scholarly journals Estimation of black carbon emissions from Siberian fires using satellite observations of absorption and extinction optical depths

2018 ◽  
Author(s):  
Igor B. Konovalov ◽  
Daria A. Lvova ◽  
Matthias Beekmann ◽  
Hiren Jethva ◽  
Eugene F. Mikhailov ◽  
...  

Abstract. Black carbon (BC) emissions from open biomass burning (BB) are known to have a considerable impact on the radiative budget of the atmosphere on global and regional scales but are poorly constrained in models by atmospheric observations, especially in remote regions. Here, we investigate the feasibility of constraining BC emissions from BB with satellite observations of the aerosol absorption optical depth (AAOD) and the aerosol extinction optical depth (AOD) retrieved from OMI (Ozone monitoring instrument) and MODIS (Moderate Resolution Imaging Spectroradiometer) measurements, respectively. We consider the case of Siberian BB BC emissions, which have a strong potential to impact the Arctic climate system. Using aerosol remote sensing data collected at Siberian sites of the Aerosol Robotic Network (AERONET) along with the results of the Fourth Fire Lab at Missoula Experiment (FLAME-4), we establish an empirical parameterization relating the ratio of the elemental carbon (EC) and organic carbon (OC) contents in BB aerosol to the ratio of AAOD and AOD at the wavelengths of the satellite observations. Applying this parameterization to the BC and OC column amounts simulated with the CHIMERE chemistry transport model, we optimize the parameters of the BB emission model based on MODIS measurements of the fire radiative power (FRP) and obtain top-down optimized estimates of the total monthly BB BC amounts emitted from intense Siberian fires that occurred in May–September 2012. The top-down estimates are compared to the corresponding values obtained using the Global Fire Emissions Database (GFED4) and the Fire Emission Inventory–northern Eurasia (FEI-NE). Our simulations using the optimized BB aerosol emissions are verified against AAOD and AOD data that were withheld from the estimation procedure. The simulations are further evaluated against in situ EC and OC measurements at the Zotino Tall Tower Observatory (ZOTTO) and also against aerosol measurement data collected on board of an aircraft in the framework of the Airborne Extensive Regional Observations (YAK-AEROSIB) experiments. We conclude that our BC and OC emission estimates, considered with their confidence intervals, are consistent with the ensemble of the measurement data analyzed in this study. Siberian fires are found to emit 0.41 ± 0.14 Tg of BC over the whole period of the five months considered; this estimate is a factor of 2 larger and a factor of 1.5 smaller compared to that the corresponding estimates based on the GFED4 (0.20 Tg) and FEI-NE (0.61 Tg) data, respectively. Our estimates of monthly BC emissions are also found to be larger than the BC amounts calculated with the GFED4 data and smaller than those calculated with the FEI-NE data for any of the five months. Especially large positive differences of our estimates of monthly BC emissions with respect to the GFED4 data are found in May and September. This finding indicates that the GFED4 database is likely to strongly underestimate BC emissions from agricultural burns and grass fires in Siberia. All these differences have important implications for climate change in the Arctic, as it is found that about a quarter of the huge BB BC mass emitted in Siberia during the fire season of 2012 was transported across the polar circle into the Arctic. Overall, the results of our analysis indicate that a combination of the available satellite observations of AAOD and AOD can provide the necessary constraints on BB BC emissions.

2018 ◽  
Vol 18 (20) ◽  
pp. 14889-14924 ◽  
Author(s):  
Igor B. Konovalov ◽  
Daria A. Lvova ◽  
Matthias Beekmann ◽  
Hiren Jethva ◽  
Eugene F. Mikhailov ◽  
...  

