scholarly journals Comparison of emissions inventories of anthropogenic air pollutants and greenhouse gases in China

2017 ◽  
Vol 17 (10) ◽  
pp. 6393-6421 ◽  
Author(s):  
Eri Saikawa ◽  
Hankyul Kim ◽  
Min Zhong ◽  
Alexander Avramov ◽  
Yu Zhao ◽  
...  

Abstract. Anthropogenic air pollutant emissions have been increasing rapidly in China, leading to worsening air quality. Modelers use emissions inventories to represent the temporal and spatial distribution of these emissions needed to estimate their impacts on regional and global air quality. However, large uncertainties exist in emissions estimates. Thus, assessing differences in these inventories is essential for the better understanding of air pollution over China. We compare five different emissions inventories estimating emissions of carbon dioxide (CO2), carbon monoxide (CO), nitrogen oxides (NOx), sulfur dioxide (SO2), and particulate matter with an aerodynamic diameter of 10 µm or less (PM10) from China. The emissions inventories analyzed in this paper include the Regional Emission inventory in ASia v2.1 (REAS), the Multi-resolution Emission Inventory for China (MEIC), the Emission Database for Global Atmospheric Research v4.2 (EDGAR), the inventory by Yu Zhao (ZHAO), and the Greenhouse Gas and Air Pollution Interactions and Synergies (GAINS). We focus on the period between 2000 and 2008, during which Chinese economic activities more than doubled. In addition to national totals, we also analyzed emissions from four source sectors (industry, transport, power, and residential) and within seven regions in China (East, North, Northeast, Central, Southwest, Northwest, and South) and found that large disagreements exist among the five inventories at disaggregated levels. These disagreements lead to differences of 67 µg m−3, 15 ppbv, and 470 ppbv for monthly mean PM10, O3, and CO, respectively, in modeled regional concentrations in China. We also find that all the inventory emissions estimates create a volatile organic compound (VOC)-limited environment and MEIC emissions lead to much lower O3 mixing ratio in East and Central China compared to the simulations using REAS and EDGAR estimates, due to their low VOC emissions. Our results illustrate that a better understanding of Chinese emissions at more disaggregated levels is essential for finding effective mitigation measures for reducing national and regional air pollution in China.

2016 ◽  
Author(s):  
Eri Saikawa ◽  
Hankyul Kim ◽  
Min Zhong ◽  
Yu Zhao ◽  
Greet Janssens-Maenhout ◽  
...  

Abstract. Anthropogenic air pollutant emissions have been increasing rapidly in China. Modelers use emissions inventories to assess temporal and spatial distribution of these emissions to estimate their impacts on regional and global air quality. However, large uncertainties exist in emissions estimates and assessing discrepancies in these inventories is essential for better understanding of the trends in air pollution over China. We compare five different emissions inventories estimating emissions of carbon monoxide (CO), nitrogen oxides (NOx), sulfur dioxide (SO2), particulate matter with an aerodynamic diameter of 10 um or less (PM10) from China. The emissions inventories analyzed in this paper include Regional Emissions inventory in ASia v2.1 (REAS); Multi-resolution Emission Inventory for China (MEIC); Emission Database for Global Atmospheric Research v4.2 (EDGAR); the inventory by Yu Zhao (ZHAO); and the Greenhouse Gas and Air Pollution Interactions and Synergies (GAINS). We focus on the period between 2000 and 2008 during which the Chinese economic activities have more than doubled. In addition to the national total, we also analyzed emissions from four source sectors (industry, transportation, power, and residential) and within seven regions in China (East, North, Northeast, Central, Southwest, Northwest, and South) and found that large disagreements (~ seven fold) exist among the five inventories at disaggregated levels. These discrepancies lead to differences of 67 ug/m3, 15 ppbv, and 470 ppbv for monthly mean PM10, O3, and CO, respectively, in modelled regional concentrations in China. We also find that MEIC inventory emissions estimates create a VOC-limited environment that produces much lower O3 mixing ratio in the East and Central China compared to the simulations using REAS and EDGAR estimates. Our results illustrate that a better understanding of Chinese emissions at more disaggregated levels is essential for finding an effective mitigation measure for reducing national and regional air pollution in China.


