Vertical Profiling of Fresh Biomass Burning Aerosol Optical Properties over the Greek Urban City of Ioannina, during the PANACEA Winter Campaign

Vertical profiling of aerosol particles was performed during the PANhellenic infrastructure for Atmospheric Composition and climatE chAnge (PANACEA) winter campaign (10 January 2020–7 February 2020) over the city of Ioannina, Greece (39.65° N, 20.85° E, 500 m a.s.l.). The middle-sized city of Ioannina suffers from wintertime air pollution episodes due to biomass burning (BB) domestic heating activities. The lidar technique was applied during the PANACEA winter campaign on Ioannina city, to fill the gap of knowledge of the spatio-temporal evolution of the vertical mixing of the particles occurring during these winter-time air pollution episodes. During this campaign the mobile single-wavelength (532 nm) depolarization Aerosol lIdAr System (AIAS) was used to measure the spatio-temporal evolution of the aerosols’ vertical profiles within the Planetary Boundary Layer (PBL) and the lower free troposphere (LFT; up to 4 km height a.s.l.). AIAS performed almost continuous lidar measurements from morning to late evening hours (typically from 07:00 to 19:00 UTC), under cloud-free conditions, to provide the vertical profiles of the aerosol backscatter coefficient (baer) and the particle linear depolarization ratio (PLDR), both at 532 nm. In this study we emphasized on the vertical profiling of very fresh (~hours) biomass burning (BB) particles originating from local domestic heating activities in the area. In total, 33 out of 34 aerosol layers in the lower free troposphere were characterized as fresh biomass burning ones of local origin, showing a mean particle linear depolarization value of 0.04 ± 0.02 with a range of 0.01 to 0.09 (532 nm) in a height region 1.21–2.23 km a.s.l. To corroborate our findings, we used in situ data, particulate matter (PM) concentrations (PM2.5) from a particulate sensor located close to our station, and the total black carbon (BC) concentrations along with the respective contribution of the fossil fuel (BCff) and biomass/wood burning (BCwb) from the Aethalometer. The PM2.5 mass concentrations ranged from 5.6 to 175.7 μg/m3, while the wood burning emissions from residential heating were increasing during the evening hours, with decreasing temperatures. The BCwb concentrations ranged from 0.5 to 17.5 μg/m3, with an extremely high mean contribution of BCwb equal to 85.4%, which in some cases during night-time reached up to 100% during the studied period.

Fine-Scale Velocity Measurement on the Wirewalker Wave-Powered Profiler

The Wirewalker (WW) ocean-wave-powered vertical profiling system allows the collection of high-resolution oceanographic data due to its rapid profiling, hydrodynamically quiet operation, and long endurance. We have assessed the potential for measuring fine-scale ocean velocities from the Wirewalker platform using commercially available acoustic velocimeters. Although the vertical profiling speed is relatively steady, platform motion affects the velocity measurements and requires correction. We present an algorithm to correct our velocity estimates using platform motion calculated from the inertial sensors – accelerometer, gyroscope, and magnetometer – on a Nortek Signature1000 Acoustic Doppler Current Profiler. This correction, carried out ping-by-ping, was effective in removing the vehicle motion from the measured velocities. The motion-corrected velocities contain contributions from surface wave orbital velocities, especially near the surface, and the background currents. To proceed, we use an averaging approach that leverages both the vertical platform profiling of the system and the ~15-20 m vertical profiling range resolution of the down-looking ADCP to separate the surface wave orbital velocities and the background flow. The former can provide information on the wave conditions. From the latter, we are able to estimate fine-scale velocity and shear with spectral wavenumber roll-off at vertical scales around 3 m, a vertical resolution several times finer than that possible from modern shipboard or fixed ADCPs with similar profiling range, and similar to recent glider measurements. When combined with a continuous time-series of buoy drift calculated from the onboard GPS, a highly-resolved total velocity field is obtained, with a unique combination of space and time resolution.

Using GEDI Waveforms for Improved TanDEM-X Forest Height Mapping: A Combined SINC + Legendre Approach

In this paper, we consider a new method for forest canopy height estimation using TanDEM-X single-pass radar interferometry. We exploit available information from sample-based, space-borne LiDAR systems, such as the Global Ecosystem Dynamics Investigation (GEDI) sensor, which offers high-resolution vertical profiling of forest canopies. To respond to this, we have developed a new extended Fourier-Legendre series approach for fusing high-resolution (but sparsely spatially sampled) GEDI LiDAR waveforms with TanDEM-X radar interferometric data to improve wide-area and wall-to-wall estimation of forest canopy height. Our key methodological development is a fusion of the standard uniform assumption for the vertical structure function (the SINC function) with LiDAR vertical profiles using a Fourier-Legendre approach, which produces a convergent series of approximations of the LiDAR profiles matched to the interferometric baseline. Our results showed that in our test site, the Petawawa Research Forest, the SINC function is more accurate in areas with shorter canopy heights (<~27 m). In taller forests, the SINC approach underestimates forest canopy height, whereas the Legendre approach avails upon simulated GEDI forest structural vertical profiles to overcome SINC underestimation issues. Overall, the SINC + Legendre approach improved canopy height estimates (RMSE = 1.29 m) compared to the SINC approach (RMSE = 4.1 m).

