scholarly journals Chemistry-climate model SOCOL: a validation of the present-day climatology

2005 ◽  
Vol 5 (1) ◽  
pp. 509-555 ◽  
Author(s):  
T. Egorova ◽  
E. Rozanov ◽  
V. Zubov ◽  
E. Manzini ◽  
W. Schmutz ◽  
...  

Abstract. In this paper we document ''SOCOL'', a new chemistry-climate model, which has been ported for regular PCs and shows good wall-clock performance. An extensive validation of the model results against present-day climate obtained from observations and assimilation data sets shows that the model describes the climatological state of the atmosphere for the late 1990s with reasonable accuracy. The model has a significant temperature bias only in the upper stratosphere and near the tropopause in the tropics and high latitudes. The latter is the result of the rather low vertical resolution of the model near the tropopause. The former can be attributed to a crude representation of the radiation heating in the middle atmosphere. A comparison of the simulated and observed link between the tropical stratospheric structure and the strength of the polar vortex shows that in general, both observations and simulations reveal a higher temperature and ozone mixing ratio in the lower tropical stratosphere for the case with stronger Polar night jet (PNJ) as predicted by theoretical studies.

2005 ◽  
Vol 5 (6) ◽  
pp. 1557-1576 ◽  
Author(s):  
T. Egorova ◽  
E. Rozanov ◽  
V. Zubov ◽  
E. Manzini ◽  
W. Schmutz ◽  
...  

Abstract. In this paper we document "SOCOL", a new chemistry-climate model, which has been ported for regular PCs and shows good wall-clock performance. An extensive validation of the model results against present-day climate data obtained from observations and assimilation data sets shows that the model describes the climatological state of the atmosphere for the late 1990s with reasonable accuracy. The model has a significant temperature bias only in the upper stratosphere and near the tropopause at high latitudes. The latter is the result of the rather low vertical resolution of the model near the tropopause. The former can be attributed to a crude representation of radiation heating in the middle atmosphere. A comparison of the simulated and observed link between the tropical stratospheric structure and the strength of the polar vortex shows that in general, both observations and simulations reveal a higher temperature and ozone mixing ratio in the lower tropical stratosphere for the case with stronger Polar night jet (PNJ) and slower Brewer-Dobson circulation as predicted by theoretical studies.


2008 ◽  
Vol 8 (21) ◽  
pp. 6505-6525 ◽  
Author(s):  
H. J. Punge ◽  
M. A. Giorgetta

Abstract. The quasi-biennial oscillation (QBO) of zonal wind is a prominent mode of variability in the tropical stratosphere. It affects not only the meridional circulation and temperature over a wide latitude range but also the transport and chemistry of trace gases such as ozone. Compared to a QBO less circulation, the long-term climatological means of these quantities are also different. These climatological net effects of the QBO can be studied in general circulation models that extend into the middle atmosphere and have a chemistry and transport component, so-called Chemistry Climate Models (CCMs). In this work we show that the CCM MAECHAM4-CHEM can reproduce the observed QBO variations in temperature and ozone mole fractions when nudged towards observed winds. In particular, it is shown that the QBO signal in transport of nitrogen oxides NOx plays an important role in reproducing the observed ozone QBO, which features a phase reversal slightly below the level of maximum of the ozone mole fraction in the tropics. We then compare two 20-year experiments with the MAECHAM4-CHEM model that differ by including or not including the QBO. The mean wind fields differ between the two model runs, especially during summer and fall seasons in both hemispheres. The differences in the wind field lead to differences in the meridional circulation, by the same mechanism that causes the QBO's secondary meridional circulation, and thereby affect mean temperatures and the mean transport of tracers. In the tropics, the net effect on ozone is mostly due to net differences in upwelling and, higher up, the associated temperature change. We show that a net surplus of up to 15% in NOx in the tropics above 10 hPa in the experiment that includes the QBO does not lead to significantly different volume mixing ratios of ozone. We also note a slight increase in the southern vortex strength as well as earlier vortex formation in northern winter. Polar temperatures differ accordingly. Differences in the strength of the Brewer-Dobson circulation and in further trace gas concentrations are analysed. Our findings underline the importance of a representation of the QBO in CCMs.


