Stratospheric water vapour as tracer for Vortex filamentation in the Arctic winter 2002/2003

Abstract. Balloon-borne frost point hygrometers measured three high-resolution profiles of stratospheric water vapour above Ny-Ålesund, Spitsbergen during winter 2002/2003. The profiles obtained on 12 December 2002 and on 17 January 2003 provide an insight into the vertical distribution of water vapour in the core of the polar vortex. The water vapour sounding on 11 February 2003 was obtained within the vortex edge region of the lower stratosphere. Here, a significant reduction of water vapour mixing ratio was observed between 16 and 19 km. The stratospheric temperatures indicate that this dehydration was not caused by the presence of polar stratospheric clouds or earlier PSC particle sedimentation. Ozone observations on this day indicate a large scale movement of the polar vortex and show laminae in the same altitude range as the water vapour profile. The link between the observed water vapour reduction and filaments in the vortex edge region is indicated in the results of the semi-lagrangian advection model MIMOSA, which show that adjacent filaments of polar and mid latitude air can be identified above the Spitsbergen region. A vertical cross-section produced by the MIMOSA model reveals that the water vapour sonde flew through polar air in the lowest part of the stratosphere below 425 K, then passed through filaments of mid latitude air with lower water vapour concentrations, before it finally entered the polar vortex above 450 K. These results indicate that on 11 February 2003 the frost point hygrometer measured different water vapour concentrations as the sonde detected air with different origins. Instead of being linked to dehydration due to PSC particle sedimentation, the local reduction in the stratospheric water vapour profile was in this case caused by dynamical processes in the polar stratosphere.

Download Full-text

Stratospheric water vapour as tracer for vortex filamentation in the Arctic winter 2002/2003

Atmospheric Chemistry and Physics Discussions ◽

10.5194/acpd-3-4393-2003 ◽

2003 ◽

Vol 3 (4) ◽

pp. 4393-4410 ◽

Cited By ~ 2

Author(s):

M. Müller ◽

R. Neuber ◽

F. Fierli ◽

A. Hauchecorne ◽

H. Vömel ◽

...

Keyword(s):

Water Vapour ◽

Large Scale ◽

Polar Vortex ◽

The Arctic ◽

Edge Region ◽

Mixing Ratio ◽

Particle Sedimentation ◽

Frost Point ◽

Contour Advection ◽

Stratospheric Water Vapour

Abstract. During winter 2002/2003, three balloon-borne frost point hygrometers measured high-resolution profiles of stratospheric water vapour above Ny-Ålesund, Spitsbergen. All measurements reveal a high H2O mixing ratio of about 7 ppmv above 24 km, thus differing significantly from the 5 ppmv that are commonly assumed for the calculation of polar stratospheric cloud existence temperatures. The profiles obtained on 12 December 2002 and on 17 January 2003 provide an insight into the vertical distribution of water vapour in the core of the polar vortex. Unlike the earlier profiles, the water vapour sounding on 11 February 2003 detected the vortex edge region in the lower part of the stratosphere. Here, a striking diminuition in H2O mixing ratio stands out between 16 and 19 km. The according stratospheric temperatures clarify that this dehydration can not be caused by the presence of polar stratospheric clouds or earlier PSC particle sedimentation. On the same day, ozone observations by lidar indicate a large scale movement of the polar vortex, while an ozone sonde measurement even shows laminae in the same altitude range as in the water vapour profile. Tracer lamination in the vortex edge region is caused by filamentation of the vortex. The link between the observed water vapour diminuition and filaments in the vortex edge region is highlighted by results of the MIMOSA contour advection model. In the altitude of interest, adjoined filaments of polar and mid-latitudinal air can be identified above the Spitsbergen region. A vertical cross-section reveals that the water vapour sonde has flown through polar air in the lowest part of the stratosphere. Where the low water vapour mixing ratio was detected, the balloon passed through air from a mid-latitudinal filament from about 425 to 445 K, before it finally entered the polar vortex above 450 K. The MIMOSA model results elucidate the correlation that on 11 February 2003 the frost point hygrometer measured strongly variable water vapour concentrations as the sonde detected air with different origins, respectively. Instead of being linked to dehydration due to PSC particle sedimentation, the local diminuition in the stratospheric water vapour profile of 11 February 2003 has been found to be caused by dynamical processes in the polar stratosphere.

