Aerosol Direct Radiative Effects over China Based on Long-Term Observations within the Sun–Sky Radiometer Observation Network (SONET)

To investigate aerosol radiative effects, the Sun–Sky Radiometer Observation Network (SONET) has performed long-term observations of columnar atmospheric aerosol properties at 20 distributed stations around China. The aerosol direct radiative forcing (RF) and efficiency (RFE, the rate at which the atmosphere is forced per unit of aerosol optical depth) were estimated using radiative transfer model simulations based on the ground-based observations dating back to 2009. Results of multi-year monthly average RF illustrated that: the dust-dominant aerosol population at arid and semi-arid sites exerted moderate cooling effects (−8.0~−31.2 W/m2) at the top and bottom of atmosphere (TOA and BOA); RF at continental background site was very weak (−0.8~−2.9 W/m2); fine-mode dominant aerosols at urban and suburban sites exerted moderate cooling effects (−9.3~−24.1 W/m2) at TOA but more significant cooling effects (−19.4~−50.6 W/m2) at BOA; RF at coastal sites was comparable with values of urban sites (−5.5~−19.5 W/m2 at TOA, and −15.6~−44.6 W/m2 at BOA), owing to combined influences by marine and urban–industrial aerosols. Differences between RFE at TOA and BOA indicated that coarse-mode dominant aerosols at arid, semi-arid, and continental background sites were less efficient to warm the atmosphere; but fine-mode dominant aerosols at urban, suburban, and coastal sites were shown to be more efficient to heat the atmosphere.

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Explicit calculation of indirect global warming potentials for halons using atmospheric models

Atmospheric Chemistry and Physics ◽

10.5194/acp-9-8719-2009 ◽

2009 ◽

Vol 9 (22) ◽

pp. 8719-8733 ◽

Cited By ~ 8

Author(s):

D. Youn ◽

K. O. Patten ◽

J.-T. Lin ◽

D. J. Wuebbles

Keyword(s):

Global Warming ◽

Ozone Depletion ◽

Radiative Forcing ◽

Radiative Transfer Model ◽

Explicit Calculation ◽

Transfer Model ◽

Atmospheric Models ◽

Pulse Emission ◽

Cooling Effects ◽

Global Warming Potentials

Abstract. The concept of Global Warming Potentials (GWPs) has been extensively used in policy consideration as a relative index for comparing the climate impact of an emitted greenhouse gas (GHG), relative to carbon dioxide with equal mass emissions. Ozone depletion due to emission of chlorinated or brominated halocarbons leads to cooling of the climate system in the opposite direction to the direct warming contribution by halocarbons as GHGs. This cooling is a key indirect effect of the halocarbons on climatic radiative forcing, which is accounted for by indirect GWPs. With respect to climate, it is critical to understand net influences considering direct warming and indirect cooling effects especially for Halons due to the greater ozone-depleting efficiency of bromine over chlorine. Until now, the indirect GWPs have been calculated using a parameterized approach based on the concept of Equivalent Effective Stratospheric Chlorine (EESC) and the observed ozone depletion over the last few decades. As a step towards obtaining indirect GWPs through a more robust approach, we use atmospheric models to explicitly calculate the indirect GWPs of Halon-1211 and Halon-1301 for a 100-year time horizon. State-of-the-art global chemistry-transport models (CTMs) were used as the computational tools to derive more realistic ozone depletion changes caused by an added pulse emission of the two major Halons at the surface. The radiative forcings on climate from the ozone changes have been calculated for indirect GWPs using an atmospheric radiative transfer model (RTM). The simulated temporal variations of global average total column Halons after a pulse perturbation follow an exponential decay with an e-folding time which is consistent with the expected chemical lifetimes of the Halons. Our calculated indirect GWPs for the two Halons are much smaller than those from past studies but are within a single standard deviation of WMO (2007) values and the direct GWP values derived agree with the published values. Our model-based assessment of the Halon indirect GWPs thus confirms the significant importance of indirect effects on climate.