2013 ◽  
Vol 26 (6) ◽  
pp. 2096-2116 ◽  
Author(s):  
Peter Hitchcock ◽  
Theodore G. Shepherd ◽  
Gloria L. Manney

Abstract A novel diagnostic tool is presented, based on polar-cap temperature anomalies, for visualizing daily variability of the Arctic stratospheric polar vortex over multiple decades. This visualization illustrates the ubiquity of extended-time-scale recoveries from stratospheric sudden warmings, termed here polar-night jet oscillation (PJO) events. These are characterized by an anomalously warm polar lower stratosphere that persists for several months. Following the initial warming, a cold anomaly forms in the middle stratosphere, as does an anomalously high stratopause, both of which descend while the lower-stratospheric anomaly persists. These events are characterized in four datasets: Microwave Limb Sounder (MLS) temperature observations; the 40-yr ECMWF Re-Analysis (ERA-40) and Modern Era Retrospective Analysis for Research and Applications (MERRA) reanalyses; and an ensemble of three 150-yr simulations from the Canadian Middle Atmosphere Model. The statistics of PJO events in the model are found to agree very closely with those of the observations and reanalyses. The time scale for the recovery of the polar vortex following sudden warmings correlates strongly with the depth to which the warming initially descends. PJO events occur following roughly half of all major sudden warmings and are associated with an extended period of suppressed wave-activity fluxes entering the polar vortex. They follow vortex splits more frequently than they do vortex displacements. They are also related to weak vortex events as identified by the northern annular mode; in particular, those weak vortex events followed by a PJO event show a stronger tropospheric response. The long time scales, predominantly radiative dynamics, and tropospheric influence of PJO events suggest that they represent an important source of conditional skill in seasonal forecasting.


2009 ◽  
Vol 9 (1) ◽  
pp. 1977-2020
Author(s):  
F. Khosrawi ◽  
R. Müller ◽  
M. H. Proffitt ◽  
R. Ruhnke ◽  
O. Kirner ◽  
...  

Abstract. 1-year data sets of monthly averaged nitrous oxide (N2O) and ozone (O3) derived from satellite measurements were used as a tool for the evaluation of atmospheric photochemical models. Two 1-year data sets, one derived from the Improved Limb Atmospheric Spectrometer (ILAS and ILAS-II) and one from the Odin Sub-Millimetre Radiometer (Odin/SMR) were employed. Here, these data sets are used for the evaluation of two Chemical Transport Models (CTMs), the Karlsruhe Simulation Model of the Middle Atmosphere (KASIMA) and the Chemical Lagrangian Model of the Stratosphere (CLaMS) as well as for one Chemistry-Climate Model (CCM), the atmospheric chemistry general circulation model ECHAM5/MESSy1 (E5M1) in the lower stratosphere with focus on the Northern Hemisphere. Since the Odin/SMR measurements cover the entire hemisphere, the evaluation is performed for the entire hemisphere as well as for the low latitudes, midlatitudes and high latitudes using the Odin/SMR 1-year data set as reference. To assess the impact of using different data sets for such an evaluation study we repeat the evaluation for the polar lower stratosphere using the ILAS/ILAS-II data set. Only small differences were found using ILAS/ILAS-II instead of Odin/SMR as a reference, thus, showing that the results are not influenced by the particular satellite data set used for the evaluation. The evaluation of CLaMS, KASIMA and E5M1 shows that all models are in good agreement with Odin/SMR and ILAS/ILAS-II. Differences are generally in the range of ±20%. Larger differences (up to −40%) are found in all models at 500±25 K for N2O mixing ratios greater than 200 ppb. Generally, the largest differences were found for the tropics and the lowest for the polar regions. However, an underestimation of polar winter ozone loss was found both in KASIMA and E5M1 both in the Northern and Southern Hemisphere.


2008 ◽  
Vol 8 (3) ◽  
pp. 12115-12162 ◽  
Author(s):  
H. J. Punge ◽  
M. A. Giorgetta

