scholarly journals Significant reduction of PM<sub>2.5</sub> in eastern China due to regional-scale emission control: evidence from SORPES in 2011–2018

2019 ◽  
Vol 19 (18) ◽  
pp. 11791-11801 ◽  
Author(s):  
Aijun Ding ◽  
Xin Huang ◽  
Wei Nie ◽  
Xuguang Chi ◽  
Zheng Xu ◽  
...  

Abstract. Haze pollution caused by PM2.5 is the largest air quality concern in China in recent years. Long-term measurements of PM2.5 and the precursors and chemical speciation are crucially important for evaluating the efficiency of emission control, understanding formation and transport of PM2.5 associated with the change of meteorology, and accessing the impact of human activities on regional climate change. Here we reported long-term continuous measurements of PM2.5, chemical components, and their precursors at a regional background station, the Station for Observing Regional Processes of the Earth System (SORPES), in Nanjing, eastern China, since 2011. We found that PM2.5 at the station has experienced a substantial decrease (−9.1 % yr−1), accompanied by even a very significant reduction of SO2 (−16.7 % yr−1), since the national “Ten Measures of Air” took action in 2013. Control of open biomass burning and fossil-fuel combustion are the two dominant factors that influence the PM2.5 reduction in early summer and winter, respectively. In the cold season (November–January), the nitrate fraction was significantly increased, especially when air masses were transported from the north. More NH3 available from a substantial reduction of SO2 and increased oxidization capacity are the main factors for the enhanced nitrate formation. The changes of year-to-year meteorology have contributed to 24 % of the PM2.5 decrease since 2013. This study highlights several important implications on air pollution control policy in China.

2019 ◽  
Author(s):  
Aijun Ding ◽  
Xin Huang ◽  
Wei Nie ◽  
Xuguang Chi ◽  
Zheng Xu ◽  
...  

Abstract. Haze pollution caused by PM2.5 is the largest air quality concern in China in recent years. Long-term measurements of PM2.5 and the precursors and chemical speciation is crucially important for evaluating the efficiency of emission control, understanding formation and transport of PM2.5 associated with the change of meteorology and for accessing the impact of human activities to regional climate change. Here we reported long-term continuous measurements of PM2.5, chemical components, and their precursors at a regional background station, the Station for Observing Regional Processes of the Earth System (SORPES), in Nanjing eastern China since 2011. We found that PM2.5 at the station has experienced a substantial decrease (−9.1 %/yr), accompanied with even much significant reduction of SO2 (−16.7 %/yr), since the national "Ten measures" for air took action in 2013. Control of open biomass burning and fossil-fuel combustion are the two dominant factors that influence the PM2.5 reduction in early summer and winter, respectively. In cold season (November–January), increased nitrate fraction was observed with more NH3 available from a substantial reduction of sulfate, and the change of year-to-year meteorology contributed to 24 % of the PM2.5 decrease since 2013. This study highlights several important implications on air pollution control policy in China.


2020 ◽  
Author(s):  
Zhixin Hao

&lt;p&gt;In China, historical documents record a large quantity of information related to climate change and grain harvest. This information can help to explore the impacts of extreme drought or flood on crop production, which can provide implications for the adaptation of agriculture to higher-probability extreme climate in the context of global warming. In this paper, reported extreme drought/flood chronologies and reconstructed grain harvest series derived from historical documents were adopted in order to investigate the association between the reported frequency of extreme drought/flood in eastern China and reconstructed poor harvests during 801&amp;#8211;1910. The results show that extreme droughts were reported more often in 801&amp;#8211;870, 1031&amp;#8211;1230, 1481&amp;#8211;1530, and 1581&amp;#8211;1650 over the whole of eastern China. On a regional scale, extreme droughts were reported more often in 1031&amp;#8211;1100, 1441&amp;#8211;1490, 1601&amp;#8211;1650, and 1831&amp;#8211;1880 in the North China Plain, 801&amp;#8211;870, 1031&amp;#8211;1120, 1161&amp;#8211;1220, and 1471&amp;#8211;1530 in Jianghuai, and 991&amp;#8211;1040, 1091&amp;#8211;1150, 1171&amp;#8211;1230, 1411&amp;#8211;1470, and 1481&amp;#8211;1530 in Jiangnan. The grain harvest was reconstructed to be generally poor in 801&amp;#8211;940, 1251&amp;#8211;1650, and 1841&amp;#8211;1910, but the reconstructed harvests were bumper in 951&amp;#8211;1250 and 1651&amp;#8211;1840, approximately. During the entire period from 801 to 1910, the frequency of reporting of extreme droughts in any subregion of eastern China was significantly associated over the long term with lower reconstructed harvests. The association between reported frequency of extreme floods and reconstructed low harvests appeared to be much weaker, while reconstructed harvest was much worse when extreme drought and extreme flood in different subregions were reported in the same year. The association between reconstructed poor harvests and reported frequency of regional extreme droughts was weak during the warm epoch of 920&amp;#8211;1300 but strong during the cold epoch of 1310&amp;#8211;1880, which could imply that a warm climate could weaken the impact of extreme drought on poor harvests; yet other historical factors may also contribute to these different patterns extracted from the two datasets.&lt;/p&gt;


