scholarly journals Discovery of a New Ozone Hole over the Tropics

2022 ◽  
Author(s):  
Qing-Bin Lu
Keyword(s):  
Lower Stratosphere ◽  
Global Climate ◽  
Ground Level ◽  
Ozone Hole ◽  
The Arctic ◽  
Ozone Loss ◽  
Global Concern ◽  
Antarctic Ozone ◽  
Stratospheric Cooling ◽  
The Tropics

Abstract This paper reveals a new ozone hole that exists in the lower stratosphere over the tropics (30°N-30°S) across the seasons since the 1980s, where an ozone hole is defined as an area of ozone loss larger than 25% compared with the undisturbed atmosphere. The depth of this all-season tropical ozone hole is comparable to that of the well-known springtime ozone hole over Antarctica, while its area is about seven times that of the latter. At the center of the deepest tropical or Antarctic ozone hole, approximately 80% of the normal ozone value is depleted, whereas annual mean ozone depletion in the lower stratosphere over the tropics due to the coldest temperature is about 1.6 times that over Antarctica and is about 7.7 times that over the Arctic. The whole-year ozone hole over the tropics could cause a serious global concern as it can lead to increases in ground-level ultraviolet radiation and affect 50% of Earth's surface area, which is home to approximately 50% of the world's population. Moreover, since ozone loss is well-known to lead to stratospheric cooling, the presence of the all-season tropical ozone hole and the seasonal polar ozone holes is equivalent to the formation of three ‘temperature holes’ in the global lower stratosphere. These findings will play a far-reaching role in understanding fundamental atmospheric processes and global climate change.

scholarly journals Differences in Arctic and Antarctic PSC occurrence as observed by lidar in Ny-Ålesund (79° N, 12° E) and McMurdo (78° S, 167° E)

2005 ◽  
Vol 5 (8) ◽  
pp. 2081-2090 ◽  
Author(s):  
M. Maturilli ◽  
R. Neuber ◽  
P. Massoli ◽  
F. Cairo ◽  
A. Adriani ◽  
...  
Keyword(s):  
Large Fraction ◽  
Particle Surface ◽  
The Arctic ◽  
Ozone Loss ◽  
Polar Stratospheric Cloud ◽  
Antarctic Ozone ◽  
Stratospheric Cooling ◽  
Hole Dimensions ◽  
Activation Rates ◽  
The Relationship

Abstract. The extent of springtime Arctic ozone loss does not reach Antarctic ``ozone hole'' dimensions because of the generally higher temperatures in the northern hemisphere vortex and consequent less polar stratospheric cloud (PSC) particle surface for heterogeneous chlorine activation. Yet, with increasing greenhouse gases stratospheric temperatures are expected to further decrease. To infer if present Antarctic PSC occurrence can be applied to predict future Arctic PSC occurrence, lidar observations from McMurdo station (78° S, 167° E) and NyÅlesund (79° N, 12° E) have been analysed for the 9 winters between 1995 (1995/1996) and 2003 (2003/2004). Although the statistics may not completely cover the overall hemispheric PSC occurrence, the observations are considered to represent the main synoptic cloud features as both stations are mostly situated in the centre or at the inner edge of the vortex. Since the focus is set on the occurrence frequency of solid and liquid particles, the analysis has been restricted to volcanic aerosol free conditions. In McMurdo, by far the largest part of PSC observations is associated with NAT PSCs. The observed persistent background of NAT particles and their potential ability to cause denoxification and irreversible denitrification is presumably more important to Antarctic ozone chemistry than the scarcely observed ice PSCs. Meanwhile in Ny-Ålesund, ice PSCs have never been observed, while solid NAT and liquid STS clouds both occur in large fraction. Although they are also found solely, the majority of observations reveals solid and liquid particle layers in the same profile. For the Ny-Ålesund measurements, the frequent occurrence of liquid PSC particles yields major significance in terms of ozone chemistry, as their chlorine activation rates are more efficient. The relationship between temperature, PSC formation, and denitrification is nonlinear and the McMurdo and Ny-Ålesund PSC observations imply that for predicted stratospheric cooling it is not possible to directly apply current Antarctic PSC occurrence to the Arctic stratosphere. Future Arctic PSC occurrence, and thus ozone loss, is likely to depend on the shape and barotropy of the vortex rather than on minimum temperature alone.

