scholarly journals Surface ozone at Nam Co in the inland Tibetan Plateau: variation, synthesis comparison and regional representativeness

2017 ◽  
Vol 17 (18) ◽  
pp. 11293-11311 ◽  
Author(s):  
Xiufeng Yin ◽  
Shichang Kang ◽  
Benjamin de Foy ◽  
Zhiyuan Cong ◽  
Jiali Luo ◽  
...  
Keyword(s):  
Tibetan Plateau ◽  
Surface Ozone ◽  
Photochemical Reactions ◽  
Transport Processes ◽  
The Tibetan Plateau ◽  
Nam Co ◽  
Air Masses ◽  
Mixing Ratios ◽  
Northern Tibetan Plateau ◽  
Ozone Levels

Abstract. Ozone is an important pollutant and greenhouse gas, and tropospheric ozone variations are generally associated with both natural and anthropogenic processes. As one of the most pristine and inaccessible regions in the world, the Tibetan Plateau has been considered as an ideal region for studying processes of the background atmosphere. Due to the vast area of the Tibetan Plateau, sites in the southern, northern and central regions exhibit different patterns of variation in surface ozone. Here, we present continuous measurements of surface ozone mixing ratios at Nam Co Station over a period of  ∼ 5 years (January 2011 to October 2015), which is a background site in the inland Tibetan Plateau. An average surface ozone mixing ratio of 47.6 ± 11.6 ppb (mean ± standard deviation) was recorded, and a large annual cycle was observed with maximum ozone mixing ratios in the spring and minimum ratios during the winter. The diurnal cycle is characterized by a minimum in the early morning and a maximum in the late afternoon. Nam Co Station represents a background region where surface ozone receives negligible local anthropogenic emissions inputs, and the anthropogenic contribution from South Asia in spring and China in summer may affect Nam Co Station occasionally. Surface ozone at Nam Co Station is mainly dominated by natural processes involving photochemical reactions, vertical mixing and downward transport of stratospheric air mass. Model results indicate that the study site is affected differently by the surrounding areas in different seasons: air masses from the southern Tibetan Plateau contribute to the high ozone levels in the spring, and enhanced ozone levels in the summer are associated with air masses from the northern Tibetan Plateau. By comparing measurements at Nam Co Station with those from other sites on the Tibetan Plateau, we aim to expand the understanding of ozone cycles and transport processes over the Tibetan Plateau. This work may provide a reference for future model simulations.

scholarly journals Surface ozone at Nam Co (4730 m a.s.l.) in the inland Tibetan Plateau: variation, synthesis comparison and regional representativeness

2017 ◽  
Author(s):  
Xiufeng Yin ◽  
Shichang Kang ◽  
Benjamin de Foy ◽  
Zhiyuan Cong ◽  
Jiali Luo ◽  
...  
Keyword(s):  
Tibetan Plateau ◽  
Surface Ozone ◽  
Early Morning ◽  
Photochemical Reactions ◽  
Transport Processes ◽  
The Tibetan Plateau ◽  
Nam Co ◽  
Mixing Ratios ◽  
Northern Tibetan Plateau ◽  
Ozone Levels

Abstract. Ozone is an important pollutant and greenhouse gas, and tropospheric ozone variations are generally associated with both natural and anthropogenic processes. As one of the most pristine and inaccessible regions in the world, the Tibetan Plateau has been considered as an ideal region for studying processes of the background atmosphere. Due to the vast area of the Tibetan Plateau, sites in the southern, northern and central regions exhibit different patterns of variation in surface ozone. Here, we present long-term measurements for ~ 5 years (January 2011 to October 2015) of surface ozone mixing ratios at Nam Co Station, which is a regional background site in the inland Tibetan Plateau. An average surface ozone mixing ratio of 47.6 ± 11.6 ppb was recorded, and a large annual cycle was observed with maximum ozone mixing ratios in the spring and minimum ratios during the winter. The diurnal cycle is characterized by a minimum in the early morning and a maximum in the late afternoon. Nam Co Station represents a background region where surface ozone receives negligible local anthropogenic emissions. Surface ozone at Nam Co Station is mainly dominated by natural processes involving photochemical reactions and potential local vertical mixing. Model results indicate that the study site is affected by the surrounding areas in different seasons and that air masses from the northern Tibetan Plateau lead to increased ozone levels in the summer. In contrast to the surface ozone levels at the edges of the Tibetan Plateau, those at Nam Co Station are less affected by stratospheric intrusions and human activities which makes Nam Co Station representative of vast background areas in the central Tibetan Plateau. By comparing measurements at Nam Co Station with those from other sites in the Tibetan Plateau and beyond, we aim to expand the understanding of ozone cycles and transport processes over the Tibetan Plateau. This work may provide a reference for model simulations in the future.