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Explicit calculation of indirect global warming potentials for halons using atmospheric models

Atmospheric Chemistry and Physics Discussions ◽

10.5194/acpd-9-15511-2009 ◽

2009 ◽

Vol 9 (4) ◽

pp. 15511-15540

Author(s):

D. Youn ◽

K. O. Patten ◽

J.-T. Lin ◽

D. J. Wuebbles

Keyword(s):

Global Warming ◽

Ozone Depletion ◽

Radiative Forcing ◽

Radiative Transfer Model ◽

Explicit Calculation ◽

Transfer Model ◽

Atmospheric Models ◽

Pulse Emission ◽

Cooling Effects ◽

Global Warming Potentials

Abstract. The concept of Global Warming Potentials (GWPs) has been extensively used in policy consideration as a relative index for comparing the climate impact of an emitted greenhouse gas (GHG), relative to carbon dioxide with equal mass emissions. Ozone depletion due to emission of chlorinated or brominated halocarbons leads to cooling of the climate system in the opposite direction to the direct warming contribution by halocarbons as GHGs. This cooling is a key indirect effect of the halocarbons on climatic radiative forcing, which is accounted for by indirect GWPs. With respect to climate, it is critical to understand net influences considering direct warming and indirect cooling effects for Halons. Until now, the indirect GWPs have been calculated using a para\\-meterized approach based on the concept of Equivalent Effective Stratospheric Chlorine (EESC) and the observed ozone depletion over the last few decades. As a step towards obtaining indirect GWPs through a more robust approach, we use atmospheric models to explicitly calculate the indirect GWPs of Halon-1211 and Halon-1301 for a 100-year time horizon. State-of-the-art global chemistry-transport models (CTMs) were used as the computational tools to derive more realistic ozone depletion changes caused by an added pulse emission of the two major Halons at the surface. The radiative forcings on climate from the ozone changes have been calculated for indirect GWPs using an atmospheric radiative transfer model (RTM). The simulated temporal variations of global average total column Halons after a pulse perturbation follow an exponential decay with an e-folding time which is consistent with the expected chemical lifetimes of the Halons. Our calculated indirect GWPs for the two Halons are smaller than past studies although direct GWPs agree with the published values. Nonetheless, our model-based assessment of the Halon indirect GWPs confirms the significant importance of indirect effects on climate.

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2-D mineral dust radiative forcing calculations from CALIPSO observations over Europe

10.5194/acp-2019-440 ◽

2019 ◽

Author(s):

Maria José Granados-Muñoz ◽

Michaël Sicard ◽

Nikolaos Papagiannopoulos ◽

Rubén Barragán ◽

Juan Antonio Bravo-Aranda ◽

...

Keyword(s):

Radiative Forcing ◽

Mineral Dust ◽

Single Point ◽

Strong Dependence ◽

Radiant Energy ◽

Radiative Properties ◽

Radiative Transfer Model ◽

Orthogonal Polarization ◽

Transfer Model ◽

Radiative Effects

Abstract. A demonstration study to examine the feasibility to retrieve dust radiative effects based on combined satellite data from MODIS (Moderate Resolution Imaging Spectroradiometer), CERES (Clouds and the Earth’s Radiant Energy System) and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) li-dar vertical profiles along their orbit is presented. The radiative transfer model GAME (Global Atmos-pheric Model) is used to estimate the shortwave and longwave dust radiative effects below the CALIP-SO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite) orbit assuming an aerosol parameterization based on CALIOP vertical distribution at a horizontal resolution of 5 km and additional AERONET (Aerosol Robotic Network) data. Two study cases are analysed; a strong long-range transport mineral dust event (AOD = 0.52) originated in the Sahara Desert and reaching the United Kingdom and a weaker event (AOD = 0.16) affecting Eastern Europe. The obtained radiative fluxes are first validated in terms of radiative forcing efficiency at a single point with space-time co-located lidar ground-based measurements from EARLINET (European Aerosol Research Lidar Network) stations below the orbit. The methodology is then applied to the full orbit. The obtained results indicate that the radiative effects show a strong dependence on the aerosol load, highlighting the need of accurate AOD measurements for forcing studies, and on the surface albedo. The calculated dust radiative effects and heating rates below the orbits are in good agreement with previous studies of mineral dust, with the forcing efficiency obtained at the surface ranging between −80.3 and −63.0 W m−2 for the weaker event and −119.1 and −79.3 W m−2 for the strong one. Results thus demonstrate the validity of the presented method to retrieve 2-D accurate radiative properties with large spatial and temporal coverage.

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Retrieval of gridded aerosol direct radiative forcing based on multiplatform datasets

Atmospheric Measurement Techniques ◽

10.5194/amt-13-575-2020 ◽

2020 ◽

Vol 13 (2) ◽

pp. 575-592 ◽

Cited By ~ 3

Author(s):

Yanyu Wang ◽

Rui Lyu ◽

Xin Xie ◽

Ze Meng ◽

Meijin Huang ◽

...