2019 ◽  
Author(s):  
Zhixin Hao ◽  
Maowei Wu ◽  
Jingyun Zheng ◽  
Jiewei Chen ◽  
Xuezhen Zhang ◽  
...  

Abstract. Chinese historical documents recorded plenty of information related with climate change and grain harvest, which are helpful to explore the impacts of extreme drought/flood on crops and the implications on adaptation for agriculture to more extreme climate probability in the context of global warming. Here, we used the reconstructed extreme drought/flood chronologies and reconstructed grain harvest series derived from historical documents to investigate the connection between the occurrences of extreme drought/flood in eastern China and poor harvest during 801–1910. The results showed that more extreme droughts occurred in 801–870, 1031–1230, 1481–1530 and 1581–1650 over whole eastern China. On regional scale, more extreme droughts occurred in 1031–1100, 1441–1490, 1601–1650 and 1831–1880 in North China, 801–870, 1031–1120, 1161–1220 and 1471–1530 in Jianghuai, 991–1040, 1091–1150, 1171–1230, 1411–1470 and 1481–1530 in Jiangnan. The grain harvest was poor in periods of 801–940, 1251–1650 and 1841 to 1910, but bumper in periods of 951–1250 and 1651–1840 approximately. For entire period of 801–1910, more occurrence of extreme drought in any sub–region of eastern China could significantly reduce harvest in the long term average, but the connection between harvest and extreme flood seemed to be much weaker. The co–occurrence of extreme drought and extreme flood in different sub–regions in the same year had a greater impact on harvest yield. However, the connection between the occurrence of poor harvest and regional extreme drought was weak in the warm epoch of 920–1300 but strong in the cold epoch of 1310–1880, which implicated warm climate might weaken the impact of extreme drought on poor harvest during historical times.


2020 ◽  
Vol 16 (1) ◽  
pp. 101-116 ◽  
Author(s):  
Zhixin Hao ◽  
Maowei Wu ◽  
Jingyun Zheng ◽  
Jiewei Chen ◽  
Xuezhen Zhang ◽  
...  

Abstract. In China, historical documents record a large quantity of information related to climate change and grain harvest. This information can help to explore the impacts of extreme drought or flood on crop production, which can provide implications for the adaptation of agriculture to higher-probability extreme climate in the context of global warming. In this paper, reported extreme drought/flood chronologies and reconstructed grain harvest series derived from historical documents were adopted in order to investigate the association between the reported frequency of extreme drought/flood in eastern China and reconstructed poor harvests during 801–1910. The results show that extreme droughts were reported more often in 801–870, 1031–1230, 1481–1530, and 1581–1650 over the whole of eastern China. On a regional scale, extreme droughts were reported more often in 1031–1100, 1441–1490, 1601–1650, and 1831–1880 in the North China Plain, 801–870, 1031–1120, 1161–1220, and 1471–1530 in Jianghuai, and 991–1040, 1091–1150, 1171–1230, 1411–1470, and 1481–1530 in Jiangnan. The grain harvest was reconstructed to be generally poor in 801–940, 1251–1650, and 1841–1910, but the reconstructed harvests were bumper in 951–1250 and 1651–1840, approximately. During the entire period from 801 to 1910, the frequency of reporting of extreme droughts in any subregion of eastern China was significantly associated over the long term with lower reconstructed harvests. The association between reported frequency of extreme floods and reconstructed low harvests appeared to be much weaker, while reconstructed harvest was much worse when extreme drought and extreme flood in different subregions were reported in the same year. The association between reconstructed poor harvests and reported frequency of regional extreme droughts was weak during the warm epoch of 920–1300 but strong during the cold epoch of 1310–1880, which could imply that a warm climate could weaken the impact of extreme drought on poor harvests; yet other historical factors may also contribute to these different patterns extracted from the two datasets.


