Characterization of interactive force acting on colloidal particles near an electrode in presence of a high-frequency (>10 kHz) AC electric field using particle diffusometry

Author(s):  
Kshitiz Gupta ◽  
Dong Hoon Lee ◽  
Steven T. Wereley ◽  
Stuart J. Williams

Colloidal particles like polystyrene beads and metallic micro and nanoparticles are known to assemble in crystal-like structures near an electrode surface under both DC and AC electric fields. Various studies have shown that this self-assembly is governed by a balance between an attractive electrohydrodynamic (EHD) force and an induced dipole-dipole repulsion (Trau et al., 1997). The EHD force originates from electrolyte flow caused by interaction between the electric field and the polarized double layers of both the particles and the electrode surface. The particles are found to either aggregate or repel from each other on application of electric field depending on the mobility of the ions in the electrolyte (Woehl et al., 2014). The particle motion in the electrode plane is studied well under various conditions however, not as many references are available in the literature that discuss the effects of the AC electric field on their out-of-plane motion, especially at high frequencies (>10 kHz). Haughey and Earnshaw (1998), and Fagan et al. (2005) have studied the particle motion perpendicular to the electrode plane and their average height from the electrode mostly in presence of DC or low frequency AC (<1 kHz) electric field. However, these studies do not provide enough insight towards the effects of high frequency (>10 kHz) electric field on the particles’ motion perpendicular to the electrode plane.  

2003 ◽  
Vol 10 (1/2) ◽  
pp. 45-52 ◽  
Author(s):  
R. E. Ergun ◽  
L. Andersson ◽  
C. W. Carlson ◽  
D. L. Newman ◽  
M. V. Goldman

Abstract. Direct observations of magnetic-field-aligned (parallel) electric fields in the downward current region of the aurora provide decisive evidence of naturally occurring double layers. We report measurements of parallel electric fields, electron fluxes and ion fluxes related to double layers that are responsible for particle acceleration. The observations suggest that parallel electric fields organize into a structure of three distinct, narrowly-confined regions along the magnetic field (B). In the "ramp" region, the measured parallel electric field forms a nearly-monotonic potential ramp that is localized to ~ 10 Debye lengths along B. The ramp is moving parallel to B at the ion acoustic speed (vs) and in the same direction as the accelerated electrons. On the high-potential side of the ramp, in the "beam" region, an unstable electron beam is seen for roughly another 10 Debye lengths along B. The electron beam is rapidly stabilized by intense electrostatic waves and nonlinear structures interpreted as electron phase-space holes. The "wave" region is physically separated from the ramp by the beam region. Numerical simulations reproduce a similar ramp structure, beam region, electrostatic turbulence region and plasma characteristics as seen in the observations. These results suggest that large double layers can account for the parallel electric field in the downward current region and that intense electrostatic turbulence rapidly stabilizes the accelerated electron distributions. These results also demonstrate that parallel electric fields are directly associated with the generation of large-amplitude electron phase-space holes and plasma waves.


2001 ◽  
Vol 114 (8) ◽  
pp. 1515-1520 ◽  
Author(s):  
A.J. Rosenspire ◽  
A.L. Kindzelskii ◽  
H.R. Petty

Previously, we have demonstrated that NAD(P)H levels in neutrophils and macrophages are oscillatory. We have also found that weak ultra low frequency AC or pulsed DC electric fields can resonate with, and increase the amplitude of, NAD(P)H oscillations in these cells. For these cells, increased NAD(P)H amplitudes directly signal changes in behavior in the absence of cytokines or chemotactic factors. Here, we have studied the effect of pulsed DC electric fields on HT-1080 fibrosarcoma cells. As in neutrophils and macrophages, NAD(P)H levels oscillate. We find that weak (~10(-)(5) V/m), but properly phased DC (pulsed) electric fields, resonate with NAD(P)H oscillations in polarized and migratory, but not spherical, HT-1080 cells. In this instance, electric field resonance signals an increase in HT-1080 pericellular proteolytic activity. Electric field resonance also triggers an immediate increase in the production of reactive oxygen metabolites. Under resonance conditions, we find evidence of DNA damage in HT-1080 cells in as little as 5 minutes. Thus the ability of external electric fields to effect cell function and physiology by acting on NAD(P)H oscillations is not restricted to cells of the hematopoietic lineage, but may be a universal property of many, if not all polarized and migratory eukaryotic cells.