Abstract. Black carbon (BC) emissions from open biomass burning (BB) are known to have a considerable impact on the radiative budget of the atmosphere at both global and regional scales; however, these emissions are poorly constrained in models by atmospheric observations, especially in remote regions. Here, we investigate the feasibility of constraining BC emissions from BB using satellite observations of the aerosol absorption optical depth (AAOD) and the aerosol extinction optical depth (AOD) retrieved from OMI (Ozone Monitoring Instrument) and MODIS (Moderate Resolution Imaging Spectroradiometer) measurements, respectively. We consider the case of Siberian BB BC emissions, which have the strong potential to impact the Arctic climate system. Using aerosol remote sensing data collected at Siberian sites of the AErosol RObotic NETwork (AERONET) along with the results of the fourth Fire Lab at Missoula Experiment (FLAME-4), we establish an empirical parameterization relating the ratio of the elemental carbon (EC) and organic carbon (OC) contents in BB aerosol to the ratio of AAOD and AOD at the wavelengths of the satellite observations. Applying this parameterization to the BC and OC column amounts simulated using the CHIMERE chemistry transport model, we optimize the parameters of the BB emission model based on MODIS measurements of the fire radiative power (FRP); we then obtain top-down optimized estimates of the total monthly BB BC amounts emitted from intense Siberian fires that occurred from May to September 2012. The top-down estimates are compared to the corresponding values obtained using the Global Fire Emissions Database (GFED4) and the Fire Emission Inventory–northern Eurasia (FEI-NE). Our simulations using the optimized BB aerosol emissions are verified against AAOD and AOD data that were withheld from the estimation procedure. The simulations are further evaluated against in situ EC and OC measurements at the Zotino Tall Tower Observatory (ZOTTO) and also against aircraft aerosol measurement data collected in the framework of the Airborne Extensive Regional Observations in SIBeria (YAK-AEROSIB) experiments. We conclude that our BC and OC emission estimates, considered with their confidence intervals, are consistent with the ensemble of the measurement data analyzed in this study. Siberian fires are found to emit 0.41±0.14 Tg of BC over the whole 5-month period considered; this estimate is a factor of 2 larger and a factor of 1.5 smaller than the corresponding estimates based on the GFED4 (0.20 Tg) and FEI-NE (0.61 Tg) data, respectively. Our estimates of monthly BC emissions are also found to be larger than the BC amounts calculated using the GFED4 data and smaller than those calculated using the FEI-NE data for any of the 5 months. Particularly large positive differences of our monthly BC emission estimates with respect to the GFED4 data are found in May and September. This finding indicates that the GFED4 database is likely to strongly underestimate BC emissions from agricultural burns and grass fires in Siberia. All of these differences have important implications for climate change in the Arctic, as it is found that about a quarter of the huge BB BC mass emitted in Siberia during the fire season of 2012 was transported across the polar circle into the Arctic. Overall, the results of our analysis indicate that a combination of the available satellite observations of AAOD and AOD can provide the necessary constraints on BB BC emissions.


2016 ◽  
Author(s):  
N. Evangeliou ◽  
Y. Balkanski ◽  
W. M. Hao ◽  
A. Petkov ◽  
R. P. Silverstein ◽  
...  

Abstract. In recent decades much attention has been given to the Arctic environment, where climate change is happening rapidly. Black carbon (BC) has been shown to be a major component of Arctic pollution that also affects the radiative balance. In the present study, we focused on how vegetation fires that occurred in Northern Eurasia during the period of 2002–2013 influenced the budget of BC in the Arctic. For simulating the transport of fire emissions from Northern Eurasia to the Arctic, we adopted BC fire emission estimates developed independently by GFED3 (Global Fire Emissions Database) and FEI-NE (Fire Emission Inventory – Northern Eurasia). Both datasets were based on fire locations and burned areas detected by MODIS (MODerate resolution Imaging Spectroradiometer) instruments on NASA's (National Aeronautics and Space Administration) Terra and Aqua satellites. Anthropogenic sources of BC were estimated using the MACCity (Monitoring Atmospheric Composition & Climate/megaCITY – Zoom for the ENvironment) emission inventory. During the 12-year period, an average area of 250,000 km2 yr−1 was burned in Northern Eurasia and the global emissions of BC ranged between 8.0 and 9.5 Tg yr−1. For the BC emitted in the Northern Hemisphere, about 70 % originated from anthropogenic sources and the rest from biomass burning (BB). Using the FEI-NE inventory, we found that 102 ± 29 kt yr−1 BC from biomass burning was deposited on the Arctic (defined here as the area north of 67º N) during the 12 years simulated, which was twice as much as when using MACCity inventory (56 ± 8 kt yr−1). The annual mass of BC deposited in the Arctic from all sources (FEI-NE in Northern Eurasia, MACCity elsewhere) is significantly higher by about 37 % in 2009 to 181 % in 2012, compared to the BC deposited using just the MACCity emission inventory. Deposition of BC in the Arctic from BB sources in the Northern Hemisphere thus represents 68 % of the BC deposited from all BC sources (the remaining being due to anthropogenic sources). Northern Eurasian vegetation fires (FEI-NE) contributed 85 % (79–91 %) to the BC deposited over the Arctic from all BB sources in the Northern Hemisphere. Arctic total BC burden showed strong seasonal variations, with highest values during the Arctic Haze season. High winter–spring values of BC burden were caused by transport of BC mainly from anthropogenic sources in Europe, whereas the peak in summer was mainly due to the fire emissions in Northern Eurasia. BC particles emitted from fires in lower latitudes (35° N–40° N) were found to remain the longest in the atmosphere due to the high release altitudes of smoke plumes, exhibit tropospheric transport resulting in a high summer peak of burden, and grow by condensation processes. In regards to the geographic contribution on the deposition of BC, we estimated that about 46 % of the BC deposited over the Arctic from vegetation fires in Northern Eurasia originated from Siberia, 6 % from Kazakhstan, 5 % from Europe, and about 1 % from Mongolia. The remaining 42 % originated from other areas in Northern Eurasia. For spring and summer, we computed that 42 % of the BC released from Northern Eurasian vegetation fires was deposited over the Arctic (annual average: 17 %). Vegetation fires in Northern Eurasia contributed to 14 % to 57 % of BC surface concentrations at the Arctic stations (Alert, Barrow, Zeppelin, Villum, and Tiksi), with fires in Siberia contributing the largest share. However, anthropogenic sources in the Northern Hemisphere remain essential, contributing 29 % to 54 % to the surface concentrations at the Arctic monitoring stations. The rest originated from North American fires.


