The Origin of High Ice Crystal Number Densities in Cirrus Clouds

2005 ◽  
Vol 62 (7) ◽  
pp. 2568-2579 ◽  
Author(s):  
C. R. Hoyle ◽  
B. P. Luo ◽  
T. Peter
Keyword(s):  
Cirrus Clouds ◽  
Small Scale ◽  
Ice Crystal ◽  
Cooling Rates ◽  
Density Distributions ◽  
In Situ Forming ◽  
Independent Particle ◽  
Scale Temperature ◽  
High Cooling Rates ◽  
Homogeneous Freezing

Abstract Recent measurements with four independent particle instruments in cirrus clouds, which formed without convective or orographic influence, report high number densities of ice particles (as high as nice = 50 cm−3) embedded in broad density distributions (nice = 0.1–50 cm−3). It is shown here that small-scale temperature fluctuations related to gravity waves, mechanical turbulence, or other small-scale air motions are required to explain these observations. These waves have typical peak-to-peak amplitudes of 1–2 K and frequencies of up to 10 h−1, corresponding to instantaneous cooling rates of up to 60 K h−1. Such waves remain unresolved in even the most advanced state-of-the-art global atmospheric models. Given the ubiquitous nature of these fluctuations, it is suggested that the character of young in situ forming cirrus clouds is mostly determined by homogeneous freezing of ice in solution droplets, driven by a broad range of small-scale fluctuations (period ∼a few minutes) with moderate to high cooling rates (1–100 K h−1).

scholarly journals Cirrus clouds in a global climate model with a statistical cirrus cloud scheme

2010 ◽  
Vol 10 (12) ◽  
pp. 5449-5474 ◽  
Author(s):  
M. Wang ◽  
J. E. Penner
Keyword(s):  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Lower Troposphere ◽  
Circulation Model ◽  
Cirrus Clouds ◽  
Cloud Formation ◽  
Cirrus Cloud ◽  
Ice Crystal ◽  
Homogeneous Freezing

Abstract. A statistical cirrus cloud scheme that accounts for mesoscale temperature perturbations is implemented in a coupled aerosol and atmospheric circulation model to better represent both subgrid-scale supersaturation and cloud formation. This new scheme treats the effects of aerosol on cloud formation and ice freezing in an improved manner, and both homogeneous freezing and heterogeneous freezing are included. The scheme is able to better simulate the observed probability distribution of relative humidity compared to the scheme that was implemented in an older version of the model. Heterogeneous ice nuclei (IN) are shown to decrease the frequency of occurrence of supersaturation, and improve the comparison with observations at 192 hPa. Homogeneous freezing alone can not reproduce observed ice crystal number concentrations at low temperatures (<205 K), but the addition of heterogeneous IN improves the comparison somewhat. Increases in heterogeneous IN affect both high level cirrus clouds and low level liquid clouds. Increases in cirrus clouds lead to a more cloudy and moist lower troposphere with less precipitation, effects which we associate with the decreased convective activity. The change in the net cloud forcing is not very sensitive to the change in ice crystal concentrations, but the change in the net radiative flux at the top of the atmosphere is still large because of changes in water vapor. Changes in the magnitude of the assumed mesoscale temperature perturbations by 25% alter the ice crystal number concentrations and the net radiative fluxes by an amount that is comparable to that from a factor of 10 change in the heterogeneous IN number concentrations. Further improvements on the representation of mesoscale temperature perturbations, heterogeneous IN and the competition between homogeneous freezing and heterogeneous freezing are needed.

scholarly journals Balloon-borne match measurements of mid-latitude cirrus clouds

2013 ◽  
Vol 13 (10) ◽  
pp. 25417-25479 ◽  
Author(s):  
A. Cirisan ◽  
B. P. Luo ◽  
I. Engel ◽  
F. G. Wienhold ◽  
U. K. Krieger ◽  
...  
Keyword(s):  
Temperature Fluctuations ◽  
Cloud Microphysics ◽  
Cirrus Clouds ◽  
Climate Feedback ◽  
Small Scale ◽  
Model Parameters ◽  
Air Mass ◽  
Upper Troposphere ◽  
Weather Model ◽  
Scale Temperature