2006 ◽  
Vol 05 (04n05) ◽  
pp. 389-394
Author(s):  
CHANGXIN CHEN ◽  
YAFEI ZHANG

Dispersed aligned single-wall carbon nanotube (SWCNT) array has been formed between electrodes by electric field assisted alignment of surface decorated SWCNTs. The surface decoration of SWCNTs with functional molecules allows them to dispersedly bridge metal electrodes and effectively obviates the entanglement between SWCNTs. The influences of solution volatility and electric-field type on the alignment are investigated. It is indicated that the well-oriented SWCNT array can be achieved by using the high-volatility solvent and the high-frequency AC electric field to align SWCNTs.


2010 ◽  
Vol 6 (1) ◽  
pp. 31 ◽  
Author(s):  
Cristina Peratta ◽  
Andres Peratta ◽  
Dragan Poljak

The paper introduces a three dimensional multidomainboundary element model of a pregnant woman and foetus for the analysis of exposure to high voltage extremely low frequency electric fields. The definition of the differentphysical and geometrical properties of the relevant tissues is established according to medical information available in existing literature. The model takes into account changes in geometry, body mass, body fat, and overall chemical composition in the body which influence the electrical properties, throughout the different gestational periods. The developed model is used to solve the case of exposure to overhead power transmission lines at different stages of pregnancy including weeks 8, 13, 26 and 38. The results obtained are in line with those published in the earlier works considering different approaches. In addition, a sensitivity analysis involving varying scenarios of conductivity, foetus postures and geometry for each stage is defined and solved. Finally, a correlation between the externally applied electric field and the current density inside the foetus is established and the zones of maximum exposure are identified.


1996 ◽  
Vol 160 ◽  
pp. 181-182
Author(s):  
Jan Kuijpers ◽  
Martin Volwerk

Radiation from a charge accelerated along its path or Linear Acceleration Emission (LAE) involves a number of subtleties (Pauli 1921; Ginzburg 1970, 1989). Potential interest of the mechanism for astrophysics has been pointed out by Wagoner (1969). Melrose (1978) and Rowe (1995) have studied amplified LAE from time-varying electric fields for radio pulsars. In contrast with the latter work our calculations are for static electric field structures or double layers (DLs) as are thought to occur in magnetospheres of neutron stars. In ordinary stellar atmospheres a LAE maser can operate in non-relativistic DLs (Kuijpers 1990) at a frequencyω≈kDLυ≈ 2π/ttr, and a wave vectorwithkDL= 2π/L(Lis the DL length,υis the particle speed, andttris the transit time of the DL by the particle). The emission process can be considered as scattering of the electrostatic electric field on fast electrons into electromagnetic radiation satisfying the resonance condition:, when the frequency of the radiated mode in the frame of the emitting electron equals the Doppler shifted frequency of the electric field of the DL (DL wave frequencyωDL≈ 0). For relativistic DLs, as are applicable to pulsar magnetospheres, the emission is expected to be beamed under an angleθ≈γ−1and the frequency of emission boosted (ω≈kDLυ(1 −υcosθ/c)−1≈γ2kDLυ).


2020 ◽  
Vol 10 (1) ◽  
Author(s):  
Jun-Yong Lee ◽  
Jeong-Seon Yu ◽  
Jong-Hyun Kim

Abstract Colloidal particles dispersed in nematic liquid crystals are aligned along the orientation that minimizes the elastic free energy. Through applying an electric field to a nematic colloidal system, the orientation of the director can change. Consequently, colloidal particles realign to minimize the total free energy, which is the sum of the elastic and electric free energies. Herein, we demonstrate that if the preferred rotation directions given by the electric and elastic free energies are different during realignment, the rotation direction of the particle can be controlled by how we apply the electric field. When the strength of the electric field gradually increases, the particles rotate in the same direction as the rotation of the director. However, when a sufficiently high electric field is suddenly applied, the particles rotate in the opposite direction. In this study, we analyzed the effect of free energy on the bidirectional rotation behavior of the particles using a theoretical model. This study provides an effective approach to control the rotational behavior of colloidal particles over a wide-angle range between two orientational local minima.