2022 ◽  
Vol 15 (1) ◽  
pp. 219-249
Author(s):  
Mahtab Majdzadeh ◽  
Craig A. Stroud ◽  
Christopher Sioris ◽  
Paul A. Makar ◽  
Ayodeji Akingunola ◽  
...  

Abstract. The photolysis module in Environment and Climate Change Canada's online chemical transport model GEM-MACH (GEM: Global Environmental Multi-scale – MACH: Modelling Air quality and Chemistry) was improved to make use of the online size and composition-resolved representation of atmospheric aerosols and relative humidity in GEM-MACH, to account for aerosol attenuation of radiation in the photolysis calculation. We coupled both the GEM-MACH aerosol module and the MESSy-JVAL (Modular Earth Submodel System) photolysis module, through the use of the online aerosol modeled data and a new Mie lookup table for the model-generated extinction efficiency, absorption and scattering cross sections of each aerosol type. The new algorithm applies a lensing correction factor to the black carbon absorption efficiency (core-shell parameterization) and calculates the scattering and absorption optical depth and asymmetry factor of black carbon, sea salt, dust and other internally mixed components. We carried out a series of simulations with the improved version of MESSy-JVAL and wildfire emission inputs from the Canadian Forest Fire Emissions Prediction System (CFFEPS) for 2 months, compared the model aerosol optical depth (AOD) output to the previous version of MESSy-JVAL, satellite data, ground-based measurements and reanalysis products, and evaluated the effects of AOD calculations and the interactive aerosol feedback on the performance of the GEM-MACH model. The comparison of the improved version of MESSy-JVAL with the previous version showed significant improvements in the model performance with the implementation of the new photolysis module and with adopting the online interactive aerosol concentrations in GEM-MACH. Incorporating these changes to the model resulted in an increase in the correlation coefficient from 0.17 to 0.37 between the GEM-MACH model AOD 1-month hourly output and AERONET (Aerosol Robotic Network) measurements across all the North American sites. Comparisons of the updated model AOD with AERONET measurements for selected Canadian urban and industrial sites, specifically, showed better correlation coefficients for urban AERONET sites and for stations located further south in the domain for both simulation periods (June and January 2018). The predicted monthly averaged AOD using the improved photolysis module followed the spatial patterns of MERRA-2 reanalysis (Modern-Era Retrospective analysis for Research and Applications – version 2), with an overall underprediction of AOD over the common domain for both seasons. Our study also suggests that the domain-wide impacts of direct and indirect effect aerosol feedbacks on the photolysis rates from meteorological changes are considerably greater (3 to 4 times) than the direct aerosol optical effect on the photolysis rate calculations.


2021 ◽  
Author(s):  
Mahtab Majdzadeh ◽  
Craig Stroud ◽  
Christopher Sioris ◽  
Paul Makar ◽  
Ayodeji Akingunola ◽  
...  

