scholarly journals Transport pathways from the Asian monsoon anticyclone to the stratosphere

2016 ◽  
Vol 16 (4) ◽  
pp. 2703-2718 ◽  
Author(s):  
Hella Garny ◽  
William J. Randel
Keyword(s):  
Large Scale ◽  
Asian Monsoon ◽  
Deep Convection ◽  
Three Dimensional ◽  
Reanalysis Data ◽  
Vertical Transport ◽  
Heating Rates ◽  
Transport Pathways ◽  
Northern Summer ◽  
The Tropics

Abstract. Transport pathways of air originating in the upper-tropospheric Asian monsoon anticyclone are investigated based on three-dimensional trajectories. The Asian monsoon anticyclone emerges in response to persistent deep convection over India and southeast Asia in northern summer, and this convection is associated with rapid transport from the surface to the upper troposphere and possibly into the stratosphere. Here, we investigate the fate of air that originates within the upper-tropospheric anticyclone from the outflow of deep convection, using trajectories driven by ERA-interim reanalysis data. Calculations include isentropic estimates, plus fully three-dimensional results based on kinematic and diabatic transport calculations. Isentropic calculations show that air parcels are typically confined within the anticyclone for 10–20 days and spread over the tropical belt within a month of their initialization. However, only few parcels (3 % at 360 K, 8 % at 380 K) reach the extratropical stratosphere by isentropic transport. When considering vertical transport we find that 31 %  or 48 % of the trajectories reach the stratosphere within 60 days when using vertical velocities or diabatic heating rates to calculate vertical transport, respectively. In both cases, most parcels that reach the stratosphere are transported upward within the anticyclone and enter the stratosphere in the tropics, typically 10–20 days after their initialization at 360 K. This suggests that trace gases, including pollutants, that are transported into the stratosphere via the Asian monsoon system are in a position to enter the tropical pipe and thus be transported into the deep stratosphere. Sensitivity calculations with respect to the initial altitude of the trajectories showed that air needs to be transported to levels of 360 K or above by deep convection to likely (≧ 50 %) reach the stratosphere through transport by the large-scale circulation.

scholarly journals Transport pathways from the Asian monsoon anticyclone to the stratosphere

2015 ◽  
Vol 15 (18) ◽  
pp. 25981-26023 ◽  
Author(s):  
H. Garny ◽  
W. J. Randel
Keyword(s):  
Large Scale ◽  
Asian Monsoon ◽  
Deep Convection ◽  
Three Dimensional ◽  
Reanalysis Data ◽  
Vertical Transport ◽  
Heating Rates ◽  
Transport Pathways ◽  
Northern Summer ◽  
The Tropics

Abstract. Transport pathways of air originating in the upper tropospheric Asian monsoon anticyclone are investigated based on three-dimensional trajectories. The Asian monsoon anticyclone emerges in response to persistent deep convection over India and southeast Asia in northern summer, and this convection is associated with rapid transport from the surface to the upper troposphere, and possibly into the stratosphere. Here, we investigate the fate of air that originates within the upper tropospheric anticyclone from the outflow of deep convection, using trajectories driven by ERA-interim reanalysis data. Calculations include isentropic estimates, plus fully three-dimensional results based on kinematic and diabatic transport calculations. Isentropic calculations show that air parcels are typically confined within the anticyclone for 10–20 days, and spread over the tropical belt within a month of their initialization. However, only few parcels (3 % at 360 K, 8 % at 380 K) reach the extratropical stratosphere by isentropic mixing. When considering vertical transport we find that 31 % (48%) of the trajectories reach the stratosphere within 60 days when using vertical velocities or diabatic heating rates to calculate vertical transport, respectively. In both cases, most parcels that reach the stratosphere are transported upward within the anticyclone and enter the stratosphere in the tropics, typically 10–20 days after their initialization at 360 K. This suggests that trace gases, including pollutants, that are transported into the stratosphere via the Asian monsoon system are in a position to enter the tropical pipe and thus be transported into the deep stratosphere. Sensitivity calculations with respect to the initial altitude of the trajectories showed that air needs to be transported to levels of 360 K or above by deep convection to likely (≧50 %) reach the stratosphere through transport by the large-scale circulation.

scholarly journals Analysis of a rapid increase of stratospheric ozone during late austral summer 2008 over Kerguelen (49.4° S, 70.3° E)