Keyword(s):

Radiative Transfer ◽

Radiative Forcing ◽

Eastern China ◽

Radiant Energy ◽

Radiative Transfer Model ◽

Transfer Model ◽

Rapid Urbanization ◽

Radiative Fluxes ◽

Direct Radiative Forcing

Abstract. Atmospheric aerosols play a crucial role in regional radiative budgets. Previous studies on clear-sky aerosol direct radiative forcing (ADRF) have mainly been limited to site-scale observations or model simulations for short-term cases, and long-term distributions of ADRF in China have not been portrayed yet. In this study, an accurate fine-resolution ADRF estimate at the surface was proposed. Multiplatform datasets, including satellite (MODIS aboard Terra and Aqua) and reanalysis datasets, served as inputs to the Santa Barbara Discrete Atmospheric Radiative Transfer (SBDART) model for ADRF simulation with consideration of the aerosol vertical profile over eastern China during 2000–2016. Specifically, single-scattering albedo (SSA) from the Modern-Era Retrospective Analysis for Research and Application, Version 2 (MERRA-2) was validated with sun photometers over eastern China. The gridded asymmetry parameter (ASY) was then simulated by matching the calculated top-of-atmosphere (TOA) radiative fluxes from the radiative transfer model with satellite observations (Clouds and the Earth's Radiant Energy System, CERES). The high correlation and small discrepancy (6–8 W m−2) between simulated and observed radiative fluxes at three sites (Baoshan, Fuzhou, and Yong'an) indicated that ADRF retrieval is feasible and has high accuracy over eastern China. Then this method was applied in each grid of eastern China, and the overall picture of ADRF distributions over eastern China during 2000–2016 was displayed. ADRF ranges from −220 to −20 W m−2, and annual mean ADRF is −100.21 W m−2, implying that aerosols have a strong cooling effect at the surface in eastern China. With the economic development and rapid urbanization, the spatiotemporal changes of ADRF during the past 17 years are mainly attributed to the changes of anthropogenic emissions in eastern China. Our method provides the long-term ADRF distribution over eastern China for the first time, highlighting the importance of aerosol radiative impact under climate change.

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Retrieval of Gridded Aerosol Direct Radiative Forcing Based on Multiplatform Datasets

10.5194/amt-2019-311 ◽

2019 ◽

Author(s):

Yanyu Wang ◽

Rui Lyu ◽

Xin Xie ◽

Meijin Huang ◽

Junshi Wu ◽

...

Keyword(s):

Radiative Transfer ◽

Radiative Forcing ◽

Radiant Energy ◽

Energy System ◽

East China ◽

Radiative Transfer Model ◽

Transfer Model ◽

Radiative Fluxes ◽

Direct Radiative Forcing

Abstract. Atmospheric aerosols play a crucial role in regional radiative budgets. Previous studies on clear-sky aerosol direct radiative forcing (ADRF) have mainly been limited to site-scale observations or model simulations for short-term cases, and long-term distributions of ADRF in China has not been portrayed yet. In this study, an accurate fine-resolution ADRF estimate at the surface was proposed. Multiplatform datasets, including satellite (Terra and Aqua) and reanalysis datasets, served as inputs to the Santa Barbara Discrete Atmospheric Radiative Transfer (SBDART) model for ADRF simulation with consideration of the aerosol vertical profile over East China during 2000–2016. Specifically, single scattering albedo (SSA) from the Modern-Era Retrospective Analysis for Research and Application, version 2 (MERRA-2) was validated with sunphotometers over East China. The gridded asymmetry parameter (ASY) was then simulated by matching the calculated top-of-atmosphere (TOA) radiative fluxes from the radiative transfer model with satellite observations (Clouds and the Earth's Radiant Energy System (CERES)). The high correlation and small discrepancy (6–8 W m-2) between simulated and observed radiative fluxes at three sites (Baoshan, Fuzhou, and Yong'an) indicated that ADRF retrieval is feasible and has high accuracy over East China. Then this method was applied in each grid of East China and the overall picture of ADRF distributions over East China during 2000–2016 was displayed. ADRF ranges from −220 to −20 W m-2, and annual mean ADRF is −100.21 W m-2, implying that aerosols have strong cooling effect at the surface during past 16 years. Finally, uncertainty analysis was also evaluated. Our method provides the long-term ADRF distribution over East China for the first time, with highlighting the importance of aerosol radiative impact under the climate change.

