scholarly journals AerGOM, an improved algorithm for stratospheric aerosol extinction retrieval from GOMOS observations – Part 2: Intercomparisons

2016 ◽  
Vol 9 (9) ◽  
pp. 4701-4718 ◽  
Author(s):  
Charles Étienne Robert ◽  
Christine Bingen ◽  
Filip Vanhellemont ◽  
Nina Mateshvili ◽  
Emmanuel Dekemper ◽  
...  
Keyword(s):  
Zenith Angle ◽  
Solar Zenith Angle ◽  
Stratospheric Aerosol ◽  
Cirrus Clouds ◽  
Apparent Temperature ◽  
Retrieval Algorithm ◽  
Aerosol Extinction ◽  
Extinction Coefficients ◽  
Wide Range

Abstract. AerGOM is a retrieval algorithm developed for the GOMOS instrument onboard Envisat as an alternative to the operational retrieval (IPF). AerGOM enhances the quality of the stratospheric aerosol extinction retrieval due to the extension of the spectral range used, refines the aerosol spectral parameterization, the simultaneous inversion of all atmospheric species as well as an improvement of the Rayleigh scattering correction. The retrieval algorithm allows for a good characterization of the stratospheric aerosol extinction for a wide range of wavelengths.In this work, we present the results of stratospheric aerosol extinction comparisons between AerGOM and various spaceborne instruments (SAGE II, SAGE III, POAM III, ACE-MAESTRO and OSIRIS) for different wavelengths. The aerosol extinction intercomparisons for λ < 700 nm and above 20 km show agreements with SAGE II version 7 and SAGE III version 4.0 within ±15 % and ±45 %, respectively. There is a strong positive bias below 20 km at λ < 700 nm, which suggests that cirrus clouds at these altitudes have a large impact on the extinction values. Comparisons performed with GOMOS IPF v6.01 alongside AerGOM show that at short wavelengths and altitudes below 20 km, IPF retrievals are more accurate when evaluated against SAGE II and SAGE III but are much less precise than AerGOM. A modified aerosol spectral parameterization can improve AerGOM in this spectral and altitude range and leads to results that have an accuracy similar to IPF retrievals. Comparisons of AerGOM aerosol extinction coefficients with OSIRIS and SAGE III measurements at wavelengths larger than 700 nm show a very large negative bias at altitudes above 25 km. Therefore, the use of AerGOM aerosol extinction data is not recommended for λ > 700 nm.Due to the unique observational technique of GOMOS, some of the results appear to be dependent on the star occultation parameters such as star apparent temperature and magnitude, solar zenith angle and latitude of observation. A systematic analysis is carried out to identify biases in the dataset, using the various spaceborne instruments as references. The quality of the aerosol retrieval is mainly influenced by the star magnitude, as well as star temperature to a lesser degree. To ensure good-quality profiles, we suggest to select occultations performed with star magnitude M < 2.5 and star temperature T > 6 × 103 K. Stray-light contamination is negligible for extinction coefficients below 700 nm using occultations performed with a solar zenith angle  > 110° but becomes important at larger wavelengths. Comparison of AerGOM results in the tropics shows an enhanced bias below 20 km that seem to confirm cirrus clouds as its cause. There are also differences between mid-latitude and tropical observations that cannot yet be explained, with a bias difference of up to 25 %.This bias characterization is extremely important for data users and might prove valuable for the production of unbiased long-term merged dataset.

scholarly journals AerGOM, an improved algorithm for stratospheric aerosol retrieval from GOMOS observations. Part 2: Intercomparisons

2016 ◽  
Author(s):  
Charles Étienne Robert ◽  
Christine Bingen ◽  
Filip Vanhellemont ◽  
Nina Mateshvili ◽  
Emmanuel Dekemper ◽  
...  
Keyword(s):  
Rayleigh Scattering ◽  
Stratospheric Aerosol ◽  
Apparent Temperature ◽  
Retrieval Algorithm ◽  
Aerosol Extinction ◽  
Systematic Analysis ◽  
Simultaneous Inversion ◽  
Atmospheric Species ◽  
Observational Technique ◽  
Wide Range