2011 ◽  
Vol 11 (1) ◽  
pp. 363-373 ◽  
Author(s):  
H. Bencherif ◽  
L. El Amraoui ◽  
G. Kirgis ◽  
J. Leclair De Bellevue ◽  
A. Hauchecorne ◽  
...  
Keyword(s):  
Potential Vorticity ◽  
Large Scale ◽  
Lower Stratosphere ◽  
Transport Model ◽  
Stratospheric Ozone ◽  
Three Dimensional ◽  
Austral Summer ◽  
Air Masses ◽  
Global Mapping ◽  
The Tropics

Abstract. This paper reports on an increase of ozone event observed over Kerguelen (49.4° S, 70.3° E) in relationship with large-scale isentropic transport. This is evidenced by ground-based observations (co-localised radiosonde and SAOZ experiments) together with satellite global observations (Aura/MLS) assimilated into MOCAGE, a Méteo-France model. The study is based on the analyses of the first ozonesonde experiment never recorded at the Kerguelen site within the framework of a French campaign called ROCK that took place from April to August 2008. Comparisons and interpretations of the observed event are supported by co-localised SAOZ observations, by global mapping of tracers (O3, N2O and columns of O3) from Aura/MLS and Aura/OMI experiments, and by model simulations of Ertel Potential Vorticity initialised by the ECMWF (European Centre for Medium-Range Weather Forecasts) data reanalyses. Satellite and ground-based observational data revealed a consistent increase of ozone in the local stratosphere by mid-April 2008. Additionally, Ozone (O3) and nitrous oxide (N2O) profiles obtained during January–May 2008 using the Microwave Limb Sounder (MLS) aboard the Aura satellite are assimilated into MOCAGE (MOdèle de Chimie Atmosphérique à Grande Echelle), a global three-dimensional chemistry transport model of Météo-France. The assimilated total O3 values are consistent with SAOZ ground observations (within ±5%), and isentropic distributions of O3 match well with maps of advected potential vorticity (APV) derived from the MIMOSA model, a high-resolution advection transport model, and from the ECMWF reanalysis. The event studied seems to be related to the isentropic transport of air masses that took place simultaneously in the lower- and middle-stratosphere, respectively from the polar region and from the tropics to the mid-latitudes. In fact, the ozone increase observed by mid April 2008 resulted simultaneously: (1) from an equator-ward departure of polar air masses characterised with a high-ozone layer in the lower stratosphere (near the 475 K isentropic level), and (2) from a reverse isentropic transport from the tropics to mid- and high-latitudes in the upper stratosphere (nearby the 700 K level). The increase of ozone observed over Kerguelen from the 16-April ozonesonde profile is thus attributed to a concomitant isentropic transport of ozone in two stratospheric layers: the tropical air moving southward and reaching over Kerguelen in the upper stratosphere, and the polar air passing over the same area but in the lower stratosphere.

scholarly journals Modeling the transport of very short-lived substances into the tropical upper troposphere and lower stratosphere

2009 ◽  
Vol 9 (5) ◽  
pp. 18511-18543 ◽  
Author(s):  
J. Aschmann ◽  
B. M. Sinnhuber ◽  
E. L. Atlas ◽  
S. M. Schauffler
Keyword(s):  
Large Scale ◽  
Lower Stratosphere ◽  
Transport Model ◽  
Three Dimensional ◽  
Chemical Transport Model ◽  
Heating Rates ◽  
Model Calculations ◽  
Upper Troposphere ◽  
Mass Fluxes ◽  
Tropical Upper Troposphere

Abstract. The transport of very short-lived substances into the tropical upper troposphere and lower stratosphere is investigated by a three-dimensional chemical transport model using archived convective updraft mass fluxes (or detrainment rates) from the European Centre for Medium-Range Weather Forecast's ERA-Interim reanalysis. Large-scale vertical velocities are calculated from diabatic heating rates. With this approach we explicitly model the large scale subsidence in the tropical troposphere with convection taking place in fast and isolated updraft events. The model calculations agree generally well with observations of bromoform and methyl iodide from aircraft campaigns and with ozone and water vapor from sonde and satellite observations. Using a simplified treatment of dehydration and bromine product gas washout we give a range of 1.6 to 3 ppt for the contribution of bromoform to stratospheric bromine, assuming a uniform source in the boundary layer of 1 ppt. We show that the most effective region for VSLS transport into the stratosphere is the West Pacific, accounting for about 55% of the bromine from bromoform transported into the stratosphere under the supposition of a uniformly distributed source.

scholarly journals The role of horizontal model resolution in assessing the transport of CO in a middle latitude cyclone using WRF-Chem

