Discovery of a New Ozone Hole over the Tropics

This paper reveals a new ozone hole that exists in the lower stratosphere over the tropics (30°N-30°S) across the seasons since the 1980s, where an ozone hole is defined as an area of ozone loss larger than 25% compared with the undisturbed atmosphere. The depth of this all-season tropical ozone hole is comparable to that of the well-known springtime ozone hole over Antarctica, while its area is about seven times that of the latter. At the center of the deepest tropical or Antarctic ozone hole, approximately 80% of the normal ozone value is depleted, whereas annual mean ozone depletion in the lower stratosphere over the tropics due to the coldest temperature is about 1.6 times that over Antarctica and is about 7.7 times that over the Arctic. The whole-year ozone hole over the tropics could cause a serious global concern as it can lead to increases in ground-level ultraviolet radiation and affect 50% of Earth's surface area, which is home to approximately 50% of the world's population. Moreover, since ozone loss is well-known to lead to stratospheric cooling, the presence of the all-season tropical ozone hole and the seasonal polar ozone holes is equivalent to the formation of three ‘temperature holes’ in the global lower stratosphere. These findings will play a far-reaching role in understanding fundamental atmospheric processes and global climate change.

Antarctic ozone recovery

Since 1976, and more so since 1985, the Antarctic ozone level has suffered considerable depletion (termed as Antarctic ozone hole), attributed to the destructive effects of CFC compounds leaking into the atmosphere from man-made gadgets. The 12-month running means of South Pole Dobson ozone (monthly means, upto 1999 end only) were subjected to spectral analysis, which showed considerable, significant amplitudes for QBO (Quasi-biennial, 2-3 years) and QTO (Quasi-triennial, 3-4 years) oscillations, with a total range of 20-30 DU. When subtracted from the original values, a fairly smooth variation was seen, with a decrease from ~260 DU in 1986 to ~230 DU in 1996 (~12% decrease in 12-month running means), and an almost steady level thereafter. Thus, the net ozone variation at South Pole consists of two parts, (i) a long-term monotonically downward trend upto 1996 and a steady level thereafter and (ii) a superposed QBO-QTO oscillation. The chemical destruction effect is not likely to disappear soon, and may even increase if greenhouse effects, major volcanic eruptions or enhanced stratospheric cooling intervene. If the long-term level (i) remains steady, an extrapolation of the QBO-QTO patterns indicates that the ozone level is due for an increase from about 1999 end to about 2001 beginning. The purpose of the present analysis is to point out that, if such an increase of 20-30 DU occurs, it should not be misinterpreted as due to a decrease in chemical destruction, which scientists are eagerly awaiting due to the indication of a reduction in the halogen load in recent years due to adherence to the Montreal Protocol. After one or two years (in 2002), the extrapolated QBO-QTO oscillation may bring down the ozone level back again to the 1999 end level, and the apparent recovery may turn out to be a false signal.

The Response of Tropical Cyclone Intensity to Temperature Profile Change

Theory indicates that tropical cyclone intensity should respond to changes in the vertical temperature profile. While the sensitivity of tropical cyclone intensity to sea surface temperature is well understood, less is known about sensitivity to the temperature profile. In this paper, we combine historical data analysis and idealised modelling to explore the extent to which historical tropospheric warming and lower stratospheric cooling can explain observed trends in the tropical cyclone intensity distribution. Observations and modelling agree that historical global temperature profile changes coincide with higher lifetime maximum intensities. But observations suggest the response depends on the tropical cyclone intensity itself. Historical lower- and upper-tropospheric temperatures in hurricane environments have warmed significantly faster than the tropical mean. In addition, hurricane-strength storms have intensified at twice the rate of weaker storms per unit warming at the surface and at 300-hPa. Idealized simulations respond in the expected sense to various imposed changes in the temperature profile and agree with tropical cyclones operating as heat engines. Yet lower stratospheric temperature changes have little influence. Idealised modelling further shows an increasing altitude of the TC outflow but little change in outflow temperature. This enables increased efficiency for strong tropical cyclones despite the warming upper troposphere. Observed sensitivities are generally larger than modelled sensitivities, suggesting that observed tropical cyclone intensity change responds to a combination of the temperature profile change and other environmental factors.