<p>The photolysis module in Environment and Climate Change Canada’s on-line chemical transport model GEM-MACH (GEM: Global Environmental Multi-scale – MACH: Modelling Air quality and Chemistry) was improved by using the on-line chemical composition and size-resolved representation of atmospheric aerosols in GEM-MACH to calculate the attenuation of radiation in the photolysis module.</p><p>We coupled both the GEM-MACH aerosol module and the MESSy-JVAL (Modular Earth Sub-Model System) photolysis routine through the use of the on-line aerosol modeled data and a new Mie lookup table for the model-generated extinction efficiency, absorption and scattering cross sections of each aerosol. The new algorithm applies a lensing correction factor to the black carbon absorption efficiency (core-shell parametrization) and calculates the scattering and absorption optical depth and asymmetry factor of black carbon, sea-salt, dust and other internally mixed components.</p><p>In order to evaluate the effects of these modifications on the performance of the GEM-MACH model, a series of simulations with the updated version of MESSy-JVAL and wildfire emission inputs from the Canadian Forest Fire Emissions Prediction System (CFFEPS) were carried out, and the model aerosol optical depth (AOD) output was compared to the previous version of MESSy-JVAL, satellite data, ground-based measurements, and re-analysis products. The comparison of the updated version of MESSy-JVAL with the previous version showed significant improvements in the model performance with the implementation of the new photolysis module and adopting the online interactive aerosol concentrations in GEM-MACH.</p>


2016 ◽  
Vol 16 (12) ◽  
pp. 7587-7604 ◽  
Author(s):  
N. Evangeliou ◽  
Y. Balkanski ◽  
W. M. Hao ◽  
A. Petkov ◽  
R. P. Silverstein ◽  
...  

Abstract. In recent decades much attention has been given to the Arctic environment, where climate change is happening rapidly. Black carbon (BC) has been shown to be a major component of Arctic pollution that also affects the radiative balance. In the present study, we focused on how vegetation fires that occurred in northern Eurasia during the period of 2002–2013 influenced the budget of BC in the Arctic. For simulating the transport of fire emissions from northern Eurasia to the Arctic, we adopted BC fire emission estimates developed independently by GFED3 (Global Fire Emissions Database) and FEI-NE (Fire Emission Inventory – northern Eurasia). Both datasets were based on fire locations and burned areas detected by MODIS (Moderate resolution Imaging Spectroradiometer) instruments on NASA's (National Aeronautics and Space Administration) Terra and Aqua satellites. Anthropogenic sources of BC were adopted from the MACCity (Monitoring Atmospheric Composition and Climate and megacity Zoom for the Environment) emission inventory.During the 12-year period, an average area of 250 000 km2 yr−1 was burned in northern Eurasia (FEI-NE) and the global emissions of BC ranged between 8.0 and 9.5 Tg yr−1 (FEI-NE+MACCity). For the BC emitted in the Northern Hemisphere (based on FEI-NE+MACCity), about 70 % originated from anthropogenic sources and the rest from biomass burning (BB). Using the FEI-NE+MACCity inventory, we found that 102 ± 29 kt yr−1 BC was deposited in the Arctic (defined here as the area north of 67° N) during the 12 years simulated, which was twice as much as when using the MACCity inventory (56 ± 8 kt yr−1). The annual mass of BC deposited in the Arctic from all sources (FEI-NE in northern Eurasia, MACCity elsewhere) is significantly higher by about 37 % in 2009 (78 vs. 57 kt yr−1) to 181 % in 2012 (153 vs. 54 kt yr−1), compared to the BC deposited using just the MACCity emission inventory. Deposition of BC in the Arctic from BB sources in the Northern Hemisphere thus represents 68 % of the BC deposited from all BC sources (the remaining being due to anthropogenic sources). Northern Eurasian vegetation fires (FEI-NE) contributed 85 % (79–91 %) to the BC deposited over the Arctic from all BB sources in the Northern Hemisphere.We estimate that about 46 % of the BC deposited over the Arctic from vegetation fires in northern Eurasia originated from Siberia, 6 % from Kazakhstan, 5 % from Europe, and about 1 % from Mongolia. The remaining 42 % originated from other areas in northern Eurasia. About 42 % of the BC released from northern Eurasian vegetation fires was deposited over the Arctic (annual average: 17 %) during spring and summer.


2021 ◽  
Vol 18 (18) ◽  
pp. 5053-5083
Author(s):  
Jessica L. McCarty ◽  
Juha Aalto ◽  
Ville-Veikko Paunu ◽  
Steve R. Arnold ◽  
Sabine Eckhardt ◽  
...  

