be assumed in the retrieval algorithm. On the other hand, if aerosol optical depth is known, it would be possible to retrieve aerosol single scattering albedo using satellite sensors.  In this study, we develop a machine learning based algorithm that retrieves aerosol single scattering albedo using joint visibility and satellite measurements. Combined with meteorology variables including relative humidity and boundary layer height, surface visibility can be converted to column aerosol optical depth. Then combining this converted aerosol optical depth with VIIRS measured TOA apparent reflectance, we retrieve aerosol single scattering albedo at over 2000 stations worldwide. The results compare well with AERONET retrieved SSA. However, compared with AERONET, visibility is recorded at every WMO meteorology station and has much more extensive coverage. We also applied our method to surface PM2.5 measurements obtained satisfactory results. Our work provides an aerosol single scattering albedo dataset with extensive coverage over land, which can be used for aerosol radiative forcing calculations and model validation.</p>

The Impact of Dust Storms on Aerosol Optical Depth and Radiative Forcing

2020 ◽  
Vol 16 (1) ◽  
pp. 1-14
Author(s):  
Monim Jiboori ◽  
Nadia Abed ◽  
Mohamed Abdel Wahab
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Radiative Forcing ◽  
Dust Storms ◽  
The Impact

scholarly journals Monitoring the Spatial Variation of Aerosol Optical Depth and Its Correlation with Land Use/Land Cover in Wuhan, China: A Perspective of Urban Planning

2021 ◽  
Vol 18 (3) ◽  
pp. 1132
Author(s):  
Qijiao Xie ◽  
Qi Sun
Keyword(s):  
Land Use ◽  
Air Quality ◽  
Urban Planning ◽  
Land Cover ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Water Bodies ◽  
Landsat 8 ◽  
Land Use Land Cover ◽  
The Impact

Aerosols significantly affect environmental conditions, air quality, and public health locally, regionally, and globally. Examining the impact of land use/land cover (LULC) on aerosol optical depth (AOD) helps to understand how human activities influence air quality and develop suitable solutions. The Landsat 8 image and Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol products in summer in 2018 were used in LULC classification and AOD retrieval in this study. Spatial statistics and correlation analysis about the relationship between LULC and AOD were performed to examine the impact of LULC on AOD in summer in Wuhan, China. Results indicate that the AOD distribution expressed an obvious “basin effect” in urban development areas: higher AOD values concentrated in water bodies with lower terrain, which were surrounded by the high buildings or mountains with lower AOD values. The AOD values were negatively correlated with the vegetated areas while positively correlated to water bodies and construction lands. The impact of LULC on AOD varied with different contexts in all cases, showing a “context effect”. The regression correlations among the normalized difference vegetation index (NDVI), normalized difference built-up index (NDBI), normalized difference water index (NDWI), and AOD in given landscape contexts were much stronger than those throughout the whole study area. These findings provide sound evidence for urban planning, land use management and air quality improvement.

scholarly journals Towards a long-term global aerosol optical depth record: applying a consistent aerosol retrieval algorithm to MODIS and VIIRS-observed reflectance

2015 ◽  
Vol 8 (10) ◽  
pp. 4083-4110 ◽  
Author(s):  
R. C. Levy ◽  
L. A. Munchak ◽  
S. Mattoo ◽  
F. Patadia ◽  
L. A. Remer ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Infrared Imaging ◽  
Quantitative Information ◽  
Environmental Data ◽  
Retrieval Algorithm ◽  
Climate Data ◽  
Data Record ◽  
Moderate Resolution ◽  
Moderate Resolution Imaging Spectroradiometer