2017 ◽  
Vol 10 (9) ◽  
pp. 3255-3276 ◽  
Author(s):  
Augustin Colette ◽  
Camilla Andersson ◽  
Astrid Manders ◽  
Kathleen Mar ◽  
Mihaela Mircea ◽  
...  

Abstract. The EURODELTA-Trends multi-model chemistry-transport experiment has been designed to facilitate a better understanding of the evolution of air pollution and its drivers for the period 1990–2010 in Europe. The main objective of the experiment is to assess the efficiency of air pollutant emissions mitigation measures in improving regional-scale air quality. The present paper formulates the main scientific questions and policy issues being addressed by the EURODELTA-Trends modelling experiment with an emphasis on how the design and technical features of the modelling experiment answer these questions. The experiment is designed in three tiers, with increasing degrees of computational demand in order to facilitate the participation of as many modelling teams as possible. The basic experiment consists of simulations for the years 1990, 2000, and 2010. Sensitivity analysis for the same three years using various combinations of (i) anthropogenic emissions, (ii) chemical boundary conditions, and (iii) meteorology complements it. The most demanding tier consists of two complete time series from 1990 to 2010, simulated using either time-varying emissions for corresponding years or constant emissions. Eight chemistry-transport models have contributed with calculation results to at least one experiment tier, and five models have – to date – completed the full set of simulations (and 21-year trend calculations have been performed by four models). The modelling results are publicly available for further use by the scientific community. The main expected outcomes are (i) an evaluation of the models' performances for the three reference years, (ii) an evaluation of the skill of the models in capturing observed air pollution trends for the 1990–2010 time period, (iii) attribution analyses of the respective role of driving factors (e.g. emissions, boundary conditions, meteorology), (iv) a dataset based on a multi-model approach, to provide more robust model results for use in impact studies related to human health, ecosystem, and radiative forcing.


2017 ◽  
Author(s):  
Augustin Colette ◽  
Camilla Andersson ◽  
Astrid Manders ◽  
Kathleen Mar ◽  
Mihaela Mircea ◽  
...  

Abstract. The Eurodelta-Trends multi-model chemistry-transport experiment has been designed to facilitate a better understanding of the evolution of air pollution and its drivers for the period 1990–2010 in Europe. The main objective of the experiment is to assess the efficiency of air pollutant emissions mitigation measures in improving regional scale air quality. The present paper formulates the main scientific questions and policy issues being addressed by the Eurodelta-Trends modelling experiment with an emphasis on how the design and technical features of the modelling experiment answer these questions. The experiment is designed in three tiers with increasing degree of computational demand in order to facilitate the participation of as many modelling teams as possible. The basic experiment consists of simulations for the years 1990, 2000 and 2010. Sensitivity analysis for the same three years using various combinations of (i) anthropogenic emissions, (ii) chemical boundary conditions and (iii) meteorology complements it. The most demanding tier consists two complete time series from 1990 to 2010, simulated using either time varying emissions for corresponding years or constant emissions. Eight chemistry-transport models have contributed with calculation results to at least one experiment tier, and three models have – to date – completed the full set of simulations (and 21-year trend calculations have been performed by four models). The modelling results are publicly available for further use by the scientific community. The main expected outcomes are (i) an evaluation of the models performances for the three reference years, (ii) an evaluation of the skill of the models in capturing observed air pollution trends for the 1990–2010 time period, (iii) attribution analyses of the respective role of driving factors (emissions/boundary conditions/meteorology), (iv) a dataset based on a multi-model approach, to provide more robust model results for use in impact studies related to human health, ecosystem and radiative forcing.


2014 ◽  
Vol 14 (18) ◽  
pp. 25617-25650 ◽  
Author(s):  
H. Y. Zhao ◽  
Q. Zhang ◽  
S. J. Davis ◽  
D. Guan ◽  
Z. Liu ◽  
...  

