Two-dimensional Au lattices featuring unique carrier transport preference and wide forbidden gap

Nanoscale ◽  
2014 ◽  
Vol 6 (17) ◽  
pp. 10118-10125 ◽  
Author(s):  
Chunmiao Zhang ◽  
Yaping Wu ◽  
Yinghui Zhou ◽  
Na Gao ◽  
Fei Guo ◽  
...  
Keyword(s):  
Large Scale ◽  
Carrier Transport ◽  
Energy Gap ◽  
Two Dimensional ◽  
Wide Energy ◽  
Forbidden Gap

Large-scale 2D Au lattices are achieved that display a unique wide energy gap and a Kagome-like transport route.

scholarly journals Production and excitation of molecules by dissipation of two-dimensional turbulence

2020 ◽  
Vol 495 (1) ◽  
pp. 816-834
Author(s):  
P Lesaffre ◽  
P Todorov ◽  
F Levrier ◽  
V Valdivia ◽  
N Dzyurkevich ◽  
...  
Keyword(s):  
Large Scale ◽  
Energy Gap ◽  
Small Scale ◽  
Two Dimensional ◽  
One Dimensional ◽  
Infrared Telescope ◽  
High Resolution Mapping ◽  
Localized Heating ◽  
Resolution Mapping ◽  
Large Scale Simulations

ABSTRACT The interstellar medium (ISM) is typically a hostile environment: cold, dilute and irradiated. Nevertheless, it appears very fertile for molecules. The localized heating resulting from turbulence dissipation is a possible channel to produce and excite molecules. However, large-scale simulations cannot resolve the dissipative scales of the ISM. Here, we present two-dimensional small-scale simulations of decaying hydrodynamic turbulence using the chemses code, with fully resolved viscous dissipation, time-dependent heating, cooling, chemistry and excitation of a few rotational levels of H2. We show that molecules are produced and excited in the wake of strong dissipation ridges. We carefully identify shocks and we assess their statistics and contribution to the molecular yields and excitation. We find that the formation of molecules is strongly linked to increased density as a result of shock compression and to the opening of endothermic chemical routes because of higher temperatures. We identify a new channel for molecule production via H2 excitation, illustrated by CH+ yields in our simulations. Despite low temperatures and the absence of magnetic fields (favouring CH+ production through ion-neutral velocity drifts), the excitation of the first few rotational levels of H2 shrinks the energy gap to form CH+. The present study demonstrates how dissipative chemistry can be modelled by statistical collections of one-dimensional steady-state shocks. Thus, the excitation of higher J levels of H2 is likely to be a direct signature of turbulence dissipation, and an indirect probe for molecule formation. We hope these results will help to bring new tools and ideas for the interpretation of current observations of H2 rotational lines carried out using the Stratospheric Observatory for Infrared Astronomy (SOFIA), and pave the way for a better understanding of the high-resolution mapping of H2 emission by future instruments, such as theJames Webb Space Telescope and the Space Infrared Telescope for Cosmology and Astrophysics.

Solution‐Processed Large‐Scale Concentric‐Ring Laser on Two‐Dimensional Ruddlesden–Popper Perovskites Thin Films

2021 ◽  
pp. 2100193
Author(s):  
Peng Liu ◽  
Bingqian Zhang ◽  
Qing Liao ◽  
Guifen Tian ◽  
Chunling Gu ◽  
...  
Keyword(s):  
Thin Films ◽  
Ring Laser ◽  
Large Scale ◽  
Two Dimensional ◽  
Concentric Ring ◽  
Solution Processed

Large-scale visualization of dispersion of liquid-exfoliated two-dimensional nanosheets

2021 ◽  
Author(s):  
Xingyu Cui ◽  
Wen ying Shi ◽  
Chao Lu
Keyword(s):  
Aqueous Solution ◽  
Large Scale ◽  
Fluorescence Microscope ◽  
Visualization Method ◽  
Two Dimensional ◽  
Non Invasive

An ultrafast, non-invasive and large-scale visualization method has been developed to evaluate the dispersion of two-dimensional nanosheets in aqueous solution with fluorescence microscope by formation of excimers from improvement of...

scholarly journals Universality class of the motility-induced critical point in large scale off-lattice simulations of active particles.

Soft Matter ◽  
2021 ◽  
Author(s):  
Claudio Maggi ◽  
Matteo Paoluzzi ◽  
Andrea Crisanti ◽  
Emanuela Zaccarelli ◽  
Nicoletta Gnan
Keyword(s):  
Phase Separation ◽  
Critical Point ◽  
Computer Simulations ◽  
Large Scale ◽  
Universality Class ◽  
Critical Behaviour ◽  
Two Dimensional ◽  
Dimensional Model ◽  
Active Particles ◽  
Two Dimensional Model

We perform large-scale computer simulations of an off-lattice two-dimensional model of active particles undergoing a motility-induced phase separation (MIPS) to investigate the systems critical behaviour close to the critical point...