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Modeling the radiative effects of desert dust on weather and regional climate

Atmospheric Chemistry and Physics ◽

10.5194/acp-13-5489-2013 ◽

2013 ◽

Vol 13 (11) ◽

pp. 5489-5504 ◽

Cited By ~ 38

Author(s):

C. Spyrou ◽

G. Kallos ◽

C. Mitsakou ◽

P. Athanasiadis ◽

C. Kalogeri ◽

...

Keyword(s):

Radiative Transfer ◽

Regional Climate ◽

Lower Troposphere ◽

Integrated Approach ◽

Dust Particles ◽

Radiative Transfer Model ◽

Limited Area ◽

Transfer Model ◽

Radiative Effects ◽

Desert Dust

Abstract. Mineral dust aerosols exert a significant effect on both solar and terrestrial radiation. By absorbing and scattering, the solar radiation aerosols reduce the amount of energy reaching the surface. In addition, aerosols enhance the greenhouse effect by absorbing and emitting outgoing longwave radiation. Desert dust forcing exhibits large regional and temporal variability due to its short lifetime and diverse optical properties, further complicating the quantification of the direct radiative effect (DRE). The complexity of the links and feedbacks of dust on radiative transfer indicate the need for an integrated approach in order to examine these impacts. In order to examine these feedbacks, the SKIRON limited area model has been upgraded to include the RRTMG (Rapid Radiative Transfer Model – GCM) radiative transfer model that takes into consideration the aerosol radiative effects. It was run for a 6 year period. Two sets of simulations were performed, one without the effects of dust and the other including the radiative feedback. The results were first evaluated using aerosol optical depth data to examine the capabilities of the system in describing the desert dust cycle. Then the aerosol feedback on radiative transfer was quantified and the links between dust and radiation were studied. The study has revealed a strong interaction between dust particles and solar and terrestrial radiation, with several implications on the energy budget of the atmosphere. A profound effect is the increased absorption (in the shortwave and longwave) in the lower troposphere and the induced modification of the atmospheric temperature profile. These feedbacks depend strongly on the spatial distribution of dust and have more profound effects where the number of particles is greater, such as near their source.

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Seasonal and interannual variations in the propagation of photosynthetically available radiation through the Arctic atmosphere

Elem Sci Anth ◽

10.1525/elementa.2020.00083 ◽

2021 ◽

Vol 9 (1) ◽

Author(s):

J. Laliberté ◽

S. Bélanger ◽

M. Babin

Keyword(s):

Large Data ◽

The Arctic ◽

Radiative Transfer Model ◽

Transfer Model ◽

The Sun ◽

Photosynthetically Available Radiation ◽

Data Set ◽

Melt Ponds ◽

Arctic Atmosphere ◽

Marine Productivity

The Arctic atmosphere–surface system transmits visible light from the Sun to the ocean, determining the annual cycle of light available to microalgae. This light is referred to as photosynthetically available radiation (PAR). A known consequence of Arctic warming is the change at the atmosphere–ocean interface (longer ice-free season, younger ice), implying an increase in the percentage of PAR being transferred to the water. However, much less is known about the recent changes in how much PAR is being transferred by the overlaying atmosphere. We studied the transfer of PAR through the atmosphere between May 21 and July 23 at a pan-Arctic scale for the period ranging from 2000 to 2016. By combining a large data set of atmospheric and surface conditions into a radiative transfer model, we computed the percentage of PAR transferred to the surface. We found that typical Arctic atmospheres convey between 60% and 70% of the incident PAR received from the Sun, meaning the Arctic atmosphere typically transmits more light than most sea ice surfaces, with the exception of mature melt ponds. We also found that the transfer of PAR through the atmosphere decreased at a rate of 2.3% per decade over the studied period, due to the increase in cloudiness and the weaker radiative interaction between the atmosphere and the surface. Further investigation is required to address how, in the warmer Arctic climate, this negative trend would compensate for the increased surface transmittance and its consequences on marine productivity.

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Radiative forcing over the Arctic of aerosols from the August 2017 Canadian and Greenlandic wildfires

10.5194/egusphere-egu21-7405 ◽

2021 ◽

Author(s):

Filippo Calì Quaglia ◽

Daniela Meloni ◽

Alcide Giorgio di Sarra ◽

Tatiana Di Iorio ◽

Virginia Ciardini ◽

...