Dynamics of key climate variables over Europe

<p>Temperature and humidity are key climatic variables for the assessment of climate variability. This study focuses on the climatic trends of temperature, specific and relative humidity both at the surface and in multiple pressure levels in the atmosphere. We present the first results of the analysis the dynamics of some key climate variables over Europe. The analysis was conducted for Europe, but it is focusing also on Greece. The main purpose of this study is to investigate whether possible changes in the basic climate variables exist over the recent years. </p><p>Data from the ERA5 reanalysis product are used for the period 1979-2018 (40 years) with spatial resolution of 0.25° x 0.25°. The Sen’s slope estimator is used to identify the climate trends at each grid point and the Mann-Kendall statistical test was applied to detect statistically significant spatial and temporal changes for the examined domain. The results indicate statistically significant warming trends at the 99% level over land and sea at surface. Regarding Greece, statistically significant warming trends at the 99% level occur during summer. In addition, positive temperature trends are also presented over land and sea, in the troposphere, over the particular domain. In contrast, in the stratosphere, statistically significant cooling trends at the 99% level are observed. Additionally, the stratospheric cooling trends increase with increasing altitude in the atmosphere. Regarding the climatic trends of the specific humidity, mainly positive values prevail up to mid-troposphere. Finally, the climatic trends of the relative humidity exhibit positive and negative values due to the relationship of humidity and temperature.</p>

Co-emission of volcanic sulfur and halogens amplifies volcanic effective radiative forcing

The evolution of volcanic sulfur and the resulting radiative forcing following explosive volcanic eruptions is well understood. Petrological evidence suggests that significant amounts of halogens may be co-emitted alongside sulfur in some explosive volcanic eruptions, and satellite evidence indicates that detectable amounts of these halogens may reach the stratosphere. In this study, we utilise an aerosol–chemistry–climate model to simulate stratospheric volcanic eruption emission scenarios of two sizes, both with and without co-emission of volcanic halogens, in order to understand how co-emitted halogens may alter the life cycle of volcanic sulfur, stratospheric chemistry, and the resulting radiative forcing. We simulate a large (10 Tg of SO2) and very large (56 Tg of SO2) sulfur-only eruption scenario and a corresponding large (10 Tg SO2, 1.5 Tg HCl, 0.0086 Tg HBr) and very large (56 Tg SO2, 15 Tg HCl, 0.086 Tg HBr) co-emission eruption scenario. The eruption scenarios simulated in this work are hypothetical, but they are comparable to Volcanic Explosivity Index (VEI) 6 (e.g. 1991 Mt Pinatubo) and VEI 7 (e.g. 1257 Mt Samalas) eruptions, representing 1-in-50–100-year and 1-in-500–1000-year events, respectively, with plausible amounts of co-emitted halogens based on satellite observations and volcanic plume modelling. We show that co-emission of volcanic halogens and sulfur into the stratosphere increases the volcanic effective radiative forcing (ERF) by 24 % and 30 % in large and very large co-emission scenarios compared to sulfur-only emission. This is caused by an increase in both the forcing from volcanic aerosol–radiation interactions (ERFari) and composition of the stratosphere (ERFclear,clean). Volcanic halogens catalyse the destruction of stratospheric ozone, which results in significant stratospheric cooling, offsetting the aerosol heating simulated in sulfur-only scenarios and resulting in net stratospheric cooling. The ozone-induced stratospheric cooling prevents aerosol self-lofting and keeps the volcanic aerosol lower in the stratosphere with a shorter lifetime. This results in reduced growth by condensation and coagulation and a smaller peak global-mean effective radius compared to sulfur-only simulations. The smaller effective radius found in both co-emission scenarios is closer to the peak scattering efficiency radius of sulfate aerosol, and thus co-emission of halogens results in larger peak global-mean ERFari (6 % and 8 %). Co-emission of volcanic halogens results in significant stratospheric ozone, methane, and water vapour reductions, resulting in significant increases in peak global-mean ERFclear,clean (> 100 %), predominantly due to ozone loss. The dramatic global-mean ozone depletion simulated in large (22 %) and very large (57 %) co-emission scenarios would result in very high levels of UV exposure on the Earth's surface, with important implications for society and the biosphere. This work shows for the first time that co-emission of plausible amounts of volcanic halogens can amplify the volcanic ERF in simulations of explosive eruptions. It highlights the need to include volcanic halogen emissions when simulating the climate impacts of past or future eruptions, as well as the necessity to maintain space-borne observations of stratospheric compounds to better constrain the stratospheric injection estimates of volcanic eruptions.

