scholarly journals How does downward planetary wave coupling affect polar stratospheric ozone in the Arctic winter stratosphere?

2017 ◽  
Vol 17 (3) ◽  
pp. 2437-2458 ◽  
Author(s):  
Sandro W. Lubis ◽  
Vered Silverman ◽  
Katja Matthes ◽  
Nili Harnik ◽  
Nour-Eddine Omrani ◽  
...  

Abstract. It is well established that variable wintertime planetary wave forcing in the stratosphere controls the variability of Arctic stratospheric ozone through changes in the strength of the polar vortex and the residual circulation. While previous studies focused on the variations in upward wave flux entering the lower stratosphere, here the impact of downward planetary wave reflection on ozone is investigated for the first time. Utilizing the MERRA2 reanalysis and a fully coupled chemistry–climate simulation with the Community Earth System Model (CESM1(WACCM)) of the National Center for Atmospheric Research (NCAR), we find two downward wave reflection effects on ozone: (1) the direct effect in which the residual circulation is weakened during winter, reducing the typical increase of ozone due to upward planetary wave events and (2) the indirect effect in which the modification of polar temperature during winter affects the amount of ozone destruction in spring. Winter seasons dominated by downward wave reflection events (i.e., reflective winters) are characterized by lower Arctic ozone concentration, while seasons dominated by increased upward wave events (i.e., absorptive winters) are characterized by relatively higher ozone concentration. This behavior is consistent with the cumulative effects of downward and upward planetary wave events on polar stratospheric ozone via the residual circulation and the polar temperature in winter. The results establish a new perspective on dynamical processes controlling stratospheric ozone variability in the Arctic by highlighting the key role of wave reflection.

2016 ◽  
Author(s):  
Sandro W. Lubis ◽  
Vered Silverman ◽  
Katja Matthes ◽  
Nili Harnik ◽  
Nour-Eddine Omrani ◽  
...  

Abstract. It is well established that variable wintertime planetary wave forcing in the stratosphere controls the variability of Arctic stratospheric ozone through changes in the strength of the polar vortex and the residual circulation. While previous studies focused on the variations in upward wave flux entering the lower stratosphere, here the impact of downward planetary wave coupling (DWC) on ozone is investigated for the first time. Utilizing the MERRA-2 reanalysis and a fully coupled chemistry-climate simulation with NCAR's Community Earth System Model (CESM1[WACCM]), we find two DWC effects on ozone: (1) the direct effect in which the residual circulation is modified and prevents the typical increase of ozone due to upward planetary wave events in winter, and (2) the indirect effect in which the modification of polar temperature during winter affects the amount of ozone destruction in spring. Winter seasons dominated by DWC events (i.e., reflective winters) are characterized by lower Arctic ozone concentration, while seasons dominated by increased upward wave events (i.e., absorptive winters) are characterized by relatively higher ozone concentration. This behavior is consistent with the cumulative effects of downward and upward planetary wave events on polar stratospheric ozone via the residual circulation and the polar temperature in winter. The results establish a new perspective on dynamical processes controlling stratospheric ozone variability in the Arctic.


2013 ◽  
Vol 70 (12) ◽  
pp. 3977-3994 ◽  
Author(s):  
John R. Albers ◽  
Terrence R. Nathan

Abstract A mechanistic chemistry–dynamical model is used to evaluate the relative importance of radiative, photochemical, and dynamical feedbacks in communicating changes in lower-stratospheric ozone to the circulation of the stratosphere and lower mesosphere. Consistent with observations and past modeling studies of Northern Hemisphere late winter and early spring, high-latitude radiative cooling due to lower-stratospheric ozone depletion causes an increase in the modeled meridional temperature gradient, an increase in the strength of the polar vortex, and a decrease in vertical wave propagation in the lower stratosphere. Moreover, it is shown that, as planetary waves pass through the ozone loss region, dynamical feedbacks precondition the wave, causing a large increase in wave amplitude. The wave amplification causes an increase in planetary wave drag, an increase in residual circulation downwelling, and a weaker polar vortex in the upper stratosphere and lower mesosphere. The dynamical feedbacks responsible for the wave amplification are diagnosed using an ozone-modified refractive index; the results explain recent chemistry–coupled climate model simulations that suggest a link between ozone depletion and increased polar downwelling. The effects of future ozone recovery are also examined and the results provide guidance for researchers attempting to diagnose and predict how stratospheric climate will respond specifically to ozone loss and recovery versus other climate forcings including increasing greenhouse gas abundances and changing sea surface temperatures.