2014 ◽  
Vol 14 (2) ◽  
pp. 609-627 ◽  
Author(s):  
C. A. Klich ◽  
H. E. Fuelberg
Keyword(s):  
Large Scale ◽  
Transport Model ◽  
Deep Convection ◽  
Middle Latitude ◽  
Convective Transport ◽  
Vertical Transport ◽  
Squall Line ◽  
Grid Spacing ◽  
Chemical Transport Model ◽  
Hysplit Model

Abstract. We use the Weather Research and Forecasting with Chemistry (WRF-Chem) online chemical transport model to simulate a middle latitude cyclone in East Asia at three different horizontal resolutions (45, 15, and 5 km grid spacing). The cyclone contains a typical warm conveyor belt (WCB) with an embedded squall line that passes through an area having large surface concentrations (> 400 ppbv) of carbon monoxide (CO). Model output from WRF-Chem is used to compare differences between the large-scale CO vertical transport by the WCB (the 45 km simulation) with the smaller-scale transport due to its convection (the 5 km simulation). Forward trajectories are calculated from WRF-Chem output using the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model. At 45 km grid spacing, the WCB exhibits gradual ascent, lofting surface CO to 6–7 km. Upon reaching the warm front, the WCB and associated CO ascend more rapidly and later turn eastward over the Pacific Ocean. Convective transport at 5 km resolution with explicitly resolved convection occurs much more rapidly, with surface CO lofted to altitudes greater than 10 km in 1 h or less. We also compute CO vertical mass fluxes over specified areas and times to compare differences in transport due to the different grid spacings. Upward CO flux exceeds 110 000 t h−1 in the domain with explicit convection when the squall line is at peak intensity, while fluxes from the two coarser resolutions are an order of magnitude smaller. Specific areas of interest within the 5 km domain are defined to compare the magnitude of convective transport to that within the entire 5 km region. Although convection encompasses only a small portion of the 5 km domain, it is responsible for ~40% of the upward CO transport. We also examine the vertical transport due to a short wave trough and its associated area of convection, not related to the cyclone, that lofts CO to the upper troposphere. Results indicate that fine-scale resolution with explicitly resolved convection is important when assessing the vertical transport of surface emissions in areas of deep convection.

scholarly journals Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere

2017 ◽  
Vol 17 (11) ◽  
pp. 7055-7066 ◽  
Author(s):  
Felix Ploeger ◽  
Paul Konopka ◽  
Kaley Walker ◽  
Martin Riese
Keyword(s):  
Asian Monsoon ◽  
Lower Stratosphere ◽  
Transport Model ◽  
Monsoon Circulation ◽  
Pollution Transport ◽  
Chemistry Transport Model ◽  
Transport Pathways ◽  
Air Mass ◽  
Mass Fractions ◽  
The Tropics

Abstract. Pollution transport from the surface to the stratosphere within the Asian monsoon circulation may cause harmful effects on stratospheric chemistry and climate. Here, we investigate air mass transport from the monsoon anticyclone into the stratosphere using a Lagrangian chemistry transport model. We show how two main transport pathways from the anticyclone emerge: (i) into the tropical stratosphere (tropical pipe), and (ii) into the Northern Hemisphere (NH) extratropical lower stratosphere. Maximum anticyclone air mass fractions reach around 5 % in the tropical pipe and 15 % in the extratropical lowermost stratosphere over the course of a year. The anticyclone air mass fraction correlates well with satellite hydrogen cyanide (HCN) and carbon monoxide (CO) observations, confirming that pollution is transported deep into the tropical stratosphere from the Asian monsoon anticyclone. Cross-tropopause transport occurs in a vertical chimney, but with the pollutants transported quasi-horizontally along isentropes above the tropopause into the tropics and NH.

scholarly journals Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere

2017 ◽  
Author(s):  
Felix Ploeger ◽  
Paul Konopka ◽  
Kaley Walker ◽  
Martin Riese
Keyword(s):  
Asian Monsoon ◽  
Lower Stratosphere ◽  
Transport Model ◽  
Monsoon Circulation ◽  
Pollution Transport ◽  
Chemistry Transport Model ◽  
Transport Pathways ◽  
Air Mass ◽  
Mass Fractions ◽  
The Tropics

Abstract. Pollution transport from the surface to the stratosphere within the Asian monsoon circulation may cause harmful effects on stratospheric chemistry and climate. Here, we investigate air mass transport from the monsoon anticyclone into the stratosphere using a Lagrangian chemistry transport model. We show how two main transport pathways from the anticyclone emerge: (i) into the tropical stratosphere (tropical pipe), and (ii) into the Northern hemisphere (NH) extra-tropical lower stratosphere. Maximum anticyclone air mass fractions reach around 5 % in the tropical pipe and 15 % in the extra-tropical lowermost stratosphere over the course of a year. The anticyclone air mass fraction correlates well with satellite hydrogen cyanide (HCN) and carbon monoxide (CO) observations, corroborating that pollution is transported deep into the tropical stratosphere from the Asian monsoon anticyclone. Cross-tropopause transport occurs in a vertical chimney, but with the emissions transported quasi-horizontally along isentropes above the tropopause into the tropics and NH.