Download Full-text

Variability of water vapour in the Arctic stratosphere

Atmospheric Chemistry and Physics Discussions ◽

10.5194/acpd-15-22013-2015 ◽

2015 ◽

Vol 15 (16) ◽

pp. 22013-22045

Author(s):

L. Thölix ◽

L. Backman ◽

R. Kivi ◽

A. Karpechko

Keyword(s):

Water Vapour ◽

Large Scale ◽

Climate Model ◽

Model Simulation ◽

Polar Vortex ◽

The Arctic ◽

Cold Pool ◽

Model Calculations ◽

Water Vapour Concentration ◽

Stratospheric Water Vapour

Abstract. This study evaluates the stratospheric water vapour distribution and variability in the Arctic. A FinROSE chemistry climate model simulation covering years 1990–2013 is compared to observations (satellite and frostpoint hygrometer soundings) and the sources of stratospheric water vapour are studied. According to observations and the simulations the water vapour concentration in the Arctic stratosphere started to increase after year 2006, but around 2011 the concentration started to decrease. Model calculations suggest that the increase in water vapour during 2006–2011 (at 56 hPa) is mostly explained by transport related processes, while the photochemically produced water vapour plays a relatively smaller role. The water vapour trend in the stratosphere may have contributed to increased ICE PSC occurrence. The increase of water vapour in the precense of the low winter temperatures in the Arctic stratosphere led to more frequent occurrence of ICE PSCs in the Arctic vortex. The polar vortex was unusually cold in early 2010 and allowed large scale formation of the polar stratospheric clouds. The cold pool in the stratosphere over the Northern polar latitudes was large and stable and a large scale persistent dehydration was observed. Polar stratospheric ice clouds and dehydration were observed at Sodankylä with accurate water vapour soundings in January and February 2010 during the LAPBIAT atmospheric sounding campaign. The observed changes in water vapour were reproduced by the model. Both the observed and simulated decrease of the water vapour in the dehydration layer was up to 1.5 ppm.

Download Full-text

Stratospheric water vapour in the vicinity of the Arctic polar vortex

Annales Geophysicae ◽

10.5194/angeo-24-1511-2006 ◽

2006 ◽

Vol 24 (6) ◽

pp. 1511-1521 ◽

Cited By ~ 6

Author(s):

M. Maturilli ◽

F. Fierli ◽

V. Yushkov ◽

A. Lukyanov ◽

S. Khaykin ◽

...

Keyword(s):

Water Vapour ◽

Climate Models ◽

Polar Vortex ◽

Relative Difference ◽

Specific Humidity ◽

The Arctic ◽

Lyman Alpha ◽

Lagrangian Advection ◽

Stratospheric Water Vapour ◽

Dry Bias

Abstract. The stratospheric water vapour mixing ratio inside, outside, and at the edge of the polar vortex has been accurately measured by the FLASH-B Lyman-Alpha hygrometer during the LAUTLOS campaign in Sodankylä, Finland, in January and February 2004. The retrieved H2O profiles reveal a detailed view on the Arctic lower stratospheric water vapour distribution, and provide a valuable dataset for the validation of model and satellite data. Analysing the measurements with the semi-lagrangian advection model MIMOSA, water vapour profiles typical for the polar vortex' interior and exterior have been identified, and laminae in the observed profiles have been correlated to filamentary structures in the potential vorticity field. Applying the validated MIMOSA transport scheme to specific humidity fields from operational ECMWF analyses, large discrepancies from the observed profiles arise. Although MIMOSA is able to reproduce weak water vapour filaments and improves the shape of the profiles compared to operational ECMWF analyses, both models reveal a dry bias of about 1 ppmv in the lower stratosphere above 400 K, accounting for a relative difference from the measurements in the order of 20%. The large dry bias in the analysis representation of stratospheric water vapour in the Arctic implies the need for future regular measurements of water vapour in the polar stratosphere to allow the validation and improvement of climate models.