2015 ◽  
Vol 15 (17) ◽  
pp. 9945-9963 ◽  
Author(s):  
N. J. Livesey ◽  
M. L. Santee ◽  
G. L. Manney

Abstract. The well-established "Match" approach to quantifying chemical destruction of ozone in the polar lower stratosphere is applied to ozone observations from the Microwave Limb Sounder (MLS) on NASA's Aura spacecraft. Quantification of ozone loss requires distinguishing transport- and chemically induced changes in ozone abundance. This is accomplished in the Match approach by examining cases where trajectories indicate that the same air mass has been observed on multiple occasions. The method was pioneered using ozonesonde observations, for which hundreds of matched ozone observations per winter are typically available. The dense coverage of the MLS measurements, particularly at polar latitudes, allows matches to be made to thousands of observations each day. This study is enabled by recently developed MLS Lagrangian trajectory diagnostic (LTD) support products. Sensitivity studies indicate that the largest influence on the ozone loss estimates are the value of potential vorticity (PV) used to define the edge of the polar vortex (within which matched observations must lie) and the degree to which the PV of an air mass is allowed to vary between matched observations. Applying Match calculations to MLS observations of nitrous oxide, a long-lived tracer whose expected rate of change is negligible on the weekly to monthly timescales considered here, enables quantification of the impact of transport errors on the Match-based ozone loss estimates. Our loss estimates are generally in agreement with previous estimates for selected Arctic winters, though indicating smaller losses than many other studies. Arctic ozone losses are greatest during the 2010/11 winter, as seen in prior studies, with 2.0 ppmv (parts per million by volume) loss estimated at 450 K potential temperature (~ 18 km altitude). As expected, Antarctic winter ozone losses are consistently greater than those for the Arctic, with less interannual variability (e.g., ranging between 2.3 and 3.0 ppmv at 450 K). This study exemplifies the insights into atmospheric processes that can be obtained by applying the Match methodology to a densely sampled observation record such as that from Aura MLS.


2021 ◽  
Author(s):  
Marina Friedel ◽  
Gabriel Chiodo ◽  
Andrea Stenke ◽  
Daniela Domeisen ◽  
Stephan Fueglistaler ◽  
...  

Abstract Massive spring ozone loss due to anthropogenic emissions of ozone depleting substances is not limited to the austral hemisphere, but can also occur in the Arctic. Previous studies have suggested a link between springtime Arctic ozone depletion and Northern Hemispheric surface climate, which might add surface predictability. However, so far it has not been possible to isolate the role of stratospheric ozone from dynamical downward impacts. For the first time, we quantify the impact of springtime Arctic ozone depletion on surface climate using observations and targeted chemistry-climate model experiments to isolate the effects of ozone feedbacks. We find that springtime stratospheric ozone depletion is followed by surface anomalies in precipitation and temperature resembling a positive Arctic Oscillation. Most notably, we show that these anomalies, affecting large portions of the Northern Hemisphere, cannot be explained by dynamical variability alone, but are to a significant degree driven by stratospheric ozone. The surface signal is linked to reduced shortwave absorption by stratospheric ozone, forcing persistent negative temperature anomalies in the lower stratosphere and a delayed breakup of the polar vortex - analogous to ozone-surface coupling in the Southern Hemisphere.These results suggest that Arctic stratospheric ozone actively forces springtime Northern Hemispheric surface climate and thus provides a source of predictability on seasonal scales.