scholarly journals Differences in Arctic and Antarctic PSC occurrence as observed by lidar in Ny-Ålesund (79° N, 12° E) and McMurdo (78° S, 167° E)

2004 ◽  
Vol 4 (5) ◽  
pp. 6837-6866 ◽  
Author(s):  
M. Müller ◽  
R. Neuber ◽  
P. Massoli ◽  
F. Cairo ◽  
A. Adriani ◽  
...  
Keyword(s):  
Large Fraction ◽  
Particle Surface ◽  
The Arctic ◽  
Type Ii ◽  
Ozone Loss ◽  
Type Ia ◽  
Antarctic Ozone ◽  
Stratospheric Cooling ◽  
Hole Dimensions ◽  
Activation Rates

Abstract. The extent of springtime Arctic ozone loss does not reach Antarctic "ozone hole" dimensions because of the generally higher temperatures in the northern hemisphere vortex and consequent less polar stratospheric cloud (PSC) particle surface for heterogeneous chlorine activation. Yet, with increasing greenhouse gases stratospheric temperatures are expected to further decrease. To infer if present Antarctic PSC occurrence can be applied to predict future Arctic PSC occurrence, lidar observations from McMurdo station (78° S, 167° E) and Ny-Ålesund (79° N, 12° E) have been analysed for the 9 winters between 1995 (1995/1996) and 2003 (2003/2004). Although the statistics may not completely cover the overall hemispheric PSC occurrence, the observations are considered to represent the main synoptic cloud features as both stations are mostly situated in the centre or at the inner edge of the vortex. Since the focus is set on the occurrence frequency of solid and liquid particles, the analysis has been restricted to volcanic aerosol free conditions. In McMurdo, by far the largest part of PSC observations is associated with PSC type Ia. The observed constant background of NAT particles and their potential ability to cause denoxification and irreversible denitrification is presumably more important to Antarctic ozone chemistry than the scarcely observed PSC type II. Meanwhile in Ny-Ålesund, PSC type II has never been observed, while type Ia and Ib both occur in large fraction. Although they are also found solely, the majority of observations reveals solid and liquid particle layers in the same profile. For the Ny-Ålesund measurements, the frequent occurrence of liquid PSC particles yields major significance in terms of ozone chemistry, as their chlorine activation rates are more efficient. The relationship between temperature, PSC formation, and denitrification is nonlinear and the McMurdo and Ny-Ålesund PSC observations imply that for predicted stratospheric cooling it is not possible to directly apply current Antarctic PSC occurrence directly to the Arctic stratosphere. Future Arctic PSC occurrence, and thus ozone loss, will depend on the shape and barotropy of the vortex rather than on the minimum temperatures.

scholarly journals Arctic on the verge of an ozone hole?

2021 ◽  
Author(s):  
Jayanarayanan Kuttippurath ◽  
Wuhu Feng ◽  
Rolf Müller ◽  
Pankaj Kumar ◽  
Sarath Raj ◽  
...  
Keyword(s):  
Ultra Violet ◽  
Ozone Hole ◽  
The Arctic ◽  
Extreme Weather Events ◽  
Ozone Loss ◽  
Ultra Violet Radiation ◽  
Weather Events ◽  
Antarctic Ozone ◽  
Near Future ◽  
First Time

Abstract. Severe vortex-wide ozone loss in the Arctic would expose nearly 650 million people and ecosystem to unhealthy ultra-violet radiation levels. Adding to these worries, and extreme weather events as the harbingers of climate change, clear signature of an ozone hole (ozone column values below 220 DU) appeared over the Arctic in March and April 2020. Sporadic occurrences of ozone hole values at different regions of vortex for almost three weeks were found for the first time in the observed history in the Arctic. Furthermore, a record-breaking ozone loss of about 2.0–3.4 ppmv triggered by an unprecedented chlorine activation (1.5–2.2 ppbv) matching to the levels of Antarctic ozone hole conditions was also observed. The polar processing situation led to the first-ever appearance of loss saturation in the Arctic. Apart from these, there were also ozone-mini holes in December 2019 and January 2020 driven by atmospheric dynamics. The large loss in ozone in the colder Arctic winters is intriguing and that demands rigorous monitoring of the region. Our study suggests that the very colder Arctic winters in near future would also very likely to experience even more ozone loss and encounter ozone hole situations, provided the stratospheric chlorine levels still stay high there.

scholarly journals Polar processing in a split vortex: early winter Arctic ozone loss in 2012/13