Download Full-text

Linking the uncertainty in simulated arctic ozone losses to modelling of tropical stratospheric water vapour

10.5194/acp-2018-310 ◽

2018 ◽

Author(s):

Laura Thölix ◽

Alexey Karpechko ◽

Leif Backman ◽

Rigel Kivi

Keyword(s):

Water Vapour ◽

Climate Models ◽

Polar Vortex ◽

The Arctic ◽

Ozone Loss ◽

Tropical Tropopause ◽

Water Vapour Concentration ◽

Vapour Concentration ◽

The Impact ◽

Stratospheric Water Vapour

Abstract. Stratospheric water vapor plays a key role in radiative and chemical processes, it e.g. influences the chemical ozone loss via controlling the polar stratospheric cloud formation in the polar stratosphere. The amount of water entering the stratosphere through the tropical tropopause differs substantially between chemistry-climate models. This is because the present-day models have difficulties in capturing the whole complexity of processes that control the water transport across the tropopause. As a result there are large differences in the stratospheric water vapour between the models. In this study we investigate the sensitivity of simulated Arctic ozone loss to the amount of water, which enters the stratosphere through the tropical tropopause. We used a chemical transport model, FinROSE-CTM, forced by ERA-Interim meteorology. The water vapour concentration in the tropical tropopause was varied between 0.5 and 1.6 times the concentration in ERA-Interim, which is similar to the range seen in chemistry climate models. The water vapour changes in the tropical tropopause led to about 1.5 and 2 ppm more water vapour in the Arctic polar vortex compared to the ERA-Interim, respectively. We found that the impact of water vapour changes on ozone loss in the Arctic polar vortex depend on the meteorological conditions. Polar stratospheric clouds form in the cold conditions within the Arctic vortex, and chlorine activation on their surface lead to ozone loss. If the cold conditions persist long enough (e.g. in 2010/11), the chlorine activation is nearly complete. In this case addition of water vapour to the stratosphere increased the formation of ICE clouds, but did not increase the chlorine activation and ozone destruction significantly. In the warm winter 2012/13 the impact of water vapour concentration on ozone loss was small, because the ozone loss was mainly NOx induced. In intermediately cold conditions, e.g. 2013/14, the effect of added water vapour was more prominent than in the other studied winters. The results show that the simulated water vapour concentration in the tropical tropopause has a significant impact on the Arctic ozone loss and deserves attention in order to improve future projections of ozone layer recovery.

Download Full-text

Variability of water vapour in the Arctic stratosphere

Atmospheric Chemistry and Physics ◽

10.5194/acp-16-4307-2016 ◽

2016 ◽

Vol 16 (7) ◽

pp. 4307-4321 ◽

Cited By ~ 5

Author(s):

Laura Thölix ◽

Leif Backman ◽

Rigel Kivi ◽

Alexey Yu. Karpechko

Keyword(s):