A Moist Static Energy Budget Analysis of Quasi-2-Day Waves Using Satellite and Reanalysis Data

2016 ◽  
Vol 73 (2) ◽  
pp. 743-759 ◽  
Author(s):  
Yukari Sumi ◽  
Hirohiko Masunaga
Keyword(s):  
Large Scale ◽  
Deep Convection ◽  
Reanalysis Data ◽  
Convective Heating ◽  
Moist Static Energy ◽  
Wave Dynamics ◽  
Vertical Advection ◽  
Budget Analysis ◽  
Static Energy ◽  
Thermodynamic Processes

Abstract A moist static energy (MSE) budget analysis is applied to quasi-2-day waves to examine the effects of thermodynamic processes on the wave propagation mechanism. The 2-day waves are defined as westward inertia–gravity (WIG) modes identified with filtered geostationary infrared measurements, and the thermodynamic parameters and MSE budget variables computed from reanalysis data are composited with respect to the WIG peaks. The composite horizontal and vertical MSE structures are overall as theoretically expected from WIG wave dynamics. A prominent horizontal MSE advection is found to exist, although the wave dynamics is mainly regulated by vertical advection. The vertical advection decreases MSE around the times of the convective peak, plausibly resulting from the first baroclinic mode associated with deep convection. Normalized gross moist stability (NGMS) is used to examine the thermodynamic processes involving the large-scale dynamics and convective heating. NGMS gradually decreases to zero before deep convection and reaches a maximum after the convection peak, where low (high) NGMS leads (lags) deep convection. The decrease in NGMS toward zero before the occurrence of active convection suggests an increasingly efficient conversion from convective heating to large-scale dynamics as the wave comes in, while the increase afterward signifies that this linkage swiftly dies out after the peak.

scholarly journals Characterizing quasi-biweekly variability of the Asian monsoon anticyclone using potential vorticity and large-scale geopotential height field

2020 ◽  
Vol 20 (22) ◽  
pp. 13857-13876
Author(s):  
Arata Amemiya ◽  
Kaoru Sato
Keyword(s):  
Potential Vorticity ◽  
Geopotential Height ◽  
Large Scale ◽  
Asian Monsoon ◽  
Reanalysis Data ◽  
Longitudinal Distribution ◽  
Middle Latitudes ◽  
Subseasonal Variability ◽  
Westward Movement ◽  
Isentropic Surface

Abstract. The spatial pattern of subseasonal variability of the Asian monsoon anticyclone is analyzed using long-term reanalysis data, focusing on the large-scale longitudinal movement. The air inside the anticyclone is quantified by a thickness-weighted low-PV (potential vorticity) area on an isentropic surface. It is shown that the longitudinal movement of the air inside the Asian monsoon anticyclone has a timescale of 1 to 2 weeks, which is shorter than the monthly dominant timescale of the variability in the anticyclone intensity. The movement of the anticyclonic air is suggested to be largely controlled by passive advection. The typical time evolution of the variability pattern, explained by two leading empirical orthogonal function (EOF) components of 100 hPa geopotential height, shows large-scale geopotential anomalies moving westward spanning from low to middle latitudes. This corresponds well with the rapid westward movement of low-PV air known as “eddy shedding” and following the eastward retreat of the anticyclonic air. The two EOF components can also explain the bimodal longitudinal distribution of geopotential maximum location.