Abstract. AerGOM is a retrieval algorithm developed for the GOMOS instrument onboard Envisat as an alternative to the operational retrieval (IPF). AerGOM enhances the quality of the stratospheric aerosol extinction retrieval due to the extension of the spectral range used, a refinement of the aerosol spectral parameterisation, the simultaneous inversion of all atmospheric species as well as an improvement of the Rayleigh scattering correction. The retrieval algorithm allows for a good characterisation of the stratospheric aerosol extinction for a wide range of wavelengths. In this work, we present the results of stratospheric aerosol extinction comparisons between AerGOM and various spaceborne instruments (SAGE II, SAGE III, POAM III, ACE-MAESTRO and OSIRIS) for different wavelengths. Due to the unique observational technique of GOMOS, some of the results appear to be dependent on the star occultation parameters such as star apparent temperature and magnitude, solar zenith angle, latitude and obliquity. A systematic analysis is carried out to identify biases in the dataset, using the various spaceborne instruments as references. This bias characterization is extremely important for data users and might prove valuable for the production of unbiased long-term merged dataset.

scholarly journals An evaluation of the SAGE III Version 4 aerosol extinction coefficient and water vapor data products

2009 ◽  
Vol 9 (5) ◽  
pp. 22177-22222
Author(s):  
L. W. Thomason ◽  
J. R. Moore ◽  
M. C. Pitts ◽  
J. M. Zawodny ◽  
E.-W. Chiou
Keyword(s):  
Water Vapor ◽  
Extinction Coefficient ◽  
Stratospheric Aerosol ◽  
Data Sets ◽  
Aerosol Extinction ◽  
Data Products ◽  
Mean Differences ◽  
Aerosol Extinction Coefficient ◽  
Polar Ozone

Abstract. Herein, we provide an assessment of the data quality of Stratospheric Aerosol and Gas Experiment (SAGE III) Version 4 aerosol extinction coefficient and water vapor data products. The evaluation is based on comparisons with data from four instruments: SAGE II, the Polar Ozone and Aerosol Measurement (POAM III), the Halogen Occultation Experiment (HALOE), and the Microwave Limb Sounder (MLS). Since only about half of the SAGE III channels have a direct comparison with measurements by other instruments, we have employed some empirical techniques to evaluate measurements at some wavelengths. We find that the aerosol extinction coefficient measurements at 449, 520, 755, 869, and 1021 nm are reliable with accuracies and precisions on the order of 10% in the primary aerosol range of 15 to 25 km. We also believe this to be true of the aerosol measurements at 1545 nm though we cannot exclude some positive bias below 15 km. We recommend use of the 385 nm measurements above 16 km where the accuracy is on par with other aerosol channels. The 601 nm measurement is much noisier (~20%) than other channels and we suggest caution in the use of these data. We believe that the 676 nm data are clearly defective particularly above 20 km (accuracy as poor as 50%) and the precision is also low (~30%). We suggest excluding this channel under most circumstances. The SAGE III Version 4 water vapor data product appears to be high quality and is recommended for science applications in the stratosphere below 45 km. In this altitude range, the mean differences with all four corroborative data sets are no bigger than 15% and often less than 10% with exceptional agreement with POAM III and MLS. Above 45 km, it seems likely that SAGE III water vapor values are increasingly too large and should be used cautiously or avoided. We believe that SAGE III meets its preflight goal of 15% accuracy and 10% precision between 15 and 45 km. We do not currently recommend limiting the SAGE III water vapor data utility in the stratosphere by aerosol loading.

scholarly journals The Ozone Mapping and Profiler Suite (OMPS) Limb Profiler (LP) Version 1 aerosol extinction retrieval algorithm: theoretical basis