Water Vapour ◽

Large Scale ◽

Decadal Variability ◽

Transport Model ◽

Model Simulation ◽

The Arctic ◽

Arctic Water ◽

Model Calculations ◽

Water Vapour Concentration ◽

Stratospheric Water Vapour

Abstract. This study evaluates the stratospheric water vapour distribution and variability in the Arctic. A FinROSE chemistry transport model simulation covering the years 1990–2014 is compared to observations (satellite and frost point hygrometer soundings), and the sources of stratospheric water vapour are studied. In the simulations, the Arctic water vapour shows decadal variability with a magnitude of 0.8 ppm. Both observations and the simulations show an increase in the water vapour concentration in the Arctic stratosphere after the year 2006, but around 2012 the concentration started to decrease. Model calculations suggest that this increase in water vapour is mostly explained by transport-related processes, while the photochemically produced water vapour plays a relatively smaller role. The increase in water vapour in the presence of the low winter temperatures in the Arctic stratosphere led to more frequent occurrence of ice polar stratospheric clouds (PSCs) in the Arctic vortex. We perform a case study of ice PSC formation focusing on January 2010 when the polar vortex was unusually cold and allowed large-scale formation of PSCs. At the same time a large-scale persistent dehydration was observed. Ice PSCs and dehydration observed at Sodankylä with accurate water vapour soundings in January and February 2010 during the LAPBIAT (Lapland Atmosphere–Biosphere facility) atmospheric measurement campaign were well reproduced by the model. In particular, both the observed and simulated decrease in water vapour in the dehydration layer was up to 1.5 ppm.

Download Full-text

Linking uncertainty in simulated Arctic ozone loss to uncertainties in modelled tropical stratospheric water vapour

Atmospheric Chemistry and Physics ◽

10.5194/acp-18-15047-2018 ◽

2018 ◽

Vol 18 (20) ◽

pp. 15047-15067

Author(s):

Laura Thölix ◽

Alexey Karpechko ◽

Leif Backman ◽

Rigel Kivi

Keyword(s):

Water Vapour ◽

Climate Models ◽

Polar Vortex ◽

The Arctic ◽

Ozone Loss ◽

Tropical Tropopause ◽

Water Vapour Concentration ◽

Vapour Concentration ◽

The Impact ◽

Stratospheric Water Vapour

Abstract. Stratospheric water vapour influences the chemical ozone loss in the polar stratosphere via control of the polar stratospheric cloud formation. The amount of water vapour entering the stratosphere through the tropical tropopause differs substantially between simulations from chemistry–climate models (CCMs). This is because the present-day models, e.g. CCMs, have difficulties in capturing the whole complexity of processes that control the water transport across the tropopause. As a result there are large differences in the stratospheric water vapour between the models. In this study we investigate the sensitivity of simulated Arctic ozone loss to the simulated amount of water vapour that enters the stratosphere through the tropical tropopause. We used a chemical transport model, FinROSE-CTM, forced by ERA-Interim meteorology. The water vapour concentration in the tropical tropopause was varied between 0.5 and 1.6 times the concentration in ERA-Interim, which is similar to the range seen in chemistry–climate models. The water vapour changes in the tropical tropopause led to about 1.5 ppmv less and 2 ppmv more water vapour in the Arctic polar vortex compared to the ERA-Interim, respectively. The change induced in the water vapour concentration in the tropical tropopause region was seen as a nearly one-to-one change in the Arctic polar vortex. We found that the impact of water vapour changes on ozone loss in the Arctic polar vortex depends on the meteorological conditions. The strongest effect was in intermediately cold stratospheric winters, such as the winter of 2013/2014, when added water vapour resulted in 2 %–7 % more ozone loss due to the additional formation of polar stratospheric clouds (PSCs) and associated chlorine activation on their surface, leading to ozone loss. The effect was less pronounced in cold winters such as the 2010/2011 winter because cold conditions persisted long enough for a nearly complete chlorine activation, even in simulations with prescribed stratospheric water vapour amount corresponding to the observed values. In this case addition of water vapour to the stratosphere led to increased areas of ICE PSCs but it did not increase the chlorine activation and ozone destruction significantly. In the warm winter of 2012/2013 the impact of water vapour concentration on ozone loss was small because the ozone loss was mainly NOx-induced. The results show that the simulated water vapour concentration in the tropical tropopause has a significant impact on the Arctic ozone loss and therefore needs to be well simulated in order to improve future projections of the recovery of the ozone layer.

Download Full-text

Record springtime stratospheric ozone depletion at 80°N in 2020

10.5194/egusphere-egu21-8892 ◽

2021 ◽

Author(s):

Ramina Alwarda ◽

Kristof Bognar ◽

Kimberly Strong ◽

Martyn Chipperfield ◽

Sandip Dhomse ◽

...