Using Climate Model Simulations to Constrain Observations

We compare atmospheric temperature changes in satellite data and in model ensembles performed under phases 5 and 6 of the Coupled Model Intercomparison Project (CMIP5 and CMIP6). In the lower stratosphere, multi-decadal stratospheric cooling during the period of strong ozone depletion is smaller in newer CMIP6 simulations than in CMIP5 or satellite data. In the troposphere, however, despite forcing and climate sensitivity differences between the two CMIP ensembles, their ensemble-average global warming over 1979-2019 is very similar. We also examine four properties of tropical behavior governed by basic physical processes. The first three are ratios between trends inwater vapor (WV) and trends in sea surface temperature (SST), lower tropospheric temperature (TLT), and mid- to upper tropospheric temperature (TMT). The fourth property is the ratio between TMT and SST trends. All four ratios are tightly constrained in CMIP simulations but diverge markedly in observations. Model trend ratios between WV and temperature are closest to observed ratios when the latter are calculated with data sets exhibiting larger tropical warming of the ocean surface and troposphere. For the TMT/SST ratio, model-data consistency depends on the combination of observations used to estimate TMT and SST trends. If model expectations of these four covariance relationships are realistic, our findings reflect either a systematic low bias in satellite tropospheric temperature trends or an overestimate of the observed atmospheric moistening signal. It is currently difficult to determine which interpretation is more credible. Nevertheless, our analysis reveals anomalous covariance behavior in several observational data sets and illustrates the diagnostic power of simultaneously considering multiple complementary variables.

Robust asymmetry of the future Arctic polar vortex is driven by tropical Pacific warming

The wintertime Arctic stratospheric polar vortex is characterized by a circumpolar westerly jet, confining the coldest temperatures over the Arctic. The future stratosphere is globally dominated by a strong radiative cooling due to the increase in greenhouse gases, enhancing the Arctic cooling. However, we find that over North America, the Arctic stratospheric cooling is suppressed or rather warming occurs, whereas over Eurasia stratospheric cooling is most pronounced, leading to an asymmetric polar vortex, based on 21st century climate model simulations. There are many causes that drive polar vortex variability, such as Arctic sea ice loss, and midlatitude and tropical Pacific warming, which make future projections highly uncertain. Our model simulations demonstrate that tropical warming induces the asymmetric polar vortex. The eastern equatorial Pacific warming causes eastward-shifted teleconnection, which strengthens the polar vortex over Eurasia and weakens over North America by enhancing the vertical wave propagation into the stratosphere. The asymmetric polar vortex is projected to markedly develop in the 2030s, and so could also affect winter surface climate over mid- to high-latitudes of Eurasia in the near future.