Abstract. High anthropogenic emissions from China have resulted in serious air pollution, and it has attracted considerable academic and public concern. The physical transport of air pollutants in the atmosphere has been extensively investigated, however, understanding the mechanisms how the pollutants were transferred through economic and trade activities remains challenge. In this work, we assessed China's virtual air pollutant transport embodied in trade, by using consumption-based accounting approach. We first constructed a consumption-based emission inventory for China's four key air pollutants (primary PM2.5, sulfur dioxide (SO2), nitrogen oxides (NOx) and non-methane volatile organic compounds (NMVOC)) in 2007, based on the bottom-up sectoral emission inventory concerning their production activities – a production-based inventory. We used a multiregional input-output (MRIO) model to integrate the sectoral production-based emissions and the associated economic and trade activities, and finally obtained consumption-based inventory. Unlike the production-based inventory, the consumption-based inventory tracked emissions throughout the supply chain related to the consumption of goods and services and hereby identified the emission flows followed the supply chains. From consumption-based perspective, emissions were significantly redistributed among provinces due to interprovincial trade. Large amount of emissions were embodied in the net imports of east regions from northern and central regions; these were determined by differences in the regional economic status and environmental policies. We also calculated the emissions embodied in exported and imported goods and services. It is found that 15–23% of China's pollutant emissions were related to exports for foreign consumption; that proportion was much higher for central and export-oriented coastal regions. It is suggested that measures should be introduced to reduce air pollution by integrating cross-regional consumers and producers in national agreements to encourage efficiency improvement in the supply chain and optimizing consumption structure internationally. The consumption-based air pollutants emission inventory developed in this work can be further used to attribute pollution to different economic activities and final demand types with the aid of air quality models.


2017 ◽  
Author(s):  
Lei Zhang ◽  
Tianliang Zhao ◽  
Sunling Gong ◽  
Shaofei Kong ◽  
Lili Tang ◽  
...  

Abstract. Air pollutant emissions play a determinant role in deteriorating air quality. However, an uncertainty in emission inventories is still the key problem for modeling air pollution. In this study, an updated emission inventory of coal-fired power plants (UEIPP) based on online monitoring data in Jiangsu province of East China for the year of 2012 was implemented in the widely used Multi-resolution Emission Inventory for China (MEIC). By employing the Weather Research and Forecasting Model with Chemistry (WRF-Chem), two simulations were executed to assess the atmospheric environmental change by using the original MEIC emission inventory and the MEIC inventory with the UEIPP. A synthetic analysis shows that (1) compared to the power emissions of MEIC, PM2.5, PM10, SO2 and NOx were lower, and CO, black carbon (BC), organic carbon (OC) and NMVOCs were higher in the UEIPP, reflecting a large discrepancy in the power emissions over East China; (2) In accordance with the changes of UEIPP, the modeled concentrations were reduced for SO2 and NO2, and increased for most areas of primary OC, BC and CO, whose concentrations in atmosphere are highly dependent on emission changes. (3) Interestingly, when the UEIPP was used, the atmospheric oxidizing capacity significantly reinforced, reflecting by increased oxidizing agents, e.g. O3 and OH, thus directly strengthened the chemical production from SO2 and NOx to sulfate and nitrate, which offset the reduction of primary PM2.5 emissions especially in the haze days. This study indicated the importance of updating air pollutant emission inventories in simulating the complex atmospheric environment changes with the implications on air quality and environmental changes.


2016 ◽  
Vol 113 (28) ◽  
pp. 7756-7761 ◽  
Author(s):  
Jun Liu ◽  
Denise L. Mauzerall ◽  
Qi Chen ◽  
Qiang Zhang ◽  
Yu Song ◽  
...  

As part of the 12th Five-Year Plan, the Chinese government has developed air pollution prevention and control plans for key regions with a focus on the power, transport, and industrial sectors. Here, we investigate the contribution of residential emissions to regional air pollution in highly polluted eastern China during the heating season, and find that dramatic improvements in air quality would also result from reduction in residential emissions. We use the Weather Research and Forecasting model coupled with Chemistry to evaluate potential residential emission controls in Beijing and in the Beijing, Tianjin, and Hebei (BTH) region. In January and February 2010, relative to the base case, eliminating residential emissions in Beijing reduced daily average surface PM2.5 (particulate mater with aerodynamic diameter equal or smaller than 2.5 micrometer) concentrations by 14 ± 7 μg⋅m−3 (22 ± 6% of a baseline concentration of 67 ± 41 μg⋅m−3; mean ± SD). Eliminating residential emissions in the BTH region reduced concentrations by 28 ± 19 μg⋅m−3 (40 ± 9% of 67 ± 41 μg⋅m−3), 44 ± 27 μg⋅m−3 (43 ± 10% of 99 ± 54 μg⋅m−3), and 25 ± 14 μg⋅m−3 (35 ± 8% of 70 ± 35 μg⋅m−3) in Beijing, Tianjin, and Hebei provinces, respectively. Annually, elimination of residential sources in the BTH region reduced emissions of primary PM2.5 by 32%, compared with 5%, 6%, and 58% achieved by eliminating emissions from the transportation, power, and industry sectors, respectively. We also find air quality in Beijing would benefit substantially from reductions in residential emissions from regional controls in Tianjin and Hebei, indicating the value of policies at the regional level.