scholarly journals Interannual variability of the boreal summer tropical UTLS in observations and CCMVal-2 simulations

2016 ◽  
Vol 16 (13) ◽  
pp. 8695-8714 ◽  
Author(s):  
Markus Kunze ◽  
Peter Braesicke ◽  
Ulrike Langematz ◽  
Gabriele Stiller
Keyword(s):  
Climate Models ◽  
Southern Oscillation ◽  
Asian Summer Monsoon ◽  
Multiple Linear Regression Model ◽  
Transport Processes ◽  
Boreal Summer ◽  
Temperature Pattern ◽  
The Tibetan Plateau ◽  
Quasi Biennial Oscillation ◽  
Mixing Ratios

Abstract. During boreal summer the upper troposphere/lower stratosphere (UTLS) in the Northern Hemisphere shows a distinct maximum in water vapour (H2O) mixing ratios and a coincident minimum in ozone (O3) mixing ratios, both confined within the Asian monsoon anticyclone (AMA). This well-known feature has been related to transport processes emerging above the convective systems during the Asian summer monsoon (ASM), further modified by the dynamics of the AMA. We compare the ability of chemistry–climate models (CCMs) to reproduce the climatological characteristics and variability of H2O, O3, and temperature in the UTLS during the boreal summer with MIPAS satellite observations and ERA-Interim reanalyses. By using a multiple linear regression model the main driving factors, the strength of the ASM, the quasi-biennial oscillation (QBO), and the El Niño–Southern Oscillation (ENSO), are separated. The regression patterns related to ENSO show a coherent, zonally asymmetric signal for temperatures and H2O mixing ratios for ERA-Interim and the CCMs and suggest a weakening of the ASM during ENSO warm events. The QBO modulation of the lower-stratospheric temperature near the Equator is well represented as a zonally symmetric pattern in the CCMs. Changes in H2O and O3 mixing ratios are consistent with the QBO-induced temperature and circulation anomalies but less zonally symmetric than the temperature pattern. Regarding the ASM, the results of the regression analysis show for ERA-Interim and the CCMs enhanced H2O and reduced O3 mixing ratios within the AMA for stronger ASM seasons. The CCM results can further confirm earlier studies which emphasize the importance of the Tibetan Plateau/southern slope of the Himalayas as the main source region for H2O in the AMA. The results suggest that H2O is transported towards higher latitudes at the north-eastern edge of the AMA rather than towards low equatorial latitudes to be fed into the tropical pipe.

scholarly journals Sediment transport processes across the Tibetan Plateau inferred from robust grain-size end members in lake sediments

2014 ◽  
Vol 10 (1) ◽  
pp. 91-106 ◽  
Author(s):  
E. Dietze ◽  
F. Maussion ◽  
M. Ahlborn ◽  
B. Diekmann ◽  
K. Hartmann ◽  
...  
Keyword(s):  
Grain Size ◽  
Sediment Transport ◽  
Tibetan Plateau ◽  
Transport Processes ◽  
The Tibetan Plateau ◽  
Dust Deposition ◽  
Northerly Wind ◽  
Near Surface ◽  
Depositional Processes ◽  
End Members

Abstract. Grain-size distributions offer powerful proxies of past environmental conditions that are related to sediment sorting processes. However, they are often of multimodal character because sediments can get mixed during deposition. To facilitate the use of grain size as palaeoenvironmental proxy, this study aims to distinguish the main detrital processes that contribute to lacustrine sedimentation across the Tibetan Plateau using grain-size end-member modelling analysis. Between three and five robust grain-size end-member subpopulations were distinguished at different sites from similarly–likely end-member model runs. Their main modes were grouped and linked to common sediment transport and depositional processes that can be associated with contemporary Tibetan climate (precipitation patterns and lake ice phenology, gridded wind and shear stress data from the High Asia Reanalysis) and local catchment configurations. The coarse sands and clays with grain-size modes >250 μm and <2 μm were probably transported by fluvial processes. Aeolian sands (~200 μm) and coarse local dust (~60 μm), transported by saltation and in near-surface suspension clouds, are probably related to occasional westerly storms in winter and spring. Coarse regional dust with modes ~25 μm may derive from near-by sources that keep in longer term suspension. The continuous background dust is differentiated into two robust end members (modes: 5–10 and 2–5 μm) that may represent different sources, wind directions and/or sediment trapping dynamics from long-range, upper-level westerly and episodic northerly wind transport. According to this study grain-size end members of only fluvial origin contribute small amounts to mean Tibetan lake sedimentation (19± 5%), whereas local to regional aeolian transport and background dust deposition dominate the clastic sedimentation in Tibetan lakes (contributions: 42 ± 14% and 51 ± 11%). However, fluvial and alluvial reworking of aeolian material from nearby slopes during summer seems to limit end-member interpretation and should be crosschecked with other proxy information. If not considered as a stand-alone proxy, a high transferability to other regions and sediment archives allows helpful reconstructions of past sedimentation history.