Abstract. To answer fundamental questions about aerosols in our changing climate, we must quantify both the current state of aerosols and how they are changing. Although NASA's Moderate Resolution Imaging Spectroradiometer (MODIS) sensors have provided quantitative information about global aerosol optical depth (AOD) for more than a decade, this period is still too short to create an aerosol climate data record (CDR). The Visible Infrared Imaging Radiometer Suite (VIIRS) was launched on the Suomi-NPP satellite in late 2011, with additional copies planned for future satellites. Can the MODIS aerosol data record be continued with VIIRS to create a consistent CDR? When compared to ground-based AERONET data, the VIIRS Environmental Data Record (V_EDR) has similar validation statistics as the MODIS Collection 6 (M_C6) product. However, the V_EDR and M_C6 are offset in regards to global AOD magnitudes, and tend to provide different maps of 0.55 μm AOD and 0.55/0.86 μm-based Ångström Exponent (AE). One reason is that the retrieval algorithms are different. Using the Intermediate File Format (IFF) for both MODIS and VIIRS data, we have tested whether we can apply a single MODIS-like (ML) dark-target algorithm on both sensors that leads to product convergence. Except for catering the radiative transfer and aerosol lookup tables to each sensor's specific wavelength bands, the ML algorithm is the same for both. We run the ML algorithm on both sensors between March 2012 and May 2014, and compare monthly mean AOD time series with each other and with M_C6 and V_EDR products. Focusing on the March–April–May (MAM) 2013 period, we compared additional statistics that include global and gridded 1° × 1° AOD and AE, histograms, sampling frequencies, and collocations with ground-based AERONET. Over land, use of the ML algorithm clearly reduces the differences between the MODIS and VIIRS-based AOD. However, although global offsets are near zero, some regional biases remain, especially in cloud fields and over brighter surface targets. Over ocean, use of the ML algorithm actually increases the offset between VIIRS and MODIS-based AOD (to ~ 0.025), while reducing the differences between AE. We characterize algorithm retrievability through statistics of retrieval fraction. In spite of differences between retrieved AOD magnitudes, the ML algorithm will lead to similar decisions about "whether to retrieve" on each sensor. Finally, we discuss how issues of calibration, as well as instrument spatial resolution may be contributing to the statistics and the ability to create a consistent MODIS → VIIRS aerosol CDR.

scholarly journals Multi-model study of mercury dispersion in the atmosphere: Vertical distribution of mercury species

2016 ◽  
Author(s):  
Johannes Bieser ◽  
Franz Slemr ◽  
Jesse Ambrose ◽  
Carl Brenninkmeijer ◽  
Steve Brooks ◽  
...  
Keyword(s):  
Vertical Distribution ◽  
Atmospheric Chemistry ◽  
Lower Troposphere ◽  
Elemental Mercury ◽  
Mercury Species ◽  
Substantial Impact ◽  
Model Studies ◽  
Model Study ◽  
The Impact ◽  
The Vertical Distribution

Abstract. Atmospheric chemistry and transport of mercury play a key role in the global mercury cycle. However, there are still considerable knowledge gaps concerning the fate of mercury in the atmosphere. This is the second part of a model inter-comparison study investigating the impact of atmospheric chemistry and emissions on mercury in the atmosphere. While the first study focused on ground based observations of mercury concentration and deposition, here we investigate the vertical distribution and speciation of mercury from the planetary boundary layer to the lower stratosphere. So far, there have been few model studies investigating the vertical distribution of mercury, mostly focusing on single aircraft campaigns. Here, we present a first comprehensive analysis based on various aircraft observations in Europe, North America, and on inter-continental flights. The investigated models proved to be able to reproduce the distribution of total and elemental mercury concentrations in the troposphere including inter-hemispheric trends. One key aspect of the study is the investigation of mercury oxidation in the troposphere. We found that different chemistry schemes were better at reproducing observed oxidized mercury (RM) patterns depending on altitude. High RM concentrations in the upper troposphere could be reproduced with oxidation by bromine while elevated concentrations in the lower troposphere were better reproduced by OH and ozone chemistry. However, the results were not always conclusive as the physical and chemical parametrizations in the chemistry transport models also proved to have a substantial impact on model results.

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