Abstract. In recent years, the pan-Arctic region has experienced increasingly extreme fire seasons. Fires in the northern high latitudes are driven by current and future climate change, lightning, fuel conditions, and human activity. In this context, conceptualizing and parameterizing current and future Arctic fire regimes will be important for fire and land management as well as understanding current and predicting future fire emissions. The objectives of this review were driven by policy questions identified by the Arctic Monitoring and Assessment Programme (AMAP) Working Group and posed to its Expert Group on Short-Lived Climate Forcers. This review synthesizes current understanding of the changing Arctic and boreal fire regimes, particularly as fire activity and its response to future climate change in the pan-Arctic have consequences for Arctic Council states aiming to mitigate and adapt to climate change in the north. The conclusions from our synthesis are the following. (1) Current and future Arctic fires, and the adjacent boreal region, are driven by natural (i.e. lightning) and human-caused ignition sources, including fires caused by timber and energy extraction, prescribed burning for landscape management, and tourism activities. Little is published in the scientific literature about cultural burning by Indigenous populations across the pan-Arctic, and questions remain on the source of ignitions above 70∘ N in Arctic Russia. (2) Climate change is expected to make Arctic fires more likely by increasing the likelihood of extreme fire weather, increased lightning activity, and drier vegetative and ground fuel conditions. (3) To some extent, shifting agricultural land use and forest transitions from forest–steppe to steppe, tundra to taiga, and coniferous to deciduous in a warmer climate may increase and decrease open biomass burning, depending on land use in addition to climate-driven biome shifts. However, at the country and landscape scales, these relationships are not well established. (4) Current black carbon and PM2.5 emissions from wildfires above 50 and 65∘ N are larger than emissions from the anthropogenic sectors of residential combustion, transportation, and flaring. Wildfire emissions have increased from 2010 to 2020, particularly above 60∘ N, with 56 % of black carbon emissions above 65∘ N in 2020 attributed to open biomass burning – indicating how extreme the 2020 wildfire season was and how severe future Arctic wildfire seasons can potentially be. (5) What works in the boreal zones to prevent and fight wildfires may not work in the Arctic. Fire management will need to adapt to a changing climate, economic development, the Indigenous and local communities, and fragile northern ecosystems, including permafrost and peatlands. (6) Factors contributing to the uncertainty of predicting and quantifying future Arctic fire regimes include underestimation of Arctic fires by satellite systems, lack of agreement between Earth observations and official statistics, and still needed refinements of location, conditions, and previous fire return intervals on peat and permafrost landscapes. This review highlights that much research is needed in order to understand the local and regional impacts of the changing Arctic fire regime on emissions and the global climate, ecosystems, and pan-Arctic communities.


2017 ◽  
Author(s):  
Ling Qi ◽  
Qinbin Li ◽  
Daven K. Henze ◽  
Hsien-Liang Tseng ◽  
Cenlin He

Abstract. We quantify source contributions to springtime (April 2008) surface black carbon (BC) in the Arctic by interpreting surface observations of BC at five receptor sites (Denali, Barrow, Alert, Zeppelin, and Summit) using a global chemical transport model (GEOS-Chem) and its adjoint. Contributions to BC at Barrow, Alert, and Zeppelin are dominated by Asian anthropogenic sources (40–43 %) before April 18 and by Siberian open biomass burning emissions (29–41 %) afterward. In contrast, Summit, a mostly free tropospheric site, has predominantly an Asian anthropogenic source contribution (24–68 %, with an average of 45 %). We compute the adjoint sensitivity of BC concentrations at the five sites during a pollution episode (April 20–25) to global emissions from March 1 to April 25. The associated contributions are the combined results of these sensitivities and BC emissions. Local and regional anthropogenic sources in Alaska are the largest anthropogenic sources of BC at Denali (63 %), and natural gas flaring emissions in the Western Extreme North of Russia (WENR) are the largest anthropogenic sources of BC at Zeppelin (26 %) and Alert (13 %). We find that long-range transport of emissions from Beijing-Tianjin-Hebei (also known as Jing-Jin-Ji), the biggest urbanized region in Northern China, contribute significantly (~ 10 %) to surface BC across the Arctic. On average it takes ~ 12 days for Asian anthropogenic emissions and Siberian biomass burning emissions to reach Arctic lower troposphere, supporting earlier studies. Natural gas flaring emissions from the WENR reach Zeppelin in about a week. We find that episodic, direct transport events dominate BC at Denali (87 %), a site outside the Arctic front, a strong transport barrier. The relative contribution of direct transport to surface BC within the Arctic front is much smaller (~ 50 % at Barrow and Zeppelin and ~ 10 % at Alert). The large contributions from Asian anthropogenic sources are predominately in the form of ‘chronic’ pollution (~ 40 % at Barrow and 65 % at Alert and 57 % at Zeppelin) on 1–2 month timescales. As such, it is likely that previous studies using 5- or 10-day trajectory analyses strongly underestimated the contribution from Asia to surface BC in the Arctic. Both finer temporal resolution of biomass burning emissions and accounting for the Wegener-Bergeron-Findeisen (WBF) process in wet scavenging improve the source attribution estimates.