2021 ◽  
Vol 13 (7) ◽  
pp. 1317
Author(s):  
Xiaodan Ma ◽  
Peng Yan ◽  
Tianliang Zhao ◽  
Xiaofang Jia ◽  
Jian Jiao ◽  
...  

The chemical composition dataset of Aerosol Reanalysis of NASA’s Modern-Era Retrospective Analysis for Research and Application, version 2 (MERRAero) has not been thoroughly evaluated with observation data in mainland China due to the lack of long-term chemical components data. Using the 5-year data of PM10 mass concentrations and chemical compositions obtained from the routine sampling measurements at the World Meteorological Organization the Global Atmosphere Watch Programme regional background stations, Jing Sha (JS) and Lin’An (LA), in central and eastern China, we comprehensively evaluate the surface PM10 concentrations and chemical compositions such as sulfate (SO42−), organic carbon (OC) and black carbon (BC) derived from MERRAero. Overall, the concentrations of PM10, SO42−, OC and BC from the MERRAero agreed well with the measurements, despite a slight and consistent overestimation of BC concentrations and a moderate and persistent underestimation of PM10 concentrations throughout the study period. The MERRAero reanalysis of aerosol compositions performs better during the summertime than wintertime. By considering the nitrate particles in PM10 reconstruction, MERRAero performance can be significantly improved. The unreasonable seasonal variations of PM10 chemical compositions at station LA by MERRAero could be causative factors for the larger MERRAero discrepancies during 2016–2017 than the period of 2011–2013.


2018 ◽  
Author(s):  
Xin Long ◽  
Naifang Bei ◽  
Jiarui Wu ◽  
Xia Li ◽  
Tian Feng ◽  
...  

Abstract. Although aggressive emission control strategies have been implemented recently in the Beijing–Tianjin–Hebei area (BTH), China, pervasive and persistent haze still frequently engulfs the region during wintertime. Afforestation in BTH, primarily concentrated in the Taihang and Yanshan Mountains, has constituted one of the controversial factors exacerbating the haze pollution due to its slowdown of the surface wind speed. We report here an increasing trend of forest cover in BTH during 2001–2013 based on long-term satellite measurements and the impact of the afforestation on the fine particles (PM2.5) level. Simulations using the Weather Research and Forecast model with chemistry reveal that the afforestation in BTH since 2001 generally deteriorates the haze pollution in BTH to some degree, enhancing PM2.5 concentrations by up to 6 % on average. Complete afforestation or deforestation in the Taihang and Yanshan Mountains would increase or decrease the PM2.5 level within 15 % in BTH. Our model results also suggest that implementing a large ventilation corridor system would not be effective or beneficial to mitigate the haze pollution in Beijing.


2019 ◽  
Author(s):  
Lei Chen ◽  
Yi Gao ◽  
Meigen Zhang ◽  
Joshua S. Fu ◽  
Jia Zhu ◽  
...  