2018 ◽  
Vol 11 (5) ◽  
pp. 2633-2651 ◽  
Author(s):  
Robert Loughman ◽  
Pawan K. Bhartia ◽  
Zhong Chen ◽  
Philippe Xu ◽  
Ernest Nyaku ◽  
...  
Keyword(s):  
Spherical Shell ◽  
Theoretical Basis ◽  
Relaxation Method ◽  
Radiative Transfer Model ◽  
Aerosol Size Distribution ◽  
Retrieval Algorithm ◽  
Transfer Model ◽  
Aerosol Extinction ◽  
Horizontal Variations

Abstract. The theoretical basis of the Ozone Mapping and Profiler Suite (OMPS) Limb Profiler (LP) Version 1 aerosol extinction retrieval algorithm is presented. The algorithm uses an assumed bimodal lognormal aerosol size distribution to retrieve aerosol extinction profiles at 675 nm from OMPS LP radiance measurements. A first-guess aerosol extinction profile is updated by iteration using the Chahine nonlinear relaxation method, based on comparisons between the measured radiance profile at 675 nm and the radiance profile calculated by the Gauss–Seidel limb-scattering (GSLS) radiative transfer model for a spherical-shell atmosphere. This algorithm is discussed in the context of previous limb-scattering aerosol extinction retrieval algorithms, and the most significant error sources are enumerated. The retrieval algorithm is limited primarily by uncertainty about the aerosol phase function. Horizontal variations in aerosol extinction, which violate the spherical-shell atmosphere assumed in the version 1 algorithm, may also limit the quality of the retrieved aerosol extinction profiles significantly.

scholarly journals Using a Parameterization of a Radiative Transfer Model to Build High-Resolution Maps of Typical Clear-Sky UV Index in Catalonia, Spain

2005 ◽  
Vol 44 (6) ◽  
pp. 789-803 ◽  
Author(s):  
Jordi Badosa ◽  
Josep-Abel González ◽  
Josep Calbó ◽  
Michiel van Weele ◽  
Richard L. McKenzie
Keyword(s):  
High Resolution ◽  
Radiative Transfer ◽  
Zenith Angle ◽  
Solar Zenith Angle ◽  
Absolute Error ◽  
Single Scattering ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Uv Index ◽  
Wide Range

Abstract To perform a climatic analysis of the annual UV index (UVI) variations in Catalonia, Spain (northeast of the Iberian Peninsula), a new simple parameterization scheme is presented based on a multilayer radiative transfer model. The parameterization performs fast UVI calculations for a wide range of cloudless and snow-free situations and can be applied anywhere. The following parameters are considered: solar zenith angle, total ozone column, altitude, aerosol optical depth, and single-scattering albedo. A sensitivity analysis is presented to justify this choice with special attention to aerosol information. Comparisons with the base model show good agreement, most of all for the most common cases, giving an absolute error within ±0.2 in the UVI for a wide range of cases considered. Two tests are done to show the performance of the parameterization against UVI measurements. One uses data from a high-quality spectroradiometer from Lauder, New Zealand [45.04°S, 169.684°E, 370 m above mean sea level (MSL)], where there is a low presence of aerosols. The other uses data from a Robertson–Berger-type meter from Girona, Spain (41.97°N, 2.82°E, 100 m MSL), where there is more aerosol load and where it has been possible to study the effect of aerosol information on the model versus measurement comparison. The parameterization is applied to a climatic analysis of the annual UVI variation in Catalonia, showing the contributions of solar zenith angle, ozone, and aerosols. High-resolution seasonal maps of typical UV index values in Catalonia are presented.

scholarly journals A Parametric Radiative Forcing Model for Contrail Cirrus

2012 ◽  
Vol 51 (7) ◽  
pp. 1391-1406 ◽  
Author(s):  
U. Schumann ◽  
B. Mayer ◽  
K. Graf ◽  
H. Mannstein
Keyword(s):  
Analytical Model ◽  
Optical Depth ◽  
Zenith Angle ◽  
Radiative Forcing ◽  
Solar Zenith Angle ◽  
Life Cycles ◽  
Radiative Transfer Model ◽  
Model Parameters ◽  
Transfer Model ◽  
Wide Range