2020 ◽  
Author(s):  
Youwen Sun ◽  
Hao Yin ◽  
Cheng Liu ◽  
Lin Zhang ◽  
Yuan Cheng ◽  
...  

Abstract. The major air pollutant emissions have decreased and the overall air quality has substantially improved across China in recent years as a consequence of active clean air policies for mitigating severe air pollution problems. As key precursors of formaldehyde (HCHO) and ozone (O3), the volatile organic compounds (VOCs) in China are still increasing because current clean air policies lack mitigation measures for VOCs. In this study, we mapped the drivers of HCHO variability over eastern China using ground-based high-resolution Fourier transform infrared (FTIR) spectrometry and GEOS-Chem model simulation. Diurnal, seasonal, and interannual variability of HCHO over eastern China was investigated and hydroxyl (OH) radical production from HCHO was evaluated. The relative contributions of emitted and photochemical sources to the observed HCHO were analysed by using ground level carbon monoxide (CO) and Ox (O3 + nitrogen oxide (NO2)) as tracers for emitted and photochemical HCHO, respectively. Contributions of various emission sectors and geographical transport to the observed HCHO summertime enhancements were determined by using a GEOS-Chem tagged-tracer simulation. The tropospheric HCHO volume mixing ratio (VMR) reached a maximum monthly mean value of (1.1 ± 0.27) ppbv in July and a minimum monthly mean value of (0.4 ± 0.11) ppbv in January. The tropospheric HCHO VMR time series from 2015–2019 shows a positive trend of (1.43 ± 0.14) % per yr. The photochemical HCHO is the dominant source of atmospheric HCHO over eastern China for most of the year (68.1 %). In the studied years, the HCHO photolysis was an important source of OH radical over eastern China during all sunlight hours of both summer and winter days. The anthropogenic emissions (fossil fuel + biofuel emissions) accounted for 31.96 % and the natural emissions (biomass burning + biogenic) accounted for 48.75 % of HCHO summertime enhancements. The observed HCHO summertime enhancements were largely attributed to the emissions within China (76.92 %), where eastern China dominated the contribution (46.24 %). The increased trend in HCHO in recent years was largely attributed to the increase in the HCHO precursors such as CH4 and nonmethane VOCs (NMVOCs). This study can provide an evaluation of recent VOC emissions and regional photochemical capacity in China. In addition, this study is also important for regulatory and control purposes and will help to improve urban air quality and contribute to the formation of new Chinese clean air policies in the future.


Author(s):  
Oleksandr Zaporozhets ◽  
Sergii Karpenko ◽  
Sergii Puzik ◽  
Bogdan Sagaidak

Development of a single method for inventory of pollutant emissions from installations based on the elaboration of existing methods for calculation of air pollution is an important scientific and practical task in the field of environmental safety. The main purpose of the study is to test and compare models of stationary emission sources and to assess air quality based on them. In the inventory of pollutant emissions, the following materials are used: direct measurements, which are based on direct instrumental measurements, and calculated measurements or combinations thereof. According to the direct measurements of NOx and CO emissions from the operation of gas turbines at the Valley compressor station with a nominal capacity of 1 to 50 MW, we found that: the actual emissions of NO and CO increase with the average load on the installation and the time of introduction into operation and date of issue and the actual values of the maximum allowable concentration of NOx (from 100.13 to 467 mg / m) and CO (from 16.08 to 444.88 mg / m) do not exceed the permissible levels of NO-500 mg / m and CO-250 mg / m according to the instructional documents. Comparison of these calculation methods showed the same results, which confirms the need for their systematization with the subsequent development of a single methodology. The distance of 106 m, where the maximum concentration of pollution in adverse weather conditions is expected, was obtained by the calculation method of determining the surface concentration of NOx and CO emissions from the installation. To assess the effectiveness of the methods for inventory of pollutant emissions into the atmosphere from gas turbines, we have developed a scheme of relationship between the object being assessed for efficiency and the object being serviced. Particularly noteworthy are the results and analysis of direct measurements of NOx and CO emissions, as well as the developed scheme for linking the inventory process for pollutant emissions into the atmosphere from installations. The actual concentration of pollutants can be estimated by measuring the background, although in this case it is impossible to exclude the influence of other neighboring and remote emission sources on the results of the air pollution assessment. Depending on the specific task, the results of computer simulation for given parameters of the external environment can also be used to assess the actual, retrospective or prospective conditions. Future conditions can be modeled only with the help of computer simulation. The method of air pollutant concentration calculation for emissions of enterprises does not consider all possible features of emission sources and, in terms of passive stationary sources and cold emissions, the algorithm needs to be clarified and the justifications in the paper indicate ways to make these improvements. Inventory is the first stage in the strategy of air quality regulation, as it provides information for the development, justification and decision-making in regulating the activities of gas turbines to reduce adverse effects on the environment and public health.