scholarly journals Atmospheric brown clouds reach the Tibetan Plateau by crossing the Himalayas

2015 ◽  
Vol 15 (11) ◽  
pp. 6007-6021 ◽  
Author(s):  
Z. L. Lüthi ◽  
B. Škerlak ◽  
S.-W. Kim ◽  
A. Lauer ◽  
A. Mues ◽  
...  
Keyword(s):  
Tibetan Plateau ◽  
Weather Prediction ◽  
Mountain Range ◽  
The Tibetan Plateau ◽  
Pollution Transport ◽  
Synoptic Scale ◽  
Gangetic Plain ◽  
Dark Light ◽  
Air Masses ◽  
Pollution Episode

Abstract. The Himalayas and the Tibetan Plateau region (HTP), despite being a remote and sparsely populated area, is regularly exposed to polluted air masses with significant amounts of aerosols including black carbon. These dark, light-absorbing particles are known to exert a great melting potential on mountain cryospheric reservoirs through albedo reduction and radiative forcing. This study combines ground-based and satellite remote sensing data to identify a severe aerosol pollution episode observed simultaneously in central Tibet and on the southern side of the Himalayas during 13–19 March 2009 (pre-monsoon). Trajectory calculations based on the high-resolution numerical weather prediction model COSMO are used to locate the source regions and study the mechanisms of pollution transport in the complex topography of the HTP. We detail how polluted air masses from an atmospheric brown cloud (ABC) over South Asia reach the Tibetan Plateau within a few days. Lifting and advection of polluted air masses over the great mountain range is enabled by a combination of synoptic-scale and local meteorological processes. During the days prior to the event, winds over the Indo-Gangetic Plain (IGP) are generally weak at lower levels, allowing for accumulation of pollutants and thus the formation of ABCs. The subsequent passing of synoptic-scale troughs leads to southwesterly flow in the middle troposphere over northern and central India, carrying the polluted air masses across the Himalayas. As the IGP is known to be a hotspot of ABCs, the cross-Himalayan transport of polluted air masses may have serious implications for the cryosphere in the HTP and impact climate on regional to global scales. Since the current study focuses on one particularly strong pollution episode, quantifying the frequency and magnitude of similar events in a climatological study is required to assess the total impact.

scholarly journals Diachronous Tibetan Plateau landscape evolution derived from lava field geomorphology

2020 ◽  
Author(s):  
Mark Allen ◽  
Robert Law
Keyword(s):  
Tibetan Plateau ◽  
Landscape Evolution ◽  
Tectonic Geomorphology ◽  
Normal Faults ◽  
The Tibetan Plateau ◽  
Lava Field ◽  
Northern Tibetan Plateau ◽  
Tectonic Processes ◽  
Stepwise Evolution

&lt;p&gt;&lt;strong&gt;Evolution of the Tibetan Plateau is important for understanding continental tectonics because of its exceptional elevation (~5 km above sea level) and crustal thickness (~70 km). Patterns of long-term landscape evolution can constrain tectonic processes, but have been hard to quantify, in contrast to established datasets for strain, exhumation and paleo-elevation. This study analyses the relief of the bases and tops of 17 Cenozoic lava fields on the central and northern Tibetan Plateau. Analyzed fields have typical lateral dimensions of 10s of km, and so have an appropriate scale for interpreting tectonic geomorphology. Fourteen of the fields have not been deformed since eruption. One field is cut by normal faults; two others are gently folded with limb dips &lt;6&lt;sup&gt;o&lt;/sup&gt;&lt;/strong&gt;&lt;strong&gt;. &lt;/strong&gt;&lt;strong&gt;Relief of the bases and tops of the fields is comparable to modern, internally-drained, parts of the plateau, and distinctly lower than externally-drained regions. The lavas preserve a record of underlying low relief bedrock landscapes at the time they were erupted, which have undergone little change since. There is an overlap in each area between younger published low-temperature thermochronology ages and the oldest eruption in each area, here interpreted as the transition &lt;/strong&gt;&lt;strong&gt;between the end of significant (&gt;3 km) exhumation and plateau landscape development. &lt;/strong&gt;&lt;strong&gt;This diachronous process took place between ~32.5&lt;sup&gt;o&lt;/sup&gt; - ~36.5&lt;sup&gt;o&lt;/sup&gt; N between ~40 and ~10 Ma, advancing northwards at a long-term rate of ~15 km/Myr. Results are consistent with incremental northwards growth of the plateau, rather than a stepwise evolution or synchronous uplift.&lt;/strong&gt;&lt;/p&gt;

