Growth of 6Li-enriched LiCl/BaCl2 eutectic as a novel neutron scintillator

In this study, Eu:6LiCl/BaCl2 with a high Li concentration was developed as a novel thermal neutron scintillator. Eu ions were doped as activators for the BaCl2 phase, and Eu:6LiCl/BaCl2 eutectics were grown via the vertical Bridgman–Stockbarger method in quartz ampoules (inner diameter = 4 mm). The Eu:6LiCl/BaCl2 eutectic exhibited a lamellar eutectic structure and optical transparency. The 400-nm emission due to the Eu2+ 4f–5d transition was observed in the BaCl2 phase by a cathode luminescence measurement. The light yield under neutrons was estimated to be over 20,200 photons/MeV. A pulse shape discrimination study was also performed using gamma and alpha-rays. The Eu:6LiCl/BaCl2 eutectic scintillator showed good potential of pulse shape discrimination.

Ratio-Based Pulse Shape Discrimination: Analytic Results for Gaussian and Poisson Noise Models

In experiments in a range of felds including fast neutron spectroscopy and astroparticle physics, one can discriminate events of interest from background events based on the shapes of electronic pulses produced by energy deposits in a detector. Here, I focus on a well-known pulse shape discrimination method based on the ratio of the temporal integral of the pulse over an early interval Xp and the temporal integral over the entire pulse Xt . For both event classes, for both a Gaussian noise model and a Poisson noise model, I present analytic expressions for the conditional distribution of Xp given knowledge of the observed value of Xt and a scaled energy deposit corresponding to the product of the full energy deposit and a relative yield factor. I assume that the energy-dependent theoretical prompt fraction for both classes are known exactly. With a Bayesian approach that accounts for imperfect knowledge of the scaled energy deposit, I determine the posterior mean background acceptance probability given the target signal acceptance probability as a function of the observed value of Xt . My method enables one to determine receiver-operating-characteristic curves by numerical integration rather than by Monte Carlo simulation for these two noise models.

Characterization of the scintillation time response of liquid argon detectors for dark matter search

The scintillation time response of liquid argon has a key role in the discrimination of electronic backgrounds in dark matter search experiments. However, its extraordinary rejection power can be affected by various detector effects such as the delayed light emission of TetraPhenyl Butadiene, the most commonly used wavelength shifter, and the electric drift field applied in Time Projection Chambers. In this work, we characterized the TetraPhenyl Butadiene delayed response and the dependence of the pulse shape discrimination on the electric field, exploiting the data acquired with the ARIS, a small-scale single-phase liquid argon detector exposed to monochromatic neutron and gamma sources at the ALTO facility of IJC Lab in Orsay.

Characterization of a medium-sized CLLB scintillator: single neutron/gamma detector for radiation monitoring

The use of a single neutron/gamma detector is an interesting solution to detect and identify gamma emitters and also special nuclear materials (SNM), being able to discriminate between the two kinds of particles and also to perform good-resolution gamma spectroscopy. In this framework, we present a comprehensive characterization of a medium sized (2" × 2") CLLB (Cs2LiLaBr6:Ce) scintillation detector, in order to give the necessary information to assess its deployment in applications regarding homeland security and radiation monitoring. In particular, the parameters studied are: energy resolution, full-energy peak gamma efficiency, time resolution, thermal neutron/gamma discrimination capability, decay time of the signals, high counting rate performance and minimum detectable activities (of 137Cs and 252Cf sources). We employed digital nuclear electronics combined with a pulse shape discrimination algorithm to acquire and analyze the data. We compared our results with reported data for smaller CLLB scintillators, finding good agreement. Experiments were combined with Monte Carlo simulations (using GEANT4 v10.6.0 and MCNP5 v1.60) in order to complement the characterization. The obtained results suggest that the 2” × 2” CLLB detector offers better performance with respect to other scintillators of the same size such as NaI(Tl), CsI, CeBr, etc. which are commonly used in a radiation monitoring systems.

Design and Fabrication of CLYC-Based Rotational Modulation Collimator (RMC) System for Gamma-Ray/Neutron Dual-Particle Imager

Background: This work aims to develop a new imaging system based on a pulse shape discrimination-capable Cs2LiYCl6:Ce (CLYC) scintillation detector combined with the rotational modulation collimator (RMC) technique for dual-particle imaging.Materials and Methods: In this study, a CLYC-based RMC system was designed based on Monte Carlo simulations, and a prototype was fabricated. Therein, a rotation control system was developed to rotate the RMC unit precisely, and a graphical user interface-based software was also developed to operate the data acquisition with RMC rotation. The RMC system was developed to allow combining various types of collimator masks and detectors interchangeably, making the imaging system more versatile for various applications and conditions.Results and Discussion: Operational performance of the fabricated system was studied by checking the accuracy and precision of the collimator rotation and obtaining modulation patterns from a gamma-ray source repeatedly.Conclusion: The prototype RMC system showed reliability in its mechanical properties and reproducibility in the acquisition of modulation patterns, and it will be further investigated for its dual-particle imaging capability with various complex radioactive source conditions.

Pulse-shape discrimination against low-energy Ar-39 beta decays in liquid argon with 4.5 tonne-years of DEAP-3600 data

The DEAP-3600 detector searches for the scintillation signal from dark matter particles scattering on a 3.3 tonne liquid argon target. The largest background comes from $$^{39}\text{ Ar }$$ 39 Ar beta decays and is suppressed using pulse-shape discrimination (PSD). We use two types of PSD estimator: the prompt-fraction, which considers the fraction of the scintillation signal in a narrow and a wide time window around the event peak, and the log-likelihood-ratio, which compares the observed photon arrival times to a signal and a background model. We furthermore use two algorithms to determine the number of photons detected at a given time: (1) simply dividing the charge of each PMT pulse by the mean single-photoelectron charge, and (2) a likelihood analysis that considers the probability to detect a certain number of photons at a given time, based on a model for the scintillation pulse shape and for afterpulsing in the light detectors. The prompt-fraction performs approximately as well as the log-likelihood-ratio PSD algorithm if the photon detection times are not biased by detector effects. We explain this result using a model for the information carried by scintillation photons as a function of the time when they are detected.