scholarly journals Sensitivity of cirrus and mixed-phase clouds to the ice nuclei spectra in McRAS-AC: single column model simulations

2012 ◽  
Vol 12 (6) ◽  
pp. 14927-14957
Author(s):  
R. Morales Betancourt ◽  
D. Lee ◽  
L. Oreopoulos ◽  
Y. C. Sud ◽  
D. Barahona ◽  
...  

Abstract. The salient features of mixed-phase and ice clouds in a GCM cloud scheme are examined using the ice formation parameterizations of Liu and Penner (LP) and Barahona and Nenes (BN). The performance of LP and BN ice nucleation parameterizations were assessed in the GEOS-5 AGCM using the McRAS-AC cloud microphysics framework in single column mode. Four dimensional assimilated data from the intensive observation period of ARM TWP-ICE campaign was used to drive the fluxes and lateral forcing. Simulation experiments where established to test the impact of each parameterization in the resulting cloud fields. Three commonly used IN spectra were utilized in the BN parameterization to described the availability of IN for heterogeneous ice nucleation. The results show large similarities in the cirrus cloud regime between all the schemes tested, in which ice crystal concentrations were within a factor of 10 regardless of the parameterization used. In mixed-phase clouds there are some persistent differences in cloud particle number concentration and size, as well as in cloud fraction, ice water mixing ratio, and ice water path. Contact freezing in the simulated mixed-phase clouds contributed to transfer liquid to ice efficiently, so that on average, the clouds were fully glaciated at T~260 K, irrespective of the ice nucleation parameterization used. Comparison of simulated ice water path to available satellite derived observations were also performed, finding that all the schemes tested with the BN parameterization predicted average values of IWP within ±15% of the observations.

2012 ◽  
Vol 12 (22) ◽  
pp. 10679-10692 ◽  
Author(s):  
R. Morales Betancourt ◽  
D. Lee ◽  
L. Oreopoulos ◽  
Y. C. Sud ◽  
D. Barahona ◽  
...  

Abstract. The salient features of mixed-phase and ice clouds in a GCM cloud scheme are examined using the ice nucleation parameterizations of Liu and Penner (LP) and Barahona and Nenes (BN). The performance of both parameterizations was assessed in the GEOS-5 AGCM using the McRAS-AC cloud microphysics framework in single column mode. Four dimensional assimilated data from the intensive observation period of ARM TWP-ICE campaign was used to drive the fluxes and lateral forcing. Simulation experiments were established to test the impact of each parameterization in the resulting cloud fields. Three commonly used IN spectra were utilized in the BN parameterization to describe the availability of IN for heterogeneous ice nucleation. The results showed large similarities in the cirrus cloud regime between all the schemes tested, in which ice crystal concentrations were within a factor of 10 regardless of the parameterization used. In mixed-phase clouds there were some persistent differences in cloud particle number concentration and size, as well as in cloud fraction, ice water mixing ratio, and ice water path. Contact freezing in the simulated mixed-phase clouds contributed to the effective transfer of liquid to ice, so that on average, the clouds were fully glaciated at T 260 K, irrespective of the ice nucleation parameterization used. Comparison of simulated ice water path to available satellite derived observations were also performed, finding that all the schemes tested with the BN parameterization predicted average values of IWP within ±15% of the observations.


2006 ◽  
Vol 63 (3) ◽  
pp. 968-982 ◽  
Author(s):  
U. Lohmann ◽  
K. Diehl

Abstract New parameterizations of contact freezing and immersion freezing in stratiform mixed-phase clouds (with temperatures between 0° and −35°C) for black carbon and mineral dust assumed to be composed of either kaolinite (simulation KAO) or montmorillonite (simulation MON) are introduced into the ECHAM4 general circulation model. The effectiveness of black carbon and dust as ice nuclei as a function of temperature is parameterized from a compilation of laboratory studies. This is the first time that freezing parameterizations take the chemical composition of ice nuclei into account. The rather subtle differences between these sensitivity simulations in the present-day climate have significant implications for the anthropogenic indirect aerosol effect. The decrease in net radiation in these sensitivity simulations at the top of the atmosphere varies from 1 ± 0.3 to 2.1 ± 0.1 W m−2 depending on whether dust is assumed to be composed of kaolinite or montmorillonite. In simulation KAO, black carbon has a higher relevancy as an ice nucleus than in simulation MON, because kaolinite is not freezing as effectively as montmorillonite. In simulation KAO, the addition of anthropogenic aerosols results in a larger ice water path, a slightly higher precipitation rate, and a reduced total cloud cover. On the contrary, in simulation MON the increase in ice water path is much smaller and globally the decrease in precipitation is dominated by the reduction in warm-phase precipitation due to the indirect cloud lifetime effect.