2015 ◽  
Vol 15 (4) ◽  
pp. 4973-5029 ◽  
Author(s):  
G. L. Manney ◽  
Z. D. Lawrence ◽  
M. L. Santee ◽  
N. J. Livesey ◽  
A. Lambert ◽  
...  
Keyword(s):  
Nitric Acid ◽  
Lower Stratosphere ◽  
Polar Vortex ◽  
The Arctic ◽  
Early Winter ◽  
Sudden Stratospheric Warming ◽  
Ozone Loss ◽  
Chlorine Monoxide ◽  
Polar Stratospheric Cloud ◽  
Vortex Split

Abstract. A sudden stratospheric warming (SSW) in early January 2013 caused the polar vortex to split. After the lower stratospheric vortex split on 8 January, the two offspring vortices – one over Canada and the other over Siberia – remained intact, well-confined, and largely at latitudes that received sunlight until they reunited at the end of January. As the SSW began, temperatures abruptly rose above chlorine activation thresholds throughout the lower stratosphere. The vortex was very disturbed prior to the SSW, and was exposed to much more sunlight than usual in December 2012 and January 2013. Aura Microwave Limb Sounder (MLS) nitric acid (HNO3) data and observations from CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) indicate extensive polar stratospheric cloud (PSC) activity, with evidence of PSCs containing solid nitric acid trihydrate particles during much of December 2012. Consistent with the sunlight exposure and PSC activity, MLS observations show that chlorine monoxide (ClO) became enhanced early in December. Despite the cessation of PSC activity with the onset of the SSW, enhanced vortex ClO persisted until mid-February, indicating lingering chlorine activation. The smaller Canadian offspring vortex had lower temperatures, lower HNO3, lower hydrogen chloride (HCl), and higher ClO in late January than the Siberian vortex. Chlorine deactivation began later in the Canadian than in the Siberian vortex. HNO3 remained depressed within the vortices after temperatures rose above the PSC existence threshold, and passive transport calculations indicate vortex-averaged denitrification of about 4 ppbv; the resulting low HNO3 values persisted until the vortex dissipated in mid-February. Consistent with the strong chlorine activation and exposure to sunlight, MLS measurements show rapid ozone loss commencing in mid-December and continuing through January. Lagrangian transport estimates suggest ~ 0.7–0.8 ppmv (parts per million by volume) vortex-averaged chemical ozone loss by late January near 500 K (~ 21 km), with substantial loss occurring from ~ 450 to 550 K. The surface area of PSCs in December 2012 was larger than that in any other December observed by CALIPSO. As a result of denitrification, HNO3 abundances in 2012/13 were among the lowest in the MLS record for the Arctic. ClO enhancement was much greater in December 2012 through mid-January 2013 than that at the corresponding time in any other Arctic winter observed by MLS. Furthermore, reformation of HCl appeared to play a greater role in chlorine deactivation than in more typical Arctic winters. Ozone loss in December 2012 and January 2013 was larger than any previously observed in those months. This pattern of exceptional early winter polar processing and ozone loss resulted from the unique combination of dynamical conditions associated with the early January 2013 SSW, namely unusually low temperatures in December 2012 and offspring vortices that remained well-confined and largely in sunlit regions for about a month after the vortex split.

The Impact of Ozone-Depleting Substances on Tropical Upwelling, as Revealed by the Absence of Lower-Stratospheric Cooling since the Late 1990s

2017 ◽  
Vol 30 (7) ◽  
pp. 2523-2534 ◽  
Author(s):  
Lorenzo M. Polvani ◽  
Lei Wang ◽  
Valentina Aquila ◽  
Darryn W. Waugh
Keyword(s):  
Greenhouse Gases ◽  
Lower Stratosphere ◽  
Stratospheric Temperature ◽  
Temperature Trends ◽  
Ozone Trends ◽  
Primary Driver ◽  
Stratospheric Cooling ◽  
Ozone Depleting Substances ◽  
The Tropics ◽  
The Impact