scholarly journals Atmospheric processes of persistent organic pollutants over a remote lake of the central Tibetan Plateau: Implications for regional cycling

2016 ◽  
Author(s):  
Jiao Ren ◽  
Xiaoping Wang ◽  
Chuanfei Wang ◽  
Ping Gong ◽  
Tandong Yao
Keyword(s):  
Tibetan Plateau ◽  
Organic Pollutants ◽  
Persistent Organic Pollutants ◽  
Secondary Source ◽  
The Tibetan Plateau ◽  
Lake Area ◽  
Nam Co ◽  
Surface Exchange ◽  
Atmospheric Processes ◽  
Water Gas

Abstract. Atmospheric processes (air-surface exchange, and atmospheric deposition and degradation) are crucial for understanding the global cycling and fate of persistent organic pollutants (POPs). However, such assessment over the Tibetan Plateau (TP) remains uncertain. More than 50 % of the Chinese lakes are located on the TP, which exerts a remarkable influence on the regional water, energy, and chemical cycling. In this study, air and water samples were simultaneously collected in Nam Co, a large lake on the TP, to test whether the lake is a "secondary source" or "sink" of POPs. Lower concentrations of organochlorine pesticides (OCPs) and polychlorinated biphenyls (PCBs) were observed in the atmosphere and lake water of Nam Co, while the levels of polycyclic aromatic hydrocarbons (PAHs) were relatively higher. Results of fugacity ratios and chiral signatures both suggest that the lake acted as the net sink of atmospheric hexachlorocyclohexanes (HCHs), following their long-range transport driven by the Indian Monsoon. Different behaviors were observed in the PAHs, which primarily originated from local biomass burning. Acenaphthylene, acenaphthene, and fluorene showed volatilization from the lake to the atmosphere; while other PAHs were deposited into the lake due to the integrated deposition process (wet/dry and air-water gas deposition) and limited atmospheric degradation. As the dominant PAH compound, phenanthrene exhibited a seasonal reversal of air-water gas exchange, which was likely related to the melting of the lake ice in May. The annual input of HCHs from air to the entire lake area (2015 km2) was estimated as 1.9 kg year−1, while those estimated for PAHs can potentially reach up to 550 kg year−1. This study highlights the significance of PAH deposition on the regional carbon cycling in the oligotrophic lakes of the TP.

scholarly journals Air-Lake Interaction Features Found in Heat and Water Exchanges over Nam Co on the Tibetan Plateau

SOLA ◽  
2009 ◽  
Vol 5 ◽  
pp. 172-175 ◽  
Author(s):  
Shigenori Haginoya ◽  
Hideyuki Fujii ◽  
Tsuneo Kuwagata ◽  
Jianqing Xu ◽  
Yasushi Ishigooka ◽  
...  
Keyword(s):  
Tibetan Plateau ◽  
The Tibetan Plateau ◽  
Nam Co

scholarly journals A numerical process study on the rapid transport of stratospheric air down to the surface over western North America and the Tibetan Plateau

2019 ◽  
Vol 19 (9) ◽  
pp. 6535-6549 ◽  
Author(s):  
Bojan Škerlak ◽  
Stephan Pfahl ◽  
Michael Sprenger ◽  
Heini Wernli
Keyword(s):  
Boundary Layer ◽  
Tibetan Plateau ◽  
Surface Ozone ◽  
Vertical Transport ◽  
The Tibetan Plateau ◽  
Near Surface ◽  
Air Mass ◽  
Ozone Concentrations ◽  
Rapid Transport ◽  
Upper Level

