Raman Lidar for Monitoring of Aerosol Pollution in the Free Troposphere

2008 ◽  
pp. 155-166 ◽  
Author(s):  
Detlef Müller ◽  
Ina Mattis ◽  
Albert Ansmann ◽  
Ulla Wandinger ◽  
Dietrich Althausen
Keyword(s):  
Free Troposphere ◽  
Raman Lidar ◽  
Aerosol Pollution

Two months of measurements with an autonomous thermodynamic Raman lidar in Lindenberg

2021 ◽  
Author(s):  
Diego Lange Vega ◽  
Andreas Behrendt ◽  
Volker Wulfmeyer
Keyword(s):  
Boundary Layer ◽  
Water Vapor ◽  
Inversion Layer ◽  
Measurement Range ◽  
High Accuracy ◽  
Free Troposphere ◽  
Raman Lidar ◽  
Backscatter Coefficient ◽  
Geophysical Research ◽  
Turbulence Scale

<p>Between 15 July 2020 and 19 September 2021, the Atmospheric Raman Temperature and Humidity Sounder (ARTHUS) collected data at the Lindenberg Observatory of the Deutscher Wetterdienst (DWD), including temperature and water vapor mixing ratio with a high temporal and range resolution.</p> <p>During the operation period, very stable 24/7 operation was achieved, and ARTHUS demonstrated that is capable to observe the atmospheric boundary layer and lower free troposphere during both daytime and nighttime up to the turbulence scale, with high accuracy and precision, and very short latency. During nighttime, the measurement range increases even up to the tropopause and lower stratosphere.</p> <p>ARTHUS measurements resolve the strength of the inversion layer at the planetary boundary layer top, elevated lids in the free troposphere, and turbulent fluctuations in water vapor and temperature, simultaneously (Lange et al., 2019, Wulfmeyer et al., 2015). In addition to thermodynamic variables, ARTHUS provides also independent profiles of the particle backscatter coefficient and the particle extinction coefficient from the rotational Raman signals at 355 nm with much better resolution than a conventional vibrational Raman lidar.</p> <p>At the conference, highlights of the measurements will be presented. Furthermore, the statistics of more than 150 comparisons with local radiosondes will be presented which confirm the high accuracy of the temperature and moisture measurements of ARTHUS.</p> <p><strong><em>Acknowledgements</em></strong></p> <p>The development of ARTHUS was supported by the Helmholtz Association of German Research Centers within the project Modular Observation Solutions for Earth Systems (MOSES). The measurements in Lindenberg were funded by DWD.</p> <p><strong><em>References </em></strong></p> <p>Lange, D., Behrendt, A., and Wulfmeyer, V. (2019). Compact operational tropospheric water vapor and temperature Raman lidar with turbulence resolution. <em>Geophysical Research Letters</em>, 46. https://doi.org/10.1029/2019GL085774</p> <p>Wulfmeyer, V., R. M. Hardesty, D. D. Turner, A. Behrendt, M. P. Cadeddu, P. Di Girolamo, P. Schlüssel, J. Van Baelen, and F. Zus (2015), A review of the remote sensing of lower tropospheric thermodynamic profiles and its indispensable role for the understanding and the simulation of water and energy cycles, <em>Rev. Geophys.</em>, 53,819–895, doi:10.1002/2014RG000476</p>

scholarly journals Validation of aerosol backscatter profiles from Raman lidar and ceilometer using balloon-borne measurements

2020 ◽  
Author(s):  
Simone Brunamonti ◽  
Giovanni Martucci ◽  
Gonzague Romanens ◽  
Yann Poltera ◽  
Frank G. Wienhold ◽  
...  
Keyword(s):  
In Situ Measurements ◽  
Spatial And Temporal Variability ◽  
Free Troposphere ◽  
Raman Lidar ◽  
Backscatter Coefficient ◽  
Custom Made ◽  
Standard Deviations ◽  
Aerosol Backscatter ◽  
Good Agreement