The impact of ozone-depleting substances on global lower-stratospheric temperature trends is widely recognized. In the tropics, however, understanding lower-stratospheric temperature trends has proven more challenging. While the tropical lower-stratospheric cooling observed from 1979 to 1997 has been linked to tropical ozone decreases, those ozone trends cannot be of chemical origin, as active chlorine is not abundant in the tropical lower stratosphere. The 1979–97 tropical ozone trends are believed to originate from enhanced upwelling, which, it is often stated, would be driven by increasing concentrations of well-mixed greenhouse gases. This study, using simple arguments based on observational evidence after 1997, combined with model integrations with incrementally added single forcings, argues that trends in ozone-depleting substances, not well-mixed greenhouse gases, have been the primary driver of temperature and ozone trends in the tropical lower stratosphere until 1997, and this has occurred because ozone-depleting substances are key drivers of tropical upwelling and, more generally, of the entire Brewer–Dobson circulation.

scholarly journals Dynamics of the Disrupted 2015/16 Quasi-Biennial Oscillation

2017 ◽  
Vol 30 (15) ◽  
pp. 5661-5674 ◽  
Author(s):  
Lawrence Coy ◽  
Paul A. Newman ◽  
Steven Pawson ◽  
Leslie R. Lait
Keyword(s):  
Lower Stratosphere ◽  
Global Climate ◽  
Quasi Biennial Oscillation ◽  
Wave Forcing ◽  
Wind Variability ◽  
Momentum Fluxes ◽  
Horizontal Momentum ◽  
The Tropics ◽  
Global Reanalysis ◽  
Biennial Oscillation

A significant disruption of the quasi-biennial oscillation (QBO) occurred during the Northern Hemisphere (NH) winter of 2015/16. Since the QBO is the major wind variability source in the tropical lower stratosphere and influences the rate of ascent of air entering the stratosphere, understanding the cause of this singular disruption may provide new insights into the variability and sensitivity of the global climate system. Here this disruptive event is examined using global reanalysis winds and temperatures from 1980 to 2016. Results reveal record maxima in tropical horizontal momentum fluxes and wave forcing of the tropical zonal mean zonal wind over the NH 2015/16 winter. The Rossby waves responsible for these record tropical values appear to originate in the NH and were focused strongly into the tropics at the 40-hPa level. Two additional NH winters, 1987/88 and 2010/11, were also found to have large tropical lower-stratospheric momentum flux divergences; however, the QBO westerlies did not change to easterlies in those cases.

scholarly journals Intercomparison of temperature trends in IPCC CMIP5 simulations with observations, reanalyses and CMIP3 models

2013 ◽  
Vol 6 (5) ◽  
pp. 1705-1714 ◽  
Author(s):  
J. Xu ◽  
L. Zhao ◽  
Keyword(s):  
Coupled Model ◽  
Temperature Trend ◽  
The Arctic ◽  
Cmip5 Models ◽  
Model Intercomparison ◽  
Model Simulations ◽  
Temperature Trends ◽  
Intercomparison Project ◽  
Stratospheric Cooling ◽  
The Tropics

Abstract. On the basis of the fifth Coupled Model Intercomparison Project (CMIP5) and the climate model simulations covering 1979 through 2005, the temperature trends and their uncertainties have been examined to note the similarities or differences compared to the radiosonde observations, reanalyses and the third Coupled Model Intercomparison Project (CMIP3) simulations. The results show noticeable discrepancies for the estimated temperature trends in the four data groups (radiosonde, reanalysis, CMIP3 and CMIP5), although similarities can be observed. Compared to the CMIP3 model simulations, the simulations in some of the CMIP5 models were improved. The CMIP5 models displayed a negative temperature trend in the stratosphere closer to the strong negative trend seen in the observations. However, the positive tropospheric trend in the tropics is overestimated by the CMIP5 models relative to CMIP3 models. While some of the models produce temperature trend patterns more highly correlated with the observed patterns in CMIP5, the other models (such as CCSM4 and IPSL_CM5A-LR) exhibit the reverse tendency. The CMIP5 temperature trend uncertainty was significantly reduced in most areas, especially in the Arctic and Antarctic stratosphere, compared to the CMIP3 simulations. Similar to the CMIP3, the CMIP5 simulations overestimated the tropospheric warming in the tropics and Southern Hemisphere and underestimated the stratospheric cooling. The crossover point where tropospheric warming changes into stratospheric cooling occurred near 100 hPa in the tropics, which is higher than in the radiosonde and reanalysis data. The result is likely related to the overestimation of convective activity over the tropical areas in both the CMIP3 and CMIP5 models. Generally, for the temperature trend estimates associated with the numerical models including the reanalyses and global climate models, the uncertainty in the stratosphere is much larger than that in the troposphere, and the uncertainty in the Antarctic is the largest. In addition, note that the reanalyses show the largest uncertainty in the lower tropical stratosphere, and the CMIP3 simulations show the largest uncertainty in both the south and north polar regions.