2015 ◽  
Vol 15 (7) ◽  
pp. 10041-10083 ◽  
Author(s):  
N. J. Livesey ◽  
M. L. Santee ◽  
G. L. Manney

Abstract. The well-established "Match" approach to quantifying chemical destruction of ozone in the polar lower stratosphere is applied to ozone observations from the Microwave Limb Sounder (MLS) on NASA's Aura spacecraft. Quantification of ozone loss requires distinguishing transport- and chemically induced changes in ozone abundance. This is accomplished in the Match approach by examining cases where trajectories indicate that the same airmass has been observed on multiple occasions. The method was pioneered using ozone sonde observations, for which hundreds of matched ozone observations per winter are typically available. The dense coverage of the MLS measurements, particularly at polar latitudes, allows matches to be made to thousands of observations each day. This study is enabled by recently developed MLS Lagrangian Trajectory Diagnostic (LTD) support products. Sensitivity studies indicate that the largest influence on the ozone loss estimates are the value of potential vorticity (PV) used to define the edge of the polar vortex (within which matched observations must lie) and the degree to which the PV of an airmass is allowed to vary between matched observations. Applying Match calculations to MLS observations of nitrous oxide, a long-lived tracer whose expected rate of change on these timescales is negligible, enables quantification of the impact of transport errors on the Match-based ozone loss estimates. Our loss estimates are generally in agreement with previous estimates for selected Arctic winters, though indicating smaller losses than many other studies. Arctic ozone losses are greatest during the 2010/11 winter, as seen in prior studies, with 2.0 ppmv (parts per million by volume) loss estimated at 450 K potential temperature. As expected, Antarctic winter ozone losses are consistently greater than those for the Arctic, with less interannual variability (e.g., ranging between 2.3 and 3.0 ppmv at 450 K). This study exemplifies the insights into atmospheric processes that can be obtained by applying the Match methodology to a densely sampled observation record such as that from Aura MLS.


Atmosphere ◽  
2021 ◽  
Vol 12 (5) ◽  
pp. 625
Author(s):  
Ansgar Schanz ◽  
Klemens Hocke ◽  
Niklaus Kämpfer ◽  
Simon Chabrillat ◽  
Antje Inness ◽  
...  

In this study, we compare the diurnal variation in stratospheric ozone of the MACC (Monitoring Atmospheric Composition and Climate) reanalysis, ECMWF Reanalysis Interim (ERA-Interim), and the free-running WACCM (Whole Atmosphere Community Climate Model). The diurnal variation of stratospheric ozone results from photochemical and dynamical processes depending on altitude, latitude, and season. MACC reanalysis and WACCM use similar chemistry modules and calculate a similar diurnal cycle in ozone when it is caused by a photochemical variation. The results of the two model systems are confirmed by observations of the Superconducting Submillimeter-Wave Limb-Emission Sounder (SMILES) experiment and three selected sites of the Network for Detection of Atmospheric Composition Change (NDACC) at Mauna Loa, Hawaii (tropics), Bern, Switzerland (midlatitudes), and Ny-Ålesund, Svalbard (high latitudes). On the other hand, the ozone product of ERA-Interim shows considerably less diurnal variation due to photochemical variations. The global maxima of diurnal variation occur at high latitudes in summer, e.g., near the Arctic NDACC site at Ny-Ålesund, Svalbard. The local OZORAM radiometer observes this effect in good agreement with MACC reanalysis and WACCM. The sensed diurnal variation at Ny-Ålesund is up to 8% (0.4 ppmv) due to photochemical variations in summer and negligible during the dynamically dominated winter. However, when dynamics play a major role for the diurnal ozone variation as in the lower stratosphere (100–20 hPa), the reanalysis models ERA-Interim and MACC which assimilate data from radiosondes and satellites outperform the free-running WACCM. Such a domain is the Antarctic polar winter where a surprising novel feature of diurnal variation is indicated by MACC reanalysis and ERA-Interim at the edge of the polar vortex. This effect accounts for up to 8% (0.4 ppmv) in both model systems. In summary, MACC reanalysis provides a global description of the diurnal variation of stratospheric ozone caused by dynamics and photochemical variations. This is of high interest for ozone trend analysis and other research which is based on merged satellite data or measurements at different local time.