2015 ◽  
Vol 54 (8) ◽  
pp. 1809-1825 ◽  
Author(s):  
Yaodeng Chen ◽  
Hongli Wang ◽  
Jinzhong Min ◽  
Xiang-Yu Huang ◽  
Patrick Minnis ◽  
...  

AbstractAnalysis of the cloud components in numerical weather prediction models using advanced data assimilation techniques has been a prime topic in recent years. In this research, the variational data assimilation (DA) system for the Weather Research and Forecasting (WRF) Model (WRFDA) is further developed to assimilate satellite cloud products that will produce the cloud liquid water and ice water analysis. Observation operators for the cloud liquid water path and cloud ice water path are developed and incorporated into the WRFDA system. The updated system is tested by assimilating cloud liquid water path and cloud ice water path observations from Global Geostationary Gridded Cloud Products at NASA. To assess the impact of cloud liquid/ice water path data assimilation on short-term regional numerical weather prediction (NWP), 3-hourly cycling data assimilation and forecast experiments with and without the use of the cloud liquid/ice water paths are conducted. It is shown that assimilating cloud liquid/ice water paths increases the accuracy of temperature, humidity, and wind analyses at model levels between 300 and 150 hPa after 5 cycles (15 h). It is also shown that assimilating cloud liquid/ice water paths significantly reduces forecast errors in temperature and wind at model levels between 300 and 150 hPa. The precipitation forecast skills are improved as well. One reason that leads to the improved analysis and forecast is that the 3-hourly rapid update cycle carries over the impact of cloud information from the previous cycles spun up by the WRF Model.


2020 ◽  
Vol 20 (6) ◽  
pp. 3459-3481 ◽  
Author(s):  
Rosa Gierens ◽  
Stefan Kneifel ◽  
Matthew D. Shupe ◽  
Kerstin Ebell ◽  
Marion Maturilli ◽  
...  

Abstract. Low-level mixed-phase clouds (MPCs) are common in the Arctic. Both local and large-scale phenomena influence the properties and lifetime of MPCs. Arctic fjords are characterized by complex terrain and large variations in surface properties. Yet, not many studies have investigated the impact of local boundary layer dynamics and their relative importance on MPCs in the fjord environment. In this work, we used a combination of ground-based remote sensing instruments, surface meteorological observations, radiosoundings, and reanalysis data to study persistent low-level MPCs at Ny-Ålesund, Svalbard, for a 2.5-year period. Methods to identify the cloud regime, surface coupling, and regional and local wind patterns were developed. We found that persistent low-level MPCs were most common with westerly winds, and the westerly clouds had a higher mean liquid (42 g m−2) and ice water path (16 g m−2) compared to those with easterly winds. The increased height and rarity of persistent MPCs with easterly free-tropospheric winds suggest the island and its orography have an influence on the studied clouds. Seasonal variation in the liquid water path was found to be minimal, although the occurrence of persistent MPCs, their height, and their ice water path all showed notable seasonal dependency. Most of the studied MPCs were decoupled from the surface (63 %–82 % of the time). The coupled clouds had 41 % higher liquid water path than the fully decoupled ones. Local winds in the fjord were related to the frequency of surface coupling, and we propose that katabatic winds from the glaciers in the vicinity of the station may cause clouds to decouple. We concluded that while the regional to large-scale wind direction was important for the persistent MPC occurrence and properties, the local-scale phenomena (local wind patterns in the fjord and surface coupling) also had an influence. Moreover, this suggests that local boundary layer processes should be described in models in order to present low-level MPC properties accurately.


2014 ◽  
Vol 14 (21) ◽  
pp. 28845-28883
Author(s):  
N. S. Umo ◽  
B. J. Murray ◽  
M. T. Baeza-Romero ◽  
J. M. Jones ◽  
A. R. Lea-Langton ◽  
...  