Abstract. Observations of persistent high supersaturations with respect to ice inside cirrus clouds are challenging our understanding of cloud microphysics and of climate feedback processes in the upper troposphere. Single measurements of a cloudy air mass provide only a snapshot from which the persistence of ice supersaturation cannot be judged. We introduce here the "cirrus match technique" to obtain information of the evolution of clouds and their saturation ratio. The aim of these coordinated balloon soundings is to analyze the same air mass twice. To this end the standard radiosonde equipment is complemented by a frost point hygrometer "SnowWhite" and a particle backscatter detector "COBALD" (Compact Optical Backscatter Aerosol Detector). Extensive trajectory calculations based on regional weather model COSMO forecasts are performed for flight planning and COSMO analyses are used as basis for comprehensive microphysical box modeling (with grid scale 2 km and 7 km, respectively). Here we present the results of matching a cirrus cloud to within 2–15 km, realized on 8 June 2010 over Payerne, Switzerland, and a location 120 km downstream close to Zurich. A thick cirrus was detected over both measurement sites. We show that in order to quantitatively reproduce the measured particle backscatter ratios, the small-scale temperature fluctuations not resolved by COSMO must be superimposed on the trajectories. The stochastic nature of the fluctuations is captured by ensemble calculations. Possibilities for further improvements in the agreement with the measured backscatter data are investigated by assuming a very slow mass accommodation of water on ice, the presence of heterogeneous ice nuclei, or a wide span of (spheroidal) particle shapes. However, the resulting improvements from microphysical refinements are moderate and comparable in magnitude with changes caused by assuming different regimes of temperature fluctuations for clear sky or cloudy sky conditions, highlighting the importance of a proper treatment of subscale fluctuations. The model yields good agreement with the measured backscatter over both sites and reproduces the measured saturation ratios with respect to ice over Payerne. Conversely, the 30% in-cloud supersaturation measured in a massive, 4-km thick cloud layer over Zurich cannot be reproduced, irrespective of the choice of meteorological or microphysical model parameters. The measured supersaturation can only be explained by either resorting to an unknown physical process, which prevents the ice particles from consuming the excess humidity, or – much more likely – by a measurement error, such as a contamination of the sensor housing of the SnowWhite hygrometer by a precipitation drop from a mixed phase cloud just below the cirrus layer or from some very slight rain in the boundary layer. This uncertainty calls for in-flight checks or calibrations of hygrometers under the extreme humidity conditions in the upper troposphere.

Jet freezing in enzyme and cosmetic research

1992 ◽  
Vol 50 (1) ◽  
pp. 756-757
Author(s):  
T. Müller ◽  
S. Moser ◽  
M. Vogt ◽  
B.E. Brooker ◽  
N. Terren
Keyword(s):  
Biological Material ◽  
Natural State ◽  
Crystal Formation ◽  
Special Device ◽  
Ice Crystal ◽  
Simultaneous Exposure ◽  
Cooling Rates ◽  
Physical Methods ◽  
Freeze Fracturing ◽  
High Cooling Rates

Freezing has turned out to be the only method capable of immobilizing biological material in its natural state. Freeze-fracturing and replication complete this preparation protocol of specimens for transmission elctron microscopy (TEM) which is based on purely physical methods. With a propane-jet, specimens of a thickness up to 20 μm can be frozen without detectable ice crystal formation, Cell and macromolecule suspensions, emulsions, liquids and polymers in a solvent can be “sandwiched” between two copper foils and kept in place while a coolant is moved very rapidly against the opposite surfaces. In the present jet freezing device (JFD 030) the temperature of the specimen, while residing in a thermostatically controlled chamber, can be monitored between 10 and 90°C immediately prior to freezing. Thus physiologically interesting situations can be immobilized and any precooling of the specimen is avoided. A special device enables the abslutely simultaneous exposure of the specimen to the double-sided jet of the coolant. High cooling rates with an exceptional reproducibility are achieved routinely (Fig.1).

scholarly journals Particle backscatter and relative humidity measured across cirrus clouds and comparison with state-of-the-art cirrus modelling

2012 ◽  
Vol 12 (4) ◽  
pp. 9553-9586
Author(s):  
M. Brabec ◽  
F. G. Wienhold ◽  
B. Luo ◽  
H. Vömel ◽  
F. Immler ◽  
...  
Keyword(s):  
Analysis Data ◽  
Cloud Microphysics ◽  
Cirrus Clouds ◽  
Temperature Fields ◽  
Small Scale ◽  
Ice Cloud ◽  
Scale Temperature ◽  
Modelling Techniques ◽  
Ice Water ◽  
Water Contents