Abstract. Fourteen chemical transport models (CTMs) participate in the MICS–Asia Phase III Topic 1. Their simulation results are compared with each other and with an extensive set of measurements, aiming to evaluate the current multi–scale air quality models’ ability in simulating aerosol species and to document similarities and differences among model performances, also to reveal the characteristics of aerosol chemical components over big cities in East Asia. In general, all participant models can reproduce the spatial distribution and seasonal variability of aerosol concentrations in the year 2010, and multi–model ensemble mean (EM) shows better performance than most individual models, with Rs ranging from 0.65 (NO3−) to 0.83 (PM2.5). Underestimations of BC (NMB = −17.0 %), SO42− (NMB = −19.1 %) and PM10 (NMB = −32.6 %) are simulated by EM, but positive biases are shown in NO3− (NMB = 4.9 %), NH4+ (NMB = 14.0 %) and PM2.5 (NMB = 4.4 %). Simulation results of BC, OC, SO42−, NO3− and NH4+ among CTMs are in good agreements, especially over polluted areas, such as the eastern China and the northern part of India. But large coefficients of variations (CV > 1.5) are also calculated over arid and semi–arid regions. This poor consistency among CTMs may attribute to their different processing capacities for dust aerosols. According to the simulation results in the six Asian cities from EM, different air–pollution control plans should be made due to their different major air pollutants in different seasons. Although a more considerable capacity for reproducing the concentrations of aerosol chemical compositions and their variation tendencies is shown in current CTMs by comparing statistics (e.g. RMSE and R) between MICS–Asia Phase II and Phase III, detailed process analysis and a fully understanding of the source–receptor relationship in each process may be helpful to explain and to reduce large diversities of simulated aerosol concentrations among CTMs, and these may be the potential development directions for future modeling studies in East Asia.


2019 ◽  
Author(s):  
Qiuji Ding ◽  
Jianning Sun ◽  
Xin Huang ◽  
Aijun Ding ◽  
Jun Zou ◽  
...  

Abstract. Aerosols can not only participate in fog formation by acting as condensation nuclei of droplets but also modify the meteorological conditions such as air temperature and moisture, planetary boundary layer height (PBLH) and regional circulation during haze event. The impact of aerosols on fog formation, yet to be revealed, can be critical in understanding and predicting of fog-haze event. In this study, we used the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) to investigate a heavy fog event during a multiday intense haze pollution episode in early December 2013 in the Yangtze River Delta (YRD) region in eastern China. Using the WRF-Chem model, we conducted four parallel numerical experiments to evaluate the roles of aerosol-radiation interaction (ARI), aerosol-cloud interaction (ACI), black carbon (BC) and none BC (non-BC) aerosols in the formation and maintenance of the heavy fog event. Only when the aerosols' feedback processes are considered can the model well capture the haze pollution and the fog event. We find that the ARI dominates this fog-haze episode while the effects of ACI are negligible. Our analyses shows that BC plays a more important role in fog formation than non-BC aerosols. The dome effect of BC leads to an increase of air moisture over the sea by reducing PBLH and weakening vertical mixing, thereby confining more water vapor in the near-surface layer. The strengthened daytime onshore flow by a cyclonic wind anomaly, induced by contrast temperature perturbation over land and sea, transports moister air to the YRD region, where the suppressed PBLH and weakened daytime vertical mixing maintain the high moisture level. Then the heave fog forms due to the surface cooling at night in this region. This study highlights the importance of anthropogenic emissions in the formation of advection-radiation fog in the polluted coastal areas.


2019 ◽  
Vol 11 (4) ◽  
pp. 467 ◽  
Author(s):  
Helga Weber ◽  
Stefan Wunderle

Explicit knowledge of different error sources in long-term climate records from space is required to understand and mitigate their impacts on resulting time series. Imagery of the heritage Advanced Very High Resolution Radiometer (AVHRR) provides unique potential for climate research dating back to the 1980s, flying onboard a series of successive National Oceanic and Atmospheric Administration (NOAA) and Meteorological Operational (MetOp) satellites. However, the NOAA satellites are affected by severe orbital drift that results in spurious trends in time series. We identified the impact and extent of the orbital drift in 1 km AVHRR long-term active fire data. This record contains data of European fire activity from 1985–2016 and was analyzed on a regional scale and extended across Europe. Inconsistent sampling of the diurnal active fire cycle due to orbital drift with a maximum delay of ∼5 h over NOAA-14 lifetime revealed a ∼90% decline in the number of observed fires. However, interregional results were less conclusive and other error sources as well as interannual variability were more pronounced. Solar illumination, measured by the sun zenith angle (SZA), related changes in background temperatures were significant for all regions and afternoon satellites with major changes in −0.03 to −0.09 K deg − 1 for ▵ B T 34 (p ≤ 0 . 001). Based on example scenes, we simulated the influence of changing temperatures related to changes in the SZA on the detection of active fires. These simulations showed a profound influence of the active fire detection capabilities dependent on biome and land cover characteristics. The strong decrease in the relative changes in the apparent number of active fires calculated over the satellites lifetime highlights that a correction of the orbital drift effect is essential even over short time periods.


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