2021 ◽  
Author(s):  
Ramina Alwarda ◽  
Kristof Bognar ◽  
Kimberly Strong ◽  
Martyn Chipperfield ◽  
Sandip Dhomse ◽  
...  

<p>The Arctic winter of 2019-2020 was characterized by an unusually persistent polar vortex and temperatures in the lower stratosphere that were consistently below the threshold for the formation of polar stratospheric clouds (PSCs). These conditions led to ozone loss that is comparable to the Antarctic ozone hole. Ground-based measurements from a suite of instruments at the Polar Environment Atmospheric Research Laboratory (PEARL) in Eureka, Canada (80.05°N, 86.42°W) were used to investigate chemical ozone depletion. The vortex was located above Eureka longer than in any previous year in the 20-year dataset and lidar measurements provided evidence of polar stratospheric clouds (PSCs) above Eureka. Additionally, UV-visible zenith-sky Differential Optical Absorption Spectroscopy (DOAS) measurements showed record ozone loss in the 20-year dataset, evidence of denitrification along with the slowest increase of NO<sub>2</sub> during spring, as well as enhanced reactive halogen species (OClO and BrO). Complementary measurements of HCl and ClONO<sub>2</sub> (chlorine reservoir species) from a Fourier transform infrared (FTIR) spectrometer showed unusually low columns that were comparable to 2011, the previous year with significant chemical ozone depletion. Record low values of HNO<sub>3</sub> in the FTIR dataset are in accordance with the evidence of PSCs and a denitrified atmosphere. Estimates of chemical ozone loss were derived using passive ozone from the SLIMCAT offline chemical transport model to account for dynamical contributions to the stratospheric ozone budget.</p>


2021 ◽  
Author(s):  
Shima Bahramvash Shams ◽  
Von P. Walden ◽  
James W. Hannigan ◽  
William J. Randel ◽  
Irina V. Petropavlovskikh ◽  
...  

Abstract. Stratospheric circulation is a critical part of the Arctic ozone cycle. Sudden stratospheric warming events (SSWs) manifest the strongest alteration of stratospheric dynamics. Changes in planetary wave propagation vigorously influence zonal mean zonal wind, temperature, and tracer concentrations in the stratosphere over the high latitudes. In this study, we examine six major SSWs from 2004 to 2020 using the Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2). Using the unique density of observations around the Greenland sector at high latitudes, we perform comprehensive comparisons of high latitude observations with the MERRA-2 ozone dataset during the six major SSWs. Our results show that MERRA-2 captures the high variability of mid stratospheric ozone fluctuations during SSWs over high latitudes. However, larger uncertainties are observed in the lower stratosphere and troposphere. The zonally averaged stratospheric ozone shows a dramatic increase of 9–29 % in total column ozone (TCO) near the time of each SSW, which lasts up to two months. The SSWs exhibit a more significant impact on ozone over high northern latitudes when the polar vortex is mostly elongated as seen in 2009 and 2018 compared to the events in which the polar vortex is displaced towards Europe. The regional impact of SSWs over Greenland has a similar structure as the zonal average, however, exhibits more intense ozone anomalies which is reflected by 15–37 % increase in TCO. The influence of SSW on mid stratospheric ozone levels persists longer than their impact on temperature. This paper is focused on the increased (suppressed) wave activity before (after) the SSWs and their impact on ozone variability at high latitudes. This includes an investigation of the different terms of tracer continuity using MERRA-2 parameters, which emphasizes the key role of vertical advection on mid-stratospheric ozone during the SSWs.