Abstract. Remote sensing measurements by light detection and ranging (lidar) instruments are fundamental for the monitoring of altitude-resolved aerosol optical properties. Here, we validate vertical profiles of aerosol backscatter coefficient (βaer) measured by two independent lidar systems using co-located balloon-borne measurements performed by Compact Optical Backscatter Aerosol Detector (COBALD) sondes. COBALD provides high-precision in-situ measurements of βaer at two wavelengths (455 and 940 nm). The two analyzed lidar systems are the research Raman Lidar for Meteorological Observations (RALMO) and the commercial CHM15K ceilometer (Lufft, Germany). We consider in total 17 RALMO and 31 CHM15K profiles, co-located with simultaneous COBALD soundings performed throughout the years 2014–2019 at the MeteoSwiss observatory of Payerne (Switzerland). The RALMO (355 nm) and CHM15K (1064 nm) measurements are converted to respectively 455 nm and 940 nm using the Angstrom exponent profiles retrieved from COBALD data. To account for the different receiver field of view (FOV) angles between the two lidars (0.01–0.02°) and COBALD (6°), we derive a custom-made correction using Mie-theory scattering simulations. Our analysis shows that both RALMO and CHM15K achieve a good agreement with COBALD measurements in the boundary layer and free troposphere, up to 6 km altitude, and including fine structures in the aerosol’s vertical distribution. For altitudes below 2 km, the mean ± standard deviation difference in βaer is + 6 % ± 40 % (+ 0.005 ± 0.319 Mm−1 sr−1) for RALMO – COBALD at 455 nm, and + 13 % ± 51 % (+ 0.038 ± 0.207 Mm−1 sr−1) for CHM15K – COBALD at 940 nm. The large standard deviations can be at least partly attributed to atmospheric variability effects, associated with the balloon’s horizontal drift with altitude (away from the lidar beam) and the different integration times of the two techniques. Combined with the high spatial and temporal variability of atmospheric aerosols, these effects often lead to a slight altitude displacement between aerosol backscatter features that are seen by both techniques. For altitudes between 2–6 km, the absolute standard deviations of both RALMO and CHM15K decrease (below 0.13 and 0.16 Mm−1sr−1, respectively), while their corresponding relative deviations increase (often exceeding 100 % COBALD of the signal). This is due to the low aerosol content (i.e. low absolute backscattered signal) in the free troposphere, and the vertically decreasing signal-to-noise ratio of the lidar measurements (especially CHM15K). Overall, we conclude that the βaer profiles measured by the RALMO and CHM15K lidar systems are in good agreement with in-situ measurements by COBALD sondes up to 6 km altitude.

scholarly journals Lidar characterization of the Arctic atmosphere during ASTAR 2007: four cases studies of boundary layer, mixed-phase and multi-layer clouds

2010 ◽  
Vol 10 (6) ◽  
pp. 2847-2866 ◽  
Author(s):  
A. Lampert ◽  
C. Ritter ◽  
A. Hoffmann ◽  
J.-F. Gayet ◽  
G. Mioche ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Case Studies ◽  
Airborne Lidar ◽  
Mixed Phase ◽  
Spherical Particles ◽  
The Arctic ◽  
Free Troposphere ◽  
Atmospheric Conditions ◽  
Raman Lidar ◽  
Tropospheric Aerosol

Abstract. During the Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR), which was conducted in Svalbard in March and April 2007, tropospheric Arctic clouds were observed with two ground-based backscatter lidar systems (micro pulse lidar and Raman lidar) and with an airborne elastic lidar. In the time period of the ASTAR 2007 campaign, an increase in low-level cloud cover (cloud tops below 2.5 km) from 51% to 65% was observed above Ny-Ålesund. Four different case studies of lidar cloud observations are analyzed: With the ground-based Raman lidar, a layer of spherical particles was observed at an altitude of 2 km after the dissolution of a cloud. The layer probably consisted of small hydrated aerosol (radius of 280 nm) with a high number concentration (around 300 cm−3) at low temperatures (−30 °C). Observations of a boundary layer mixed-phase cloud by airborne lidar and concurrent airborne in situ and spectral solar radiation sensors revealed the localized process of total glaciation at the boundary of different air masses. In the free troposphere, a cloud composed of various ice layers with very different optical properties was detected by the Raman lidar, suggesting large differences of ice crystal size, shape and habit. Further, a mixed-phase double layer cloud was observed by airborne lidar in the free troposphere. Local orography influenced the evolution of this cloud. The four case studies revealed relations of cloud properties and specific atmospheric conditions, which we plan to use as the base for numerical simulations of these clouds.

scholarly journals Forest Fire Smoke Layers Observed in the Free Troposphere over Portugal with a Multiwavelength Raman Lidar: Optical and Microphysical Properties

2014 ◽  
Vol 2014 ◽  
pp. 1-11 ◽  
Author(s):  
Sérgio Nepomuceno Pereira ◽  
Jana Preißler ◽  
Juan Luis Guerrero-Rascado ◽  
Ana Maria Silva ◽  
Frank Wagner
Keyword(s):  
Single Scattering ◽  
Effective Radius ◽  
Free Troposphere ◽  
Depolarization Ratio ◽  
Raman Lidar ◽  
Extinction Coefficients ◽  
Smoke Particles ◽  
Microphysical Properties ◽  
Fire Smoke ◽  
Lidar Ratio