Abstract. Advanced measurement and modelling techniques are employed to determine the partitioning of atmospheric water between the gas phase and the condensed phase in and around cirrus clouds, and thus to identify in-cloud and out-of-cloud supersaturations with respect to ice. In November 2008 the newly developed balloon-borne backscatter sonde COBALD (Compact Optical Backscatter and AerosoL Detector) was flown 14 times together with a CFH (Cryogenic Frost point Hygrometer) from Lindenberg, Germany (52° N, 14° E). The case discussed here in detail shows two cirrus layers with in-cloud relative humidities with respect to ice between 50% and 130%. Global operational analysis data of ECMWF (roughly 1° × 1° horizontal and 1 km vertical resolution, 6-hourly stored fields) fail to represent ice water contents and relative humidities. Conversely, regional COSMO-7 forecasts (6.6 km × 6.6 km, 5-min stored fields) capture the measured humidities and cloud positions remarkably well. The main difference between ECMWF and COSMO data is the resolution of small-scale vertical features responsible for cirrus formation. Nevertheless, ice water contents in COSMO-7 are still off by factors 2–10, likely reflecting limitations in COSMO's ice phase bulk scheme. Significant improvements can be achieved by comprehensive size-resolved microphysical and optical modelling along backward trajectories based on COSMO-7 wind and temperature fields, which allow accurate computation of humidities, ice particle size distributions and backscatter ratios at the COBALD wavelengths. However, only by superimposing small-scale temperature fluctuations, which remain unresolved by the NWP models, can we obtain a satisfying agreement with the observations and reconcile the measured in-cloud non-equilibrium humidities with conventional ice cloud microphysics.

scholarly journals Modelling of cirrus clouds – Part 1b: Structuring cirrus clouds by dynamics

2009 ◽  
Vol 9 (2) ◽  
pp. 707-719 ◽  
Author(s):  
P. Spichtinger ◽  
K. M. Gierens
Keyword(s):  
Large Scale ◽  
Cirrus Clouds ◽  
Small Scale ◽  
Linear Processes ◽  
Microphysics Scheme ◽  
Scale Temperature ◽  
Sensitivity Studies ◽  
Cloud Evolution ◽  
Cloud Ice ◽  
The Impact

Abstract. A recently developed and validated bulk microphysics scheme for modelling cirrus clouds (Spichtinger and Gierens, 2009), implemented into the anelastic non-hydrostatic model EULAG is used for investigation of the impact of dynamics on the evolution of an arctic cirrostratus. Sensitivity studies are performed, using variation of large-scale updraughts as well as addition of small-scale temperature fluctuations and wind shear. The results show the importance of sedimentation of ice crystals on cloud evolution. Due to non-linear processes like homogeneous nucleation situations can arise where small changes in the outer parameters have large effects on the resulting cloud structure. In-cloud ice supersaturation is a common feature of all our simulations, and we show that dynamics is as least as important for its appearance than is microphysics.

scholarly journals The roles of dynamical variability and aerosols in cirrus cloud formation

2003 ◽  
Vol 3 (3) ◽  
pp. 823-838 ◽  
Author(s):  
B. Kärcher ◽  
J. Ström
Keyword(s):  
Gravity Waves ◽  
Probability Distributions ◽  
Cirrus Clouds ◽  
Cloud Formation ◽  
Small Scale ◽  
Cirrus Cloud ◽  
Ice Crystal ◽  
Mesoscale Variability ◽  
Cloud Properties

Abstract. The probability of occurrence of ice crystal number densities in young cirrus clouds is examined based on airborne measurements. The observations have been carried out at midlatitudes in both hemispheres at equivalent latitudes (52-55°N/S) during the same season (local autumn in 2000). The in situ measurements considered in the present study include temperatures, vertical velocities, and total ice crystal concentrations, the latter determined with high precision and accuracy using a counterflow virtual impactor. Most young cirrus clouds typically contain high number densities (1-10 cm-3) of small (diameter <20 mm) ice crystals. This mode dominates the probability distributions and is shown to be caused by rapid cooling rates associated with updraft speeds in the range 10-100 cm s-1. A second mode containing larger crystals extends from ~1 cm-3 to low concentrations close to the detection threshold (~3 x 10-4 cm-3) and could be associated with lower updraft speeds. Results of a statistical analysis provide compelling evidence that the dynamical variability of vertical air motions on the mesoscale is the key factor determining the observed probability distributions of pristine ice crystal concentrations in cirrus. Other factors considered are changes of temperature as well as size, number, and ice nucleation thresholds of the freezing aerosol particles. The variability in vertical velocities is caused by atmospheric gravity waves leading to small-scale temperature fluctuations. Inasmuch as gravity waves are widespread, mesoscale variability in vertical velocities can be viewed as a universal feature of young cirrus clouds. Large-scale models that do not account for this subgrid-scale variability yield erroneous predictions of the variability of basic cirrus cloud properties. Climate change may bring about changes in the global distribution of updraft speeds, mean air temperatures, and aerosol properties. As shown in this work, these changes could significantly modify the probability distribution of cirrus ice crystal concentrations. This study emphasizes the key role of vertical velocities and mesoscale variability in vertical velocities in controlling cirrus properties. The results suggest that, in any effort to ascribe cause to trends of cirrus cloud properties, a careful evaluation of dynamical changes in cloud formation should be done before conclusions regarding the role of other anthropogenic factors, such as changes in aerosol composition, are made.