AbstractA new parameterized analytical model is presented to compute the instantaneous radiative forcing (RF) at the top of the atmosphere (TOA) produced by an additional thin contrail cirrus layer (called “contrail” below). The model calculates the RF using as input the outgoing longwave radiation and reflected solar radiation values at TOA for a contrail-free atmosphere, so that the model is applicable for both cloud-free and cloudy ambient atmospheres. Additional input includes the contrail temperature, contrail optical depth (at 550 nm), effective particle radius, particle habit, solar zenith angle, and the optical depth of cirrus above the contrail layer. The model parameters (5 for longwave and 10 for shortwave) are determined from least squares fits to calculations from the “libRadtran” radiative transfer model over a wide range of atmospheric and surface conditions. The correlation coefficient between model and calculations is larger than 98%. The analytical model is compared with published results, including a 1-yr simulation of global RF, and is found to agree well with previous studies. The fast analytical model is part of a larger modeling system to simulate contrail life cycles (“CoCiP”) and can allow for the rapid simulation of contrail cirrus RF over a wide range of meteorological conditions and for a given size-dependent habit mixture. Ambient clouds are shown to have large local impact on the net RF of contrails. Net RF of contrails may both increase and decrease and even change sign in the presence of higher-level cirrus, depending on solar zenith angle.

scholarly journals AerGOM, an improved algorithm for stratospheric aerosol extinction retrieval from GOMOS observations. Part 1: Algorithm development

2016 ◽  
Author(s):  
Filip Vanhellemont ◽  
Nina Mateshvili ◽  
Laurent Blanot ◽  
Charles E. Robert ◽  
Christine Bingen ◽  
...  
Keyword(s):  
Stratospheric Aerosol ◽  
Quality Data ◽  
Retrieval Algorithm ◽  
Aerosol Extinction ◽  
Data Inversion ◽  
Aerosol Retrieval ◽  
Stellar Occultation ◽  
Algorithmic Problems ◽  
The Subject ◽  
Level 2

Abstract. The GOMOS instrument on EnviSat has succesfully demonstrated that a UV/Vis/NIR spaceborne stellar occultation instrument is capable of delivering quality data on the gaseous and particulate composition of Earth's atmosphere. Still, some problems related to data inversion remained to be treated. In the past, it was found that the aerosol extinction profile retrievals in the upper troposphere and stratosphere are of good quality at a reference wavelength of 500 nm, but suffer from anomalous, retrieval-related perturbations at other wavelengths. Identification of algorithmic problems and subsequent improvement was therefore necessary. This work has been carried out; the resulting AerGOM Level 2 retrieval algorithm together with the first data version AerGOMv1.0 forms the subject of this paper. First, a brief overview of the operational IPFv6.01 GOMOS algorithm is given, since the AerGOM algorithm is to a certain extent similar. Then, the discussion on the AerGOM algorithm specifically focuses on the new aspects that were implemented to tackle the aerosol retrieval problems. Finally, a first assess- ment of the obtained aerosol extinction data quality is presented, clearly showing significant improvement of aerosol profile shape, spectral behaviour and similarity to SAGE II data.

scholarly journals Stratospheric aerosol particle size information in Odin-OSIRIS limb scatter spectra

2013 ◽  
Vol 6 (3) ◽  
pp. 5065-5099
Author(s):  
L. A. Rieger ◽  
A. E. Bourassa ◽  
D. A. Degenstein
Keyword(s):  
Particle Size ◽  
Particle Size Distribution ◽  
Size Distribution ◽  
Imaging System ◽  
Stratospheric Aerosol ◽  
Retrieval Algorithm ◽  
Aerosol Layer ◽  
Aerosol Extinction ◽  
Model Calculations ◽  
Size Information