Vertically resolved optical and microphysical properties of biomass burning aerosols, measured in 2011 with a multiwavelength Raman lidar, are presented. The transportation time, within 1-2 days (or less), pointed towards the presence of relatively fresh smoke particles over the site. Some strong layers aloft were observed with particle backscatter and extinction coefficients (at 355 nm) greater than 5 Mm−1 sr−1and close to 300 Mm−1, respectively. The particle intensive optical properties showed features different from the ones reported for aged smoke, but rather consistent with fresh smoke. The Ångström exponents were generally high, mainly above 1.4, indicating a dominating accumulation mode. Weak depolarization values, as shown by the small depolarization ratio of 5% or lower, were measured. Furthermore, the lidar ratio presented no clear wavelength dependency. The inversion of the lidar signals provided a set of microphysical properties including particle effective radius below 0.2 μm, which is less than values previously observed for aged smoke particles. Real and imaginary parts of refractive index of about 1.5-1.6 and 0.02i, respectively, were derived. The single scattering albedo was in the range between 0.85 and 0.93; these last two quantities indicate the nonnegligible absorbing characteristics of the observed particles.

scholarly journals Vertical aerosol distribution in the Southern hemispheric Midlatitudes as observed with lidar at Punta Arenas, Chile (53.2° S and 70.9° W) during ALPACA

2018 ◽  
Author(s):  
Andreas Foth ◽  
Thomas Kanitz ◽  
Ronny Engelmann ◽  
Holger Baars ◽  
Martin Radenz ◽  
...  
Keyword(s):  
Long Range Transport ◽  
Free Troposphere ◽  
Marine Aerosol ◽  
Raman Lidar ◽  
Aerosol Distribution ◽  
Range Transport ◽  
Aerosol Sources ◽  
Ground Based Lidar ◽  
Lidar Observations ◽  
Measurement Period

Abstract. Within this publication, lidar observations of the vertical aerosol distribution above Punta Arenas, Chile (53.2° S and 50.9° W) which have been performed with the Raman lidar PollyXT from December 2009 to April 2010 are presented. Pristine marine aerosol conditions related to the prevailing westerly circulation dominated the measurements. Lofted aerosol layers could only be observed eight times during the whole measurement period. Two case studies are presented showing long-range transport of smoke from biomass burning in Australia and regionally transported dust from the Patagonian Desert, respectively. The aerosol sources are identified by trajectory analyses with HYSPLIT and FLEXPART. However, seven of the eight analysed cases with lofted layers show an aerosol optical thickness of less than 0.05. From the lidar observations a mean planetary boundary layer (PBL) top height of 1150 ± 350 m was determined. An analysis of particle backscatter coefficients confirms that the majority of the aerosol is attributed to the PBL while the free troposphere is characterized by a very low background aerosol concentration. The ground-based lidar observations at 532 and 1064 nm are supplemented by the AERONET Sun photometers and the space-borne lidar CALIOP on board of CALIPSO. The averaged AOT determined by CALIOP was 0.02 ± 0.01 at Punta Arenas from 2009 to 2010.

scholarly journals Optical characteristics of biomass burning aerosols over Southeastern Europe determined from UV-Raman lidar measurements

2009 ◽  
Vol 9 (7) ◽  
pp. 2431-2440 ◽  
Author(s):  
V. Amiridis ◽  
D. S. Balis ◽  
E. Giannakaki ◽  
A. Stohl ◽  
S. Kazadzis ◽  
...  
Keyword(s):  
Biomass Burning ◽  
Hot Spot ◽  
Optical Parameters ◽  
Free Troposphere ◽  
Raman Lidar ◽  
Smoke Particles ◽  
Tropospheric Aerosol ◽  
Smoke Plumes ◽  
Lidar Measurements ◽  
Uv Raman