scholarly journals Cloud chamber experiments on the origin of ice crystal complexity in cirrus clouds

2016 ◽  
Vol 16 (8) ◽  
pp. 5091-5110 ◽  
Author(s):  
Martin Schnaiter ◽  
Emma Järvinen ◽  
Paul Vochezer ◽  
Ahmed Abdelmonem ◽  
Robert Wagner ◽  
...  
Keyword(s):  
Light Scattering ◽  
Cloud Chamber ◽  
Cirrus Clouds ◽  
Small Scale ◽  
Atmospheric Conditions ◽  
Ice Crystal ◽  
Ice Clouds ◽  
Microphysical Properties ◽  
Institute Of Technology ◽  
Low Sensitivity

Abstract. This study reports on the origin of small-scale ice crystal complexity and its influence on the angular light scattering properties of cirrus clouds. Cloud simulation experiments were conducted at the AIDA (Aerosol Interactions and Dynamics in the Atmosphere) cloud chamber of the Karlsruhe Institute of Technology (KIT). A new experimental procedure was applied to grow and sublimate ice particles at defined super- and subsaturated ice conditions and for temperatures in the −40 to −60 °C range. The experiments were performed for ice clouds generated via homogeneous and heterogeneous initial nucleation. Small-scale ice crystal complexity was deduced from measurements of spatially resolved single particle light scattering patterns by the latest version of the Small Ice Detector (SID-3). It was found that a high crystal complexity dominates the microphysics of the simulated clouds and the degree of this complexity is dependent on the available water vapor during the crystal growth. Indications were found that the small-scale crystal complexity is influenced by unfrozen H2SO4 / H2O residuals in the case of homogeneous initial ice nucleation. Angular light scattering functions of the simulated ice clouds were measured by the two currently available airborne polar nephelometers: the polar nephelometer (PN) probe of Laboratoire de Métérologie et Physique (LaMP) and the Particle Habit Imaging and Polar Scattering (PHIPS-HALO) probe of KIT. The measured scattering functions are featureless and flat in the side and backward scattering directions. It was found that these functions have a rather low sensitivity to the small-scale crystal complexity for ice clouds that were grown under typical atmospheric conditions. These results have implications for the microphysical properties of cirrus clouds and for the radiative transfer through these clouds.

scholarly journals Characterization of Arctic mixed-phase cloud properties at small scale and coupling with satellite remote sensing

2017 ◽  
Author(s):  
Guillaume Mioche ◽  
Olivier Jourdan ◽  
Julien Delanoë ◽  
Christophe Gourbeyre ◽  
Guy Febvre ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Crystal Size ◽  
Mixed Phase ◽  
Ice Crystals ◽  
Small Scale ◽  
Vertical Profiles ◽  
Liquid Droplets ◽  
Ice Crystal ◽  
High Concentration ◽  
Ice Crystal Size

Abstract. This study aims to characterize the microphysical and optical properties of ice crystals and supercooled liquid droplets within low-level Arctic mixed-phase clouds (MPC). We compiled and analyzed cloud in situ measurements from 4 airborne campaigns (18 flights, 71 vertical profiles in MPC) over the Greenland Sea and the Svalbard region. Cloud phase discrimination and representative vertical profiles of number, size, mass and shapes of ice crystals and liquid droplets are assessed. The results show that the liquid phase dominates the upper part of the MPC with high concentration of small droplets (120 cm−3, 15&amp;tinsp;μm), and averaged LWC around 0.2 g m−3. The ice phase is found everywhere within the MPC layers, but dominates the properties in the lower part of the cloud and below where ice crystals precipitate down to the surface. The analysis of the ice crystal morphology highlights that irregulars and rimed are the main particle habit followed by stellars and plates. We hypothesize that riming and condensational growth processes (including the Wegener-Bergeron-Findeisein mechanism) are the main growth mechanisms involved in MPC. The differences observed in the vertical profiles of MPC properties from one campaign to another highlight that large values of LWC and high concentration of smaller droplets are possibly linked to polluted situations which lead to very low values of ice crystal size and IWC. On the contrary, clean situations with low temperatures exhibit larger values of ice crystal size and IWC. Several parameterizations relevant for remote sensing or modeling are also determined, such as IWC (and LWC) – extinction relationship, ice and liquid integrated water paths, ice concentration and liquid water fraction according to temperature. Finally, 4 flights collocated with active remote sensing observations from CALIPSO and CloudSat satellites are specifically analyzed to evaluate the cloud detection and cloud thermodynamical phase DARDAR retrievals. This comparison is valuable to assess the sub-pixel variability of the satellite measurements as well as their shortcomings/performance near the ground.

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