Abstract. Ice nucleating particles can modify cloud properties with implications for climate and the hydrological cycle; hence, it is important to understand which aerosol particle types nucleate ice and how efficiently they do so. It has been shown that aerosol particles such as natural dusts, volcanic ash, bacteria and pollen can act as ice nucleating particles, but the ice nucleating ability of combustion ashes has not been studied. Combustion ashes are major by-products released during the combustion of solid fuels and a significant amount of these ashes are emitted into the atmosphere either during combustion or via aerosolization of bottom ashes. Here, we show that combustion ashes (coal fly ash, wood bottom ash, domestic bottom ash, and coal bottom ash) nucleate ice in the immersion mode at conditions relevant to mixed-phase clouds. Hence, combustion ashes could play an important role in primary ice formation in mixed-phase clouds, especially in clouds that are formed near the emission source of these aerosol particles. In order to quantitatively assess the impact of combustion ashes on mixed-phase clouds, we propose that the atmospheric abundance of combustion ashes should be quantified since up to now they have mostly been classified together with mineral dust particles. Also, in reporting ice residue compositions, a distinction should be made between natural mineral dusts and combustion ashes in order to quantify the contribution of combustion ashes to atmospheric ice nucleation.


2018 ◽  
Vol 18 (18) ◽  
pp. 13345-13361 ◽  
Author(s):  
Matthew S. Norgren ◽  
Gijs de Boer ◽  
Matthew D. Shupe

Abstract. The interactions that occur between aerosols and a mixed-phase cloud system, and the subsequent alteration of the microphysical state of such clouds, are a problem that has yet to be well constrained. Advancing our understanding of aerosol–ice processes is necessary to determine the impact of natural and anthropogenic emissions on Earth's climate and to improve our capability to predict future climate states. This paper deals specifically with how aerosols influence ice mass production in low-level Arctic mixed-phase clouds. In this study, a 9-year record of aerosol, cloud and atmospheric state properties is used to quantify aerosol influence on ice production in mixed-phase clouds. It is found that mixed-phase clouds present in a clean aerosol state have higher ice water content (IWC) by a factor of 1.22 to 1.63 at cloud base than do similar clouds in cases with higher aerosol loading. We additionally analyze radar-derived mean Doppler velocities to better understand the drivers behind this relationship, and we conclude that aerosol induced reduction of the ice crystal nucleation rate, together with decreased riming rates in polluted clouds, are likely influences on the observed reductions in IWC.


2013 ◽  
Vol 6 (5) ◽  
pp. 8187-8233 ◽  
Author(s):  
J. Gong ◽  
D. L. Wu

Abstract. Ice water path (IWP) and cloud top height (ht) are two of the key variables to determine cloud radiative and thermodynamical properties in the climate models. Large uncertainty remains among IWP measurements from satellite sensors, in large part due to the assumptions made for cloud microphysics in these retrievals. In this study, we develop a fast algorithm to retrieve IWP from the 157, 183.3 ± 3 and 190.3 GHz radiances of Microwave Humidity Sounder (MHS) such that the MHS cloud ice retrieval is consistent with CloudSat IWP measurements. This retrieval is obtained by constraining the forward models between collocated-and-coincident measurements of CloudSat IWP and MHS cloud-induced radiance depression (Tcir) at these channels. The empirical forward model is represented by a look-up-table (LUT) of Tcir–IWP relationships as a function of ht and frequency channel. With ht simultaneously retrieved, the IWP is found to be more accurate. The useful range of the MHS IWP retrieval is between 0.5 and 10 kg m−2, and agrees well with CloudSat in terms of normalized probability density function (PDF). Compared to the empirical model, current radiative transfer models (RTMs) still have significant uncertainties in characterizing the observed Tcir–IWP relationships. Therefore, the empirical LUT method developed here remains as an effective approach to retrieving ice cloud properties from the MHS-like microwave channels.


2015 ◽  
Vol 15 (9) ◽  
pp. 5195-5210 ◽  
Author(s):  
N. S. Umo ◽  
B. J. Murray ◽  
M. T. Baeza-Romero ◽  
J. M. Jones ◽  
A. R. Lea-Langton ◽  
...  

Abstract. Ice-nucleating particles can modify cloud properties with implications for climate and the hydrological cycle; hence, it is important to understand which aerosol particle types nucleate ice and how efficiently they do so. It has been shown that aerosol particles such as natural dusts, volcanic ash, bacteria and pollen can act as ice-nucleating particles, but the ice-nucleating ability of combustion ashes has not been studied. Combustion ashes are major by-products released during the combustion of solid fuels and a significant amount of these ashes are emitted into the atmosphere either during combustion or via aerosolization of bottom ashes. Here, we show that combustion ashes (coal fly ash, wood bottom ash, domestic bottom ash, and coal bottom ash) nucleate ice in the immersion mode at conditions relevant to mixed-phase clouds. Hence, combustion ashes could play an important role in primary ice formation in mixed-phase clouds, especially in clouds that are formed near the emission source of these aerosol particles. In order to quantitatively assess the impact of combustion ashes on mixed-phase clouds, we propose that the atmospheric abundance of combustion ashes should be quantified since up to now they have mostly been classified together with mineral dust particles. Also, in reporting ice residue compositions, a distinction should be made between natural mineral dusts and combustion ashes in order to quantify the contribution of combustion ashes to atmospheric ice nucleation.