The impact of sudden stratospheric warmings (SSWs) on UTLS composition, local radiative effects and air quality

2020 ◽  
Author(s):  
Ryan Williams ◽  
Michaela Hegglin ◽  
Patrick Jöckel ◽  
Hella Garny ◽  
Keith Shine ◽  
...  
Keyword(s):  
Air Quality ◽  
Atmospheric Chemistry ◽  
Large Scale ◽  
Lower Stratosphere ◽  
Weather Prediction ◽  
Onset Date ◽  
Identification Algorithm ◽  
Heating Rates ◽  
Transport Pathways ◽  
The Impact

<p>Midwinter sudden stratospheric warmings (SSWs), characterised by the reversal of the temperature gradient poleward of 60°N and the 10 hPa climatological zonal mean wind from westerly to easterly at 60°N, are known to have pronounced impacts on tropospheric circulation which lead to regional changes in temperature, precipitation and other meteorological variables. Such abrupt events are furthermore known to be associated with large-scale changes in the distribution of stratospheric chemistry constituents, such as ozone (O<sub>3</sub>) and water vapour (H<sub>2</sub>O), although the implications for stratosphere-troposphere exchange (STE) have not been previously investigated. The evolution of O<sub>3</sub> and H<sub>2</sub>O anomalies during an SSW life cycle are first examined from the surface up to 1 hPa using specified-dynamics simulations from the European Centre for Medium-Range Weather Forecasts – Hamburg (ECHAM)/Modular Earth Submodel System (MESSy) Atmospheric Chemistry (EMAC) model over the period 1979-2013. We show that significant positive anomalies in O<sub>3</sub> occur around the onset of an SSW in the middle to lower stratosphere, with persistence timescales of around 50 days in the upper troposphere-lower stratosphere (UTLS). Similarly, we find significant H<sub>2</sub>O anomalies in the lowermost stratosphere (± 25 %) for up to 75 days. The extent and magnitude of the anomalies are largely confirmed in both Copernicus Atmospheric Monitoring Service (CAMS) reanalysis and ozonesonde measurements at five different Arctic stations. These chemical perturbations result in local temperature changes of up to 2 K, which may impact numerical weather prediction (NWP) of the tropospheric response to SSWs. Evaluation of the vertical residual velocity (w*) support the notion of transport changes being the driver of the temporal evolution of the anomalies. Using a stratospheric-tagged O<sub>3</sub> tracer, a signal for enhanced STE of ozone is subsequently inferred (~ 5-10 %), which is maximised around 50 days after the SSW onset date. We furthermore attempt to elucidate STE transport pathways using a tropopause fold identification algorithm applied to ERA-Interim during this period, and assess such changes in folding frequency and distribution during such events. Our results highlight that SSWs can induce significantly disturbed O<sub>3</sub> and H<sub>2</sub>O distributions in the UTLS, leading to enhanced STE of O<sub>3</sub>, with potentially significant implications for radiative fluxes, atmospheric heating rates and air quality.</p>

scholarly journals Relationship between Asian monsoon strength and transport of surface aerosols to the Asian Tropopause Aerosol Layer (ATAL): Interannual variability and decadal changes

2018 ◽  
Author(s):  
Cheng Yuan ◽  
William K. M. Lau ◽  
Zhanqing Li ◽  
Maureen Cribb ◽  
Tijian Wang
Keyword(s):  
Interannual Variability ◽  
Asian Monsoon ◽  
Asian Summer Monsoon ◽  
Deep Convection ◽  
Reanalysis Data ◽  
Aerosol Layer ◽  
Carbonaceous Aerosols ◽  
South Asian Summer Monsoon ◽  
Gangetic Plain ◽  
Monsoon Strength

Abstract. In this study, we have investigated the interannual variability and the decadal trend of carbon monoxide (CO), carbonaceous aerosols (CA), and mineral dust in the Asian Tropopause Aerosol Layer (ATAL) in relation to varying strengths of the South Asian summer monsoon (SASM) using MERRA2 reanalysis data (2001–2015). Results show that during this period, the aforementioned ATAL constituents exhibit strong interannual variability and rising trends connected to the variations of the strength of SASM. During strong monsoon years, the Asian Monsoon Anticyclone (AMA) is more expansive and shifted northward compared to weak years. In spite of effect of quenching of biomass burning emissions of CO and CA by increased precipitation, as well as the removal of CA and dust by increased washout from the surface to mid-troposphere in monsoon regions, all three constituents are found to be more abundant in an elongated accumulation zone at ATAL, on the southern flank of the expanded AMA. Enhanced transport to the ATAL by overshooting deep convection is found over preferred pathways along the foothills of the Himalayan-Gangetic Plain (HGP), and the Sichuan Basin (SB). The long-term positive trends of ATAL CO and CA are robust, while ATAL dust trend is weak due to its large interannual variability. The ATAL trends are associated with increasing strength of the AMA, with earlier and enhanced vertical transport of ATAT constituents by enhanced overshooting convection over the HGP and SB regions, out-weighing the strong reduction of CA and dust from surface to the mid-troposphere.

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