Keyword(s):

Ozone Depletion ◽

Transport Model ◽

Stratospheric Ozone ◽

Polar Vortex ◽

The Arctic ◽

Optical Absorption Spectroscopy ◽

Chemical Transport Model ◽

Polar Stratospheric Clouds ◽

Ozone Loss ◽

Stratospheric Clouds

The Arctic winter of 2019-2020 was characterized by an unusually persistent polar vortex and temperatures in the lower stratosphere that were consistently below the threshold for the formation of polar stratospheric clouds (PSCs). These conditions led to ozone loss that is comparable to the Antarctic ozone hole. Ground-based measurements from a suite of instruments at the Polar Environment Atmospheric Research Laboratory (PEARL) in Eureka, Canada (80.05&#176;N, 86.42&#176;W) were used to investigate chemical ozone depletion. The vortex was located above Eureka longer than in any previous year in the 20-year dataset and lidar measurements provided evidence of polar stratospheric clouds (PSCs) above Eureka. Additionally, UV-visible zenith-sky Differential Optical Absorption Spectroscopy (DOAS) measurements showed record ozone loss in the 20-year dataset, evidence of denitrification along with the slowest increase of NO2 during spring, as well as enhanced reactive halogen species (OClO and BrO). Complementary measurements of HCl and ClONO2 (chlorine reservoir species) from a Fourier transform infrared (FTIR) spectrometer showed unusually low columns that were comparable to 2011, the previous year with significant chemical ozone depletion. Record low values of HNO3 in the FTIR dataset are in accordance with the evidence of PSCs and a denitrified atmosphere. Estimates of chemical ozone loss were derived using passive ozone from the SLIMCAT offline chemical transport model to account for dynamical contributions to the stratospheric ozone budget.

Download Full-text

Global Hawk dropsonde observations of the Arctic atmosphere obtained during the Winter Storms and Pacific Atmospheric Rivers (WISPAR) field campaign

Atmospheric Measurement Techniques ◽

10.5194/amt-7-3917-2014 ◽

2014 ◽

Vol 7 (11) ◽

pp. 3917-3926 ◽

Cited By ~ 9

Author(s):

J. M. Intrieri ◽

G. de Boer ◽

M. D. Shupe ◽

J. R. Spackman ◽

J. Wang ◽

...

Keyword(s):

Large Scale ◽

Polar Vortex ◽

Unmanned Aircraft ◽

The Arctic ◽

Winter Storms ◽

Field Campaign ◽

Atmospheric Rivers ◽

The North ◽

Aircraft System ◽

Global Hawk

Abstract. In February and March of 2011, the Global Hawk unmanned aircraft system (UAS) was deployed over the Pacific Ocean and the Arctic during the Winter Storms and Pacific Atmospheric Rivers (WISPAR) field campaign. The WISPAR science missions were designed to (1) mprove our understanding of Pacific weather systems and the polar atmosphere; (2) evaluate operational use of unmanned aircraft for investigating these atmospheric events; and (3) demonstrate operational and research applications of a UAS dropsonde system at high latitudes. Dropsondes deployed from the Global Hawk successfully obtained high-resolution profiles of temperature, pressure, humidity, and wind information between the stratosphere and surface. The 35 m wingspan Global Hawk, which can soar for ~ 31 h at altitudes up to ~ 20 km, was remotely operated from NASA's Dryden Flight Research Center at Edwards Air Force Base (AFB) in California. During the 25 h polar flight on 9–10 March 2011, the Global Hawk released 35 sondes between the North Slope of Alaska and 85° N latitude, marking the first UAS Arctic dropsonde mission of its kind. The polar flight transected an unusually cold polar vortex, notable for an associated record-level Arctic ozone loss, and documented polar boundary layer variations over a sizable ocean–ice lead feature. Comparison of dropsonde observations with atmospheric reanalyses reveal that, for this day, large-scale structures such as the polar vortex and air masses are captured by the reanalyses, while smaller-scale features, including low-level jets and inversion depths, are mischaracterized. The successful Arctic dropsonde deployment demonstrates the capability of the Global Hawk to conduct operations in harsh, remote regions. The limited comparison with other measurements and reanalyses highlights the potential value of Arctic atmospheric dropsonde observations where routine in situ measurements are practically nonexistent.