Unusually High Ion Conductivity in Large-Scale Patternable Two-Dimensional MoS2 Film

ACS Nano ◽  
2021 ◽  
Author(s):  
Juhong Park ◽  
Sanket Bhoyate ◽  
Young-Hoon Kim ◽  
Young-Min Kim ◽  
Young Hee Lee ◽  
...  
Keyword(s):  
Large Scale ◽  
Ion Conductivity ◽  
Two Dimensional ◽  
Mos2 Film

scholarly journals Fabrication of Ultrathin MoS2 Nanosheets and Application on Adsorption of Organic Pollutants and Heavy Metals

Processes ◽  
2020 ◽  
Vol 8 (5) ◽  
pp. 504 ◽  
Author(s):  
Siyi Huang ◽  
Ziyun You ◽  
Yanting Jiang ◽  
Fuxiang Zhang ◽  
Kaiyang Liu ◽  
...  
Keyword(s):  
Heavy Metals ◽  
Electrostatic Interactions ◽  
Large Scale ◽  
Layer Structure ◽  
Structural Characteristics ◽  
Hexagonal Phase ◽  
Two Dimensional ◽  
Mos2 Nanosheets ◽  
Hybrid Strategy ◽  
Ultrathin Mos2 Nanosheets

Owing to their peculiar structural characteristics and potential applications in various fields, the ultrathin MoS2 nanosheets, a typical two-dimensional material, have attracted numerous attentions. In this paper, a hybrid strategy with combination of quenching process and liquid-based exfoliation was employed to fabricate the ultrathin MoS2 nanosheets (MoS2 NS). The obtained MoS2 NS still maintained hexagonal phase (2H-MoS2) and exhibited evident thin layer-structure (1–2 layers) with inconspicuous wrinkle. Besides, the MoS2 NS dispersion showed excellent stability (over 60 days) and high concentration (0.65 ± 0.04 mg mL−1). The MoS2 NS dispersion also displayed evident optical properties, with two characteristic peaks at 615 and 670 nm, and could be quantitatively analyzed with the absorbance at 615 nm in the range of 0.01–0.5 mg mL−1. The adsorption experiments showed that the as-prepared MoS2 NS also exhibited remarkable adsorption performance on the dyes (344.8 and 123.5 mg g−1 of qm for methylene blue and methyl orange, respectively) and heavy metals (185.2, 169.5, and 70.4 mg g−1 of qm for Cd2+, Cu2+, and Ag+). During the adsorption, the main adsorption mechanisms involved the synergism of physical hole-filling effects and electrostatic interactions. This work provided an effective way for the large-scale fabrication of the two-dimensional nanosheets of transition metal dichalcogenides (TMDs) by liquid exfoliation.

Large scale simulations of two-dimensional nonpremixed methane jet flames

2000 ◽  
Vol 123 (4) ◽  
pp. 465-487 ◽  
Author(s):  
S. James ◽  
F.A. Jaberi
Keyword(s):  
Large Scale ◽  
Two Dimensional ◽  
Jet Flames ◽  
Large Scale Simulations

Room Temperature Solvent-Free Synthesis of Monodisperse Magnetite Nanocrystals

2006 ◽  
Vol 6 (3) ◽  
pp. 852-856 ◽  
Author(s):  
X. R. Ye ◽  
C. Daraio ◽  
C. Wang ◽  
J. B. Talbot ◽  
S. Jin
Keyword(s):  
Oleic Acid ◽  
Solid State ◽  
Large Scale ◽  
Room Temperature ◽  
Solvent Free ◽  
Two Dimensional ◽  
New Process ◽  
High Boiling Point ◽  
Magnetite Nanocrystals ◽  
Solvent Free Synthesis

We have successfully demonstrated a facile, solvent-free synthesis of highly crystalline and monodisperse Fe3O4 nanocrystallites at ambient temperature avoiding any heating. Solid state reaction of inorganic Fe(II) and Fe(III) salts with NaOH was found to produce highly crystalline Fe3O4 nanoparticles. The reaction, if carried out in the presence of surfactant such as oleic acid–oleylamine adduct, generated monodisperse Fe3O4 nanocrystals extractable directly from the reaction mixture. The extracted nanoparticles were capable of forming self-assembled, two-dimensional and uniform periodic array. The new process utilizes inexpensive and nontoxic starting materials, and does not require a use of high boiling point and toxic solvents, thus is amenable to an environmentally desirable, large-scale synthesis of nanocrystals.

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