Abstract. The influence of smoke on the aerosol loading in the free troposphere over Thessaloniki, Greece is examined in this paper. Ten cases during 2001–2005 were identified when very high aerosol optical depth values in the free troposphere were observed with a UV-Raman lidar. Particle dispersion modeling (FLEXPART) and satellite hot spot fire detection (ATSR) showed that these high free tropospheric aerosol optical depths are mainly attributed to the advection of smoke plumes from biomass burning regions over Thessaloniki. The biomass burning regions were found to extend across Russia in the latitudinal belt between 45° N–55° N, as well as in Eastern Europe (Baltic countries, Western Russia, Belarus, and the Ukraine). The highest frequency of agricultural fires occurred during the summer season (mainly in August). The data collected allowed the optical characterization of the smoke aerosols that arrived over Greece, where limited information has so far been available. Two-wavelength backscatter lidar measurements showed that the backscatter-related Ångström exponent ranged between 0.5 and 2.4 indicating a variety of particle sizes. UV-Raman lidar measurements showed that for smoke particles the extinction to backscatter ratios (so-called lidar ratios) varied between 40 sr for small particles to 100 sr for large particles. Dispersion model estimations of the carbon monoxide tracer concentration profiles for smoke particles indicate that the variability of the optical parameters is a function of the age of the smoke plumes. This information could be useful on the lidar community for reducing uncertainty in the aerosol backscatter coefficient determination due to the lidar ratio assumption, starting from a simply elastic backscatter lidar as the first satellite-borne lidar CALIPSO.

scholarly journals Comparison of Raman Lidar Observations of Water Vapor with COSMO-DE Forecasts during COPS 2007

2011 ◽  
Vol 26 (6) ◽  
pp. 1056-1066 ◽  
Author(s):  
Christian Herold ◽  
Dietrich Althausen ◽  
Detlef Müller ◽  
Matthias Tesche ◽  
Patric Seifert ◽  
...  
Keyword(s):  
Water Vapor ◽  
Short Range ◽  
Residual Layer ◽  
Small Scale ◽  
Free Troposphere ◽  
Raman Lidar ◽  
Mixing Ratios ◽  
Performance Check ◽  
Water Vapor Mixing Ratio ◽  
Range Forecasts

Abstract Water vapor measurements with the multiwavelength Raman lidar Backscatter Extinction Lidar-Ratio Temperature Humidity Profiling Apparatus (BERTHA) were performed during the Convective and Orographically-induced Precipitation Study (COPS) in the Black Forest, Germany, from June to August 2007. For quality assurance, profiles of the water vapor mixing ratio measured with BERTHA are compared to simultaneous measurements of a radiosonde and an airborne differential absorption lidar (DIAL) on 31 July 2007. The differences from the radiosonde observations are found to be on average 1.5% and 2.5% in the residual layer and in the free troposphere, respectively. During the two overflights at 1937 and 2018 UTC, the differences from the DIAL results are −2.2% and −3.7% in the residual layer and 2.1% and −2.6% in the free troposphere. After this performance check, short-range forecasts from the German Meteorological Service’s (Deutscher Wetterdienst, DWD) version of the Consortium for Small-Scale Modeling (COSMO-DE) model are compared to the BERTHA measurements for two case studies. Generally, it is found that water vapor mixing ratios from short-range forecasts are on average 7.9% drier than the values measured in the residual layer. In the free troposphere, modeled values are 9.7% drier than the measurements.

scholarly journals Profiling of CH<sub>4</sub> background mixing ratio in the lower troposphere with Raman lidar: a feasibility experiment

2018 ◽  
Author(s):  
Igor Veselovskii ◽  
Philippe Goloub ◽  
Qiaoyun Hu ◽  
Thierry Podvin ◽  
David N. Whiteman ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Elastic Scattering ◽  
Nd:Yag Laser ◽  
Counting Rate ◽  
Photon Counting ◽  
Lower Troposphere ◽  
Free Troposphere ◽  
Mixing Ratio ◽  
Raman Lidar ◽  
Additional Control

Abstract. We present the results of methane profiling in the lower troposphere using LILAS Raman lidar from Lille University observatory platform (France). The lidar is based on a tripled Nd:YAG laser and nighttime profiling up to 4000 m with 100 m height resolution is possible for methane. Agreement between measured the photon counting rate in the CH4 Raman channel in the free troposphere and numerical simulations for a typical CH4 background mixing ratio (2 ppm) confirms that CH4 Raman scattering is observed. Within the planetary boundary layer, an increase of the CH4 mixing ratio, up to a factor of 2, is observed. Different possible interfering factors, such as leakage of the elastic signal and aerosol fluorescence have been taken into consideration. Tests using backscattering from clouds confirmed that the filters in the Raman channel provide sufficient rejection of elastic scattering. The measured methane profiles do not correlate with aerosol backscattering, which corroborates the hypothesis that, in the PBL, not aerosol fluorescence but CH4 is observed. However, the fluorescence contribution cannot be completely excluded and, for future measurements, we plan to install an additional control channel close to 393 nm where no strong Raman lines exist and only fluorescence can be observed.

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