2020 ◽  
Author(s):  
Junghwa Lee ◽  
Patric Seifert ◽  
Tempei Hashino ◽  
Roland Schrödner ◽  
Michael Weger ◽  
...  

<p>Ice- and mixed-phase clouds largely contribute to global precipitation due to their high spatiotemporal coverage. It has been highlighted that aerosol-cloud interaction is a critical factor. However, our current understanding of the complexity of their microphysical properties is still rather limited.  </p><p>In this talk, we will discuss the impact of perturbations of the cloud condensation nuclei (CCN) and ice-nucleating particle (INP) on the structure and composition of mixed-phase clouds. The main methods are ground-based observations (i.e., Ka-band polarimetric cloud radar) as well as the spectral-bin microphysical methodology called AMPS (Advanced Microphysics Prediction System). Until now, significant efforts have been underway to improve microphysical processes in AMPS, such as the schemes for immersion freezing and habit prediction. Despite these endeavors, it is still challenging using modeling alone to resolve such complexity of microphysical processes due to many parameterizations and assumptions. In particular, the ice habit prediction system in AMPS is sensitive to the 3-D Eulerian advection scheme. Meanwhile, the Doppler-spectra derived from polarimetric cloud radar enables us to retrieve the hydrometeor habit of the significant signal peak in the Doppler spectrum of mixed-phase clouds. The synergy between the above mentioned advanced modeling approach and state-of-the-art observation techniques are in our study used to evaluate the effects of the CCN and INP perturbations on mixed-phase clouds. </p><p>The steps are as follows. First of all, we will present the evaluation of a case study of a mixed-phase cloud by observation data. In the course of the work, AMPS is coupled with the German weather prediction system COSMO (Consortium for Small-scale Modeling) model. We choose an observation dataset from the ACCEPT (Analysis of the Composition of Clouds with Extended Polarization Techniques) field campaign in Cabauw, Netherlands, which was conducted during fall 2014. Also, we use the radar forward operator CR-SIM (Cloud Resolving Model Radar Simulator) that translates the dataset of simulation output into radar variables. Therefore, we will present direct comparisons between ground-based observation and modeling datasets. In the next step, AMPS is coupled with a simple 1-D dynamic core KiD (Kinematic Driver for microphysics intercomparison), so-called KiD-AMPS. In doing so, we will discuss the comparison with other schemes (i.e., Morrison 2-moment). Finally, in the frame of KiD-AMPS, we will debate the impact of the CCN and INP perturbations on mixed-phase clouds. </p>


2013 ◽  
Vol 52 (11) ◽  
pp. 2582-2599 ◽  
Author(s):  
Anne Garnier ◽  
Jacques Pelon ◽  
Philippe Dubuisson ◽  
Ping Yang ◽  
Michaël Faivre ◽  
...  

AbstractThis paper describes the version-3 level-2 operational analysis of the Imaging Infrared Radiometer (IIR) data collected in the framework of the Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) mission to retrieve cirrus cloud effective diameter and ice water path in synergy with the Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) collocated observations. The analysis uses a multisensor split-window technique relying on the concept of microphysical index applied to the two pairs of channels (12.05, 10.6 μm) and (12.05, 8.65 μm) to retrieve cirrus microphysical properties (effective diameter, ice water path) at 1-km pixel resolution. Retrievals are performed for three crystal families selected from precomputed lookup tables identified as representative of the main relationships between the microphysical indices. The uncertainties in the microphysical indices are detailed and quantified, and the impact on the retrievals is simulated. The possible biases have been assessed through consistency checks that are based on effective emissivity difference. It has been shown that particle effective diameters of single-layered cirrus clouds can be retrieved, for the first time, down to effective emissivities close to 0.05 when accurate measured background radiances can be used and up to 0.95 over ocean and land, as well as over low opaque clouds. The retrieval of the ice water path from the IIR effective optical depth and the effective diameter is discussed. Taking advantage of the cloud boundaries retrieved by CALIOP, an IIR power-law relationship between ice water content and extinction is established for four temperature ranges and shown to be consistent with previous results on average for the chosen dataset.


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