2020 ◽  
Vol 117 (32) ◽  
pp. 18984-18990 ◽  
Author(s):  
Zander S. Venter ◽  
Kristin Aunan ◽  
Sourangsu Chowdhury ◽  
Jos Lelieveld

The lockdown response to coronavirus disease 2019 (COVID-19) has caused an unprecedented reduction in global economic and transport activity. We test the hypothesis that this has reduced tropospheric and ground-level air pollution concentrations, using satellite data and a network of >10,000 air quality stations. After accounting for the effects of meteorological variability, we find declines in the population-weighted concentration of ground-level nitrogen dioxide (NO2: 60% with 95% CI 48 to 72%), and fine particulate matter (PM2.5: 31%; 95% CI: 17 to 45%), with marginal increases in ozone (O3: 4%; 95% CI: −2 to 10%) in 34 countries during lockdown dates up until 15 May. Except for ozone, satellite measurements of the troposphere indicate much smaller reductions, highlighting the spatial variability of pollutant anomalies attributable to complex NOxchemistry and long-distance transport of fine particulate matter with a diameter less than 2.5 µm (PM2.5). By leveraging Google and Apple mobility data, we find empirical evidence for a link between global vehicle transportation declines and the reduction of ambient NO2exposure. While the state of global lockdown is not sustainable, these findings allude to the potential for mitigating public health risk by reducing “business as usual” air pollutant emissions from economic activities. Explore trends here:https://nina.earthengine.app/view/lockdown-pollution.


Atmosphere ◽  
2018 ◽  
Vol 9 (11) ◽  
pp. 449 ◽  
Author(s):  
Agapol Junpen ◽  
Jirataya Pansuk ◽  
Orachorn Kamnoet ◽  
Penwadee Cheewaphongphan ◽  
Savitri Garivait

Crop residue burning negatively impacts both the environment and human health, whether in the aspect of air pollution, regional and global climate change, or transboundary air pollution. Accordingly, this study aims to assess the level of air pollutant emissions caused by the rice residue open burning activities in 2018, by analyzing the remote sensing information and country specific data. This research also aims to analyze the trend of particulate matter 10 microns or less in diameter (PM10) concentration air quality sites in provinces with large paddy rice planting areas from 2010–2017. According to the results, 61.87 megaton (Mt) of rice residue were generated, comprising 21.35 Mt generated from the irrigated fields and 40.53 Mt generated from the rain-fed field. Only 23.0% of the total rice residue generated were subject to open burning—of which nearly 32% were actually burned in the fields. The emissions from such rice residue burning consisted of: 5.34 ± 2.33 megaton (Mt) of CO2, 44 ± 14 kiloton (kt) of CH4, 422 ± 179 kt of CO, 2 ± 2 kt of NOX, 2 ± 2 kt of SO2, 38 ± 22 kt of PM2.5, 43 ± 29 kt of PM10, 2 ± 1 kt of black carbon (BC), and 14 ± 5 kt of organic carbon (OC). According to the air quality trends, the results shows the higher level of PM10 concentration was due to the agricultural burning activities, as reflected in the higher monthly averages of the months with the agricultural burning, by around 1.9–2.1 times. The result also shows the effect of government’s policy for farmers on the crop burning activities and air quality trends.


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