scholarly journals Effects of injected ice particles in the lower stratosphere on the Antarctic ozone hole

2015 ◽  
Vol 3 (5) ◽  
pp. 143-158 ◽  
Author(s):  
H. Nagase ◽  
D. E. Kinnison ◽  
A. K. Petersen ◽  
F. Vitt ◽  
G. P. Brasseur
Keyword(s):  
Lower Stratosphere ◽  
Ozone Hole ◽  
Ice Particles ◽  
Antarctic Ozone ◽  
The Antarctic ◽  
Antarctic Ozone Hole

scholarly journals Three-dimensional model study of the arctic ozone loss in 2002/2003 and comparison with 1999/2000 and 2003/2004

2004 ◽  
Vol 4 (5) ◽  
pp. 5045-5074
Author(s):  
W. Feng ◽  
M. P. Chipperfield ◽  
S. Davies ◽  
B. Sen ◽  
G. Toon ◽  
...  
Keyword(s):  
Lower Stratosphere ◽  
Transport Model ◽  
Current Model ◽  
Vertical Motion ◽  
Horizontal Resolution ◽  
The Arctic ◽  
Chemical Transport Model ◽  
Three Dimensional Model ◽  
Vertical Coordinate ◽  
Ozone Loss

Abstract. We have used the SLIMCAT 3-D off-line chemical transport model (CTM) to quantify the Arctic chemical ozone loss in the year 2002/2003 and compare it with similar calculations for the winters 1999/2000 and 2003/2004. Recent changes to the CTM have improved the model's ability to reproduce polar chemical and dynamical processes. The updated CTM uses σ-θ as a vertical coordinate which allows it to extend down to the surface. The CTM has a detailed stratospheric chemistry scheme and now includes a simple NAT-based denitrification scheme in the stratosphere. In the model runs presented here the model was forced by ECMWF ERA40 and operational analyses. The model used 24 levels extending from the surface to ~55 km and a horizontal resolution of either 7.5°×7.5° or 2.8°×2.8°. Two different radiation schemes, MIDRAD and the CCM scheme, were used to diagnose the vertical motion in the stratosphere. Based on tracer observations from balloons and aircraft, the more sophisticated CCM scheme gives a better representation of the vertical transport in this model which includes the troposphere. The higher resolution model generally produces larger chemical O3 depletion, which agrees better with observations. The CTM results show that very early chemical ozone loss occurred in December 2002 due to extremely low temperatures and early chlorine activation in the lower stratosphere. Thus, chemical loss in this winter started earlier than in the other two winters studied here. In 2002/2003 the local polar ozone loss in the lower stratosphere was ~40% before the stratospheric final warming. Larger ozone loss occurred in the cold year 1999/2000 which had a persistently cold and stable vortex during most of the winter. For this winter the current model, at a resolution of 2.8°×2.8°, can reproduce the observed loss of over 70% locally. In the warm and more disturbed winter 2003/2004 the chemical O3 loss was generally much smaller, except above 620 K where large losses occurred due to a period of very low minimum temperatures at these altitudes.

Peatlands

Ecology ◽  
2012 ◽  
Author(s):  
Dale H. Vitt
Keyword(s):  
Global Climate Change ◽  
Land Surface ◽  
Net Primary Production ◽  
Global Climate ◽  
High Water ◽  
The Arctic ◽  
Nutrient Inputs ◽  
C And N ◽  
The Tropics

Peatland ecosystems are characterized by a substantial accumulation of organic matter in soil (peat), resulting from long-term excess of net primary production at the surface compared to decomposition throughout the peat column. Globally, peatlands cover 3–4 percent of the earth’s land surface, yet they store 25–30 percent of the world’s soil carbon (about 455 Pg of C) and 9–16 percent of the world’s soil nitrogen (8–15 Pg of N) in peat. These large stores of C and N are especially vulnerable to global climate change. Although peatlands occur from the tropics to the Arctic, it is in the boreal region where peatlands are most abundant. The presence of a well-developed ground layer of mosses along with either abundant shrubs or sedges makes the population and community ecology of these ecosystems interesting and challenging. The high water table, presence of anoxia, and isolation from all nutrient inputs—except the atmosphere in some peatlands (bogs)—present unique opportunities to study the hydrology and biogeochemistry.

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