Abstract. Upper-level fronts are often associated with the rapid transport of stratospheric air along tilted isentropes to the middle or lower troposphere, where this air leads to significantly enhanced ozone concentrations. These plumes of originally stratospheric air can only occasionally be observed at the surface because (i) stable boundary layers prevent an efficient vertical transport down to the surface, and (ii) even if boundary layer turbulence were strong enough to enable this transport, the originally stratospheric air mass can be diluted by mixing, such that only a weak stratospheric signal can be recorded at the surface. Most documented examples of stratospheric air reaching the surface occurred in mountainous regions. This study investigates two such events, using a passive stratospheric air mass tracer in a mesoscale model to explore the processes that enable the transport down to the surface. The events occurred in early May 2006 in the Rocky Mountains and in mid-June 2006 on the Tibetan Plateau. In both cases, a tropopause fold associated with an upper-level front enabled stratospheric air to enter the troposphere. In our model simulation of the North American case, the strong frontal zone reaches down to 700 hPa and leads to a fairly direct vertical transport of the stratospheric tracer along the tilted isentropes to the surface. In the Tibetan Plateau case, however, no near-surface front exists and a reservoir of high stratospheric tracer concentrations initially forms at 300–400 hPa, without further isentropic descent. However, entrainment at the top of the very deep boundary layer (reaching to 300 hPa over the Tibetan Plateau) and turbulence within the boundary layer allows for downward transport of stratospheric air to the surface. Despite the strongly differing dynamical processes, stratospheric tracer concentrations at the surface reach peak values of 10 %–20 % of the imposed stratospheric value in both cases, corroborating the potential of deep stratosphere-to-troposphere transport events to significantly influence surface ozone concentrations in these regions.

scholarly journals Developing a novel hybrid model for the estimation of surface 8 h ozone (O<sub>3</sub>) across the remote Tibetan Plateau during 2005–2018

2020 ◽  
Vol 20 (10) ◽  
pp. 6159-6175 ◽  
Author(s):  
Rui Li ◽  
Yilong Zhao ◽  
Wenhui Zhou ◽  
Ya Meng ◽  
Ziyu Zhang ◽  
...  
Keyword(s):  
Tibetan Plateau ◽  
Hybrid Model ◽  
Additive Model ◽  
World Health ◽  
The Tibetan Plateau ◽  
The Novel ◽  
Slow Increase ◽  
Potential Health ◽  
Generalised Additive Model ◽  
Northern Tibetan Plateau

Abstract. We developed a two-stage model called the random-forest–generalised additive model (RF–GAM), based on satellite data, meteorological factors, and other geographical covariates, to predict the surface 8 h O3 concentrations across the remote Tibetan Plateau. The 10-fold cross-validation result suggested that RF–GAM showed excellent performance, with the highest R2 value (0.76) and lowest root-mean-square error (RMSE) (14.41 µg m−3), compared with other seven machine-learning models. The predictive performance of RF–GAM showed significant seasonal discrepancy, with the highest R2 value observed in summer (0.74), followed by winter (0.69) and autumn (0.67), and the lowest one in spring (0.64). Additionally, the unlearning ground-observed O3 data collected from open-access websites were applied to test the transferring ability of the novel model and confirmed that the model was robust in predicting the surface 8 h O3 concentration during other periods (R2=0.67, RMSE = 25.68 µg m−3). RF–GAM was then used to predict the daily 8 h O3 level over the Tibetan Plateau during 2005–2018 for the first time. It was found that the estimated O3 concentration displayed a slow increase, from 64.74±8.30 µg m−3 to 66.45±8.67 µg m−3 from 2005 to 2015, whereas it decreased from the peak to 65.87±8.52 µg m−3 during 2015–2018. Besides this, the estimated 8 h O3 concentrations exhibited notable spatial variation, with the highest values in some cities of the northern Tibetan Plateau, such as Huangnan (73.48±4.53 µg m−3) and Hainan (72.24±5.34 µg m−3), followed by the cities in the central region, including Lhasa (65.99±7.24 µg m−3) and Shigatse (65.15±6.14 µg m−3), and the lowest O3 concentration occurred in a city of the southeastern Tibetan Plateau called Aba (55.17±12.77 µg m−3). Based on the 8 h O3 critical value (100 µg m−3) provided by the World Health Organization (WHO), we further estimated the annual mean nonattainment days over the Tibetan Plateau. It should be noted that most of the cities on the Tibetan Plateau had excellent air quality, while several cities (e.g. Huangnan, Haidong, and Guoluo) still suffered from more than 40 nonattainment days each year, which should be given more attention in order to alleviate local O3 pollution. The results shown herein confirm that the novel hybrid model improves the prediction accuracy and can be applied to assess the potential health risk, particularly in remote regions with few monitoring sites.

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