2021 ◽  
Author(s):  
Jezabel Curbelo ◽  
Gang Chen ◽  
Carlos R. Mechoso

<div>The evolution of the Northern Hemisphere stratosphere during late winter and early spring of 2020 was punctuated by outstanding events both in dynamics and tracer evolution. It provides an ideal case for study of the Lagrangian properties of the evolving flow and its connections with the troposphere. The events ranged from an episode of polar warming at upper levels in March, a polar vortex split into two cyclonic vortices at middle and lower levels in April, and a remarkably deep and persistent mass of ozone poor air within the westerly circulation throughout the period. The latter feature was particularly remarkable during 2020, which showed the lowest values of stratospheric ozone on record.</div><div> </div><div>We focus on the vortex split in April 2020 and we examine this split at middle as well as lower stratospheric levels, and the interactions that occurred between the resulting two vortices which determined the distribution of ozone among them. We also examine the connections among stratospheric and tropospheric events during the period.</div><div> </div><div>Our approach for analysis will be based on the application of Lagrangian tools to the flow field, based on following air parcels trajectories, examining barriers to the flow, and the activity and propagation of planetary waves. Our findings confirm the key role for the split played by a flow configuration with a polar hyperbolic trajectory and associated manifolds. A trajectory analysis illustrates the transport of ozone between the vortices during the split. We argue that these stratospheric events were linked to strong synoptic scale disturbances in the troposphere forming a wave train from the north Pacific to North America and Eurasia.</div><div><strong> </strong></div><div><strong>Reference:</strong><strong> </strong>J. Curbelo, G. Chen,  C. R. Mechoso. Multi-level analysis of the northern polar vortex split in April 2020 during development of the Arctic ozone hole. Earth and Space Science Open Archive. doi: 10.1002/essoar.10505516.1</div><div> </div><div><strong>Acknowledgements:</strong> NSF Grant AGS-1832842, RYC2018-025169 and EIN2019-103087.</div>


2019 ◽  
Vol 19 (15) ◽  
pp. 10303-10317 ◽  
Author(s):  
Yuke Wang ◽  
Valerii Shulga ◽  
Gennadi Milinevsky ◽  
Aleksey Patoka ◽  
Oleksandr Evtushevsky ◽  
...  

Abstract. The impact of a major sudden stratospheric warming (SSW) in the Arctic in February 2018 on the midlatitude mesosphere is investigated by performing the microwave radiometer measurements of carbon monoxide (CO) and zonal wind above Kharkiv, Ukraine (50.0∘ N, 36.3∘ E). The mesospheric peculiarities of this SSW event were observed using a recently designed and installed microwave radiometer in eastern Europe for the first time. Data from the ERA-Interim and MERRA-2 reanalyses, as well as the Aura microwave limb sounder measurements, are also used. Microwave observations of the daily CO profiles in January–March 2018 allowed for the retrieval of mesospheric zonal wind at 70–85 km (below the winter mesopause) over the Kharkiv site. Reversal of the mesospheric westerly from about 10 m s−1 to an easterly wind of about −10 m s−1 around 10 February was observed. The local microwave observations at our Northern Hemisphere (NH) midlatitude site combined with reanalysis data show wide-ranging daily variability in CO, zonal wind, and temperature in the mesosphere and stratosphere during the SSW of 2018. The observed local CO variability can be explained mainly by horizontal air mass redistribution due to planetary wave activity. Replacement of the CO-rich polar vortex air by CO-poor air of the surrounding area led to a significant mesospheric CO decrease over the station during the SSW and fragmentation of the vortex over the station at the SSW start caused enhanced stratospheric CO at about 30 km. The results of microwave measurements of CO and zonal wind in the midlatitude mesosphere at 70–85 km altitudes, which still are not adequately covered by ground-based observations, are useful for improving our understanding of the SSW impacts in this region.


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