1986 ◽  
Vol 73 ◽  
Author(s):  
Alan J. Hurd

ABSTRACTA technique for inducing ordered, close-packed arrangements of various symmetries among colloidal particles is discussed. An external alternating electric field applied to the colloid induces dipole interactions of variable strength by polarizing either the dielectric material of the particles or their electrostatic double layers. Ordering in various symmetries can be obtained by switching the field rapidly between pairs of electrodes, thereby changing the orientation of the induced dipoles. A small dc bias serves to deposit and compact the aligned particles.


Author(s):  
Minami Yoda ◽  
Necmettin Cevheri

Manipulating suspended neutrally buoyant colloidal particles of radii a = O(0.1 μm–1 μm) near solid surfaces, or walls, is a key technology in various microfluidics devices. These particles, suspended in an aqueous solution at rest near a solid surface, or wall, are subject to wall-normal “lift” forces described by the DLVO theory of colloid science. The particles experience additional lift forces, however, when suspended in a flowing solution. A fundamental understanding of such lift forces could therefore lead to new methods for the transport and self-assembly of particles near and on solid surfaces. Various studies have reported repulsive electroviscous and hydrodynamic lift forces on colloidal particles in Poiseuille flow (with a constant shear rate γ̇ near the wall) driven by a pressure gradient. A few studies have also observed repulsive dielectrophoretic-like lift forces in electroosmotic (EO) flows driven by electric fields. Recently, evanescent-wave particle tracking has been used to quantify near-wall lift forces on a = 125 nm–245 nm polystyrene (PS) particles suspended in a monovalent electrolyte solution in EO flow, Poiseuille flow, and combined Poiseuille and EO flow through ∼30 μm deep fused-silica channels. In Poiseuille flow, the repulsive lift force appears to be proportional to γ̇, a scaling consistent with hydrodynamic, vs. electroviscous, lift. In combined Poiseuille and EO flow, the lift forces can be repulsive or attractive, depending upon whether the EO flow is in the same or opposite direction as the Poiseuille flow, respectively. The magnitude of the force appears to be proportional to the electric field magnitude. Moreover, the force in combined flow exceeds the sum of the forces observed in EO flow for the same electric field or in Poiseuille flow for the same γ̇. Initial results also imply that this force, when repulsive, scales as γ̇1/2. These results suggest that the lift force in combined flow is fundamentally different from electroviscous, hydrodynamic, or dielectrophoretic-like lift. Moreover, for the case when the EO flow opposes the Poiseuille flow, the particles self-assemble into dense stable periodic streamwise bands with an average width of ∼6 μm and a spacing of 2–4 times the band width when the electric field magnitude exceeds a threshold value. These results are described and reviewed here.


Author(s):  
Chunzhen Ye ◽  
Dongqing Li

This paper considers the electrophoretic motion of multiple spheres in an aqueous electrolyte solution in a straight rectangular microchannel, where the size of the channel is close to that of the particles. This is a complicated 3-D transient process where the electric field, the flow field and the particle motion are coupled together. The objective is to numerically investigate how one particle influences the electric field and the flow field surrounding the other particle and the particle moving velocity. It is also aimed to investigate and demonstrate that the effects of particle size and electrokinetic properties on particle moving velocity. Under the assumption of thin electrical double layers, the electroosmotic flow velocity is used to describe the flow in the inner region. The model governing the electric field and the flow field in the outer region and the particle motion is developed. A direct numerical simulation method using the finite element method is adopted to solve the model. The numerical results show that the presence of one particle influences the electric field and the flow field adjacent to the other particle and the particle motion, and that this influences weaken when the separation distance becomes bigger. The particle motion is dependent on its size, with the smaller particle moving a little faster. In addition, the zeta potential of particle has an effective influence on the particle motion. For a faster particle moving from behind a slower one, numerical results show that the faster moving particle will climb and then pass the slower moving particle then two particles’ centers are not located on a line parallel to the electric field.


1980 ◽  
Vol 239 (5) ◽  
pp. R424-R427 ◽  
Author(s):  
A. A. Marino ◽  
J. M. Cullen ◽  
M. Reichmanis ◽  
R. O. Becker ◽  
F. X. Hart

The action of a 60-Hz, 5 kV/m electric field on erythrocyte parameters in mice was determined. No effects attributable to the magnitude of the field were found, but a transition either from or to an environment containing the field caused decreased red blood cell concentrations and decreased hematocrits. The failure of others to observe effects on erythrocyte parameters following exposure to low-frequency electric fields may have been due to an inappropriate choice of duration of exposure.


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