Co-emission of volcanic sulfur and halogens amplifies volcanic effective radiative forcing

The evolution of volcanic sulfur and the resulting radiative forcing following explosive volcanic eruptions is well understood. Petrological evidence suggests that significant amounts of halogens may be co-emitted alongside sulfur in some explosive volcanic eruptions, and satellite evidence indicates that detectable amounts of these halogens may reach the stratosphere. In this study, we confront an aerosol-chemistry-climate model with four stratospheric volcanic eruption emission scenarios (56 Tg SO2 ± 15 Tg HCl & 0.086 Tg HBr and 10 Tg SO2 ± 1.5 Tg HCl & 0.0086 Tg HBr) in order to understand how co-emitted halogens may alter the life cycle of volcanic sulfur, stratospheric chemistry and the resulting radiative forcing. The eruption sizes simulated in this work are hypothetical Volcanic Explosivity Index (VEI) 7 (e.g. 1257 Mt. Samalas) and VEI 6 (e.g. 1991 Mt. Pinatubo) eruptions, representing 1 in 500–1000 year and 1 in 50–100 year events respectively, with plausible amounts of co-emitted halogens based on satellite observations and volcanic plume modelling. We show that co-emission of volcanic halogens and sulfur into the stratosphere increases the volcanic ERF by 24–30 % compared to sulfur-only emission. This is caused by an increase in both the forcing from volcanic aerosol-radiation interactions (ERFari) and composition of the stratosphere (ERFclear,clean). Volcanic halogens catalyse the destruction of stratospheric ozone which results in significant stratospheric cooling (1.5–3 K); counteracting the typical stratospheric radiative heating from volcanic sulfate aerosol. The ozone induced stratospheric cooling prevents aerosol self-lofting and keeps the volcanic aerosol lower in the stratosphere with a shorter lifetime, resulting in reduced growth due to condensation and coagulation and smaller peak global-mean effective radius compared to sulfur-only simulations. The smaller effective radius found in both co-emission scenarios is closer to the peak scattering efficiency radius of sulfate aerosol, thus, co-emission of halogens results in larger peak global-mean ERFari (6–8 %). Co-emission of volcanic halogens results in significant stratospheric ozone, methane and water vapour reductions, resulting in significant increases in peak global-mean ERFclear,clean (> 100 %), predominantly due to ozone loss. The dramatic global-mean ozone depletion simulated in both co-emission simulations (22 %, 57 %) would result in very high levels of UV exposure on the Earth's surface, with important implications for society and the biosphere. This work shows for the first time that co-emission of plausible amounts of volcanic halogens can amplify the volcanic ERF in simulations of explosive eruptions; highlighting the need to include volcanic halogens fluxes when simulating the climate impacts of past or future eruptions and providing motivation to better quantify the degassing budgets and stratospheric injection estimates for volcanic eruptions.

The HadGEM3-GA7.1 radiative kernel: the importance of a well-resolved stratosphere

We present top-of-atmosphere and surface radiative kernels based on the atmospheric component (GA7.1) of the HadGEM3 general circulation model developed by the UK Met Office. We show that the utility of radiative kernels for forcing adjustments in idealised CO2 perturbation experiments is greatest where there is sufficiently high resolution in the stratosphere in both the target climate model and the radiative kernel. This is because stratospheric cooling to a CO2 perturbation continues to increase with height, and low-resolution or low-top kernels or climate model output are unable to fully resolve the full stratospheric temperature adjustment. In the sixth phase of the Coupled Model Intercomparison Project (CMIP6), standard atmospheric model data are available up to 1 hPa on 19 pressure levels, which is a substantial advantage compared to CMIP5. We show in the IPSL-CM6A-LR model where a full set of climate diagnostics are available that the HadGEM3-GA7.1 kernel exhibits linear behaviour and the residual error term is small, as well as from a survey of kernels available in the literature that in general low-top radiative kernels underestimate the stratospheric temperature response. The HadGEM3-GA7.1 radiative kernels are available at https://doi.org/10.5281/zenodo.3594673 (Smith, 2019).