Abstract. The Optical Spectrograph and InfraRed Imaging System (OSIRIS) on-board the Odin satellite has now taken over a decade of limb scatter measurements that have been used to retrieve the Version 5 stratospheric aerosol extinction product. This product is retrieved using a representative particle size distribution to calculate scattering cross sections and scattering phase functions for the forward model calculations. In this work the information content of OSIRIS measurements with respect to stratospheric aerosol is systematically examined for the purpose of retrieving particle size information along with the extinction coefficient. The benefit of using measurements at different wavelengths and scattering angles in the retrieval is studied and it is found that incorporation of the 1530 nm radiance measurement is key for a robust retrieval of particle size information. It is also found that using OSIRIS measurements at different solar geometries simultaneously provides little additional benefit. Based on these results, an improved aerosol retrieval algorithm is developed that couples the retrieval of aerosol extinction and mode radius of a log-normal particle size distribution. Comparison of these results with coincident measurements from SAGE III show agreement in retrieved extinction to within approximately 10% over the bulk of the aerosol layer, which is comparable to Version 5. The retrieved particle size, when converted to Ångström coefficient, shows good qualitative agreement with SAGE II measurements made at somewhat shorter wavelengths.

scholarly journals Stratospheric aerosol characteristics from space-borne observations: extinction coefficient and Ångström exponent

2018 ◽  
Author(s):  
Elizaveta Malinina ◽  
Alexei Rozanov ◽  
Landon Rieger ◽  
Adam Bourassa ◽  
Heinrich Bovensmann ◽  
...  
Keyword(s):  
Extinction Coefficient ◽  
Simple Relation ◽  
Stratospheric Aerosol ◽  
Accurate Information ◽  
Aerosol Extinction ◽  
Data Set ◽  
Extinction Coefficients ◽  
Angstrom Exponent ◽  
Ångström Exponent ◽  
Ångstrom Exponent

Abstract. Stratospheric aerosols are of a great importance to the scientific community, predominantly because of their role in climate, but also because accurate knowledge of aerosol characteristics is relevant for trace gases retrievals from remote sensing instruments. There are several data sets published which provide aerosol extinction coefficients in the stratosphere. However, for the instruments measuring in the limb viewing geometry, the use of this parameter is associated with uncertainties resulting from the need to assume an aerosol particle size distribution (PSD) within the retrieval process. These uncertainties can be mitigated if PSD information is retrieved. While occultation instruments provide more accurate information on the aerosol extinction coefficient, in this study, it was shown that limb instruments have better potential for the PSD retrieval, especially during the background aerosol loading periods. A data set containing PSD information was recently retrieved from SCIAMACHY limb measurements and provides two parameters of the log-normal PSD for the SCIAMACHY operational period (2002–2012). In this study, the data set is expanded by aerosol extinction coefficients and Ångström exponents calculated from the retrieved PSD parameters. Errors in the Ångström exponents and aerosol extinction coefficients are assessed using synthetic retrievals. For the extinction coefficient the resulting accuracy is within ±25 %, and for the Ångström exponent, it is better than 10 %. The recalculated SCIAMACHY aerosol extinction coefficients are compared to those from SAGE II. The differences between the instruments vary from 0 to 25 % depending on the wavelength. Ångström exponent comparison with SAGE II shows differences between 10 % at 31 km and 40 % at 18 km. Comparisons with SAGE II, however, suffer from the low amount of collocated profiles. Furthermore, the Ångström exponents obtained from the limb viewing instrument OSIRIS are used for the comparison. This comparison shows an average difference within 7 %. The time series of these differences do not show signatures of any remarkable events. Besides, the temporal behavior of the Ångström exponent in the tropics is analyzed using the SCIAMACHY data set. It is shown, that there is no simple relation between the Ångström exponent and the PSD because the same value of Ångström exponent can be obtained from an infinite number of combinations of the PSD parameters.