Abstract. The quasi-biennial oscillation (QBO) of zonal wind is a prominent mode of variability in the tropical stratosphere. It affects not only the meridional circulation and temperature over a wide latitude range but also the transport and chemistry of trace gases such as ozone. Compared to a QBO less circulation, the long-term climatological means of these quantities are also different. These climatological net effects of the QBO can be studied in general circulation models that extend into the middle atmosphere and have a chemistry and transport component, so-called Chemistry Climate Models (CCMs). In this work we show that the CCM MAECHAM4-CHEM can reproduce the observed QBO variations in temperature and ozone mole fractions when nudged towards observed winds. In particular, it is shown that the QBO signal in transport of nitrogen oxides NOx plays an important role in reproducing the observed ozone QBO, which features a phase reversal slightly below the maximum of the ozone mole fraction in the tropics. We then compare two 20-year experiments with the MAECHAM4-CHEM model that differ by including or not including the QBO. The mean wind fields differ between the two model runs, especially during summer and fall on both hemispheres. The differences in the wind field lead to differences in the meridional circulation, by the same mechanism that causes the QBO's secondary meridional circulation, and thereby affecting mean temperatures and the mean transport of tracers. In the tropics, the net effect on ozone is mostly due to net differences in upwelling and, higher up, the associated temperature change. We show that a net surplus of up to 15% in NOx in the tropics above 10 hPa in the experiment that includes the QBO does not lead to significantly different volume mixing ratios of ozone. We also note a slight increase in the southern vortex strength as well as earlier vortex formation in northern winter. Polar temperatures differ accordingly. Differences in the strength of the Brewer-Dobson circulation and in further trace gas concentrations are analysed. Our findings underline the importance of a representation of the QBO in CCMs.


2010 ◽  
Vol 10 (10) ◽  
pp. 24853-24917 ◽  
Author(s):  
K. Semeniuk ◽  
V. I. Fomichev ◽  
J. C. McConnell ◽  
C. Fu ◽  
S. M. L. Melo ◽  
...  

Abstract. The impact of NOx and HOx production by three types of energetic particle precipitation (EPP), aurora, solar proton events and galactic cosmic rays is examined using a chemistry climate model. Ensemble simulations forced by transient EPP derived from observations with one-year repeating sea surface temperatures and fixed chemical boundary conditions were conducted for cases with and without solar cycle in irradiance. Our model results show a wintertime polar stratosphere ozone reduction of between 3 and 10% in agreement with previous studies. EPP is found to modulate the radiative solar cycle effect in the middle atmosphere in a significant way, bringing temperature and ozone variations closer to observed patterns. The Southern Hemisphere polar vortex undergoes an intensification from solar minimum to solar maximum instead of a weakening. This changes the solar cycle variation of the Brewer-Dobson circulation, with a weakening during solar maxima compared to solar minima. In response, the tropical tropopause temperature manifests a statistically significant solar cycle variation resulting in about 4% more water vapour transported into the lower tropical stratosphere during solar maxima compared to solar minima. This has implications for surface temperature variation due to the associated change in radiative forcing.


2020 ◽  
Author(s):  
Markus Kunze ◽  
Tim Kruschke ◽  
Ulrike Langematz ◽  
Miriam Sinnhuber ◽  
Thomas Reddmann ◽  
...  

Abstract. Variations of the solar spectral irradiance (SSI) with the 11-year sunspot cycle have been shown to have a significant impact on temperatures and the mixing ratios of atmospheric constituents in the stratosphere and mesosphere. Uncertainties in modelling the effects of SSI variations arise from uncertainties in the empirical models reconstructing the prescribed SSI data set as well as from uncertainties in the chemistry-climate model (CCM) formulation. In this study CCM simulations with the ECHAM MESSy Atmospheric Chemistry (EMAC) model and the Community Earth System Model 1 (CESM1) – Whole Atmosphere Chemistry Climate Model (WACCM) have been performed to quantify the uncertainties of the solar responses in chemistry and dynamics that are due to the usage of five different SSI data sets or the two CCMs. We apply a two-way analysis of variance (ANOVA) to separate the influence of the SSI data sets and the CCMs on the variability of the solar response in shortwave heating rates, temperature and ozone. The ANOVA identifies the SSI data set with the strongest influence on the variability of the solar signal in shortwave heating rates in the upper mesosphere and in the upper stratosphere/lower mesosphere. The strongest influence on the variability of the solar signal in ozone and temperature is identified in the upper stratosphere/lower mesosphere. The largest influence of the CCMs on variability of the solar responses can be identified in the upper mesosphere. The solar response in the lower stratosphere also depends on the CCM used, especially in the tropics and northern hemispheric subtropics and mid latitudes, where the model dynamics modulate the solar responses.


2019 ◽  
Vol 19 (14) ◽  
pp. 9485-9494 ◽  
Author(s):  
Pavle Arsenovic ◽  
Alessandro Damiani ◽  
Eugene Rozanov ◽  
Bernd Funke ◽  
Andrea Stenke ◽  
...  