Download Full-text

Multilevel Cloud Structures over Svalbard

Monthly Weather Review ◽

10.1175/mwr-d-16-0214.1 ◽

2017 ◽

Vol 145 (4) ◽

pp. 1149-1159 ◽

Cited By ~ 16

Author(s):

Andreas Dörnbrack ◽

Sonja Gisinger ◽

Michael C. Pitts ◽

Lamont R. Poole ◽

Marion Maturilli

Keyword(s):

Large Scale ◽

Wave Structure ◽

Horizontal Resolution ◽

Temperature Fields ◽

The Arctic ◽

Mountain Waves ◽

Air Masses ◽

Flow Features ◽

Stratospheric Clouds ◽

Lidar Observations

Abstract The presented picture of the month is a superposition of spaceborne lidar observations and high-resolution temperature fields of the ECMWF Integrated Forecast System (IFS). It displays complex tropospheric and stratospheric clouds in the Arctic winter of 2015/16. Near the end of December 2015, the unusual northeastward propagation of warm and humid subtropical air masses as far north as 80°N lifted the tropopause by more than 3 km in 24 h and cooled the stratosphere on a large scale. A widespread formation of thick cirrus clouds near the tropopause and of synoptic-scale polar stratospheric clouds (PSCs) occurred as the temperature dropped below the thresholds for the existence of cloud particles. Additionally, mountain waves were excited by the strong flow at the western edge of the ridge across Svalbard, leading to the formation of mesoscale ice PSCs. The most recent IFS cycle using a horizontal resolution of 8 km globally reproduces the large-scale and mesoscale flow features and leads to a remarkable agreement with the wave structure revealed by the spaceborne observations.

Download Full-text

An Atlantic streamer in stratospheric ozone observations and SD-WACCM simulation data

10.5194/acp-2016-996 ◽

2016 ◽

Author(s):

Klemens Hocke ◽

Franziska Schranz ◽

Eliane Maillard Barras ◽

Lorena Moreira ◽

Niklaus Kämpfer

Keyword(s):

Water Vapour ◽

Central Europe ◽

Large Scale ◽

Surf Zone ◽

Middle Atmosphere ◽

Stratospheric Ozone ◽

Polar Vortex ◽

Transport Processes ◽

Sudden Increase ◽

Nonlinear Transport

Abstract. Observation and simulation of individual ozone streamers are important for the description and understanding of nonlinear transport processes in the middle atmosphere. A sudden increase in mid-stratospheric ozone occurred above Central Europe on December 4, 2015. The GROunbased Millimeter-wave Ozone Spectrometer (GROMOS) and the Stratospheric Ozone MOnitoring RAdiometer (SOMORA) in Switzerland measured an ozone enhancement of about 30 % at 34 km altitude from December 1 to December 4. A similar ozone increase is simulated by the Specified Dynamics-Whole Atmosphere Community Climate (SD-WACCM) model. Further, the global ozone fields at 34 km altitude from SD-WACCM and the satellite experiment Aura/MLS show a remarkable agreement for the location and the timing of an ozone streamer (large-scale tongue like structure) extending from the subtropics in Northern America over the Atlantic to Central Europe. This agreement indicates that SD-WACCM can inform us about the wind inside the Atlantic ozone streamer. SD-WACCM shows an eastward wind of about 100 m/s inside the Atlantic streamer in the mid-stratosphere. SD-WACCM shows that the Atlantic streamer flows along the edge region of the polar vortex. The Atlantic streamer turns southward at an erosion region of the polar vortex located above the Caspian Sea. The spatial distribution of stratospheric water vapour indicates a filament outgoing from this erosion region. The Atlantic streamer, the polar vortex erosion region and the water vapour filament belong to the process of planetary wave breaking in the so-called surf zone of the Northern mid-latitude winter stratosphere.

Download Full-text