scholarly journals RETRIEVAL OF AEROSOL PHASE FUNCTION AND POLARIZED PHASE FUNCTION FROM POLARIZATION OF SKYLIGHT FOR DIFFERENT OBSERVATION GEOMETRIES

2018 ◽  
Vol XLII-3 ◽  
pp. 857-863
Author(s):  
L. Li ◽  
L. L. Qie ◽  
H. Xu ◽  
Z. Q. Li
Keyword(s):  
Zenith Angle ◽  
Phase Function ◽  
Solar Zenith Angle ◽  
Stokes Parameter ◽  
Principal Plane ◽  
Stokes Parameters ◽  
Retrieval Algorithm ◽  
Optical Parameters ◽  
Skylight Polarization ◽  
Observation Geometry

The phase function and polarized phase function are important optical parameters, which describe scattering properties of atmospheric aerosol particles. Polarization of skylight induced by the scattering processes is sensitive to the scattering properties of aerosols. The Stokes parameters <i>I, Q, U</i> and the polarized radiance <i>L<sub>p</sub></i> of skylight measured by the CIMEL dual-polar sun-sky radiometer CE318- DP can be use to retrieve the phase function and polarized phase function, respectively. Two different observation geometries (i.e., the principal plane and almucantar) are preformed by the CE318-DP to detect skylight polarization. Polarization of skylight depends on the illumination and observation geometries. For the same solar zenith angle, retrievals of the phase function and the polarized phase function are still affected by the observation geometry. The performance of the retrieval algorithm for the principal plane and almucantar observation geometries was assessed by the numerical experiments at two typical high and low sun’s positions (i.e. solar zenith angles are equal to 45&amp;deg; and 65&amp;deg;). Comparing the results for the principal plane and almucantar geometries, it is recommended to utilize the principal plane observations to retrieve the phase function when the solar zenith angle is small. The Stokes parameter <i>U</i> and the polarized radiance <i>L<sub>p</sub></i> from the almucantar observations are suggested to retrieve the polarized phase function, especially for short wavelength channels (e.g., 440 and 500&amp;thinsp;nm).

scholarly journals Global stratospheric aerosol extinction profile retrievals from SCIAMACHY limb-scatter observations

2012 ◽  
Vol 5 (4) ◽  
pp. 5993-6035 ◽  
Author(s):  
F. Ernst ◽  
C. von Savigny ◽  
A. Rozanov ◽  
V. Rozanov ◽  
K.-U. Eichmann ◽  
...  
Keyword(s):  
Surface Albedo ◽  
Optimal Estimation ◽  
Stratospheric Aerosol ◽  
Visible Spectral Range ◽  
Radiative Transfer Model ◽  
Retrieval Algorithm ◽  
Transfer Model ◽  
Aerosol Extinction ◽  
Index Approach ◽  
The Impact

Abstract. Stratospheric aerosol extinction profiles are retrieved from SCIAMACHY/Envisat limb-scatter observations in the visible spectral range. The retrieval algorithm is based on a colour-index approach using the normalized limb-radiance profiles at 470 nm and 750 nm wavelength. The optimal estimation approach in combination with the radiative transfer model SCIATRAN is employed for the retrievals. This study presents a detailed description of the retrieval algorithm, and a sensitivity analysis investigating the impact of the most important parameters that affect the aerosol extinction profile retrieval accuracy. It is found that the parameter with the largest impact is surface albedo, particularly for SCIAMACHY observations in the Southern Hemisphere where the error in stratospheric aerosol extinction can be up to 50% if the surface albedo is not well known. The effect of errors in the assumed ozone and neutral density profiles on the aerosol profile retrievals is with generally less than 6% relatively small. The aerosol extinction profiles retrieved from SCIAMACHY are compared with co-located SAGE II solar occultation measurements of stratospheric aerosol extinction during the period 2003–2005. The mean aerosol extinction profiles averaged over all co-locations agree to within 20% between 15 and 35 km altitude. However, larger differences are observed at specific latitudes.

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