2020 ◽  
Author(s):  
Anu-Maija Sundström ◽  
Tomi Karppinen ◽  
Antti Arola ◽  
Larisa Sogacheva ◽  
Hannakaisa Lindqvist ◽  
...  

<p>Climate change is proceeding fastest in the Arctic region. During past years Arctic summers have been warmer and drier elevating the risk for extensive forest fire episodes. In fact, satellite observations show, that during past two summers (2018, 2019) an increase is seen in the number of fires occurring above the Arctic Circle, especially in Siberia. While human-induced emissions of long-lived greenhouse gases are the main driving factor of global warming, short-lived climate forcers or pollutants emitted from the forest fires are also playing an important role especially in the Arctic. Absorbing aerosols can cause direct arctic warming locally. They can also alter radiative balance when depositing onto snow/ice and decreasing the surface albedo, resulting in subsequent warming. Aerosol-cloud interaction feedbacks can also enhance warming. Forest fire emissions also affect local air quality and photochemical processes in the atmosphere. For example, CO contributes to the formation of tropospheric ozone and affects the abundance of greenhouse gases such as methane and CO<sub>2</sub>.</p><p>This study focuses on analyzing fire episodes in the Arctic for the past 10 years, as well as investigating the transport of forest fire CO and smoke aerosols to the Arctic. Smoke plumes and their transport are analyzed using Absorbing Aerosol Index (AAI) from several satellite instruments: GOME-2 onboard Metop A and B, OMI onboard Aura, and TROPOMI onboard Copernicus Sentinel-5P satellite. Observations of CO are obtained from IASI (Metop A and B) as well as from TROPOMI, while the fire observations are obtained from MODIS instruments onboard Aqua and Terra, as well as from VIIRS onboard Suomi NPP.  In addition, observations e.g. from a space-borne lidar, CALIPSO, is used to obtain vertical distribution of smoke and to estimate plume heights.</p>


2004 ◽  
Vol 4 (7) ◽  
pp. 1857-1868 ◽  
Author(s):  
N. Spichtinger ◽  
R. Damoah ◽  
S. Eckhardt ◽  
C. Forster ◽  
P. James ◽  
...  

Abstract. Forest fire emissions have a strong impact on the concentrations of trace gases and aerosols in the atmosphere. In order to quantify the influence of boreal forest fire emissions on the atmospheric composition, the fire seasons of 1997 and 1998 are compared in this paper. Fire activity in 1998 was very strong, especially over Canada and Eastern Siberia, whereas it was much weaker in 1997. According to burned area estimates the burning in 1998 was more than six times as intense as in 1997. Based on hot spot locations derived from ATSR (Along Track Scanning Radiometer) data and official burned area data, fire emissions were estimated and their transport was simulated with a Lagrangian tracer transport model. Siberian and Canadian forest fire tracers were distinguished to investigate the transport of both separately. The fire emissions were transported even over intercontinental distances. Due to the El Niño induced meteorological situation, transport from Siberia to Canada was enhanced in 1998. Siberian fire emissions were transported towards Canada and contributed concentrations more than twice as high as those due to Canada's own CO emissions by fires. In 1998 both tracers arrive at higher latitudes over Europe, which is due to a higher North Atlantic Oscillation (NAO) index in 1998. The simulated emission plumes are compared to CMDL (Climate Monitoring and Diagnostics Laboratory) CO2 and CO data, Total Ozone Mapping Spectrometer (TOMS) aerosol index (AI) data and Global Ozone Monitoring Experiment (GOME) tropospheric NO2 and HCHO columns. All the data show clearly enhanced signals during the burning season of 1998 compared to 1997. The results of the model simulation are in good agreement with ground-based as well as satellite-based measurements.


Sign in / Sign up

Export Citation Format

Share Document