Large and increasing methane emissions from eastern Amazonia derived from satellite data, 2010–2018

We use a global inverse model, satellite data and flask measurements to estimate methane (CH4) emissions from South America, Brazil and the basin of the Amazon River for the period 2010–2018. We find that emissions from Brazil have risen during this period, most quickly in the eastern Amazon basin, and that this is concurrent with increasing surface temperatures in this region. Brazilian CH4 emissions rose from 49.8 ± 5.4 Tg yr−1 in 2010–2013 to 55.6 ± 5.2 Tg yr−1 in 2014–2017, with the wet season of December–March having the largest positive trend in emissions. Amazon basin emissions grew from 41.7 ± 5.3 to 49.3 ± 5.1 Tg yr−1 during the same period. We derive no significant trend in regional emissions from fossil fuels during this period. We find that our posterior distribution of emissions within South America is significantly and consistently changed from our prior estimates, with the strongest emission sources being in the far north of the continent and to the south and south-east of the Amazon basin, at the mouth of the Amazon River and nearby marsh, swamp and mangrove regions. We derive particularly large emissions during the wet season of 2013/14, when flooding was prevalent over larger regions than normal within the Amazon basin. We compare our posterior CH4 mole fractions, derived from posterior fluxes, to independent observations of CH4 mole fraction taken at five lower- to mid-tropospheric vertical profiling sites over the Amazon and find that our posterior fluxes outperform prior fluxes at all locations. In particular the large emissions from the eastern Amazon basin are shown to be in good agreement with independent observations made at Santarém, a location which has long displayed higher mole fractions of atmospheric CH4 in contrast with other basin locations. We show that a bottom-up wetland flux model can match neither the variation in annual fluxes nor the positive trend in emissions produced by the inversion. Our results show that the Amazon alone was responsible for 24 ± 18 % of the total global increase in CH4 flux during the study period, and it may contribute further in future due to its sensitivity to temperature changes.

A Concept of 2U Spaceborne Multichannel Heterodyne Spectroradiometer for Greenhouse Gases Remote Sensing

We present the project of a 2U CubeSat format spaceborne multichannel laser heterodyne spectroradiometer (MLHS) for studies of the Earth’s atmosphere upper layers in the near-infrared (NIR) spectral range (1258, 1528, and 1640 nm). A spaceborne MLHS operating in the solar occultation mode onboard CubeSat platform, is capable of simultaneous vertical profiling of CO2, H2O, CH4, and O2, as well as Doppler wind measurements, in the tangent heights range of 5–50 km. We considered the low Earth orbit for the MLHS deployment and analyzed the expected surface coverage and spatial resolution during one year of operations. A ground-based prototype of the MLHS for CO2 and CH4 molecular absorption measurements with an ultra-high spectral resolution of 0.0013 cm−1 is presented along with the detailed description of its analytical characteristics and capabilities. Implementation of a multichannel configuration of the heterodyne receiver (four receivers per one spectral channel) provides a significant improvement of the signal-to-noise ratio with the reasonable exposure time typical for observations in the solar occultation mode. Finally, the capability of building up a tomographic picture of sounded gas concentration distributions provided by high spectral resolution is discussed.

The Spectral Nature of Earth’s Reflected Radiation: Measurement and Science Applications

This paper introduces the aerosol, clouds, convection and precipitation (ACCP) program that is currently in the process of defining a number of measurement objectives for NASA that are to be implemented toward the end of the current decade. Since a (solar) visible-shortwave infrared (VSWIR) spectrometer is being considered as part of the ACCP architecture, illustrations of the different ways these measurements will contribute to this program and how these measurements can be expected to advance the science objectives of ACCP are highlighted. These contributions range from 1) constraining cloud radiative process and related estimates of radiative fluxes, 2) scene discrimination, 3) providing aerosol and cloud optical properties, and 4) providing other enhanced information such as the phase of water in clouds, and total column water vapor. The spectral measurements also offer new capabilities that will further enhance the ACCP science such as the discrimination of dust aerosol and the potential for the vertical profiling cloud droplet size in shallow clouds. The areas where the maturity of approaches is lacking is also highlighted as a way of emphasizing research topics to be a focus in the coming years.