Keyword(s):

Radiative Transfer ◽

Radiative Forcing ◽

Solar Zenith Angle ◽

Surface Albedo ◽

High Arctic ◽

The Arctic ◽

Radiative Transfer Model ◽

Transfer Model ◽

Aerosol Layer ◽

Radiative Effect

Extended and intense wildfires occurred in Northern Canada and, unexpectedly, on the Greenlandic West coast during summer 2017. The thick smoke plume emitted into the atmosphere was transported to the high Arctic, producing one of the largest impacts ever observed in the region. Evidence of Canadian and Greenlandic wildfires was recorded at the Thule High Arctic Atmospheric Observatory (THAAO, 76.5&#176;N, 68.8&#176;W, www.thuleatmos-it.it) by a suite of instruments managed by ENEA, INGV, Univ. of Florence, and NCAR. Ground-based observations of the radiation budget have allowed quantification of the surface radiative forcing at THAAO.&#160;Excess biomass burning chemical tracers such as CO, HCN, H2CO, C2H6, and NH3 were&#160; measured in the air column above Thule starting from August 19 until August 23. The aerosol optical depth (AOD) reached a peak value of about 0.9 on August 21, while an enhancement of wildfire compounds was&#160; detected in PM10. The measured shortwave radiative forcing was -36.7 W/m2 at 78&#176; solar zenith angle (SZA) for AOD=0.626.MODTRAN6.0 radiative transfer model (Berk et al., 2014) was used to estimate the aerosol radiative effect and the heating rate profiles at 78&#176; SZA. Measured temperature profiles, integrated water vapour, surface albedo, spectral AOD and aerosol extinction profiles from CALIOP onboard CALIPSO were used as model input. The peak&#160; aerosol heating rate (+0.5 K/day) was&#160; reached within the aerosol layer between 8 and 12 km, while the maximum radiative effect (-45.4 W/m2) is found at 3 km, below the largest aerosol layer.The regional impact of the event that occurred on August 21 was investigated using a combination of atmospheric radiative transfer modelling with measurements of AOD and ground surface albedo from MODIS. The aerosol properties used in the radiative transfer model were constrained by in situ measurements from THAAO. Albedo data over the ocean have been obtained from Jin et al. (2004). Backward trajectories produced through HYSPLIT simulations (Stein et al., 2015) were also employed to trace biomass burning plumes.The radiative forcing efficiency (RFE) over land and ocean was derived, finding values spanning from -3 W/m2 to -132 W/m2, depending on surface albedo and solar zenith angle. The fire plume covered a vast portion of the Arctic, with large values of the daily shortwave RF (< -50 W/m2) lasting for a few days. This large amount of aerosol is expected to influence cloud properties in the Arctic, producing significant indirect radiative effects.

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Polar Stratospheric Clouds detection at Belgrano II Antarctic station from DOAS measurements

10.5194/egusphere-egu21-3054 ◽

2021 ◽

Author(s):

Laura Gómez Martín ◽

Daniel Toledo ◽

Margarita Yela ◽

Cristina Prados-Román ◽

José Antonio Adame ◽

...

Keyword(s):

Radiative Transfer ◽

Color Index ◽

Radiative Transfer Model ◽

Optical Absorption Spectroscopy ◽

Transfer Model ◽

Meteorological Model ◽

Weather Forecasts ◽

Stratospheric Temperature ◽

Stratospheric Clouds

Ground-based zenith DOAS (Differential Optical Absorption Spectroscopy) measurements have been used to detect and estimate the altitude of PSCs over Belgrano II Antarctic station during the polar sunrise seasons of 2018 and 2019. The method used in this work studies the evolution of the color index (CI) during twilights. The CI has been defined here as the ratio of the recorded signal at 520 and 420 nm. In the presence of PSCs, the CI shows a maximum at a given solar zenith angle (SZA). The value of such SZA depends on the altitude of the PSC. By using a spherical Monte Carlo radiative transfer model (RTM), the method has been validated and a function relating the SZA of the CI maximum and the PSC altitude has been calculated. Model simulations also show that PSCs can be detected and their altitude can be estimated even in presence of optically thin tropospheric clouds or aerosols. Our results are in good agreement with the stratospheric temperature evolution obtained through the ERA5 data reanalysis from the global meteorological model ECMWF (European Centre for Medium Range Weather Forecasts) and the PSCs observations from CALIPSO (Cloud-Aerosol-Lidar and Infrared Pathfinder Satellite Observations).The methodology used in this work could also be applied to foreseen and/or historical measurements obtained with ground-based spectrometers such e. g. the DOAS instruments dedicated to trace gas observation in Arctic and Antarctic sites. This would also allow to investigate the presence and long-term evolution of PSCs.Keywords: Polar stratospheric clouds; color index; radiative transfer model; visible spectroscopy.

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