Abstract. Energetic particle precipitation (EPP) affects the chemistry of the polar middle atmosphere by producing reactive nitrogen (NOy) and hydrogen (HOx) species, which then catalytically destroy ozone. Recently, there have been major advances in constraining these particle impacts through a parametrization of NOy based on high-quality observations. Here we investigate the effects of low (auroral) and middle (radiation belt) energy range electrons, separately and in combination, on reactive nitrogen and hydrogen species as well as on ozone during Southern Hemisphere winters from 2002 to 2010 using the SOCOL3-MPIOM chemistry-climate model. Our results show that, in the absence of solar proton events, low-energy electrons produce the majority of NOy in the polar mesosphere and stratosphere. In the polar vortex, NOy subsides and affects ozone at lower altitudes, down to 10 hPa. Comparing a year with high electron precipitation with a quiescent period, we found large ozone depletion in the mesosphere; as the anomaly propagates downward, 15 % less ozone is found in the stratosphere during winter, which is confirmed by satellite observations. Only with both low- and middle-energy electrons does our model reproduce the observed stratospheric ozone anomaly.


2009 ◽  
Vol 9 (9) ◽  
pp. 3001-3009 ◽  
Author(s):  
M. A. Thomas ◽  
M. A. Giorgetta ◽  
C. Timmreck ◽  
H.-F. Graf ◽  
G. Stenchikov

Abstract. The sensitivity of the climate impact of Mt. Pinatubo eruption in the tropics and extratropics to different QBO phases is investigated. Mt. Pinatubo erupted in June 1991 during the easterly phase of the QBO at 30 hPa and the phase change to westerly took place in August 1992. Here, the consequences are analyzed if the QBO phase had been in the opposite phase during the eruption of Mt. Pinatubo. Hence, in this study, simulations are carried out using the middle atmosphere configuration of ECHAM5 general circulation model for two cases – one with the observed QBO phase and the other with the opposite QBO phase. The response of temperature and geopotential height in the lower stratosphere is evaluated for the following cases – (1) when only the effects of the QBO are included and (2) when the effects of aerosols, QBO and SSTs (combined response) are included. The tropical QBO signature in the lower stratospheric temperature is well captured in the pure QBO responses and in the combined (aerosol + ocean + QBO) responses. The response of the extratropical atmosphere to the QBO during the second winter after the eruption is captured realistically in the case of the combined forcing showing a strengthening of the polar vortex when the QBO is in its westerly phase and a warm, weak polar vortex in the easterly QBO phase. The vortex is disturbed during the first winter irrespective of the QBO phases in the combined responses and this may be due to the strong influences of El Niño during the first winters after eruption. However, the pure QBO experiments do not realistically reproduce a strengthening of the polar vortex in the westerly QBO phase, even though below normal temperatures in the high latitudes are seen in October-November-December months when the opposite QBO phase is prescribed instead of the December-January-February winter months used here for averaging.


2015 ◽  
Vol 15 (12) ◽  
pp. 6879-6895 ◽  
Author(s):  
A. Kuchar ◽  
P. Sacha ◽  
J. Miksovsky ◽  
P. Pisoft

Abstract. This study focusses on the variability of temperature, ozone and circulation characteristics in the stratosphere and lower mesosphere with regard to the influence of the 11-year solar cycle. It is based on attribution analysis using multiple nonlinear techniques (support vector regression, neural networks) besides the multiple linear regression approach. The analysis was applied to several current reanalysis data sets for the 1979–2013 period, including MERRA, ERA-Interim and JRA-55, with the aim to compare how these types of data resolve especially the double-peaked solar response in temperature and ozone variables and the consequent changes induced by these anomalies. Equatorial temperature signals in the tropical stratosphere were found to be in qualitative agreement with previous attribution studies, although the agreement with observational results was incomplete, especially for JRA-55. The analysis also pointed to the solar signal in the ozone data sets (i.e. MERRA and ERA-Interim) not being consistent with the observed double-peaked ozone anomaly extracted from satellite measurements. The results obtained by linear regression were confirmed by the nonlinear approach through all data sets, suggesting that linear regression is a relevant tool to sufficiently resolve the solar signal in the middle atmosphere. The seasonal evolution of the solar response was also discussed in terms of dynamical causalities in the winter hemispheres. The hypothetical mechanism of a weaker Brewer–Dobson circulation at solar maxima was reviewed together with a discussion of polar vortex behaviour.


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